Photocatalysis: science and technology
Gespeichert in:
| Format: | Buch |
|---|---|
| Sprache: | English |
| Veröffentlicht: |
Berlin [u.a.]
Springer
2002
Tokyo Kodansha |
| Schriftenreihe: | Biological and medical physics series
Physics and astronomy online library |
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | XVI, 356 S. Ill., graph. Darst. |
| ISBN: | 3540434739 4062106159 |
Internformat
MARC
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| 245 | 1 | 0 | |a Photocatalysis |b science and technology |c Masao Kaneko ... (eds.) |
| 264 | 1 | |a Berlin [u.a.] |b Springer |c 2002 | |
| 264 | 1 | |a Tokyo |b Kodansha | |
| 300 | |a XVI, 356 S. |b Ill., graph. Darst. | ||
| 336 | |b txt |2 rdacontent | ||
| 337 | |b n |2 rdamedia | ||
| 338 | |b nc |2 rdacarrier | ||
| 490 | 0 | |a Biological and medical physics series | |
| 490 | 0 | |a Physics and astronomy online library | |
| 650 | 7 | |a Catálise |2 larpcal | |
| 650 | 7 | |a Fotoquímica |2 larpcal | |
| 650 | 7 | |a Photocatalyse |2 ram | |
| 650 | 4 | |a Photocatalysis | |
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| 700 | 1 | |a Kaneko, Masao |d 1942- |e Sonstige |0 (DE-588)123824516 |4 oth | |
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Datensatz im Suchindex
| _version_ | 1804129347969220608 |
|---|---|
| adam_text | Contents
List of Contributors
....................................................................................
v
Preface
.........................................................................................................
vii
1
Introduction
....................................................................................... 1
1.1
Background
................................................................................ 1
1.2
Aim and Outline of This Volume
............................................. 2
1.3
Summary
.................................................................................... 4
1.4
Future Perspectives
.................................................................... 4
References
............................................................................................ 5
I Fundamental Aspects of Photocatalysts
Photoelectrochemical Processes of Semiconductors
9
2.1
Semiconductor Electrodes for Solar Energy Conversion
........ 11
2.2
Reduction of CO2 at Illuminated Semiconductor Electrodes
··
IS
2.3
Photocatalysis
............................................................................ 18
2.3.1
General Remarks
........................................................... 18
2.3.2
Mechanistic Studies
...................................................... 19
2.3.3
Low Intensity Illumination
........................................... 22
2.3.4
Applications
................................................................... 24
References
............................................................................................ 26
Design, Preparation and Characterization of Highly Active Metal
Oxide Photocatalysts
29
3.1
Introduction
................................................................................ 29
3.2
Photocatalytic Activity
.............................................................. 29
3.2.1
Effect of Surface Area on Photocatalytic Activity
...... 30
3.2.2
Effect of Electron-hole Recombination on Photocatalytic
Activity
..........................................................................
3.2.3
Design of Photocatalysts of High Activity
3.3
Preparation of Titanium(IV) Oxide Powders
3.3.1 Sulfate
Method
..............................................................
3.3.2
Chloride Method (Vapor Method)
3.3.3
Alkoxide Method
...........................................................
