Electronic defect states in alkali halides: effects of interaction with molecular ions
Gespeichert in:
| 1. Verfasser: | |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Berlin [u.a.]
Springer
2003
|
| Schriftenreihe: | Springer tracts in modern physics
185 |
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | Includes bibliographical references and index. |
| Beschreibung: | XII, 196 S. graph. Darst. |
| ISBN: | 3540004718 |
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| 245 | 1 | 0 | |a Electronic defect states in alkali halides |b effects of interaction with molecular ions |c Volkmar Dierolf |
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| 300 | |a XII, 196 S. |b graph. Darst. | ||
| 336 | |b txt |2 rdacontent | ||
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| 490 | 1 | |a Springer tracts in modern physics |v 185 | |
| 500 | |a Includes bibliographical references and index. | ||
| 650 | 7 | |a Física moderna |2 larpcal | |
| 650 | 4 | |a Alkali metal halides | |
| 650 | 4 | |a Crystals |x Defects | |
| 650 | 4 | |a Energy-band theory of solids | |
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| 650 | 0 | 7 | |a Molekülion |0 (DE-588)4039973-4 |2 gnd |9 rswk-swf |
| 650 | 0 | 7 | |a Gitterbaufehler |0 (DE-588)4125030-8 |2 gnd |9 rswk-swf |
| 650 | 0 | 7 | |a Wechselwirkung |0 (DE-588)4064937-4 |2 gnd |9 rswk-swf |
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Datensatz im Suchindex
| _version_ | 1804129902897659904 |
|---|---|
| adam_text | VOLKMA
R DIEROL
F
ELECTRONIC
DEFECT STATES
IN ALKALI HALIDES
EFFECTS OF INTERACTION WITH MOLECULAR IONS
WITH 80 FIGURES AN
D 22 TABLES
T
U DARMSTADT
TEILBIBLIOTHEK CHEMIE/
MATERIALWISSENSCHAFT
SPRINGER
CONTENT
S
INTRODUCTIO
N AND HISTORICA
L OVERVIE
W
1
1.1 THE INITIAL IDEA 1
1.2 THE UNEXPECTED NEW RESULTS 2
1.3 THE DREAM COMES TRUE 4
1.4 WHAT TO EXPECT? 4
REFERENCES
7
F CENTER
S AND RARE-EART
H IO
N DEFECT
S
IN ALKALI HALIDE
S
9
2.1 F-CENTER-RELATED DEFECTS 9
2.2 DIVALENT RARE-EARTH IONS IN ALKALI HALIDES 11
2.2.1 ISOLATED YB
2
+
IONS 11
2.2.2 ISOLATED EU
2
+
IONS 15
2.2.3 ISOLATED SM
2
+
IONS 16
REFERENCES 20
PROPERTIE
S OF MOLECULA
R DEFECT
S
23
3.1 TRANSITION ENERGIES 23
3.1.1 FREE MOLECULES 23
3.1.2 TRANSITION ENERGIES OF MOLECULAR IONS IN A SOLID 24
3.2 ABSORPTION INTENSITY AND OSCILLATOR STRENGTHS 26
3.2.1 FREE MOLECULE 26
3.2.2 TRANSITION PROBABILITIES FOR MOLECULAR IONS IN A SOLID.
. 28
3.3 MOLECULES IN ALKALI HALIDES 30
REFERENCES 31
THEORETICA
L MODEL
S FOR E-
V TRANSFER
33
4.1 COMMON FEATURES 33
4.2 FORSTER-DEXTER-TYPE MODELS 36
4.3 MODELS FOR ELECTRONIC-VIBRATIONAL COUPLING 38
4.3.1 RADIATIVE TRANSITIONS
INCLUDING ELECTRONIC-VIBRATIONAL COUPLING 39
4.3.2 SUPERMOLECULE MODEL (HORIZONTAL TUNNELING) 42
4.3.3 THE SUDDEN APPROXIMATION 43
X CONTENTS
4.4 COMPARISON 45
4.5 POTENTIAL ENERGY SURFACES 47
REFERENCES 48
5
FH(CN~
)
CENTER
S
51
5.1 BASIC SPECTROSCOPIC PROPERTIES 51
5.1.1 OVERVIEW 51
5.1.2 ELECTRONIC TRANSITIONS 52
5.1.3 VIBRATIONAL TRANSITIONS 53
5.2 ENERGY TRANSFER: RELATIVE AND ABSOLUTE E-
V TRANSFER RATES . 54
5.2.1 E-
V TRANSFER EFFICIENCY IN KC1 55
5.2.2 E-
V TRANSFER IN CSCL:
TIME-DEPENDENT MEASUREMENT OF TH
E EL AND VL 57
5.3 V-
E ENERGY TRANSFER 60
5.4 VIBRATIONAL COUPLING OF F CENTERS T
O TH
E CN~ STRETCHMODE . 61
5.4.1 KC1 61
5.4.2 CSCL AND CSBR 63
5.5 THE NATUR
E OF TH
E RELAXED EXCITED STAT
E 65
5.6 PUTTIN
G IT ALL TOGETHER:
COMPARING E-
V TRANSFER RATES WITH THEORETICAL MODELS ...
. 66
5.6.1 FD MODEL 67
5.6.2 HORIZONTAL-TUNNELING MODEL 67
5.6.3 RELATIVE TRANSFER RATES 68
REFERENCES 69
6 CN
~ NEX
T T
O A
N ANIO
N VACANC
Y
OCCUPIE
D B
Y N
O ELECTRO
N OR TW
O ELECTRON
S
71
6.1 BACKGROUND 71
6.2 EXPERIMENTAL RESULTS 72
6.3 CREATION KINETICS 74
6.4 SHIFT IN SPECTRAL POSITION 75
6.5 CHANGES IN ABSORPTION CROSS SECTION 76
REFERENCES 76
7 F
H
(OH-
)
