Magnetism: molecules to materials: 2 Molecule-based materials
Saved in:
| Format: | Book |
|---|---|
| Language: | English |
| Published: |
Weinheim [u.a.]
WILEY-VCH
2001
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| Subjects: | |
| Online Access: | Inhaltsverzeichnis |
| Physical Description: | XIV, 489 S. zahlr. graph. Darst. |
| ISBN: | 3527303014 |
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Record in the Search Index
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|---|---|
| adam_text | MAGNETISM: MOLECULES TO MATERIALS II MOLECULE-BASED MATERIALS EDITED BY
JOEL S. MILLER AND MARC DRILLON WILEY-VCH WEINHEIM * NEW YORK *
CHICHESTER BRISBANE * SINGAPORE * TORONTO CONTENTS 1 NITROXIDE-BASED
ORGANIC MAGNETS 1 1.1 INTRODUCTION 1 1.2 UNCONJUGATED NITROXIDES 5 1.2.1
MONO-NITROXIDES 5 1.2.2 OLIGO-NITROXIDES 10 1.3 CONJUGATED NITROXIDES 12
1.3.1 MONO-NITROXIDES 12 1.3.2 OLIGO-NITROXIDES 14 1.4 NITRONYL
NITROXIDES 18 1.4.1 MONO-NITRONYL NITROXIDES 18 1.4.2 OLIGO-NITRONYL
NITROXIDES 35 1.4.3 CO-CRYSTALLIZATION OF NITRONYL NITROXIDES 40 1.5
IMINO NITROXIDES 44 1.6 POLY(NITROXIDES) 46 1.7 OUTLOOK 49 REFERENCES 51
2 MAGNETIC ORDERING IN METAL COORDINATION COMPLEXES WITH AMINOXYL
RADICALS 61 2.1 INTRODUCTION 61 2.2 AMINOXYL RADICALS 61 2.2.1
ELECTRONIC STRUCTURE AND BASICITY 62 2.2.2 AMINOXYL RADICALS WITH
ANOTHER BASIC CENTER 63 2.2.3 HIGH-SPIN DI- AND POLY(AMINOXYL) RADICALS
64 2.3 MAGNETIC INTERACTION BETWEEN TRANSITION METAL IONS AND AMINOXYL
RADICALS 65 2.3.1 INDIRECT COUPLING (EXTENDED SUPEREXCHANGE) 65 2.3.2
COMPLEXES WITH DIRECT METAL-AMINOXYL COORDINATION .... 70 2.3.3 CYCLIC
COMPLEXES 72 2.4 DESIGN STRATEGY FOR VARIOUS CRYSTYL STRUCTURES 74 2.5
PREPARATION OF 3D TRANSITION METAL-POLY(AMINOXYL) RADICAL COMPLEXES 77
2.6 ONE-DIMENSIONAL METAL-AMINOXYL SYSTEMS 80 2.6.1 STRUCTURE AND
MAGNETIC PROPERTIES OF FERRIMAGNETIC 1D CHAINS FORMED BY MANGANESE(II)
AND NITRONYL NITROXIDES 81 CONTENTS 2.6.2 STRUCTURE AND MAGNETIC
PROPERTIES OF FERRIMAGNETIC 1D CHAINS FORMED BY MANGANESE(II) AND
TRIPLET BIS-AMINOXYL RADICALS 82 2.7 TWO-DIMENSIONAL METAL-AMINOXYL
SYSTEMS 88 2.7.1 STRUCTURE AND MAGNETIC PROPERTIES OF FERRIMAGNETIC 2D
SHEETS FORMED BY MANGANESE(II) AND NITRONYL NITROXIDES 89 2.7.2
STRUCTURE AND MAGNETIC PROPERTIES OF FERRIMAGNETIC 2D SHEETS FORMED BY
MANGANESE(II) AND HIGH-SPIN TRIS-AMINOXYL RADICALS 90 2.7.3 CONCLUSION
97 2.8 THREE-DIMENSIONAL METAL-AMINOXYL SYSTEMS 97 2.8.1 CRYSTAL AND
MOLECULAR STRUCTURE OF THE 3D SYSTEM 98 2.8.2 MAGNETIC PROPERTIES OF THE
