Verfügbarkeit: Basic principles in applied catalysis

Basic principles in applied catalysis:

Gespeichert in:

Bibliographische Detailangaben
Format:	Buch
Sprache:	English
Veröffentlicht:	Berlin [u.a.] Springer 2004
Schriftenreihe:	Springer series in chemical physics 75
Schlagworte:	Biokatalyse Catalyse Físico-química Katalysatoren Katalyse Reactiekinetiek Catalysis Katalysator Aufsatzsammlung
Online-Zugang:	Inhaltsverzeichnis
Beschreibung:	X, 557 S. Ill., graph. Darst.
ISBN:	3540441352 3540402616

Internformat

MARC


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Datensatz im Suchindex

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adam_text	CONTENTS PART I SYNTHETIC APPROACHES TO NANOMOLECULAR SYSTEMS 1 DYNAMIC REDOX SYSTEMS: TOWARDS THE REALIZATION OF UNIMOLECULAR MEMORY TAKANORI SUZUKI, HIROKI HIGUCHI, TAKASHI TSUJI, JUN-ICHI NISHIDA, YOSHIRO YAMASHITA, TSUTOMU MIYASHI ............................. 3 1.1 INTRODUCTION . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 3 1.2 REDOX SYSTEMS THAT EXHIBIT DRASTIC GEOMETRICAL CHANGES UPON ET 4 1.2.1 FOLDEDPLANAR STRUCTURAL CHANGE . . . . . . . . . . . . . . . . . . . . . . . 5 1.2.2 PLANARTWISTED STRUCTURAL CHANGE . . . . . . . . . . . . . . . . . . . . . . 5 1.2.3 TWISTEDTWISTED STRUCTURAL CHANGE . . . . . . . . . . . . . . . . . . . . . 7 1.2.4 FOLDEDTWISTED STRUCTURAL CHANGE . . . . . . . . . . . . . . . . . . . . . . 9 1.3 REDOX SYSTEMS THAT UNDERGO R EVERSIBLE BOND MAKING/BREAKING UPON ET . . . . . . . . . . . . . . . . . . . 11 1.3.1 REVERSIBLE BOND MAKING / BREAKING BETWEEN HETEROATOMS UPON ET . . . . . . . . . . . . . . . . . . . . . . . . . 12 1.3.2 * -ELECTRON SYSTEMS THAT UNDERGO CC BOND MAKING UPON IONIZATION . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 12 1.3.3 -ELECTRON SYSTEMS THAT UNDERGO CC BOND BREAKING UPON IONIZATION . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 16 1.4 TOWARD THE R EALIZATION OF UNIMOLECULAR MEMORY . . . . . . . . . . . . . . . 19 R EFERENCES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 20 2 PHOTOSWITCHING OF INTRAMOLECULAR MAGNETIC INTERACTION USING PHOTOCHROMIC COMPOUNDS KENJI MATSUDA, MASAHIRO IRIE ..................................... 25 2.1 INTRODUCTION . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 25 2.2 PHOTOCHROMIC COMPOUNDS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 26 2.3 INTRAMOLECULAR MAGNETIC INTERACTION . . . . . . . . . . . . . . . . . . . . . . . . . . . 26 2.4 PHOTOSWITCHING USING A SINGLE PHOTOCHROMIC MOLECULE . . . . . . . . . . . . . . . . . . . . . . . . . 28 2.4.1 MOLECULAR DESIGN . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 28 2.4.2 SWITCHING OF MAGNETIC INTERACTION DETECTED BY SUSCEPTIBILITY MEASUREMENT . . . . . . . . . . . . . . . . . . 30 X CONTENTS 2.4.3 SWITCHING OF MAGNETIC INTERACTION DETECTED BY ESRSPECTRA 32 2.5 PHOTOSWITCHING USING AN ARRAY OF PHOTOCHROMIC MOLECULES . . . . . . 36 2.6 CONCLUDING R EMARKS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 39 ACKNOWLEDGMENTS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 39 R EFERENCES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 39 3 SINGLE-MOLECULE MAGNETS KEIJI TAKEDA, KUNIO AWAGA ...................................... 41 3.1 SINGLE-DOMAIN MAGNETS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 41 3.2 TWELVE-NUCLEUS MANGANESE CLUSTERS. . . . . . . . . . . . . . . . . . . . . . . . . . . 43 3.3 THERMAL RELAXATION IN MN 12 . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 45 3.4 JAHNTELLER ISOMERS IN MN 12 . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 47 3.4.1 MAGNETIC PROPERTIES OF THE SLOWER AND FASTER MOLECULES . . . . 47 3.4.2 MOLECULAR STRUCTURE OF THE SLOWER AND FASTER MOLECULES . . . . 49 3.5 QUANTUM RELAXATION IN MN 12 . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 51 3.5.1 QUANTUM R ELAXATION OF THE SLOWER-R ELAXATION MOLECULE . . . . 51 3.5.2 QUANTUM R ELAXATION OF THE FASTER-R ELAXATION MOLECULE . . . . 52 3.6 QUANTUM COMPUTING WITH SMMS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 53 3.7 SUMMARY . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 54 R EFERENCES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 55 4 ATOMIC RESOLUTION OF PORPHYRINS: SINGLE-MOLECULE OBSERVATIONS OF PORPHYRINOID COMPOUNDS BY SCANNING TUNNELING MICROSCOPY KEN-ICHI SUGIURA, HITOSHI MIYASAKA, TOMOHIKO ISHII, MASAHIRO YAMASHITA ............................................. 59 4.1 INTRODUCTION . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 59 4.2 WHY PORPHYRINS? . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 59 4.3 PHTHALOCYANINES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 62 4.3.1 COPPER PHTHALOCYANINE . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 62 4.3.2 EFFECT OF SUBSTRATE. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 62 4.3.3 EFFECT OF INCORPORATED METALS . . . . . . . . . . . . . . . . . . . . . . . . . . . 63 4.3.4 CHEMICALLY MODIFIED PHTHALOCYANINES . . . . . . . . . . . . . . . . . . . . 64 4.4 PORPHYRINS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 65 4.4.1 TETRAPHENYLPORPHYRINS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 65 4.4.2 OTHER SIMPLE PORPHYRINS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 69 4.4.3 PORPHYRIN OLIGOMERS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 69 R EFERENCES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 70 CONTENTS XI PART II SURFACE MOLECULAR SYSTEMS 5 CARBOXYLATES ADSORBED ON TIO 2 (110) HIROSHI ONISHI .................................................. 75 5.1 INTRODUCTION . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 75 5.2 RUTILE TIO 2 (110), THE SUBSTRATE . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 76 5.3 FORMATE ON TIO 2 (110) . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 78 5.4 OTHER CARBOXYLATES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 82 5.5 CARBOXYLATE MONOLAYERS OF MIXED COMPOSITION . . . . . . . . . . . . . . . . . 84 5.6 PROSPECTS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 85 ACKNOWLEDGMENTS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 86 R EFERENCES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 86 6 SELF-ASSEMBLED MONOLAYERS FOR MOLECULAR NANOELECTRONICS TAKAO ISHIDA ................................................... 91 6.1 INTRODUCTION . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 91 6.2 BASIC PROPERTIES OF ORGANOSULFUR SAMS ON AU SURFACES . . . . . . . . . . 92 6.3 STM OBSERVATION OF ORGANOSULFUR SAMS . . . . . . . . . . . . . . . . . . . . . . 94 6.4 NANOSTRUCTURE FORMATION USING SAMS . . . . . . . . . . . . . . . . . . . . . . . . . 98 6.5 ELECTRICAL-CONDUCTION MEASUREMENTS OF SAMS . . . . . . . . . . . . . . . . . . 99 6.6 STABILITY OF SAMS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 102 6.7 CONCLUSIONS AND FUTURE EXPECTATIONS. . . . . . . . . . . . . . . . . . . . . . . . . . 103 ACKNOWLEDGMENTS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 103 R EFERENCES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 104 7 SUPRAMOLECULAR CHEMISTRY ON SOLID SURFACES TAKUYA MATSUMOTO, TOMOJI KAWAI, TAKASHI YOKOYAMA .............. 107 7.1 SUPRAMOLECULAR ASSEMBLY IN MOLECULAR-SCALE ELECTRONICS . . . . . . . . . 107 7.2 SUPRAMOLECULAR APPROACH . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 108 7.3 DIPOLEDIPOLE INTERACTIONS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 109 7.4 HYDROGEN BONDS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 114 7.5 -STACKING INTERACTIONS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 115 7.6 CONCLUDING R EMARKS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 120 R EFERENCES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 121 8 SEMICONDUCTOR AND MOLECULAR-ASSEMBLY NANOWIRES TOMOYUKI AKUTAGAWA, TAKAYOSHI NAKAMURA ........................ 