Verfügbarkeit: Selective spectroscopy of single molecules

Selective spectroscopy of single molecules:

Gespeichert in:

Bibliographische Detailangaben
1. Verfasser:	Osad'ko, Igor' S. (VerfasserIn)
Format:	Buch
Sprache:	English Russian
Veröffentlicht:	Berlin [u.a.] Springer 2003
Schriftenreihe:	Springer series in chemical physics 69
Schlagworte:	Físico-química Molecular spectroscopy Tunneling (Physics) Einzelmolekülspektroskopie
Online-Zugang:	Inhaltsverzeichnis
Beschreibung:	XII, 382 S. graph. Darst.
ISBN:	3540441018

Internformat

MARC


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Datensatz im Suchindex

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adam_text	CONTENTS INTRODUCTION .................................................. 1 PART I. SINGLE ATOM IN TRANSVERSE ELECTROMAGNETIC FIELD 1. QUANTUM PRINCIPLES OF TWO-LEVEL ATOMIC SPECTROSCOPY ... 7 1.1 HAMILTONIAN OF AN ELECTRONPHOTON SYSTEM . . . . . . . . . . . . . . . . 7 1.2 TRANSVERSE ELECTROMAGNETIC FIELD AS A PHOTON GAS . . . . . . . . . . 9 1.3 ELECTRONPHOTON INTERACTION. RABI FREQUENCY . . . . . . . . . . . . . . 13 1.4 EQUATIONS FOR TRANSITION AMPLITUDES . . . . . . . . . . . . . . . . . . . . . . 16 1.5 DENSITY MATRIX OF THE SYSTEM. RELATION TO TRANSITION AMPLITUDES . . . . . . . . . . . . . . . . . . . . . . . . 18 2. TWO-PHOTON STARTSTOP CORRELATOR ....................... 21 2.1 PHOTON COUNTING IN THE STARTSTOP REGIME . . . . . . . . . . . . . . . . 21 2.2 SPONTANEOUS FLUORESCENCE. TEMPORAL EVOLUTION OF FLUORESCENCE LINE SHAPE . . . . . . . . . . . . 22 2.3 OPTICAL ABSORPTION LINE. EQUATIONS FOR TRANSITION AMPLITUDES . . . . . . . . . . . . . . . . . . . . . . 27 2.4 TEMPORAL EVOLUTION OF PROBABILITIES. . . . . . . . . . . . . . . . . . . . . . . 30 2.5 TEMPORAL EVOLUTION OF ABSORPTION LINE SHAPE . . . . . . . . . . . . . 33 2.6 TWO-PHOTON STARTSTOP CORRELATOR . . . . . . . . . . . . . . . . . . . . . . . 35 3. FULL TWO-PHOTON CORRELATOR .............................. 39 3.1 COUNTING ALL PHOTON PAIRS. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 39 3.2 INFINITE SET OF EQUATIONS FOR TRANSITION AMPLITUDES. DISCUSSION OF MAIN APPROXIMATIONS . . . . . . . . . . . . . . . . . . . . . . . 40 3.3 EQUATIONS GOVERNING THE FULL TWO-PHOTON CORRELATOR . . . . . . . 43 3.4 RELATING THE FULL AND STARTSTOP TWO-PHOTON CORRELATORS . . . . . . . . . . . . . . . . . . . 46 3.5 FREQUENCY AND TIME DEPENDENCE OF FULL AND STARTSTOP TWO-PHOTON CORRELATORS . . . . . . . . . . . . 48 VIII CONTENTS PART II. PHONONS AND TUNNELING EXCITATIONS 4. ADIABATIC INTERACTION ..................................... 55 4.1 THEORETICAL DESCRIPTION OF INTERACTING ELECTRONS AND NUCLEI . . 55 4.2 FRANCKCONDON AND HERZBERGTELLER INTERACTIONS . . . . . . . . . . . 57 5. NATURAL VIBRATIONS OF SOLIDS .............................. 61 5.1 ACOUSTIC AND OPTICAL PHONONS . . . . . . . . . . . . . . . . . . . . . . . . . . . 61 5.2 LOCALIZED PHONON MODES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 65 6. TUNNELING SYSTEMS IN SOLIDS .............................. 75 6.1 TUNNELING DEGREES OF FREEDOM IN COMPLEX MOLECULES AND AMORPHOUS SOLIDS . . . . . . . . . . . . . . 75 6.2 RATE EQUATIONS FOR TUNNELING SYSTEMS . . . . . . . . . . . . . . . . . . . . 78 6.3 ONE-PHONON TRANSITION PROBABILITIES IN TUNNELING SYSTEMS . . 