Islands, mounds, and atoms: patterns and processes in crystal growth far from equilibrium
Gespeichert in:
| Hauptverfasser: | , |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Berlin [u.a.]
Springer
2004
|
| Schriftenreihe: | Springer series in surface sciences
42 |
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | Literaturverz. S. 287 - 305 |
| Beschreibung: | XVIII, 313 S. Ill., graph. Darst. |
| ISBN: | 9783642622373 3540407286 |
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| 100 | 1 | |a Michely, Thomas |e Verfasser |4 aut | |
| 245 | 1 | 0 | |a Islands, mounds, and atoms |b patterns and processes in crystal growth far from equilibrium |c T. Michely ; J. Krug |
| 264 | 1 | |a Berlin [u.a.] |b Springer |c 2004 | |
| 300 | |a XVIII, 313 S. |b Ill., graph. Darst. | ||
| 336 | |b txt |2 rdacontent | ||
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| 490 | 1 | |a Springer series in surface sciences |v 42 | |
| 490 | 0 | |a Physics and astronomy online library | |
| 500 | |a Literaturverz. S. 287 - 305 | ||
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Datensatz im Suchindex
| _version_ | 1804130290331811840 |
|---|---|
| adam_text | CONTENTS LIST OF FREQUENTLY USED SYMBOLS ..............................
XV 1. INTRODUCTION .............................................. 1 1.1
ATOMS, CRYSTALS AND VISUALIZATION . . . . . . . . . . . . . . . . . . .
. . . . . 1 1.2 CRYSTAL GROWTH FAR FROM EQUILIBRIUM . . . . . . . . . .
. . . . . . . . . . . 5 1.3 EPITAXY . . . . . . . . . . . . . . . . . .
. . . . . . . . . . . . . . . . . . . . . . . . . . . . . 8 1.4 ABOUT
THIS BOOK . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .
. . . . . . . . 10 2. CONDENSATION, DIFFUSION AND NUCLEATION
.................. 13 2.1 ARRIVING AT THE SURFACE: STICKING AND
TRANSIENT MOBILITY . . . . . . . . . . . . . . . . . . . . . . . . . .
13 2.2 MOVING ON: SURFACE DIFFUSION . . . . . . . . . . . . . . . . . .
. . . . . . . . . . . 16 2.2.1 THE SURFACE DIFFUSION COEFFICIENT . . . .
. . . . . . . . . . . . . . . 16 2.2.2 TRANSITION STATE THEORY . . . . .
. . . . . . . . . . . . . . . . . . . . . . 18 2.2.3 DIRECT OBSERVATION
OF ADATOM DIFFUSION . . . . . . . . . . . . . 20 2.2.4 THE ONSET METHOD
. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 22 2.2.5
THEORETICAL ESTIMATES OF DIFFUSION PARAMETERS ON PT(111) . . . . . . . .
. . . . . . . . . 24 2.3 GETTING TOGETHER: TWO-DIMENSIONAL NUCLEATION .
. . . . . . . . . . . 25 2.3.1 ATOMISTIC NUCLEATION THEORY . . . . . . .
. . . . . . . . . . . . . . . 25 2.3.2 THE ISLAND SIZE DISTRIBUTION . .
. . . . . . . . . . . . . . . . . . . . . 29 2.3.3 EXPERIMENTAL TEST OF
NUCLEATION THEORY . . . . . . . . . . . . 31 2.3.4 BINDING ENERGIES FROM
ISLAND DENSITIES . . . . . . . . . . . . . . 35 2.4 SUPPLEMENTARY
TOPICS. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .
. . 41 2.4.1 CONDENSATION ON CLUSTERS AND AT STEPS . . . . . . . . . . .
. . . 41 2.4.2 EXCHANGE DIFFUSION . . . . . . . . . . . . . . . . . . .
. . . . . . . . . . . . 46 2.4.3 NUCLEATION AND RANDOM WALKS . . . . . .
. . . . . . . . . . . . . . . 47 2.4.4 NUCLEATION WITH MOBILE CLUSTERS.
. . . . . . . . . . . . . . . . . . . 49 2.4.5 ADATOM*ADATOM
INTERACTIONS AND NUCLEATION THEORY . 51 2.4.6 ADSORBATE INFLUENCED
DIFFUSION AND NUCLEATION . . . . . . . 54 3. ISLAND SHAPES
............................................. 61 3.1 ISLAND SHAPES AND
THE HIERARCHY OF DIFFUSION PROCESSES. . . . . . . . . . . . . . . . . .