CENTER
S
77
7.1 CS HALIDES 77
7.1.1 ELECTRONIC ABSORPTION 77
7.1.2 MAGNETIC RESONANCE 80
7.1.3 VIBRATIONAL PROPERTIES 81
7.1.4 THE RELAXED EXCITED STAT
E 81
7.2
FH
2
CENTER 81
7.3 K AND RB HALIDES: OPTICAL BISTABILITY 82
7.3.1 ELECTRONIC ABSORPTION 82
7.3.2 VIBRATIONAL ABSORPTION 84
7.3.3 MICROSCOPIC STRUCTURE 86
CONTENTS XI
7.3.4 ENTROPY-DRIVEN BISTABILITY: TWO-CENTER MODEL 88
7.3.5 THREE-CENTER-TYPE MODEL 88
7.3.6 CHANGES IN VIBRATIONAL ABSORPTION CROSS-SECTION 90
7.4 E-V ENERGY TRANSFER 91
7.5 DYNAMIC PROPERTIES 91
REFERENCES 93
8 INTERACTION BETWEE
N F ELECTRON
S
AND DISTAN
T OH
MOLECULE
S
95
8.1 THE MAIN IDEA 95
8.2 OH~ DEFECTS WITH A CAPTURED EXTR
A ELECTRON 97
8.2.1 ABSORPTION RESULTS 97
8.2.2 OPTICALLY DETECTED MAGNETIC RESONANCE 100
8.3 VIBRATIONAL PROPERTIES OF MOLECULAR ELECTRON TRAPS 101
8.3.1 SHIFT IN TRANSITION ENERGY
AND ENHANCEMENT OF ABSORPTION INTENSITY 101
8.3.2 MECHANICAL AND ELECTRICAL ANHARMONICITY 104
8.3.3 LIBRATIONAL SIDEBANDS 104
8.3.4 SUMMARY 105
8.4 ELECTRON TRAPPING BY OH~ PAIRS 105
8.5 ELECTRON TUNNELING FROM F CENTERS
TO OH~-RELATED DEFECTS 107
8.6 E-V TRANSFER BETWEEN DISTANT F-CENTERS AND OH~DEFECTS ..
. 108
8.7 CONCLUSIONS AND OUTLOOK 110
8.8 FURTHER OH~-TYPE CENTERS IN CSL IL
L
REFERENCES 112
9 YTTERBIU
M IONS AN
D CN
~ MOLECULE
S
115
9.1 CRYSTAL GROWTH AND SAMPLE CHARACTERIZATION 115
9.2 YB
2+
:(CN~)
N
DEFECT COMPLEXES: ELECTRONIC TRANSITIONS 116
9.2.1 ABSORPTION AND EMISSION PROPERTIES 117
9.3 VIBRATIONAL TRANSITIONS OF CN~ MOLECULES
WITHIN YB
2
+:(CN-)
N
COMPLEXES 122
9.3.1 TEMPERATURE DEPENDENCE 123
9.4 OPTICALLY INDUCED BISTABILITY . ! 128
9.5 CENTER MODEL 130
9.6 INTERPRETATION OF THE SPECTRAL SHIFTS 132
9.6.1 LIGAND FELD STRENGTH 132
9.7 VIBRATIONAL LUMINESCENCE AND E-
V ENERGY TRANSFER 138
9.7.1 TYPE OF CENTER INVOLVED IN THE E-V ENERGY TRANSFER. . 141
9.8 DYNAMICS OF THE E-
V TRANSFER 142
9.8.1 TEMPERATURE DEPENDENCE 147
9.8.2 CONCENTRATION VARIATION 149
9.9 PROPERTIES OF YB
2
+
IONS WITH EXCITED CN~ NEIGHBORS 152
9.9.1 EXPERIMENTAL RESULTS AND THEIR INTERPRETATION 153
XII CONTENTS
9.9.2 ORIGIN OF ENHANCEMENT
OF ELECTRONIC TRANSITION PROBABILITY 155
9.10 PUTTIN
G IT ALL TOGETHER:
COMPARING E-V TRANSFER RATES WITH THEORETICAL MODELS ...
. 156
9.10.1 THE FORSTER-DEXTER MODEL
AND THE RELATIVE TRANSFER RATES 157
9.10.2 FD MODEL: ABSOLUTE TRANSFER RATES 158
9.10.3 HORIZONTAL-TUNNELING MODEL: RELATIVE TRANSFER RATES . 158