80 6.4 KINETICS OF TUNNELING SYSTEMS . . . . . . . . . . . . . . . . . . . . . . . . . . . 84 6.5 TUNNELING SYSTEMS IN POLYMERS AND GLASSES. . . . . . . . . . . . . . . . 86 6.6 TWO-LEVEL SYSTEMS (TLS). TUNNELONS. TUNNELONPHONON AND ELECTRONTUNNELON INTERACTION . . . . . . . 90 PART III. SPECTROSCOPY OF A SINGLE IMPURITY CENTER 7. DENSITY MATRIX FOR AN IMPURITY CENTER ................... 95 7.1 TRANSITION AMPLITUDES IN THE ELECTRONPHONONTUNNELON SYSTEM . . . . . . . . . . . . . . . . . 95 7.2 EQUATIONS FOR THE DENSITY MATRIX . . . . . . . . . . . . . . . . . . . . . . . . . 99 7.3 REDUCING EQUATIONS FOR THE FULL DENSITY MATRIX TO THE OPTICAL BLOCH EQUATIONS . . . . . . . . . . . . . . . . . . . . . . . . . . . 104 8. ONE- AND TWO-PHOTON COUNTING METHODS IN THE SPECTROSCOPY OF A SINGLE IMPURITY CENTER .......... 109 8.1 TWO-PHOTON CORRELATOR FOR A TWO-LEVEL IMPURITY CENTER . . . . 109 8.2 INFLUENCE OF A TRIPLET LEVEL ON THE TWO-PHOTON CORRELATOR. PHOTON BUNCHING AND ANTIBUNCHING . . . . . . . . . . . . . . . . . . . . . . 112 8.3 ONE-PHOTON COUNTING METHOD. QUANTUM TRAJECTORIES . . . . . . . 119 CONTENTS IX PART IV. OPTICAL BAND SHAPE THEORY FOR IMPURITY CENTERS 9. STOCHASTIC THEORIES OF LINE BROADENING ................... 125 9.1 DYNAMIC AND STOCHASTIC APPROACHES TO THE LINE-BROADENING PROBLEM . . . . . . . . . . . . . . . . . . . . . . . . . . 125 9.2 STOCHASTIC THEORY DUE TO ANDERSON AND WEISS . . . . . . . . . . . . . 126 9.3 ANDERSON THEORY FOR OPTICAL LINES . . . . . . . . . . . . . . . . . . . . . . . 129 9.4 EXCHANGE MODEL FOR LINE BROADENING . . . . . . . . . . . . . . . . . . . . . 131 10. DYNAMICAL THEORY OF ELECTRONPHONON BANDS ............ 137 10.1 ABSORPTION CROSS-SECTION AND THE PROBABILITY OF LIGHT EMISSION . . . . . . . . . . . . . . . . . . . . . 138 10.2 ELECTRONPHONON OPTICAL TRANSITIONS IN A CONDON APPROXIMATION AT T = 0 . . . . . . . . . . . . . . . . . . . . . 139 10.3 ZERO-PHONON LINE AND PHONON SIDE BAND . . . . . . . . . . . . . . . . . 142 10.4 INFLUENCE OF TEMPERATURE ON THE ZPL INTENSITY . . . . . . . . . . . . . 149 10.5 OPTICAL BANDS FOR STRONG ELECTRONPHONON COUPLING . . . . . . . . 150 11. VIBRONIC SPECTRA OF COMPLEX MOLECULES .................. 153 11.1 VIBRONIC SPECTRA IN THE CONDON APPROXIMATION. SIMILARITY RULE IN VIBRONIC SPECTRA . . . . . . . . . . . . . . . . . . . . . . . 153 11.2 INFLUENCE OF THE HT INTERACTION ON OPTICAL BANDS . . . . . . . . . . . 156 11.3 INTERFERENCE OF HT AND FC AMPLITUDES. BREAKDOWN OF THE MIRROR SYMMETRY OF CONJUGATE ABSORPTION AND FLUORESCENCE BANDS . . . . . . . . . . . 158 11.4 THEORETICAL TREATMENT OF ELECTRONPHONON AND VIBRONIC SPECTRA . . . . . . . . . . . . . . . . . 161 12. DYNAMICAL THEORY OF LINE BROADENING .................... 167 12.1 SPECIFIC FEATURES OF THE QUADRATIC FC INTERACTION . . . . . . . . . . . 168 12.2 CUMULANT EXPANSION OF THE DIPOLAR CORRELATOR . . . . . . . . . . . . . 170 12.3 BROADENING AND SHIFT OF THE ZPL AT WEAK COUPLING WITH ACOUSTIC AND LOCALIZED PHONONS . . . . . . . . . . . . . . . . . . . . . 173 12.4 QUANTUM PHONON GREEN FUNCTIONS . . . . . . . . . . . . . . . . . . . . . . . 177 12.5 TEMPERATURE BROADENING AND SHIFT OF THE ZPL AT ARBITRARY STRENGTH OF THE QUADRATIC FC INTERACTION . . . . . . 