. 61 XII CONTENTS 3.2 THE EQUILIBRIUM SHAPE OF ADATOM AND VACANCY
ISLANDS . . . . . . . . . . . . . . . . . . . . . . . . . . 66 3.2.1
DEFINITION AND THE WULFF CONSTRUCTION. . . . . . . . . . . . . . . 66
3.2.2 EXPERIMENTAL REALIZATION OF 2D EQUILIBRIUM SHAPES . . 69 3.2.3 THE
ISING MODEL AND THE AWNING APPROXIMATION . . . . . 72 3.2.4 ABSOLUTE
ENERGY VALUES FOR STEPS AND KINKS . . . . . . . . . 78 3.3
FRACTAL-DENDRITIC ISLANDS . . . . . . . . . . . . . . . . . . . . . . .
. . . . . . . . . 81 3.4 COMPACT, TRIANGULAR ISLANDS . . . . . . . . . .
. . . . . . . . . . . . . . . . . . . 88 3.5 ADSORBATES AND ISLAND
SHAPES . . . . . . . . . . . . . . . . . . . . . . . . . . . . 94 3.6
SHAPE INSTABILITIES AND THE DIFFUSION FIELD . . . . . . . . . . . . . .
. . . 99 3.7 SUPPLEMENTARY TOPICS. . . . . . . . . . . . . . . . . . . .
. . . . . . . . . . . . . . . 109 3.7.1 MIGRATION ALONG ROUGH ISLAND
EDGES . . . . . . . . . . . . . . . 109 3.7.2 THE TRANSITION FROM
FRACTAL-DENDRITIC TO COMPACT ISLANDS: THEORY VERSUS EXPERIMENT . . . . .
. 112 3.7.3 STABILITY CRITERIA FOR COMPACT ISLANDS . . . . . . . . . . .
. . . . 116 4. PATTERN FORMATION IN MULTILAYER GROWTH .................
121 4.1 THE TEMPERATURE DEPENDENCE OF MULTILAYER GROWTH . . . . . . . .
121 4.1.1 GROWTH MODES ON PT(111): TEAS . . . . . . . . . . . . . . . .
. . 124 4.1.2 GROWTH MODES ON PT(111): STM . . . . . . . . . . . . . . .
. . . . 126 4.1.3 ROUGHNESS MEASURES . . . . . . . . . . . . . . . . . .
. . . . . . . . . . . . 127 4.2 STATISTICAL GROWTH AND THE SHAPE OF
WEDDING CAKES . . . . . . . . 129 4.3 INTERLAYER TRANSPORT . . . . . . .
. . . . . . . . . . . . . . . . . . . . . . . . . . . . . 138 4.3.1 THE
STEP EDGE BARRIER AND SOME OF ITS CONSEQUENCES . 138 4.3.2 THEORY OF
SECOND LAYER NUCLEATION . . . . . . . . . . . . . . . . . 142 4.3.3
EXPERIMENTAL DETERMINATION OF THE STEP EDGE BARRIER . 146 4.3.4
THEORETICAL ESTIMATES OF STEP CROSSING RATES ON PT(111)155 4.4 STEP
ATOMIC STRUCTURE AND GROWTH MODES ON PT(111) . . . . . . . . . . . . . .
. . . . . . . . . . . . . 158 4.4.1 A MODEL FOR THE EFFECTIVE STEP EDGE
BARRIER . . . . . . . . . 158 4.4.2 FILM THICKNESS DEPENDENCE OF *E EFF
S AT 440 K . . . . . . . 159 4.4.3 LOW TEMPERATURE GROWTH ON PT(111) . .
. . . . . . . . . . . . . 161 4.4.4 GROWTH BIFURCATION AROUND 500 K . .
. . . . . . . . . . . . . . . . 163 4.4.5 CO ADSORPTION AND MOUND GROWTH
ON PT(111) . . . . . . 165 4.4.6 A CRITERION FOR MOUND GROWTH . . . . .
. . . . . . . . . . . . . . . . 167 4.5 MOUND FORMATION WITH WEAK
BARRIERS . . . . . . . . . . . . . . . . . . . . 168 4.5.1 DIFFUSION
BIAS AND THE GROWTH-INDUCED CURRENT . . . . . . 169 4.5.2 WEAK BARRIERS:
ONSET OF THE INSTABILITY . . . . . . . . . . . . . . 171 4.5.3 WEAK
BARRIERS: MOUND SHAPES . . . . . . . . . . . . . . . . . . . . . 175 4.6
LONG TIME EVOLUTION OF THE MOUND MORPHOLOGY. . . . . . . . . . . . 176
4.6.1 SLOPE SELECTION . . . . . . . . . . . . . . . . . . . . . . . . .
. . . . . . . . . . 176 4.6.2 COARSENING . . . . . . . . . . . . . . . .