3D SYSTEM 99 2.8.3 CONCLUSION 104 2.9 SUMMARY AND PROGNOSIS 104
REFERENCES 105 ORGANIC KAGOME ANTIFERROMAGNETS 109 3.1 INTRODUCTION 109
3.2 INORGANIC KAGOME ANTIFERROMAGNETS 110 3.2.1 SRGA L2 . X CR X 0 19
(SCGO(X)) 110 3.2.2 JAROSITE, AM 3 (OH) 6 (S0 4 )2 (A = NA+, K+, RB+,
AG+, NH+, H 3 0+,ETC.,ANDM = FE 3 +ORCR 3+ ) 111 3.3 ORGANIC KAGOME
ANTIFERROMAGNET, M-MPYNN * X 111 3.3.1 CRYSTAL STRUCTURE 111 3.3.2
MAGNETIC SUSCEPTIBILITY 113 3.3.3 HEAT CAPACITY 115 3.3.4 POSITIVE MUON
SPIN ROTATION 116 3.3.5 DISTORTED KAGOME LATTICES 117 3.3.6 SUMMARY 120
REFERENCES 120 MAGNETISM IN TDAE-C 60 123 4.1 INTRODUCTION 123 4.2
SYNTHESIS AND STRUCTURE 124 4.2.1 SYNTHESIS 124 4.2.2 THE LATTICE
STRUCTURE 126 4.3 THE ELECTRONIC STRUCTURE 128 4.4 THE MAGNETIC
PROPERTIES 130 4.4.1 THE BULK MAGNETIC PROPERTIES 130 4.4.2 THE
SPIN-GLASS BEHAVIOR OF A -TDAE-C 60 134 4.4.3 ELECTRON-SPIN RESONANCE
135 4.4.4 FERROMAGNETIC RESONANCE 137 4.5 CONCLUSION 144 REFERENCES 145
CONTENTS VII 5 TRIARYLMETHYL AND AMINE RADICALS 149 5.1 INTRODUCTION 149
5.2 MONORADICALS(S = L/2) 149 5.3 DIRADICALS (S = 1) 153 5.4 TRIRADICALS
(S = 3/2) 161 5.5 MONODISPERSE HIGH-SPIN OLIGOMERS (S = 2 - CA. 10) 163
5.6 HIGH-SPIN POLYMERS (UP TO 5 N = CA. 48) 179 5.7 CONCLUSIONS AND
PROSPECTS (BEYOND S = CA. 48?) 182 REFERENCES 185 6 HIGH-SPIN
METAL-ION-CONTAINING MOLECULES 189 6.1 INTRODUCTION 189 6.2
SELF-ASSEMBLY OF MOLECULAR CLUSTERS 190 6.2.1 COMPETING INTERACTIONS AND
SPIN FRUSTRATION 190 6.2.2 THE CARBOXYLATE FAMILY 192 6.2.3 THE
HYDROXYPYRIDONATE FAMILY 197 6.3 HOST-GUEST APPROACH 201 6.3.1
HEXANUCLEAR IRON(III) RINGS 202 6.3.2 HEXANUCLEAR MANGANESE RINGS 203
6.4 STEP-BY-STEP RATIONALE APPROACH 204 6.4.1 COMPLEX AS LIGAND AND
COMPLEX AS METAL 206 6.4.2 PREDICTING THE SPIN GROUND STATE 207 6.4.3
ANTIFERROMAGNETIC APPROACH 208 6.4.4 FERROMAGNETIC APPROACH 211 6.4.5
ROLE OF THE ORGANIC LIGAND 214 6.4.6 MOLECULES WITH TWO SHELLS OF
PARAMAGNETIC SPECIES 217 6.5 CONCLUSION 223 REFERENCES 223 7 ELECTRONIC
STRUCTURE AND MAGNETIC BEHAVIOR IN POLYNUCLEAR TRANSITION-METAL
COMPOUNDS 227 7.1 INTRODUCTION 227 7.2 PHENOMENOLOGICAL DESCRIPTION OF
EXCHANGE COUPLING: THE HEISENBERG HAMILTONIAN 228 7.3 QUALITATIVE MODELS
OF THE EXCHANGE COUPLING MECHANISM 230 7.3.1 ORTHOGONAL MAGNETIC
ORBITALS 230 7.3.2 NATURAL MAGNETIC ORBITALS 234 7.4 QUANTITATIVE
EVALUATION OF EXCHANGE COUPLING CONSTANTS 235 7.4.1 PERTURBATIVE AND
VARIATIONAL CALCULATIONS OF STATE ENERGY DIFFERENCES 236 7.4.2 AB INITIO