ι
Contents
3.3.4
Specific Methods
........................................................... 34
3.3.5
Activation of TiO2 Photocatalysts
................................ 36
3.4
Preparation of Other Photocatalysts
......................................... 38
3.5
Characterization of TiO2 Photocatalysts of Both High Crystallinity
and Large Surface Area
............................................................. 38
3.5.1
Photocatalytic Activity of HyCOM TiO2 in Aqueous
Suspension Systems
...................................................... 38
3.5.2
Correlation Between Physical Properties and Photocatalytic
Activity of HyCOM TiO2
39
3.5.3
Novel Hypothesis for Activity of Photocatalyst
.......... 43
3.6
Preparation and Characterization of Photocatalytic Thin Films
................................................................................................... 44
3.6.1
Preparation of Photocatalytic TiO2 Thin Films
........... 44
3.6.2
Characterization of Photocatalytic Thin Films Prepared
from HyCOM TiO2 Powders
........................................ 45
3.7
Summary
.................................................................................... 47
References
............................................................................................ 47
4
Photoelectrochemistry at Semiconductor/Liquid Interfaces
···■ 51
4.1
Introduction
................................................................................ 51
4.2
Basic Properties of Semiconductor/Liquid Interface
............... 52
4.2.1
Band Bending
................................................................ 52
4.2.2
Barrier Height and Flat Band Potential
........................ 54
4.2.3
Electron Transfer and Corrosion Reactions
................. 57
4.3
Photoelectrochemistry at Atomically Well-defined Surfaces
■ 59
4.3.1
Atomically Flat H-terminated Si Surfaces
59
4.3.2
Selective Exposition of
( 100)
Face on
n-TiO2
(Rutile)
by
Photoetching
.................................................................. 62
4.4
Photoelectrochemistry at Metal Dot-coated Semiconductors
·· 64
4.4.1
Ideal Semiconductor Electrodes
................................... 64
4.4.2
Metal-loaded TiO2 Electrodes
....................................... 66
References
............................................................................................ 67
5 Photoelectrochemical
Reactions at Semiconductor Microparticle
■ 69
5.1
Introduction
................................................................................ 69
5.2
Energy Structure of Semiconductor Microparticle
.................. 69
5.2.1
Depletion Layer
............................................................. 69
5.2.2
Electric Heterogeneity of Surface
................................ 71
5.2.3
Size Quantization Effect
............................................... 72
5.3
Kinetics at Semiconductor Microparticle
.................................... 72
5.3.1
Recombination Model
................................................... 73
5.3.2
2D Ladder Model
.......................................................... 74
5.3.3
Effect of Size
................................................................. 76
5.4
Observation of Primary Reaction Intermediates
......................... 77
5.4.1
ESR Analysis for Irradiated TiO2 Particles
.................. 78
5.4.2
Direct Observation of Intermediate Radicals
............... 81
5.4.3
Chemiluminescent Probe for Active Oxygens
............. 83
References
.............................................................................
..............
g5
Contents xi
6 New
Approaches in Solution-phase
Processing
of Semiconductor
Thin
Films .......................................................................................... 87
6.1
Introduction
................................................................................ 87
6.2
Previous Methods for Solution-phase Deposition of Semiconductor
Thin Films
.................................................................................. 89
6.2.1
Chemical Bath Deposition of Metal
Sulfide
Thin Films
............................................................................................ 89
6.2.2
Electrodeposition of Metal
Sulfide
Thin Films
........... 90
6.2.3
Chemical and Electrochemical Deposition of Metal Oxide
Thin Films
...................................................................... 92
6.3
Electrochemically Induced Chemical Deposition (EICD) of CdS
Thin Films
.................................................................................. 93
6.3.1
Idea
................................................................................. 93
6.3.2
Morphological and Structural Analysis
........................ 94
6.3.3
Growth Kinetics and Mechanism of EICD Process
..... 95
6.3.4
Modification of EICD Process
...................................... 97
6.4
True Electrodeposition of Metal
Sulfide
Thin Films by Reduction
of Thiocyanato Complexes
........................................................ 97
6.4.1
Idea
................................................................................. 97
6.4.2
Thermodynamic Consideration
..................................... 98
6.4.3
Electrochemical Layer-by-layer Growth of CdS
Thin Films
...................................................................... 98
6.4.4
Electrodeposition of Other Metal
Sulfides ................... 100
6.5
Electrochemical Self-assembly of ZnO/Dye Hybrid
Thin Films
.................................................................................. 100
6.5.1
Idea
................................................................................. 100
6.5.2
Electrochemical Self-assembly of ZnO/Dye Hybrid
Structure
......................................................................... 102
6.5.3
Mechanism of Electrochemical Self-assembly
............ 104
6.6
Summary
.................................................................................... 104
References
............................................................................................ 105
II Application to Environmental Cleaning
7
Self-cleaning Properties of TiCVcoated Substrates
109
7.1
Introduction
................................................................................ 109
7.2
Photocatalytic Decomposition
.................................................. 110
7.2.1
Air Purifying Effect
...................................................... 110
7.2.2
Sterilization Effect
........................................................