. . . . . . . . . . . . . . . . . . . . . . 179 4.7 GROWTH INSTABILITIES
OF VICINAL SURFACES. . . . . . . . . . . . . . . . . . . . 186 4.7.1
STABILITY OF A STEP TRAIN. . . . . . . . . . . . . . . . . . . . . . . .
. . . 187 4.7.2 STEP MEANDERING: THE BALES*ZANGWILL INSTABILITY . . . .
. 188 CONTENTS XIII 4.7.3 STEP MEANDERING: EXPERIMENTS AND ALTERNATIVE
MECHANISMS . . . . . . . . . . . 191 4.7.4 THE ULTIMATE FATE OF STEP
FLOW . . . . . . . . . . . . . . . . . . . . 195 4.8 SELF*AFFINE GROWTH
. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .
. 197 4.8.1 UNIVERSALITY CLASSES OF KINETIC ROUGHENING . . . . . . . . .
. 200 4.8.2 CONSERVED AND NONCONSERVED GROWTH . . . . . . . . . . . . .
. . 201 4.8.3 KINETIC ROUGHENING AND MOUND FORMATION . . . . . . . . . .
204 4.9 SUPPLEMENTARY TOPICS. . . . . . . . . . . . . . . . . . . . . .
. . . . . . . . . . . . . 206 4.9.1 GROWTH REGIMES AND SURFACE ATOMIC
STRUCTURE . . . . . . 206 4.9.2 RIPPLE FORMATION IN HOMOEPITAXIAL GROWTH
. . . . . . . . . 209 4.9.3 DERIVATION OF THE STEP EDGE BOUNDARY
CONDITION . . . . . 211 4.9.4 SECOND LAYER NUCLEATION AND RATE EQUATIONS
. . . . . . . . 213 4.9.5 SECOND LAYER NUCLEATION WITH REVERSIBLE
AGGREGATION . 214 4.9.6 FURTHER EXPERIMENTAL SIGNATURES OF THE STEP EDGE
BARRIER . . . . . . . . . . . . . . . . . . . . . . . . . . 215 4.9.7
DIFFUSION BIAS WITHOUT A STEP EDGE BARRIER . . . . . . . . . 218 4.9.8
CONTINUUM THEORY OF MOUND COARSENING . . . . . . . . . . . . 219 4.9.9
STABILITY OF VICINAL SURFACES: CONTINUUM APPROACH . . . 225 5.
LAYER*BY*LAYER GROWTH AND GROWTH MANIPULATION
................................ 227 5.1 BASIC CONCEPTS . . . . . . . .
. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 227
5.2 LAYER*BY*LAYER GROWTH BY SURFACTANTS . . . . . . . . . . . . . . . .
. . . 230 5.3 LAYER*BY*LAYER GROWTH THROUGH GROWTH MANIPULATION. . . . .
236 5.4 LAYER*BY*LAYER GROWTH THROUGH SURFACE RECONSTRUCTION . . . 238
5.5 THEORY OF PULSED DEPOSITION . . . . . . . . . . . . . . . . . . . .
. . . . . . . . . 245 5.6 KINETIC ROUGHENING AND LAYER*BY*LAYER GROWTH.
. . . . . . . . . . 248 6. METHODS
.................................................. 253 6.1 DEPOSITION
AND VACUUM . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .
. . 253 6.2 MICROSCOPY . . . . . . . . . . . . . . . . . . . . . . . . .
. . . . . . . . . . . . . . . . . . . 256 6.2.1 SCANNING TUNNELING
MICROSCOPY . . . . . . . . . . . . . . . . . . . . 257 6.2.2 FIELD ION
MICROSCOPY . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 261
6.3 DIFFRACTION . . . . . . . . . . . . . . . . . . . . . . . . . . . .
. . . . . . . . . . . . . . . . . 264 6.4 TOTAL ENERGY CALCULATIONS . .
. . . . . . . . . . . . . . . . . . . . . . . . . . . . . 269 6.4.1
DENSITY FUNCTIONAL THEORY . . . . . . . . . . . . . . . . . . . . . . .
. 270 6.4.2 SEMI-EMPIRICAL MANY BODY POTENTIALS . . . . . . . . . . . .
. . 273 6.5 GROWTH SIMULATIONS. . . . . . . . . . . . . . . . . . . . .
. . . . . . . . . . . . . . . . 277 6.5.1 MOLECULAR DYNAMICS . . . . . .
. . . . . . . . . . . . . . . . . . . . . . . . 277 6.5.2 THE KINETIC
MONTE CARLO METHOD . . . . . . . . . . . . . . . . . . 278 6.5.3
CONSTRUCTING KMC MODELS . . . . . . . . . . . . . . . . . . . . . . . .