CALCULATIONS OF STATE ENERGIES 240 7.4.3 CALCULATIONS USING
BROKEN-SYMMETRY FUNCTIONS 242 7.5 EXCHANGE COUPLING IN POLYNUCLEAR
TRANSITION-METAL COMPLEXES . . . 249 7.5.1 HOMODINUCLEAR COMPOUNDS 249
7.5.2 HETERODINUCLEAR COMPOUNDS 261 VIII CONTENTS 7.5.3 POLYNUCLEAR
COMPOUNDS 263 7.5.4 SOLID-STATE COMPOUNDS: THE CASEOFCU 2 (OH) 3 N0 3
266 REFERENCES 271 8 VALENCE TAUTOMERISM IN DIOXOLENE COMPLEXES OF
COBALT 281 8.1 INTRODUCTION - BISTABILITY, HYSTERESIS, AND
ELECTRONICALLY LABILE MATERIALS 281 8.1.1 BISTABILITY AND HYSTERESIS 281
8.1.2 ELECTRONICALLY LABILE MATERIALS 281 8.2 VALENCE TAUTOMERISM IN
DIOXOLENE COMPLEXES OF COBALT 284 8.2.1 VALENCE TAUTOMERISM - A GENERAL
CHEMICAL DESCRIPTION . . 284 8.2.2 VALENCE TAUTOMERISM - A SIMPLIFIED MO
DESCRIPTION .... 287 8.2.3 VT THERMODYNAMICS 288 8.2.4 EXPERIMENTAL
DETERMINATION OF THERMODYNAMIC PARAMETERS 290 8.2.5 DEPENDENCE OF KYR
EQUILIBRIUM ON ANCILLARY LIGANDS . . . 292 8.2.6 PRESSURE-INDUCED VT 297
8.2.7 LIGHT-INDUCED VT AND RATES OF VT 299 8.2.8 VT COMPLEXES OF OTHER
QUINONE LIGANDS AND REDOX CHEMISTRY OF VT COMPLEXES 300 8.2.9 POLYMERIE
VT MATERIALS 302 8.3 FUTURE DIRECTIONS 303 REFERENCES 304 9
MOLECULE-BASED MAGNETS DERIVED FROM NI 11 AND MN AZIDO BRIDGING LIGAND
AND RELATED COMPOUNDS 307 9.1 INTRODUCTION 307 9.2 SYNTHETIC PROCEDURES
308 9.3 EXCHANGE-COUPLING PARAMETER 309 9.4 MOLECULAR-BASED MAGNETIC
MATERIALS 309 9.5 ONE-DIMENSIONAL SYSTEMS 312 9.5.1 WITH 1,3-AZIDO
BRIDGING LIGANDS (AF, UNIFORM) 312 9.5.2 WITH 1,3-AZIDO BRIDGING LIGANDS
(AF, ALTERNATING) 313 9.5.3 WITH 1,1-AZIDO BRIDGING LIGANDS
(FERROMAGNETIC) 316 9.5.4 WITH 1,3-N 3 AND 1,1-N 3 BRIDGES 319 9.6
TWO-DIMENSIONAL SYSTEMS 322 9.6.1 WITH ONLY AZIDO AS BRIDGING LIGAND 322
9.7 THREE-DIMENSIONAL SYSTEMS 329 9.8 CONCLUSIONS 334 REFERENCES 335 10
OXALATE-BASED 2D AND 3D MAGNETS 339 10.1 INTRODUCTION 339 10.2 BASIC
PRINCIPLES OF SPECIFIC 2D AND 3D NETWORK CONFIGURATIONS . . . 339 10.3
STRUCTURAL STUDIES ON 2D OXALATO BRIDGED COMPOUNDS 344 10.4 MAGNETIC
STUDIES ON 2D OXALATO BRIDGED COMPOUNDS 346 10.5 STRUCTURAL STUDIES ON
3D OXALATO BRIDGED COMPOUNDS 349 CONTENTS IX 10.6 MAGNETIC STUDIES ON 3D
OXALATO BRIDGED COMPOUNDS 352 10.7 SUMMARY 354 REFERENCES 355 11 HYBRID
ORGANIC-INORGANIC MULTILAYER COMPOUNDS: TOWARDS CONTROUABLE AND/OR
SWITCHABLE MAGNETS 357 11.1 INTRODUCTION 357 11.2 HYDROXIDE-BASED
LAYERED COMPOUNDS 358 11.3 ANION-EXCHANGE REACTIONS 360 11.4 INFLUENCE
OF ORGANIC SPACERS IN HYDROXIDE-BASED COMPOUNDS . . . . 361 11.4.1 THE