Ill
7.2.3
Anti-fouling Effect
........................................................ 113
7.2.4
Photo-induced High Amphiphilicity
............................ 114
7.3
Conclusions
................................................................................ 120
References
............................................................................................ 121
8
Cleaning Atmospheric Environment
............................................. 123
8.1
Introduction
................................................................................ 123
8.2
Photocatalytic Activities of TiO2
.............................................. 124
xii Contents
8.2.1
Oxidation of Air Pollutants by
Photogenerated
Active
Oxygen Species
............................................................. 124
8.2.2
Photocatalytic Reactions of Volatile Hydrocarbons
·■·■ 125
8.2.3
Photocatalytic Reactions of Halogenated Hydrocarbons
............................................................................................ 136
8.2.4
Nitrogen Oxides (NO,)
.................................................. 143
8.3
Development of Air Purifying Materials Based on
Photocatalyst
.............................................................................. 147
8.3.1
Immobilization of Powder Photocatalysts
................... 147
8.3.2
Preparation of Air-purifying Materials
........................ 148
8.3.3
Performance Characteristics of Air-purifying
Materials
........................................................................ 149
8.4
Application of Photocatalysis to Cleaning of Atmospheric
Environment
............................................................................... 151
8.4.1
Passive Purification of Polluted Air
151
8.4.2
Active Air Purification of Closed Space
...................... 153
8.5
Summary
.................................................................................... 154
References
............................................................................................ 155
9
Water Purification
—
Degradation of Aqueous Pollutant and
Application to Water Treatment
.................................................... 157
9.1
Introduction
............................................................................... 157
9.2
Photocatalytic Characteristics of Titanium Dioxide
................ 157
9.3
Photocatalytic Degradation of Pollutant
160
9.3.1
Volatile Organohalide Compound
160
9.3.2
Pesticides
....................................................................... 162
9.3.3
Other Organic Compounds
........................................... 164
9.3.4
Environmental Hormones (Endocrine Disruptors)
...... 165
9.4
Enhancement of Degradation Rate
........................................... 166
9.4.1
Pt-loading
....................................................................... 166
9.4.2
Addition of H2O2
........................................................... 167
9.4.3
Ozone
............................................................................. 169
9.4.4
Increase in Adsorption
.................................................. 169
9.5
Solar System for Water Treatment
........................................... 171
9.6
Immobilization of TiO2 and Instrumentation
........................... 171
9.7
Conclusion and Outlook
............................................................ 172
References
............................................................................................ 172
10
Second-generation TiO2 Photocatalysts Able to Initiate Reactions
Under Visible Light Irradiation
..................................................... 175
10.1
Introduction
................................................................................ 175
10.2
Experimental Section
................................................................. 175
10.3
Results and Discussion
.............................................................. 176
10.4
Conclusion
................................................................................. 182
References
............................................................................................ 182
Contents
III
Application
to Photoenergy Conversion
11
Photocatalytic Organic Syntheses Using Semiconductor
Particles
.............................................................................................. 185
11.1
Introduction
................................................................................ 185
11.2
Principle of Photocatalysis by Semiconductor Particles
.......... 186
11.3
Photocatalytic Reactions by Semiconductor Suspension
........ 187
11.4
Redox
Combined Photocatalytic Processes for Nitrogen-containing
Substrates
................................................................................... 189
11.5
Further Development to Stereoselective Organic Synthesis of
Nitrogen-containing Compounds
.............................................. 191
11.6
Introduction of Oxygen Atoms into Organic Compounds
....... 194
11.6.1
Stereospecific Epoxidation of 2-hexene on Photoirradiated
TiO2 Powders Using Molecular Oxygen as
Oxidant
— 195
11.6.2
Selective Oxidation of Naphthalene by Molecular Oxygen
and Water Using
ТЮг
Photocatalysts
.......................... 196
11.6.3
Photocatalytic
Oxygénation:
Summary
........................ 198
11.7
Concluding Remarks
................................................................. 199
References
............................................................................................ 199
12
Sonophotocatalysis
—
Joint System of Sonochemical and
Photocatalytic Reactions
................................................................. 203
12.1
Introduction
—
What is Sonophotocatalysis?
