Chemistry for the 21st century:
Gespeichert in:
| Format: | Buch |
|---|---|
| Sprache: | English |
| Veröffentlicht: |
Weinheim [u.a.]
Wiley-VCH
2001
|
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | XIV, 293 S. Ill., graph. Darst. |
| ISBN: | 3527302352 |
Internformat
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Datensatz im Suchindex
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|---|---|
| adam_text | CHEMISTRY FOR THE 21 ST CENTURY EDITED BY EHUD KEINEM, ISRAEL SCHECHTER
WILEY-VCH WEINHEIM - NEW-YORK - CHICHESTER - BRISBANE - SINGAPORE -
TORONTO CONTENTS 1 SOME REFLECTIONS ON CHEMISTRY - MOLECULAR,
SUPRAMOLECULAR AND BEYOND 1 1.1 FROM STRUCTURE TO INFORMATION. THE
CHALLENGE OF INSTRUCTED CHEMISTRY 1 1.2 STEPS TOWARDS COMPLEXITY 3 1.3
CHEMISTRY AND BIOLOGY, CREATIVITY AND ART 5 2 CHEMICAL SYNTHESIS AND
BIOLOGICAL STUDIES OF THE EPOTHILONES - MICROTUBULE STABILIZING AGENTS
WITH ENHANCED ACTIVITY AGAINST MULTIDRUG-RESISTANT CELL LINES AND TUMORS
8 2.1 INTRODUCTION 8 2.2 TOTAL SYNTHESIS OF EPOTHILONES 9 2.3 FIRST
GENERATION SYNTHESES OF EPOTHILONES A AND B 9 2.4 FIRST GENERATION
SYNTHESIS OF THE ACYL DOMAIN 10 2.5 INVESTIGATION OF C9-C10 BOND
CONSTRUCTION THROUGH RING CLOSING METATHESIS 12 2.6 B-ALKYL SUZUKI
STRATEGY 12 2.7 MACROLACTONIZATION AND MACROALDOLIZATION APPROACHES 16
2.8 A NEW AND MORE EFFICIENT SYNTHESIS OFEPOTHILONE B 18 2.9 DIANION
EQUIVALENTS CORRESPONDING TO THE POLYPROPIONATE DOMAIN OF EPOTHILONE B
19 2.10 B-ALKYL SUZUKI MERGER 20 2.11 STEREOSELECTIVE NOYORI REDUCTION
21 2.12 DISCOVERY OF A REMARKABLE LONG-RANGE EFFECT ON THE DOUBLE
DIASTEREOFACE SELECTIVITY IN AN ALDOL CONDENSATION 22 2.13 PREPARATIONOF
OTHER EPOTHILONE ANALOGS 25 2.14 BIOLOGICAL EVALUATION OF EPOTHILONES 26
2.15 SAR ANALYSIS OF EPOTHILONES: THE ZONE APPROACH 26 2.16 IN VITRO
ANALYSIS COMPARISON TO PACLITAXEL AND RELATED AGENTS 28 2.17 IN VIVO
ANALYSIS: COMPARISONS TO PACLITAXEL 30 2.18 CONCLUSIONS 33 2.19
ACKNOWLEDGEMENTS 33 VI CONTENTS 3 THE SPIROTETRAHYDROFURAN MOTIF: ITS
ROLE IN ENHANCING LIGATION IN BEITED LONOPHORES, BIASING CYCLOHEXANE
CONFORMATION, AND RESTRICTING NUCLEOSIDE/IMUCLEOTIDE CONFORMATION 37 3.1
INTRODUCTION 37 3.2 SYN-L,3,5-ORIENTATION ON A CYCLOHEXANE CORE 40 3.3
MAXIMALLY SUBSTITUTED HEXA(SPIROTETRAHYDROFURANYL)-CYCLOHEXANES 43 3.4
SPIROCYCLIC RESTRICTION OF NUCLEOSIDES/NUCLEOTIDES 49 3.5
ACKNOWLEDGEMENT 51 4 HETEROGENEOUS CATALYSIS: FROM BLACK ART TO ATOMIC
UNDERSTANDING 54 4.1 INTRODUCTION 54 4.2 A CASE STUDY: AMMONIA SYNTHESIS
55 4.3 THE SURFACE SCIENCE APPROACH 57 4.4 THE ATOMIC MECHANISM OF A
CATALYTIC REACTION: OXIDATION OF CARBON MONOXIDE 62 4.5 FURTHER ASPECTS
