Verfügbarkeit: Quantum phenomena in clusters and nanostructures

Quantum phenomena in clusters and nanostructures: with ... 8 tables

Gespeichert in:

Bibliographische Detailangaben
Format:	Buch
Sprache:	English
Veröffentlicht:	Berlin [u.a.] 2003
Schriftenreihe:	Springer series in cluster physics Physics and astronomy online library
Schlagworte:	Cluster Nanostruktur Quantenphysik Quanteneffekt Clusterphysik
Online-Zugang:	Inhaltsverzeichnis
Beschreibung:	XII, 265 S. Ill., graph. Darst.
ISBN:	3540000151

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Datensatz im Suchindex

_version_	1804129575106510848
adam_text	CONTENTS 1 CLUSTER AND NANOSCALE SCIENCE: OVERVIEW AND PERSPECTIVE A.W. CASTLEMAN, JR., S.N. KHANNA ................................ 1 1.1 INTRODUCTION . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 1 1.2 CLUSTER TYPES: FORMATION AND STUDY . . . . . . . . . . . . . . . . . . . . . . . . . . 2 1.3 THEORETICAL DEVELOPMENTS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 3 1.4 THEME OF THE BOOK . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 3 2 QUANTUM AND CLASSICAL SIZE EFFECTS IN THERMODYNAMIC PROPERTIES R.S. BERRY ..................................................... 7 2.1 INTRODUCTION . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 7 2.2 QUANTUM PROPERTIES OF SMALL SYSTEMS . . . . . . . . . . . . . . . . . . . . . . . . 10 2.3 PHASES OF FINITE SYSTEMS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 12 2.4 PHASE DIAGRAMS OF FINITE SYSTEMS . . . . . . . . . . . . . . . . . . . . . . . . . . . . 19 2.5 CONCLUSION . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 26 REFERENCES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 26 3PHOTOELECTRON SPECTROSCOPY G. GANTEF¨ OR .................................................... 29 3 .1 INTRODUCTION . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 29 3 .2 PHYSICS OF PHOTOELECTRON SPECTROSCOPY . . . . . . . . . . . . . . . . . . . . . . . . 3 1 3 .3 EXPERIMENTAL SET UP . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 3 6 3 .3 .1 CLUSTER SOURCE . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 3 7 3.3.2 TIME-OF-FLIGHT MASS SPECTROMETER . . . . . . . . . . . . . . . . . . . . . . 3 7 3 .3 .3 LASER . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 3 7 3 .3 .4 PHOTOELECTRON SPECTROMETER . . . . . . . . . . . . . . . . . . . . . . . . . . . 3 8 3 .4 RESULTS. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 3 9 3.4.1 EXAMPLE: ELECTRONIC SHELLS IN CLUSTERS OF SIMPLE METALS . . . 39 3 .4.2 EXAMPLE: THE SIZE DEPENDENCE OF THE BAND GAP . . . . . . . . . 42 3 .4.3 EXAMPLE: CHEMICAL REACTIVITY AND ELECTRONIC STRUCTURE. . . . . 45 3 .4.4 EXAMPLE: DYNAMICS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 48 3 .5 CONCLUSION AND OUTLOOK . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 51 VIII CONTENTS 4 QUANTUM TUNNELING OF THE MAGNETIZATION IN MOLECULAR NANOCLUSTERS R. SESSOLI, D. GATTESCHI, W. WERNSDORFER ........................... 55 4.1 INTRODUCTION . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 55 4.2 THE MAGNETIC ANISOTROPY OF MOLECULAR CLUSTERS . . . . . . . . . . . . . . . . 57 4.3 THE SUPERPARAMAGNETIC BEHAVIOR. . . . . . . . . . . . . . . . . . . . . . . . . . . . . 61 4.4 LONGITUDINAL FIELD DEPENDENCE OF THE RELAXATION RATE: THE STEPPED HYSTERESIS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 63 4.5 TRANSVERSE FIELD DEPENDENCE OF THE RELAXATION RATE: THE BERRY PHASE . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 65 4.6 THE ROLE OF DIPOLAR FIELDS: THE NON-EXPONENTIAL RELAXATION . . . . 69 4.7 THE ROLE OF THE NUCLEAR MAGNETIC MOMENTS: THE ISOTOPE EFFECT . . 74 4.8 CONCLUSIONS. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 78 REFERENCES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 79 5 MAGNETISM OF FREE AND SUPPORTED METAL CLUSTERS J.P. BUCHER .................................................... 83 5.1 INTRODUCTION . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 84 5.2 SIMPLE CONSIDERATIONS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 86 5.2.1 COMMON IDEAS ON MAGNETISM . . . . . . . . . . . . . . . . . . . . . . . . . . 86 5.2.2 IMPLICATIONS FOR CLUSTER MAGNETISM . . . . . . . . . . . . . . . . . . . . . 87 5.3 THE STERN-GERLACH EXPERIMENTS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 89 5.3 .1 EXPERIMENTAL PRINCIPLES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 89 5.3.2 MAGNETIC MOMENT MEASUREMENTS OF UNSUPPORTED CLUSTERS . 91 5.3 .3 A HIGH RESOLUTION EXPERIMENT: NICKEL . . . . . . . . . . . . . . . . . . 92 5.3 .4 TEMPERATURE DEPENDENCE OF THE GIANT MOMENTS. . . . . . . . . . 93 5.3 .5 CLUSTERS OF NON-FERROMAGNETIC TRANSITION METALS . . . . . . . . . 96 5.3 .6 LOCKED MOMENT CLUSTERS AND SPIN CANTING . . . . . . . . . . . . . . 97 5.4 INTERPRETATION OF THE BEAM EXPERIMENTS . . . . . . . . . . . . . . . . . . . . . . . 99 5.4.1 MAGNETIC ANISOTROPY . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 100 5.4.2 COUPLING BETWEEN MAGNETIC MOMENT AND LATTICE: DEFLECTION PROFILE . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 100 5.5 GROWTH KINETICS OF CLUSTERS ON SURFACES . . . . . . . . . . . . . . . . . . . . . . . 102 5.5.1 TUNING THE CLUSTERS DENSITY . . . . . . . . . . . . . . . . . . . . . . . . . . . 102 5.5.2 ISLAND SHAPES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 104 5.6 THERMODYNAMIC GROWTH MODES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 106 5.6.1 GROWTH CRITERIA . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 106 5.6.2 ELASTIC AND STRUCTURAL CONSIDERATIONS . . . . . . . . . . . . . . . . . . . 107 5.7 ORGANIZED GROWTH . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 108 5.7.1 INCOMMENSURATE MODULATED LAYERS . . . . . . . . . . . . . . . . . . . . . 108 5.7.2 ATOMIC SCALE TEMPLATE . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 110 5.7.3 SELF ORGANIZATION . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 112 5.7.4 PERIODIC PATTERNING BY STRESS RELAXATION . . . . . . . . . . . . . . . . 113 CONTENTS IX 5.7.5 ORGANIZATION ON VICINAL SURFACES . . . . . . . . . . . . . . . . . . . . . . . 115 5.7.6 LOW TEMPERATURE GROWTH . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 115 5.8 MAGNETIC PROPERTIES OF NANOSTRUCTURES . . . . . . . . . . . . . . . . . . . . . . . . 116 5.8.1 ISOLATED CLUSTERS ON SURFACES . . . . . . . . . . . . . . . . . . . . . . . . . . . 117 5.8.2 INTERACTING ISLANDS AND CHAINS . . . . . . . . . . . . . . . . . . . . . . . . . 120 5.8.3 THE TWO-DIMENSIONAL LIMIT . . . . . . . . . . . . . . . . . . . . . . . . . . . 125 5.9 CONCLUSION AND OUTLOOK . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 13 0 REFERENCES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 13 2 6 MAGNETISM IN FREE CLUSTERS AND IN MN 12 O 12 -ACETATE NANOMAGNETS S.N. KHANNA, C. ASHMAN, M.R. PEDERSON, J. KORTUS ................ 139 6.1 INTRODUCTION . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 13 9 6.2 MAGNETIC MOMENT OF FREE CLUSTERS IN BEAMS . . . . . . . . . . . . . . . . . . . 140 6.3OSCILLATORY CHANGE IN THE MAGNETIC MOMENT OF NI N CLUSTERS UPON H ADSORPTION . . . . . . . . . . . . . . . . . . . . . . . . . . . 143 6.4 QUANTUM TUNNELING AND ATOMIC, ELECTRONIC AND MAGNETIC STRUCTURE OF MN 12 O 12 -ACETATE . . . . . . . . . . . . . . . . . . . 146 6.5 DETAILS OF THEORETICAL STUDIES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 149 6.6 GEOMETRY AND ELECTRONIC STRUCTURE OF ISOLATED MN 12 O 12 CLUSTERS . 150 6.6.1 VIBRATIONAL FREQUENCIES OF THE HEXAGONAL TOWER . . . . . . . . . . 151 6.7 ELECTRONIC STRUCTURE OF MN 12 O 12 -ACETATE . . . . . . . . . . . . . . . . . . . . . . 152 6.8 MAGNETIC ANISOTROPY ENERGY . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 154 6.9 CONCLUSIONS AND EXTENSION TO FE 8 NANOMAGNETS . . . . . . . . . . . . . . . . 156 REFERENCES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 157 7 SIZE EFFECTS IN CATALYSIS BY SUPPORTED METAL CLUSTERS A.A. KOLMAKOV, D.W. GOODMAN .................................. 159 7.1 INTRODUCTION . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 159 7.2 METHODOLOGY. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 160 7.2.1 THIN OXIDE FILMS AS A MODEL SUPPORT . . . . . . . . . . . . . . . . . . 160 7.2.2 CLUSTER DEPOSITION: DENSITY, SIZE AND CONTROL OF MORPHOLOGY . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 161 7.2.3 ANALYTICAL TOOLS: SPECTROSCOPY AND MICROSCOPY. . . . . . . . . . . 164 7.3 CLUSTER SIZE AND REACTIVITY . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 170 7.3 .1 GEOMETRIC FACTORS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 170 7.3 .2 ELECTRONIC FACTORS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 174 7.4 EXAMPLES OF SIZE EFFECTS IN CLUSTER REACTIVITY . . . . . . . . . . . . . . . . . . 181 7.4.1 ONSET OF THE REACTIVITY OF AU/TIO 2 WITH METAL-NONMETAL TRANSITIONS AND THE DIMENSIONALITY OF SUPPORTED CLUSTERS . . . . . . . . . . . . 181 7.4.2 CO DISSOCIATION ON STRUCTURAL DEFECTS OF RH/AL 2 O 3 /NIAL (110) . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 186 7.4.3CO OXIDATION OVER A PT/MGO MONODISPERSED CATALYST . . . 189 X CONTENTS 7.5 CONCLUDING REMARKS AND FUTURE PROSPECTS . . . . . . . . . . . . . . . . . . . . 192 REFERENCES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 193 8 DELAYED IONIZATION E.E.B. CAMPBELL, R.D. LEVINE .................................... 199 8.1 INTRODUCTION . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 199 8.2 TRANSITION STATE THEORY . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 200 8.3 DETAILED BALANCE . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 203 8.4 EXPERIMENTAL: THE RATE OF THERMIONIC EMISSION . . . . . . . . . . . . . . . 210 8.5 EXPERIMENTAL: DYNAMICS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 213 8.6 KINETIC MODEL . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 217 8.7 CONCLUDING REMARKS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 219 9 CLUSTER DYNAMICS: INFLUENCES OF SOLVATION AND AGGREGATION Q. ZHONG, A.W. CASTLEMAN, JR. ................................... 223 9.1 INTRODUCTION . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 223 9.2 CHARGE-TRANSFER REACTIONS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 224 9.2.1 PHOTO-INDUCED ELECTRON-TRANSFER REACTIONS . . . . . . . . . . . . . . 224 9.2.2 EXCITED-STATE PROTON-TRANSFER . . . . . . . . . . . . . . . . . . . . . . . . . 226 9.2.3 EXCITED-STATE DOUBLE PROTON-TRANSFER . . . . . . . . . . . . . . . . . . . 229 9.3 CAGING DYNAMICS. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 231 9.3 .1 CAGING DYNAMICS IN NEUTRAL CLUSTERS . . . . . . . . . . . . . . . . . . . 23 2 9.3 .2 CAGING DYNAMICS IN ANIONIC CLUSTERS . . . . . . . . . . . . . . . . . . . 23 4 9.4 COULOMB EXPLOSION PROCESS IN CLUSTERS . . . . . . . . . . . . . . . . . . . . . . . 23 8 9.4.1 ROLE OF CLUSTERS IN THE COULOMB EXPLOSION PROCESS . . . . . . . 23 8 9.4.2 MODELING OF COULOMB EXPLOSION PROCESS . . . . . . . . . . . . . . . . . 240 9.4.3 COULOMB EXPLOSION IMAGING . . . . . . . . . . . . . . . . . . . . . . . . . . . 243 9.5 ELECTRONIC EXCITATION, RELAXATION AND IONIZATION OF MET-CARS . . . . 245 9.5.1 MET-CARS: A UNIQUE MOLECULAR CLUSTER SYSTEM . . . . . . . . . . . 246 9.5.2 DELAYED IONIZATION . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 246 9.5.3 ULTRAFAST SPECTROSCOPY . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 248 9.6 CONCLUSION . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 251 REFERENCES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 252 10 FUTURE DIRECTIONS A.W. CASTLEMAN, JR., S.N. KHANNA ................................ 259 INDEX ......................................................... 263
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id	DE-604.BV014799324
illustrated	Illustrated
indexdate	2024-07-09T19:07:19Z
institution	BVB
isbn	3540000151
language	English
oai_aleph_id	oai:aleph.bib-bvb.de:BVB01-010015298
oclc_num	249221816
open_access_boolean
owner	DE-703 DE-355 DE-BY-UBR DE-11
owner_facet	DE-703 DE-355 DE-BY-UBR DE-11
physical	XII, 265 S. Ill., graph. Darst.