............................ 203
12.2
Utilization of Sonophotocatalytic Reaction
............................. 204
12.2.1
Sonophotocatalysis of Water
........................................ 204
12.2.2
Sonophotocatalysis of Artificial Seawater
................... 216
12.2.3
Sonophotocatalyses of Organic Compounds
................ 219
12.3
Conclusion and Future Scopes
.................................................. 220
References
............................................................................................ 221
13
Gas-phase Water Photolysis by NaOH-coated Photocatalysts
223
13.1
Introduction
................................................................................ 223
13.2
Water Photolysis by Pt/TiO2
..................................................... 224
13.3
Water Photolysis by Metallized Semiconductor Powders
....... 226
13.3.1
Gas-phase Water Photolysis by NaOH-coating
226
13.3.2
Factors Influencing Yield of Water Photolysis
229
13.4
Concluding Remarks
................................................................. 233
References
............................................................................................ 234
14
Water Photolysis by TiO2 Particles—Significant Effect of
Na2CO3 Addition on Water Splitting
235
14.1
Introduction
................................................................................ 235
14.2
Significant Effect of Carbonate Salt Addition on Water Splitting
from Pt/TiO2 Water Suspension
................................................ 236
14.3
Role of Carbonate Salts on Water Splitting and Reaction
Mechanism
................................................................................. 240
xiv Contents
14.4
Effective
Screening of Active Photocatalysts for Water Splitting
Using Na2CO} Addition Method
............................................... 242
14.5
Solar Hydrogen Production Using NajCOj Addition Method
246
14.6
Conclusion
................................................................................. 248
References
............................................................................................ 248
15
Water Photolysis by Titanates with Tunnel Structures
249
15.1
Water Photolysis by RuOj/BaTuO, with Pentagonal Prism
Tunnel Structure
........................................................................ 250
15.2
Water Photolysis by RuCb/^TUO,
,
with Rectangular Tunnel
Structure
..................................................................................... 257
References
............................................................................................ 260
16
Water Photolysis by Layered Compounds
................................... 261
16.1
Introduction
................................................................................ 261
16.2
Layered Oxides of Transition Metals
....................................... 261
16.3
K4NDA7
.................................................................................... 263
16.3.1
Structure and Physico-chemical Properties
.................. 263
16.3.2
Photocatalytic Overall Water Splitting
265
16.3.3
Structure of Ni-loaded K4Nb6O17 and Reaction
Mechanism
..................................................................... 267
16.4
Perovskite-related Layered Oxides
........................................... 268
16.5
Summary
.................................................................................... 276
References
............................................................................................ 276
17
Splitting of Water by Combining Two Photocatalytic Reactions
via Quinone
Redox
Couple Dissolved in Oil Phase: Artificial
Photosynthesis
................................................................................... 279
17.1
Introduction
................................................................................ 279
17.2
Strategy for Water Splitting by Mimicking Photosynthesis
280
17.3
Photocatalytic Hydrogen and Oxygen Evolution in Separate
Systems
...................................................................................... 281
17.3.1
Photooxidation of Water Using
ТІО2
Particles
282
17.3.2
Photoreduction of Water Using Pt-loaded TiO2
Particles
.......................................................................... 285
17.4
Approaches to Electrochemical and Chemical Combinations of
Two Photocatalytic Reactions
