New concepts for enantioselective transition metal catalysts: chiral-AT-rhenium donor ligands as design elements
Gespeichert in:
| 1. Verfasser: | |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
2002
|
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | Erlangen-Nürnberg, Univ., Diss., 2003 |
| Beschreibung: | XXII, 183 S. graph. Darst. |
Internformat
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| 245 | 1 | 0 | |a New concepts for enantioselective transition metal catalysts |b chiral-AT-rhenium donor ligands as design elements |c von Klemenz Kromm |
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| 500 | |a Erlangen-Nürnberg, Univ., Diss., 2003 | ||
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Datensatz im Suchindex
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|---|---|
| adam_text |
TABLE
OF
CONTENTS
ZUSAMMENFASSUNG
VII
ABSTRACT
XI
LIST
OF
TABLES
XVII
LIST
OF
FIGURES
XVIII
LIST
OF
SCHEMES
XXI
1
GENERAL
INTRODUCTION
1
2
A
NEW
FAMILY
OF
CHELATING
DIPHOSPHINES
WITH
A
"CHIRAL-AT
RHENIUM"
LIGAND
BACKBONE
9
2.1
INTRODUCTION
9
2.2
RESULTS
13
2.2.1
FIRST
GENERATION
SYSTEMS:
"CHIRAL-AT-RHENIUM"
LIGANDS
13
2.2.2
SECOND
GENERATION
SYSTEMS:
"CHIRAL-AT-RHENIUM
AND
CARBON"
32
2.2.3
APPLICATIONS
TO
ENANTIOSELECTIVE
CATALYSIS
48
2.3
DISCUSSION
56
2.3.1
SYNTHESES
AND
ELECTRONIC
PROPERTIES
56
2.3.2
STRUCTURES
OF
17-20
59
2.3.3
EPIMERIZATION
OF
17
60
2.3.4
OTHER
REACTIONS
62
2.3.5
ENANTIOSELECTIVE
CATALYSIS
65
2.3.6
CONCLUSION
69
2.4
EXPERIMENTAL
SECTION
70
2.4.1
GENERAL
DATA
70
2.4.2
EXPERIMENTAL
PROCEDURES
71
3
SYNTHESES
AND
CHARACTERIZATION
OF
CHELATING
LIGANDS
CONTAI
NING
FOUR
"CHIRAL-AT-RHENIUM"
SPECTATOR
GROUPS
95
3.1
INTRODUCTION
95
3.2
RESULTS
101
3.2.1
LIGAND
SYNTHESES
101
3.2.2
CRYSTAL
STRUCTURE
OF
(5R
E
5R
E
SR
E
SRE)"59
110
3.2.3
CHELATE
FORMATION
112
XVI
3.3
DISCUSSION
114
3.3.1
SYNTHESES
AND
PROPERTIES
114
3.3.2
STEREOCHEMICAL
ANALYSIS
115
3.3.3
MOLECULAR
STRUCTURE
117
3.3.4
CHELATE
FORMATION
121
3.3.5
RELATED
LITERATURE
COMPOUNDS
123
3.3.6
RELEVANCE
TO
CATALYSIS
124
3.4
EXPERIMENTAL
SECTION
125
3.4.1
GENERAL
DATA
125
3.4.2
EXPERIMENTAL
PROCEDURES
126
4
CRYSTALLOGRAPHY
135
4.1
DATA
COLLECTION
AND
STRUCTURE
REFINEMENT
135
4.2
DATA
DEPOSITION
136
4.3
CIYSTALLOGRAPHIC
TABLES
137
5
REFERENCES
AND
NOTES
143
6
APPENDIX.
SYNTHESES
AND
CHARACTERIZATION
OF
PALLADACYCLES
CONTAINING
A
"CHIRAL-AT-RHENIUM"
LIGAND
BACKBONE
169
6.1
INTRODUCTION
169
6.2
RESULTS
171
6.3
EXPERIMENTAL
SECTION
179
6.3.1
GENERAL
DATA
179
6.3.2
EXPERIMENTAL
PROCEDURES
179 |
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| genre | (DE-588)4113937-9 Hochschulschrift gnd-content |
| genre_facet | Hochschulschrift |
| id | DE-604.BV017121982 |
| illustrated | Illustrated |
| indexdate | 2024-08-16T00:08:28Z |
| institution | BVB |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-010321987 |
| oclc_num | 643394554 |
| open_access_boolean | |
| owner | DE-29 DE-29T DE-12 DE-355 DE-BY-UBR |
| owner_facet | DE-29 DE-29T DE-12 DE-355 DE-BY-UBR |
| physical | XXII, 183 S. graph. Darst. |
| publishDate | 2002 |
| publishDateSearch | 2002 |
| publishDateSort | 2002 |
| record_format | marc |
| spelling | Kromm, Klemenz 1970- Verfasser (DE-588)124696007 aut New concepts for enantioselective transition metal catalysts chiral-AT-rhenium donor ligands as design elements von Klemenz Kromm 2002 XXII, 183 S. graph. Darst. txt rdacontent n rdamedia nc rdacarrier Erlangen-Nürnberg, Univ., Diss., 2003 Übergangsmetallverbindungen (DE-588)4061385-9 gnd rswk-swf Katalysator (DE-588)4029919-3 gnd rswk-swf Enantioselektivität (DE-588)4315368-9 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Katalysator (DE-588)4029919-3 s Übergangsmetallverbindungen (DE-588)4061385-9 s Enantioselektivität (DE-588)4315368-9 s DE-604 DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=010321987&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Kromm, Klemenz 1970- New concepts for enantioselective transition metal catalysts chiral-AT-rhenium donor ligands as design elements Übergangsmetallverbindungen (DE-588)4061385-9 gnd Katalysator (DE-588)4029919-3 gnd Enantioselektivität (DE-588)4315368-9 gnd |
| subject_GND | (DE-588)4061385-9 (DE-588)4029919-3 (DE-588)4315368-9 (DE-588)4113937-9 |
| title | New concepts for enantioselective transition metal catalysts chiral-AT-rhenium donor ligands as design elements |
| title_auth | New concepts for enantioselective transition metal catalysts chiral-AT-rhenium donor ligands as design elements |
| title_exact_search | New concepts for enantioselective transition metal catalysts chiral-AT-rhenium donor ligands as design elements |
| title_full | New concepts for enantioselective transition metal catalysts chiral-AT-rhenium donor ligands as design elements von Klemenz Kromm |
| title_fullStr | New concepts for enantioselective transition metal catalysts chiral-AT-rhenium donor ligands as design elements von Klemenz Kromm |
| title_full_unstemmed | New concepts for enantioselective transition metal catalysts chiral-AT-rhenium donor ligands as design elements von Klemenz Kromm |
| title_short | New concepts for enantioselective transition metal catalysts |
| title_sort | new concepts for enantioselective transition metal catalysts chiral at rhenium donor ligands as design elements |
| title_sub | chiral-AT-rhenium donor ligands as design elements |
| topic | Übergangsmetallverbindungen (DE-588)4061385-9 gnd Katalysator (DE-588)4029919-3 gnd Enantioselektivität (DE-588)4315368-9 gnd |
| topic_facet | Übergangsmetallverbindungen Katalysator Enantioselektivität Hochschulschrift |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=010321987&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT krommklemenz newconceptsforenantioselectivetransitionmetalcatalystschiralatrheniumdonorligandsasdesignelements |