66 5 DRUGS FOR A NEW MILLENNIUM 70 5.1 INTRODUCTION 70 5.2 CELL DEATH 70
5.3 STROKE AND MYOCARDIAL INFARCT 71 5.4 SCHIZOPHRENIA 75 5.4.1
NEUROLEPTIC DRUG DEVELOPMENT 76 5.4.2 DRUG PSYCHOSES 79 5.5 DRUGS OF
ABUSE 81 5.5.1 DEFMITIONS AND VARIETIES 81 5.5.2 APPROACHES TO
TREATMENT: FOCUS ON COCAINE 83 5.6 CONCLUSIONS AND NEW DIRECTIONS 85 5.7
ACKNOWLEDGEMENTS 87 6 PROTEIN FOLDING AND BEYOND 89 6.1 INTRODUCTION 89
6.1.1 COMPUTATIONAL PROTEIN FOLDING 91 6.1.2 AU-ATOM SIMULATIONS OF
PROTEIN UNFOLDING AND SHORT PEPTIDE FOLDING 92 6.2 ALL-ATOM SIMULATIONS
OF FOLDING OF SMALL PROTEINS 93 6.2.1 CONCOMITANT HYDROPHOBIE COLLAPSE
AND PARTIAL HELIX FORMATION 93 6.2.2 A MARGINALLY STABLE INTERMEDIATE
STATE 94 6.3 A PERSPECTIVE VIEW 96 7 THE ENZYMOLOGY OF BIOLOGICAL
NITROGEN FIXATION 102 7.1 EARLY HISTORY 102 7.2 PRACTICAL APPLICATIONS
103 7.3 BIOCHEMISTRY OF N 2 FIXATION 104 7.4 FIRST PRODUCTOFN 2 FIXATION
105 7.5 STUDIES WITH 15 N AS A TRACER 105 7.6 N 2 FIXATION WITH
CELL-FREE PREPARATIONS 206 7.7 NITROGENASE CONSISTS OF TWO PROTEINS 107
7.8 ATP FURNISHES ENERGY FOR FIXATION 108 7.9 H 2 AN OBLIGATORY PRODUCT
OF THE NITROGENASE REACTION 108 7.10 N 2 AND HD FORMATION 109 7.11
ELECTRON TRANSFER SEQUENCE 109 7.12 ALTERNATIVE SUBSTRATES 110 7.13 N 2
FIXATION IN NON-LEGUMINOUS PLANTS 110 7.14 CONTROL OF NITROGENASE 111
7.15 MAGNITUDE OF CHEMICAL AND BIOLOGICALN 2 FIXATION 111 7.16
ASSOCIATIVE BIOLOGICAL N 2 FIXATION 112 7.17 GENETICSOF BIOLOGICAL N 2
FIXATION 112 7.18 COMPOSITION AND STRUCTUREOF NITROGENASES 113 7.19
SELECTIONOFN 2 FIXERS 113 8 THE CHEMISTRY OF NITROGEN IN SOILS 117 8.1
INTRODUCTION 117 8.2 NITROGEN FIXATION AND ENSUING REACTIONS 117 8.3
AMINO ACIDS, AMINO SUGARS, AND AMMONIA IN SOILS 118 8.4 NUCLEIC ACID
BASES IN SOILS 121 8.5 BIOAVAILABILITY OF THE NH-N FRACTION 121 8.6
CHEMISTRY OF THE UH-N FRACTION 122 8.7 CHEMISTRY OF THE NH-N FRACTION
122 8.8 PYROLYSIS-FIELD IONIZATION MASS SPECTROMETRY (PY-FIMS) AND
CURIE-POINT PYROLYSIS-GAS CHROMATOGRAPHY/MASS SPECTROMETRY (CPPY-GC/MS)
OF SOILS 124 8.9 ORIGINS OF MAJOR N COMPOUNDS IDENTIFIED 325 8.10 15 NMR
ANALYSIS OF SOILS 126 8.11 DISTRIBUTION OFN IN SOILS 127 8.12 CONCLUDING
COMMENTS 127 9 SPHERICAL MOLECUIAR ASSEMBLIES: A CLASS OF HOSTS FOR THE
NEXT MILLENNIUM 130 9.1 INTRODUCTION 130 9.1.1 SUPRAMOLECULAR CHEMISTRY
130 9.1.2 TOWARDS SUPRAMOLECULAR SYNTHESIS 131 9.1.3 SELF-ASSEMBLY 131
9.2 OVERVIEW 132 9.3 A SPHERICAL MOLECUIAR ASSEMBLY HELD TOGETHER BY 60
HYDROGEN BONDS 132 9.3.1 POLYHEDRON MODEL - SNUB CUBE 133 9.4 GENERAL
PRINCIPLES FOR SPHERICAL HOST DESIGN 234 9.4.1 SPHEROID DESIGN 134 9.4.2
SELF-ASSEMBLY 134 9.4.3 SUBUNITS FOR SPHEROID DESIGN AND SELF-ASSEMBLY