................................................... 286
17.5
Splitting of Water by a Combination of Two Photocatalytic
Reactions via DDQ/DDHQ
....................................................... 289
17.6
Conclusions
................................................................................ 291
References
............................................................................................ 291
18
Sensitization by Metal Complexes Towards Future Artificial
Photosynthesis
................................................................................... 293
18.1
Introduction
................................................................................ 293
18.2
Photoinduced Hydrogen Evolution in Homogeneous
Four-component Systems
.......................................................... 294
Contents xv
18.2.1
Photoinduced Hydrogen Evolution with
Porphyrin
Metal
Complexes and Hydrogenase
........................................ 294
18.2.2
Photoinduced Hydrogen Evolution Using Cytochrome
Cj as Electron Carrier
.................................................... 296
18.2.3
Photoinduced Hydrogen Evolution Using
Chemically-modified Chlorophyll
................................ 298
18.3
Photoinduced Hydrogen Evolution with Viologen-linked
orphyrin Metal Complexes
........................................................ 299
18.3.1
Photoinduced Hydrogen Evolution with Water-soluble
Viologen-linked Cationic Porphyrin Metal Complexes
and Hydrogenase
........................................................... 300
18.3.2
Photoinduced Hydrogen Evolution with Water-soluble
Viologen-linked
Anionie
Porphyrin and Hydrogenase
........................................................................................ 302
18.4
Other Systems for Hydrogen Evolution Using Natural
Photosensitizers
......................................................................... 303
18.5
Conclusion
................................................................................. 306
References
............................................................................................ 306
19
Catalyses and Sensitization for Water Reaction Towards Future
Artificial Photosynthesis
309
19.1
Introduction
................................................................................ 309
19.2
Design of Artificial Photosynthesis
309
19.2.1
Photosynthesis and Energy Cycle on Earth
................. 309
19.2.2
Artificial Photosynthesis
311
19.3
Molecular Catalysts for Water Reactions and CO2 Reduction
312
19.3.1
Catalysis in Water Oxidation
312
19.3.2
Catalysis in Proton Reduction
...................................... 316
19.3.3
Catalysis in Carbon Dioxide Reduction
....................... 316
19.4
Photoexcited State Electron Transfer in Heterogeneous Phases
.................................................................................................... 317
19.5
Sensitization of TiO2 Powders and Films in Water
................. 320
19.6
Conclusion and Future Prospects
.............................................. 322
References
............................................................................................ 323
20
Photoelectric TiO2 Solar Cells
325
20.1
Introduction
................................................................................ 325
20.2
Dye-sensitization of Semiconductors
....................................... 325
20.2.1
History
........................................................................... 325
20.2.2
Innovative Dye-sensitized Solar Cells
........................ 327
20.2.3
Fabrication of Dye-sensitized TiO2 Solar Cells
328
20.2.4
Characterization of Innovative Dye-sensitized
TiO2 Solar Cells
............................................................. 329
20.3
Electron-transfer Sensitization on TiO2
.................................... 330
20.3.1
Bonding Structure of Dye on TiO2 Influencing rjt,
331
20.3.2
Dynamics in Electron Transfer from Photoexcited Dye
2
to TiO2
............................................................................ 331
Contents
20.3.3 Electron Transfer
Between Oxidized Dye
2
and
Г/Ь
Electrolyte
...................................................................... 332
20.4
Electron Transport in Porous TiO2 Electrodes
333
20.4.1
Electron Transport Models for High
ηα
....................... 334
20.4.2
Time-course Analysis