281 6.5.4 HYBRID APPROACHES . . . . . . . . . . . . . . . . . . . . . .
. . . . . . . . . 285 REFERENCES
.................................................... 287 INDEX
......................................................... 307
|
| any_adam_object | 1 |
| author | Michely, Thomas Krug, Joachim |
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| ctrlnum | (OCoLC)52749966 (DE-599)BVBBV017491843 |
| dewey-full | 548/.5 |
| dewey-hundreds | 500 - Natural sciences and mathematics |
| dewey-ones | 548 - Crystallography |
| dewey-raw | 548/.5 |
| dewey-search | 548/.5 |
| dewey-sort | 3548 15 |
| dewey-tens | 540 - Chemistry and allied sciences |
| discipline | Chemie / Pharmazie Physik |
| format | Book |
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| id | DE-604.BV017491843 |
| illustrated | Illustrated |
| indexdate | 2024-07-09T19:18:41Z |
| institution | BVB |
| isbn | 9783642622373 3540407286 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-010537669 |
| oclc_num | 52749966 |
| open_access_boolean | |
| owner | DE-20 DE-19 DE-BY-UBM DE-703 DE-91G DE-BY-TUM DE-29T DE-634 DE-83 DE-11 DE-188 |
| owner_facet | DE-20 DE-19 DE-BY-UBM DE-703 DE-91G DE-BY-TUM DE-29T DE-634 DE-83 DE-11 DE-188 |
| physical | XVIII, 313 S. Ill., graph. Darst. |
| publishDate | 2004 |
| publishDateSearch | 2004 |
| publishDateSort | 2004 |
| publisher | Springer |
| record_format | marc |
| series | Springer series in surface sciences |
| series2 | Springer series in surface sciences Physics and astronomy online library |
| spelling | Michely, Thomas Verfasser aut Islands, mounds, and atoms patterns and processes in crystal growth far from equilibrium T. Michely ; J. Krug Berlin [u.a.] Springer 2004 XVIII, 313 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Springer series in surface sciences 42 Physics and astronomy online library Literaturverz. S. 287 - 305 Crystal growth Homoepitaxie (DE-588)4457865-9 gnd rswk-swf Kristallwachstum (DE-588)4123579-4 gnd rswk-swf Irreversibler Prozess (DE-588)4027687-9 gnd rswk-swf Homoepitaxie (DE-588)4457865-9 s Kristallwachstum (DE-588)4123579-4 s Irreversibler Prozess (DE-588)4027687-9 s DE-604 Krug, Joachim Verfasser aut Springer series in surface sciences 42 (DE-604)BV000600785 42 SWB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=010537669&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Michely, Thomas Krug, Joachim Islands, mounds, and atoms patterns and processes in crystal growth far from equilibrium Springer series in surface sciences Crystal growth Homoepitaxie (DE-588)4457865-9 gnd Kristallwachstum (DE-588)4123579-4 gnd Irreversibler Prozess (DE-588)4027687-9 gnd |
| subject_GND | (DE-588)4457865-9 (DE-588)4123579-4 (DE-588)4027687-9 |
| title | Islands, mounds, and atoms patterns and processes in crystal growth far from equilibrium |
| title_auth | Islands, mounds, and atoms patterns and processes in crystal growth far from equilibrium |
| title_exact_search | Islands, mounds, and atoms patterns and processes in crystal growth far from equilibrium |
| title_full | Islands, mounds, and atoms patterns and processes in crystal growth far from equilibrium T. Michely ; J. Krug |
| title_fullStr | Islands, mounds, and atoms patterns and processes in crystal growth far from equilibrium T. Michely ; J. Krug |
| title_full_unstemmed | Islands, mounds, and atoms patterns and processes in crystal growth far from equilibrium T. Michely ; J. Krug |
| title_short | Islands, mounds, and atoms |
| title_sort | islands mounds and atoms patterns and processes in crystal growth far from equilibrium |
| title_sub | patterns and processes in crystal growth far from equilibrium |
| topic | Crystal growth Homoepitaxie (DE-588)4457865-9 gnd Kristallwachstum (DE-588)4123579-4 gnd Irreversibler Prozess (DE-588)4027687-9 gnd |
| topic_facet | Crystal growth Homoepitaxie Kristallwachstum Irreversibler Prozess |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=010537669&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| volume_link | (DE-604)BV000600785 |
| work_keys_str_mv | AT michelythomas islandsmoundsandatomspatternsandprocessesincrystalgrowthfarfromequilibrium AT krugjoachim islandsmoundsandatomspatternsandprocessesincrystalgrowthfarfromequilibrium |