179 12.6 GENERAL EXPRESSION FOR THE CUMULANT FUNCTION OF AN ELECTRONPHONON SYSTEM . . . . . . . . . . . . . . . . . . . . . . . . . . . 186 12.7 THEORETICAL TREATMENT OF EXPERIMENTAL DATA FOR TEMPERATURE BROADENING OF THE ZPL . . . . . . . . . . . . . . . . . . . 187 X CONTENTS PART V. METHODS OF SELECTIVE SPECTROSCOPY 13. FLUORESCENCE LINE NARROWING ............................. 195 13.1 FREQUENCY SELECTION OF MOLECULES BY LASER EXCITATION . . . . . . . 195 13.2 FLUORESCENCE LINE NARROWING AND ITS RELATION TO THE FULL TWO-PHOTON CORRELATOR . . . . . . . . . 198 13.3 LASER FLUORESCENCE ANALYSIS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 202 14. SPECTRAL HOLE BURNING IN INHOMOGENEOUS OPTICAL BANDS .. 205 14.1 TRANSIENT SPECTRAL HOLE BURNING. RELATION TO THE FULL TWO-PHOTON CORRELATOR. . . . . . . . . . . . . . . . 205 14.2 PERSISTENT SPECTRAL HOLES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 209 14.3 KINETICS OF PERSISTENT HOLE BURNING. HOLE SHAPE IN THE SHORT TIME LIMIT . . . . . . . . . . . . . . . . . . . . . . 213 14.4 HOLE BURNING WITH PHOTOACTIVE PHOTOPRODUCT. ANTIHOLES. . . . . 216 14.5 POLARIZATION ASPECTS IN SPECTRAL HOLES AND ANTIHOLES . . . . . . . . 221 14.6 PHOTON-GATED PERSISTENT SPECTRAL HOLE BURNING . . . . . . . . . . . . 226 PART VI. TRANSIENT COHERENT PHENOMENA IN SOLIDS 15. COHERENT RADIATION OF MOLECULAR ENSEMBLES .............. 233 15.1 DEPHASING AND ENERGY RELAXATION. COHERENT SPONTANEOUS EMISSION . . . . . . . . . . . . . . . . . . . . . . . . . . 233 15.2 FAST OPTICAL DEPHASING . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 237 16. PHOTON ECHO .............................................. 241 16.1 INTERACTION OF A SINGLE ATOM WITH A CLASSICAL ELECTROMAGNETIC FIELD . . . . . . . . . . . . . . . . . . . . 241 16.2 MOLECULE INTERACTING WITH A CLASSICAL ELECTROMAGNETIC FIELD, PHONONS, AND TUNNELONS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 244 16.3 SIMPLEST THEORY OF THE TWO-PULSE PHOTON ECHO . . . . . . . . . . . . 246 16.4 BLOCH VECTOR AND ITS TEMPORAL EVOLUTION . . . . . . . . . . . . . . . . . . 249 16.5 EXPONENTIAL TWO-PULSE PHOTON ECHO . . . . . . . . . . . . . . . . . . . . . . 251 16.6 THREE-PULSE PHOTON ECHO. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 255 16.7 LONG-LIVED 3PE . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 258 16.8 SPACE ANISOTROPY OF ECHO RADIATION . . . . . . . . . . . . . . . . . . . . . . 261 17. NONEXPONENTIAL PHOTON ECHO ............................. 263 17.1 GENERALIZED BLOCH VECTOR . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 263 17.2 LONG-LIVED STIMULATED PHOTON ECHO . . . . . . . . . . . . . . . . . . . . . . 265 17.3 PICOSECOND SPE . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 271 17.4 TWO-PULSE FEMTOSECOND PHOTON ECHO . . . . . . . . . . . . . . . . . . . . . 272 17.5 3PE AT ARBITRARY WAITING TIME T W . . . . . . . . . . . . . . . . . . . . . . . 278 CONTENTS XI PART VII. LOW TEMPERATURE SPECTRAL DIFFUSION IN POLYMERS AND GLASSES 18. THEORY OF ELECTRONTUNNELON OPTICAL BAND ............... 283 18.1 GENERAL EXPRESSION FOR THE CUMULANT FUNCTION OF THE ELECTRONTUNNELON SYSTEM . . . . . . . . . . . . . . . . . . . . . . . . . 284 18.2 TUNNELON GREEN FUNCTION . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 288 18.3 TEMPERATURE BROADENING OF THE ZERO TUNNELON OPTICAL LINE . 