CU 2 (OH) 3 X SERIES 361 11.4.2 THE CO 2 (OH) 3 X SERIES 364 11.4.3
DIPOLAR INTERACTION AND LONG-RANGE MAGNETIC ORDER 367 11.5 DIFUNCTIONAL
ORGANIC ANIONS CONNECTING MAGNETIC LAYERS 370 11.6 METAL-RADICAL-BASED
LAYERED MAGNETS 376 11.7 CONTROUABLE MAGNETIC PROPERTIES OF LAYERED
COPPER HYDROXIDES . . 380 11.7.1 SOLVENT-MEDIATED MAGNETISM 380 11.7.2
PHOTOISOMERISM OF AZOBENZENES IN LAYERED COPPER HYDROXIDES 384 11.8
LAYERED PEROVSKITE FERROMAGNETS 385 11.8.1 HIGH-PRESSURE EFFECTS 386
11.8.2 SPONTANEOUS MAGNETIZATION IN LAYERED PEROVSKITE FERROMAGNETS 389
REFERENCES 393 12 INTERCALATION-INDUCED MAGNETIZATION IN MPS3 LAYERED
COMPOUNDS 397 12.1 INTRODUCTION AND SCOPE 397 12.2 STRUCTURAL AND
ELECTRONIC ASPECTS 397 12.3 MAGNETIC PROPERTIES OF THE PRISTINE MPS 3
PHASES (M = MN, FE, NI) . 399 12.4 ION-EXCHANGE INTERCALATION INTO THE
MPS3 COMPOUNDS 401 12.5 THE MAGNETIC PROPERTIES OF THE MNPS3
INTERCALATES 402 12.5.1 GENERAL 402 12.5.2 X-RAY AND NEUTRON-DIFFRACTION
STUDY OF SELECTED INTERCALATES 405 12.5.3 A FERRIMAGNETIC MODEL OF THE
MNPS3 INTERCALATES: IMBALANCING OF SPINS 407 12.6 THE MAGNETIC
PROPERTIES OF THE FEPS3 INTERCALATES 410 12.6.1 GENERAL 410 12.6.2
SPECTROSCOPIC CHARACTERIZATION OF THE FEPS3 INTERCALATES . . 413 12.6.3
DISCUSSION ON THE ROLE OF INTERCALATION INTO FEPS3 415 12.6.4 MAGNETIC
PROPERTIES OF IRON-DILUTED FEI_ X CD X PS3 COMPOUNDS 416 12.6.5
DISCUSSION 417 12.7 THE NIPS3-COBALTOCENE INTERCALATION COMPOUND 419 X
CONTENTS 12.8 MULTI-PROPERTY MATERIALS: ASSOCIATING MAGNETISM AND
NON-LINEAR OPTICS 420 12.9 CONCLUSION AND PERSPECTIVES 421 REFERENCES
421 13 TRANSITION METAL ION PHOSPHONATES AS HYBRID ORGANIC-INORGANIC
MAGNETS 425 13.1 INTRODUCTION 425 13.2 SYNTHESIS OF THE LIGANDS 426 13.3
VANADIUM PHOSPHONATES 426 13.3.1 PREPARATION 426 13.3.2 CRYSTAL
STRUCTURES 427 13.3.3 MAGNETIC PROPERTIES 427 13.4 DIVALENT METAL
PHOSPHONATES 430 13.4.1 SYNTHESIS 430 13.4.2 CRYSTAL STRUCTURES 432
13.4.3 MAGNETIC PROPERTIES 437 13.5 METAL(II) DIPHOSPHONATES 449 13.5.1
SYNTHESIS 449 13.5.2 CRYSTAL STRUCTURES 450 13.5.3 MAGNETIC PROPERTIES
452 REFERENCES 454 14 MAGNETIC LANGMUIR-BLODGETT FILMS 457 14.1
INTRODUCTION 457 14.2 THE LANGMUIR-BLODGETT TECHNIQUE 459 14.2.1
FABRICATION OF LANGMUIR-BLODGETT FILMS 459 14.2.2 STRUCTURAL AND
PHYSICAL CHARACTERIZATION OF LANGMUIR AND LB FILMS 461 14.3 MAGNETIC
SYSTEMS: A MOLECULAR APPROACH 462 14.3.1 HYBRID LB FILMS WITH MAGNETIC
CLUSTERS 462 14.3.2 SPIN-TRANSITION SYSTEMS 465 14.3.3 COMMENTS ON