123 8.1 INTRODUCTION . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 123 8.2 SEMICONDUCTOR NANOWIRES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 126 8.2.1 PREPARATION AND ASSEMBLY . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 127 8.2.2 ELECTRICAL PROPERTIES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 132 8.2.3 P * N JUNCTIONS AND FET DEVICES . . . . . . . . . . . . . . . . . . . . . . . . . 134 XII CONTENTS 8.3 NANOWIRES OF MOLECULAR ASSEMBLIES . . . . . . . . . . . . . . . . . . . . . . . . . . . . 136 8.3.1 MOLECULAR CONDUCTORS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 138 8.3.2 TTF*BR NANOCRYSTALS. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 139 8.3.3 CROWN-ETHER-FUSED PHTHALOCYANINE . . . . . . . . . . . . . . . . . . . . . . 140 8.3.4 TTF MACROCYCLE . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 142 8.4 SUMMARY . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 143 R EFERENCES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 144 9 CONTROL OF DYE AGGREGATES IN MICROSCOPIC POLYMER MATRICES OLAF KARTHAUS .................................................. 149 9.1 CYANINE DYES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 149 9.2 DEWETTING-ASSISTED POLYMER MICRODOME FORMATION . . . . . . . . . . . . . 151 9.3 R ESULTS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 151 9.3.1 MICROSCOPY OF POLYSTYRENE MATRICES . . . . . . . . . . . . . . . . . . . . . 151 9.3.2 SPECTROSCOPY . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 154 9.3.3 MICROSCOPY OF LIQUID CRYSTALLINE MATRICES . . . . . . . . . . . . . . . 158 9.4 OUTLOOK . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 160 R EFERENCES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 160 PART III THEORY OF NANOMOLECULAR SYSTEMS 10 THEORETICAL CALCULATIONS OF ELECTRICAL PROPERTIES OF NANOSCALE SYSTEMS UNDER THE INFLUENCE OF ELECTRIC FIELDS AND CURRENTS SATOSHI WATANABE . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 165 10.1 PROBLEMS OF CONVENTIONAL METHODS. . . . . . . . . . . . . . . . . . . . . . . . . . . . 165 10.2 METHODS TO TREAT NANOMOLECULAR SYSTEMS UNDER THE INFLUENCE OF ELECTRIC FIELDS AND CURRENTS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 167 10.2.1 METHOD FOR CASES WITHOUT ELECTRIC CURRENTS . . . . . . . . . . . . . . 167 10.2.2 METHODS FOR CASES WITH ELECTRIC CURRENTS . . . . . . . . . . . . . . . . 169 10.3 APPLICATIONS TO SIMPLE NANOSCALE SYSTEMS . . . . . . . . . . . . . . . . . . . . . 172 10.3.1 FIELD EMISSION FROM METAL SURFACES . . . . . . . . . . . . . . . . . . . . . . 172 10.3.2 ATOMIC WIRES BETWEEN METAL ELECTRODES . . . . . . . . . . . . . . . . . 174 10.4 APPROACHES TO NANOMOLECULAR SYSTEMS . . . . . . . . . . . . . . . . . . . . . . . . 177 10.4.1 EMPIRICAL APPROACHES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 177 10.4.2 SELF-CONSISTENT APPROACHES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 178 10.5 CONCLUDING R EMARKS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 179 ACKNOWLEDGMENTS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 180 R EFERENCES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 180 CONTENTS XIII 11 NANODEVICES FOR QUANTUM COMPUTING USING PHOTONS SHIGEKI TAKEUCHI ................................................ 183 11.1 QUANTUM COMMUNICATION AND QUANTUM INFORMATION PROCESSING . . 183 11.2 QUANTUM CRYPTOGRAPHY . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 184 11.2.1 THE MECHANISM OF QUANTUM CRYPTOGRAPHY . . . . . . . . . . . . . . . 