.................................................... 335
20.4.3
Frequency Analysis
....................................................... 335
20.4.4
Effect of TiOj Films on Performance of Dye-sensitized
Solar Cells
..................................................................... 337
20.5
Sensitization Dyes
..................................................................... 337
20.5.1
Ruthenium Polypyridine Complexes
............................ 337
20.5.2
Other Metal Complexes
................................................ 339
20.5.3
Organic Dyes
................................................................. 340
20.5.4
Natural Dyes
.................................................................. 342
20.6
Recent Research Progress in Dye-sensitized Solar Cells
........ 343
20.7
Future Work on Dye-sensitized Solar Cells
............................. 344
20.8
Concluding Remarks
................................................................. 345
References
............................................................................................ 346
Index
..................................................................................................... 349
|
| any_adam_object | 1 |
| author_GND | (DE-588)123824516 |
| building | Verbundindex |
| bvnumber | BV014569152 |
| callnumber-first | J - Political Science |
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| callnumber-sort | JK 3271 |
| callnumber-subject | JK - United States |
| classification_rvk | UM 4500 VE 8300 |
| classification_tum | CHE 167f CHE 189f |
| ctrlnum | (OCoLC)50023751 (DE-599)BVBBV014569152 |
| dewey-full | 541.3/95 |
| dewey-hundreds | 500 - Natural sciences and mathematics |
| dewey-ones | 541 - Physical chemistry |
| dewey-raw | 541.3/95 |
| dewey-search | 541.3/95 |
| dewey-sort | 3541.3 295 |
| dewey-tens | 540 - Chemistry and allied sciences |
| discipline | Chemie / Pharmazie Physik Chemie |
| format | Book |
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| id | DE-604.BV014569152 |
| illustrated | Illustrated |
| indexdate | 2024-07-09T19:03:42Z |
| institution | BVB |
| isbn | 3540434739 4062106159 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-009906281 |
| oclc_num | 50023751 |
| open_access_boolean | |
| owner | DE-703 DE-29T DE-1046 DE-M49 DE-BY-TUM DE-384 DE-11 |
| owner_facet | DE-703 DE-29T DE-1046 DE-M49 DE-BY-TUM DE-384 DE-11 |
| physical | XVI, 356 S. Ill., graph. Darst. |
| publishDate | 2002 |
| publishDateSearch | 2002 |
| publishDateSort | 2002 |
| publisher | Springer Kodansha |
| record_format | marc |
| series2 | Biological and medical physics series Physics and astronomy online library |
| spelling | Photocatalysis science and technology Masao Kaneko ... (eds.) Berlin [u.a.] Springer 2002 Tokyo Kodansha XVI, 356 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Biological and medical physics series Physics and astronomy online library Catálise larpcal Fotoquímica larpcal Photocatalyse ram Photocatalysis Fotokatalyse (DE-588)4193873-2 gnd rswk-swf Fotokatalyse (DE-588)4193873-2 s DE-604 Kaneko, Masao 1942- Sonstige (DE-588)123824516 oth Digitalisierung UB Bayreuth application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=009906281&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Photocatalysis science and technology Catálise larpcal Fotoquímica larpcal Photocatalyse ram Photocatalysis Fotokatalyse (DE-588)4193873-2 gnd |
| subject_GND | (DE-588)4193873-2 |
| title | Photocatalysis science and technology |
| title_auth | Photocatalysis science and technology |
| title_exact_search | Photocatalysis science and technology |
| title_full | Photocatalysis science and technology Masao Kaneko ... (eds.) |
| title_fullStr | Photocatalysis science and technology Masao Kaneko ... (eds.) |
| title_full_unstemmed | Photocatalysis science and technology Masao Kaneko ... (eds.) |
| title_short | Photocatalysis |
| title_sort | photocatalysis science and technology |
| title_sub | science and technology |
| topic | Catálise larpcal Fotoquímica larpcal Photocatalyse ram Photocatalysis Fotokatalyse (DE-588)4193873-2 gnd |
| topic_facet | Catálise Fotoquímica Photocatalyse Photocatalysis Fotokatalyse |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=009906281&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT kanekomasao photocatalysisscienceandtechnology |