9.10.4 HORIZONTAL-TUNNELING MODEL: ABSOLUTE TRANSFER RATES . 159
9.11 POSSIBLE APPLICATION AS A PHOSPHOR 159
REFERENCES 162
10 EUROPIUM AND CN
~ MOLECULE
S
165
10.1 EU
2+
:(CN-)
N
COMPLEXES 165
10.2 POSSIBLE APPLICATION AS A PHOSPHOR 168
10.3 SUMMARY AND INTERPRETATION OF EXPERIMENTAL RESULTS 168
REFERENCES 169
11 SAMARIUM AND CN
~ MOLECULE
S
171
11.1 INTRODUCTION 171
11.2 COMPLEXES INVOLVING A SINGLE CN~ MOLECULE 172
11.2.1 SPECTROSCOPIC CHARACTERIZATION 172
11.2.2 PRELIMINARY CENTER MODEL 175
11.2.3 ENERGY-LEVEL SCHEME 176
11.3 COMPLEXES INVOLVING SEVERAL CN~ MOLECULES 176
11.3.1 ENERGY-LEVEL SCHEME 177
11.4 E-
V ENERGY TRANSFER 177
11.4.1 VIBRATIONAL LUMINESCENCE 178
11.4.2 INTERPRETATION 179
11.4.3 SUMMARY AND OUTLOOK 181
REFERENCES 181
12 OTHER DEFEC
T COMPLEXE
S
183
12.1 NS
2
IONS (T1+ AND PB
2+
) AND CN~ MOLECULES 183
12.2 CU+ IONS AND OH
MOLECULES 185
REFERENCES 185
13 SUMMARY
187
13.1 COMPARISON OF THE DEFECT SYSTEMS 187
13.2 POTENTIAL APPLICATIONS 190
REFERENCE 191
INDE
X
193
|
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| id | DE-604.BV016992670 |
| illustrated | Illustrated |
| indexdate | 2024-07-09T19:12:31Z |
| institution | BVB |
| isbn | 3540004718 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-010258098 |
| oclc_num | 51818743 |
| open_access_boolean | |
| owner | DE-29T DE-91G DE-BY-TUM DE-19 DE-BY-UBM DE-703 DE-11 DE-188 |
| owner_facet | DE-29T DE-91G DE-BY-TUM DE-19 DE-BY-UBM DE-703 DE-11 DE-188 |
| physical | XII, 196 S. graph. Darst. |
| publishDate | 2003 |
| publishDateSearch | 2003 |
| publishDateSort | 2003 |
| publisher | Springer |
| record_format | marc |
| series | Springer tracts in modern physics |
| series2 | Springer tracts in modern physics |
| spelling | Dierolf, Volkmar Verfasser aut Electronic defect states in alkali halides effects of interaction with molecular ions Volkmar Dierolf Berlin [u.a.] Springer 2003 XII, 196 S. graph. Darst. txt rdacontent n rdamedia nc rdacarrier Springer tracts in modern physics 185 Includes bibliographical references and index. Física moderna larpcal Alkali metal halides Crystals Defects Energy-band theory of solids Alkalihalogenide (DE-588)4226772-9 gnd rswk-swf Elektronenzustand (DE-588)4263453-2 gnd rswk-swf Molekülion (DE-588)4039973-4 gnd rswk-swf Gitterbaufehler (DE-588)4125030-8 gnd rswk-swf Wechselwirkung (DE-588)4064937-4 gnd rswk-swf Alkalihalogenide (DE-588)4226772-9 s Gitterbaufehler (DE-588)4125030-8 s Elektronenzustand (DE-588)4263453-2 s Molekülion (DE-588)4039973-4 s Wechselwirkung (DE-588)4064937-4 s DE-604 Springer tracts in modern physics 185 (DE-604)BV000000153 185 DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=010258098&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Dierolf, Volkmar Electronic defect states in alkali halides effects of interaction with molecular ions Springer tracts in modern physics Física moderna larpcal Alkali metal halides Crystals Defects Energy-band theory of solids Alkalihalogenide (DE-588)4226772-9 gnd Elektronenzustand (DE-588)4263453-2 gnd Molekülion (DE-588)4039973-4 gnd Gitterbaufehler (DE-588)4125030-8 gnd Wechselwirkung (DE-588)4064937-4 gnd |
| subject_GND | (DE-588)4226772-9 (DE-588)4263453-2 (DE-588)4039973-4 (DE-588)4125030-8 (DE-588)4064937-4 |
| title | Electronic defect states in alkali halides effects of interaction with molecular ions |
| title_auth | Electronic defect states in alkali halides effects of interaction with molecular ions |
| title_exact_search | Electronic defect states in alkali halides effects of interaction with molecular ions |
| title_full | Electronic defect states in alkali halides effects of interaction with molecular ions Volkmar Dierolf |
| title_fullStr | Electronic defect states in alkali halides effects of interaction with molecular ions Volkmar Dierolf |
| title_full_unstemmed | Electronic defect states in alkali halides effects of interaction with molecular ions Volkmar Dierolf |
| title_short | Electronic defect states in alkali halides |
| title_sort | electronic defect states in alkali halides effects of interaction with molecular ions |
| title_sub | effects of interaction with molecular ions |
| topic | Física moderna larpcal Alkali metal halides Crystals Defects Energy-band theory of solids Alkalihalogenide (DE-588)4226772-9 gnd Elektronenzustand (DE-588)4263453-2 gnd Molekülion (DE-588)4039973-4 gnd Gitterbaufehler (DE-588)4125030-8 gnd Wechselwirkung (DE-588)4064937-4 gnd |
| topic_facet | Física moderna Alkali metal halides Crystals Defects Energy-band theory of solids Alkalihalogenide Elektronenzustand Molekülion Gitterbaufehler Wechselwirkung |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=010258098&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| volume_link | (DE-604)BV000000153 |
| work_keys_str_mv | AT dierolfvolkmar electronicdefectstatesinalkalihalideseffectsofinteractionwithmolecularions |