184 11.2.2 DEVICES FOR QUANTUM CRYPTOGRAPHY . . . . . . . . . . . . . . . . . . . . . 187 11.3 QUANTUM COMPUTATION . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 187 11.3.1 THE MECHANISM OF QUANTUM COMPUTATION . . . . . . . . . . . . . . . . 187 11.3.2 TOWARDS THE R EALIZATION OF QUANTUM COMPUTERS . . . . . . . . . . 189 11.3.3 A HARD BOTTLENECK: DECOHERENCE . . . . . . . . . . . . . . . . . . . . . . . . 189 11.4 NANODEVICES FOR QUANTUM COMPUTING USING PHOTONS . . . . . . . . . . . . 190 11.4.1 SINGLE-PHOTON SOURCES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 190 11.4.2 PHOTONIC QUANTUM PHASE GATES . . . . . . . . . . . . . . . . . . . . . . . . . 191 11.5 CONCLUSION . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 192 ACKNOWLEDGMENTS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 192 R EFERENCES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 192 INDEX ......................................................... 195
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genre_facet	Aufsatzsammlung
id	DE-604.BV017323049
illustrated	Illustrated
indexdate	2024-07-09T19:16:37Z
institution	BVB
isbn	3540441352 3540402616
language	English
oai_aleph_id	oai:aleph.bib-bvb.de:BVB01-010441704
oclc_num	53038183
open_access_boolean
owner	DE-703 DE-91G DE-BY-TUM DE-384 DE-29T DE-634 DE-83 DE-11 DE-188
owner_facet	DE-703 DE-91G DE-BY-TUM DE-384 DE-29T DE-634 DE-83 DE-11 DE-188
physical	X, 557 S. Ill., graph. Darst.
publishDate	2004
publishDateSearch	2004
publishDateSort	2004
publisher	Springer
record_format	marc
series	Springer series in chemical physics
series2	Springer series in chemical physics Physics and astronomy online library
spelling	Basic principles in applied catalysis M. Baerns (ed.) Berlin [u.a.] Springer 2004 X, 557 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Springer series in chemical physics 75 Physics and astronomy online library Biokatalyse gtt Catalyse Físico-química larpcal Katalysatoren gtt Katalyse gtt Reactiekinetiek gtt Catalysis Katalyse (DE-588)4029921-1 gnd rswk-swf Katalysator (DE-588)4029919-3 gnd rswk-swf (DE-588)4143413-4 Aufsatzsammlung gnd-content Katalyse (DE-588)4029921-1 s DE-604 Katalysator (DE-588)4029919-3 s Baerns, Manfred 1934-2021 Sonstige (DE-588)106670425 oth Springer series in chemical physics 75 (DE-604)BV000000670 75 SWB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=010441704&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis
spellingShingle	Basic principles in applied catalysis Springer series in chemical physics Biokatalyse gtt Catalyse Físico-química larpcal Katalysatoren gtt Katalyse gtt Reactiekinetiek gtt Catalysis Katalyse (DE-588)4029921-1 gnd Katalysator (DE-588)4029919-3 gnd
subject_GND	(DE-588)4029921-1 (DE-588)4029919-3 (DE-588)4143413-4
title	Basic principles in applied catalysis
title_auth	Basic principles in applied catalysis
title_exact_search	Basic principles in applied catalysis
title_full	Basic principles in applied catalysis M. Baerns (ed.)
title_fullStr	Basic principles in applied catalysis M. Baerns (ed.)
title_full_unstemmed	Basic principles in applied catalysis M. Baerns (ed.)
title_short	Basic principles in applied catalysis
title_sort	basic principles in applied catalysis
topic	Biokatalyse gtt Catalyse Físico-química larpcal Katalysatoren gtt Katalyse gtt Reactiekinetiek gtt Catalysis Katalyse (DE-588)4029921-1 gnd Katalysator (DE-588)4029919-3 gnd
topic_facet	Biokatalyse Catalyse Físico-química Katalysatoren Katalyse Reactiekinetiek Catalysis Katalysator Aufsatzsammlung
url	http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=010441704&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA
volume_link	(DE-604)BV000000670
work_keys_str_mv	AT baernsmanfred basicprinciplesinappliedcatalysis

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