publishDate	2003
publishDateSearch	2003
publishDateSort	2003
record_format	marc
series2	Springer series in cluster physics Physics and astronomy online library
spelling	Quantum phenomena in clusters and nanostructures with ... 8 tables S. N. Khanna ; A. W. Castleman Berlin [u.a.] 2003 XII, 265 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Springer series in cluster physics Physics and astronomy online library Cluster (DE-588)4010318-3 gnd rswk-swf Nanostruktur (DE-588)4204530-7 gnd rswk-swf Quantenphysik (DE-588)4266670-3 gnd rswk-swf Quanteneffekt (DE-588)4356922-5 gnd rswk-swf Clusterphysik (DE-588)4616587-3 gnd rswk-swf Clusterphysik (DE-588)4616587-3 s Quanteneffekt (DE-588)4356922-5 s DE-604 Nanostruktur (DE-588)4204530-7 s Cluster (DE-588)4010318-3 s Quantenphysik (DE-588)4266670-3 s Khanna, Shiv N. Sonstige oth Castleman, Albert W. 1936- Sonstige (DE-588)14345997X oth SWB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=010015298&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis
spellingShingle	Quantum phenomena in clusters and nanostructures with ... 8 tables Cluster (DE-588)4010318-3 gnd Nanostruktur (DE-588)4204530-7 gnd Quantenphysik (DE-588)4266670-3 gnd Quanteneffekt (DE-588)4356922-5 gnd Clusterphysik (DE-588)4616587-3 gnd
subject_GND	(DE-588)4010318-3 (DE-588)4204530-7 (DE-588)4266670-3 (DE-588)4356922-5 (DE-588)4616587-3
title	Quantum phenomena in clusters and nanostructures with ... 8 tables
title_auth	Quantum phenomena in clusters and nanostructures with ... 8 tables
title_exact_search	Quantum phenomena in clusters and nanostructures with ... 8 tables
title_full	Quantum phenomena in clusters and nanostructures with ... 8 tables S. N. Khanna ; A. W. Castleman
title_fullStr	Quantum phenomena in clusters and nanostructures with ... 8 tables S. N. Khanna ; A. W. Castleman
title_full_unstemmed	Quantum phenomena in clusters and nanostructures with ... 8 tables S. N. Khanna ; A. W. Castleman
title_short	Quantum phenomena in clusters and nanostructures
title_sort	quantum phenomena in clusters and nanostructures with 8 tables
title_sub	with ... 8 tables
topic	Cluster (DE-588)4010318-3 gnd Nanostruktur (DE-588)4204530-7 gnd Quantenphysik (DE-588)4266670-3 gnd Quanteneffekt (DE-588)4356922-5 gnd Clusterphysik (DE-588)4616587-3 gnd
topic_facet	Cluster Nanostruktur Quantenphysik Quanteneffekt Clusterphysik
url	http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=010015298&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA
work_keys_str_mv	AT khannashivn quantumphenomenainclustersandnanostructureswith8tables AT castlemanalbertw quantumphenomenainclustersandnanostructureswith8tables

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