135 9.4.4 PIATONIC SOLIDS 137 CONTENTS VII VIII CONTENTS 9.4.5
ARCHIMEDEAN SOLIDS 238 9.4.6 MODELS FOR SPHEROID DESIGN 139 9.5 EXAMPLES
FROM THE LABORATORY AND FROM NATURE 140 9.5.1 PIATONIC SOLIDS 140
9.5.1.1 TETRAHEDRAL SYSTEMS (T D , T H , T) 140 9.5.1.2 OCTAHEDRAL
SYSTEMS (O H , O) 141 9.5.1.3 ICOSAHEDRAL SYSTEMS (I H , I) 142 9.5.2
ARCHIMEDEAN SOLIDS 143 9.5.2.1 TRUNCTATED TETRAHEDRON (I) 143 9.5.2.2
CUBOCTAHEDRON (2) 144 9.5.2.3 TRUNCTATED OCTAHEDRON (4) 144 9.5.2.4
RHOMBICUBOCTAHEDRON (5) 145 9.5.2.5 SNUBCUBE(6) 245 9.5.2.6 TRUNCTATED
ICOSAHEDRON (10) 245 9.5.3 ARCHIMEDEAN DUALS AND IRREGULAER POLYGONS 246
9.5.3.1 RHOMBIC DODECAHEDRON (2) 246 9.5.4 IRREGULAER POLYGONS 247 9.6
WHY THE PIATONIC AND ARCHIMEDEAN SOLIDS? 247 9.7 CONCLUSION 248 10 THE
COMBINATORIAL APPROACH TO MATERIALS DISCOVERY 252 10.1 INTRODUCTION 252
10.2 HISTORY OF RAPID SYNTHESIS APPROACHES IN MATERIALS RESEARCH 252
10.2.1 EARLY WORK 252 10.2.3 RECENT INNOVATIONS 254 10.2.4 THE
CONTINUOUS COMPOSITIONAL SPREAD (CCS) APPROACH 256 10.3 SYSTEMATIZED
SEARCH FOR A NEW HIGH-E THIN-FILM MATERIAL 258 10.3.1 GENERAL
CONSIDERATIONS FOR INVESTIGATING NEW MATERIALS SYSTEMS 258 10.3.2 THE
PROBLEM: FINDING NEW HIGH DIELECTRIC-CONSTANT MATERIALS 259 10.3.3
MEASUREMENT STRATEGY AND FIGUREOF MERIT 262 10.3.4 ELECTRICAL AND
COMPOSITIONAL EVALUATION 262 10.4 IDENTIFICATION OFA PROMISING CANDIDATE
AND DISCUSSION OF TRENDS 264 10.4.1 INITIAL SURVEY 264 10.4.2 THE
ZR-SN-TI-0 SYSTEM 264 10.4.3 SINGLE-TARGET SYNTHESIS AND DETAILED
ELECTRICAL CHARACTERIZATION 267 10.4.4 HFTT ANALOG 168 10.4.5 OTHER
SYSTEMS 168 10.4.6 OTHER PROBLEMS FOR WHICH A COMBINATORIAL APPROACH IS
WELL SUITED 272 10.4.7 NEW MAGNETIC MATERIALS 272 10.4.8 SUPERCONDUCTORS
172 10.4.9 THERMOELECTRIC MATERIALS 272 10.4.10 PIEZOELECTRIC MATERIALS
172 10.4.11 FERROELECTRIC MATERIALS 273 10.4.12 OPTICAL MATERIALS 273
10.4.13 CATALYSTS 173 10.5 CONCLUDING COMMENTS 173 11 ON ONE HAND BUT
NOT THE OTHER: THE CHALLENGE OF THE ORIGIN AND SURVIVAL OF HOMOCHIRALITY
IN PREBIOTIC CHEMISTRY 175 11.1 SYMMETRY BREAKING AND CHIRAL INDUCTION
177 11.1.1 IS IT INTRINSIC? 177 11.1.2 IS IT FLUCTUATIONAL? 179 11.1.3
IS IT EXTRINSIC? 181 11.2 EXPERIMENTAL STUDIES OF CHIRAL INDUCTION 181
11.2.1 INTRINSIC MECHANISMS 182 11.2.2 FLUCTUATIONAL MECHANISMS 183
11.2.3 EXTRINSIC MECHANISMS 385 11.3 CHIRAL AMPLIFICATION AND TAKEOVER
386 11.3.1 AUTOAMPLIFICATION BY POLYMERIZATION/DEPOLYMERIZATION 187
11.3.2 ENANTIOMERIC AMPLIFICATION BY CHANGE OF PHASE 189 11.3.3
METAL-ASSISTED ENANTIOMERIC AMPLIFICATION 389 11.3.4 AMPLIFICATION BY
MOLECULAR PROPAGATION FROM A CHIRAL CENTER 393 11.3.5 AMPLIFICATION BY