MOLECULAR MAGNETISM IN LB FILMS 468 14.4 EXTENDED SYSTEMS AND
COOPERATIVE EFFECTS 469 14.4.1 LITERALLY TWO-DIMENSIONAL MAGNETS 469
14.4.2 METAL PHOSPHONATE LB FILMS 470 14.4.3 ORGANIC AND INORGANIC DUAL
NETWORK FILMS 473 14.4.4 BIMETALLIC COMPOUNDS 475 14.5 COMPARISON WITH
OTHER LAMELLAR AND COLLOIDAL SYSTEMS 478 14.5.1 HYBRID LAMELLAR SYSTEMS
479 14.5.2 SELF-ORGANIZED MEDIA 480 14.6 CONCLUSION 481 REFERENCES 482
INDEX 485
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| id | DE-604.BV013757523 |
| illustrated | Illustrated |
| indexdate | 2024-07-09T18:51:29Z |
| institution | BVB |
| isbn | 3527303014 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-009405608 |
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| owner_facet | DE-29T DE-703 DE-384 DE-20 DE-91G DE-BY-TUM DE-634 DE-11 DE-188 |
| physical | XIV, 489 S. zahlr. graph. Darst. |
| publishDate | 2001 |
| publishDateSearch | 2001 |
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| publisher | WILEY-VCH |
| record_format | marc |
| spelling | Magnetism: molecules to materials 2 Molecule-based materials ed. by Joel S. Miller ... Molecule based materials Weinheim [u.a.] WILEY-VCH 2001 XIV, 489 S. zahlr. graph. Darst. txt rdacontent n rdamedia nc rdacarrier (DE-588)1071861417 Konferenzschrift gnd-content Miller, Joel S. Sonstige (DE-588)122681541 oth (DE-604)BV013757522 2 GBV Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=009405608&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Magnetism: molecules to materials |
| subject_GND | (DE-588)1071861417 |
| title | Magnetism: molecules to materials |
| title_alt | Molecule based materials |
| title_auth | Magnetism: molecules to materials |
| title_exact_search | Magnetism: molecules to materials |
| title_full | Magnetism: molecules to materials 2 Molecule-based materials ed. by Joel S. Miller ... |
| title_fullStr | Magnetism: molecules to materials 2 Molecule-based materials ed. by Joel S. Miller ... |
| title_full_unstemmed | Magnetism: molecules to materials 2 Molecule-based materials ed. by Joel S. Miller ... |
| title_short | Magnetism: molecules to materials |
| title_sort | magnetism molecules to materials molecule based materials |
| topic_facet | Konferenzschrift |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=009405608&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| volume_link | (DE-604)BV013757522 |
| work_keys_str_mv | AT millerjoels magnetismmoleculestomaterials2 AT millerjoels moleculebasedmaterials |