289 18.4 DIPOLAR CORRELATOR FOR A CHROMOPHORETLS SYSTEM. SOLUTION OF THE INTEGRAL EQUATION . . . . . . . . . . . . . . . . . . . . . . . . . 292 18.5 ELECTRONTUNNELON OPTICAL BAND SHAPE FUNCTION . . . . . . . . . . . 294 19. CHROMOPHORE INTERACTING WITH PHONONS AND TLSS WHICH ARE NOT IN THERMAL EQUILIBRIUM ................... 297 19.1 HAMILTONIAN OF THE ELECTRONPHONONTUNNELON SYSTEM . . . . . . 297 19.2 EQUATIONS FOR THE DENSITY MATRIX OF THE ELECTRONPHONONTUNNELON SYSTEM . . . . . . . . . . . . . . . . . 299 19.3 SPONTANEOUS AND LIGHT-INDUCED TRANSITIONS IN TLSS . . . . . . . . 305 19.4 INTERACTION WITH ONE TLS. APPROXIMATE SOLUTION . . . . . . . . . . . 307 19.5 INTERACTION WITH MANY TLSS UNDERGOING SPONTANEOUS TUNNELING . . . . . . . 310 20. DYNAMICAL THEORY OF SPECTRAL DIFFUSION .................. 313 20.1 ABSORPTION COEFFICIENT OF A SINGLE GUEST MOLECULE INTERACTING WITH NONEQUILIBRIUM TLSS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 313 20.2 DEPENDENCE OF THE OPTICAL DEPHASING TIME T 2 ON THE TIME SCALE OF THE EXPERIMENT. . . . . . . . . . . . . . . . . . . . . . 317 20.3 LOGARITHMIC TEMPORAL LINE BROADENING. DEVIATION FROM THE LOGARITHMIC TEMPORAL LAW . . . . . . . . . . . . . 321 21. THEORY OF TUNNELING TRANSITIONS IN TLSS ................. 325 21.1 GENERAL FORMULAS FOR THE TUNNELING PROBABILITY . . . . . . . . . . . . 325 21.2 INELASTIC TUNNELING ASSISTED BY ACOUSTIC AND LOCALIZED PHONON MODES . . . . . . . . . 328 21.3 ELASTIC TUNNELING . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 332 22. INVESTIGATING TLS RELAXATION BY SINGLE-MOLECULE SPECTROSCOPY .......................... 333 22.1 TWO-PHOTON CORRELATOR OF A MOLECULE INTERACTING WITH TLSS . 333 22.2 SPONTANEOUS AND LIGHT-INDUCED JUMPS OF THE OPTICAL LINE. RELATION TO HOLE BURNING . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 336 22.3 ANALYSIS OF COMPLICATED SPECTRAL TRAJECTORIES USING THE TWO-PHOTON CORRELATOR . . . . . . . . . . . . . . . . . . . . . . . . 338 XII CONTENTS 22.4 SINGLE-MOLECULE CHEMICAL REACTIONS . . . . . . . . . . . . . . . . . . . . . . 340 22.5 MANIFESTATION OF SPECTRAL DIFFUSION IN THE TWO-PHOTON CORRELATOR . . . . . . . . . . . . . . . . . . . . . . . . . . . . 341 22.6 DIVERSITY OF THE LOCAL DYNAMICS OF INDIVIDUAL MOLECULES . . . . . 342 22.7 CONTRIBUTION TO THE OPTICAL BAND FROM DIFFERENT TYPES OF TLS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 345 22.8 DEVIATIONS FROM THE STANDARD TLS MODEL . . . . . . . . . . . . . . . . . 346 APPENDICES ................................................... 349 A. CALCULATION OF THE FUNCTION * ( * ) . . . . . . . . . . . . . . . . . . . . . . . . . 349 B. PROBABILITY OF SPONTANEOUS PHOTON EMISSION . . . . . . . . . . . . . . . 350 C. UNITARITY OF AMPLITUDES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 351 D. DERIVATION OF (3.8) . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 351 E. DERIVATION OF (3.24) . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 352 F. PROOF OF THE APPROXIMATION (7.16) . . . . . . . . . . . . . . . . . . . . . . . . 352 G. THE WICKBLOCHDOMINICIS THEOREM FOR BOSONS . . . . . . . . . . . 353 H. INFLUENCE OF FC AND HT INTERACTIONS ON THE OPTICAL BAND SHAPE FUNCTION . . . . . . . . . . . . . . . . . . . . . . 355 I. CUMULANT EXPANSION . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 359 J. RELATION BETWEEN PHONON GREEN FUNCTIONS . . . . . . . . . . . . . . . . 361 K. SHIFT OF THE ZPL AT T = 0 . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 363 L. DERIVATION OF (17.65) . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 364 M. THE WICKBLOCHDOMINICIS THEOREM FOR FERMIONS . . . . . . . . . . 365 N. DERIVATION OF (18.37) AND (18.38) . . . . . . . . . . . . . . . . . . . . . . . . . 367 O. DERIVATION OF (18.53) . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 368 P. DERIVATION OF (18.60) . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 369 Q. STOCHASTIC APPROACH TO SPECTRAL DIFFUSION . . . . . . . . . . . . . . . . . 370 BIBLIOGRAPHY .................................................. 375 INDEX ......................................................... 381
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id	DE-604.BV014685958
illustrated	Illustrated
indexdate	2024-07-09T19:05:02Z
institution	BVB
isbn	3540441018
language	English Russian
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owner	DE-703 DE-384 DE-11 DE-188
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physical	XII, 382 S. graph. Darst.
publishDate	2003
publishDateSearch	2003
publishDateSort	2003
publisher	Springer
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series	Springer series in chemical physics
series2	Springer series in chemical physics Physics and astronomy online library
spelling	Osad'ko, Igor' S. Verfasser aut Selective spectroscopy of single molecules Igor S. Osad'ko Berlin [u.a.] Springer 2003 XII, 382 S. graph. Darst. txt rdacontent n rdamedia nc rdacarrier Springer series in chemical physics 69 Physics and astronomy online library Físico-química larpcal Molecular spectroscopy Tunneling (Physics) Einzelmolekülspektroskopie (DE-588)4396226-9 gnd rswk-swf Einzelmolekülspektroskopie (DE-588)4396226-9 s DE-604 Springer series in chemical physics 69 (DE-604)BV000000670 69 SWB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=009959882&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis
spellingShingle	Osad'ko, Igor' S. Selective spectroscopy of single molecules Springer series in chemical physics Físico-química larpcal Molecular spectroscopy Tunneling (Physics) Einzelmolekülspektroskopie (DE-588)4396226-9 gnd
subject_GND	(DE-588)4396226-9
title	Selective spectroscopy of single molecules
title_auth	Selective spectroscopy of single molecules
title_exact_search	Selective spectroscopy of single molecules
title_full	Selective spectroscopy of single molecules Igor S. Osad'ko
title_fullStr	Selective spectroscopy of single molecules Igor S. Osad'ko
title_full_unstemmed	Selective spectroscopy of single molecules Igor S. Osad'ko
title_short	Selective spectroscopy of single molecules
title_sort	selective spectroscopy of single molecules
topic	Físico-química larpcal Molecular spectroscopy Tunneling (Physics) Einzelmolekülspektroskopie (DE-588)4396226-9 gnd
topic_facet	Físico-química Molecular spectroscopy Tunneling (Physics) Einzelmolekülspektroskopie
url	http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=009959882&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA
volume_link	(DE-604)BV000000670
work_keys_str_mv	AT osadkoigors selectivespectroscopyofsinglemolecules

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