CPL PHOTOINDUCTION 392 11.4 THE SEQUESTRATION OFCHIRALITY 193 11.4.1
POROUS MINERALS 394 11.4.2 AMPHIPHILIC VESICLES 195 11.5 SETTING THE
SCENE FOR LIFE 396 11.6 THE ROCKY ROAD TO LIFE? 198 11.7 CONCLUDING
REMARKS 202 11.8 ACKNOWLEDGMENTS 202 12 CHEMICAL REACTION DYNAMICS LOOKS
TO THE UNDERSTANDING OF COMPLEX SYSTEMS 209 ACKNOWLEDGEMENT 217 13 THE
PAST, PRESENT, AND FUTURE OF QUANTUM CHEMISTRY 219 INTRODUCTION 219 13.2
THE HISTORY AND PRESENT STATUS OF QUANTUM CHEMISTRY 223 13.2.1 THE
GAUSSIAN PROGRAMS 223 13.2.2 COUPLED CLUSTER THEORY 222 13.2.3
MULTIREFERENCE APPROACHES 224 13.2.4 ANALYTIC GRADIENT TECHNIQUES 226
13.2.5 DENSITY-FUNCTIONAL THEORY 228 13.2.6 INTEGRAL-DIRECT METHODS 230
13.3 THE FUTURE OF QUANTUM CHEMISTRY 231 13.3.1 EXTENSIONS TO LARGE
SYSTEMS 232 13.3.2 PURSUIT OF SPECTROSCOPIC ACCURACY 235 13.3.3
POTENTIAL ENERGY SURFACES FOR REACTION DYNAMICS 238 13.4 CONCLUSIONS 243
CONTENTS IX X CONTENTS 13.5 ACKNOWLEDGEMENTS 242 13.6 APPENDIX:
NOMENCLATURE 242 14 QUANTUM ALCHEMY 247 14.1 FROM ALCHEMY TO QUANTUM
THEORY 247 14.2 APPLYING QUANTUM THEORY 248 14.3 TOTAL ENERGY
CALCULATIONS 256 14.4 NOVEL MATERIALS 262 14.5 THE FUTURE 266
ACKNOWLEDGEMENTS 268 15 QUANTUM THEORY PROJECT 271 15.1 INTRODUCTION 271
15.2 BACKGROUND 271 15.3 WAVE FUNCTION THEORY 274 15.4 DENSITY
FUNCTIONAL THEORY 278 15.5 AB INITIO DENSITY FUNCTIONAL THEORY 281
15.5.1 EXACT EXCHANGE 281 15.5.2 EXACT CORRELATION 283 ACKNOWLEDGEMENTS
284 INDEX 287
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| id | DE-604.BV013486137 |
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| indexdate | 2024-07-09T18:46:42Z |
| institution | BVB |
| isbn | 3527302352 |
| language | English |
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| spelling | Chemistry for the 21st century ed. by Ehud Keinan ... Weinheim [u.a.] Wiley-VCH 2001 XIV, 293 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Chemie Chemistry Chemistry trends Chemie (DE-588)4009816-3 gnd rswk-swf (DE-588)4143413-4 Aufsatzsammlung gnd-content Chemie (DE-588)4009816-3 s DE-604 Keinan, Ehud Sonstige (DE-588)123115477 oth GBV Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=009205070&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Chemistry for the 21st century Chemie Chemistry Chemistry trends Chemie (DE-588)4009816-3 gnd |
| subject_GND | (DE-588)4009816-3 (DE-588)4143413-4 |
| title | Chemistry for the 21st century |
| title_auth | Chemistry for the 21st century |
| title_exact_search | Chemistry for the 21st century |
| title_full | Chemistry for the 21st century ed. by Ehud Keinan ... |
| title_fullStr | Chemistry for the 21st century ed. by Ehud Keinan ... |
| title_full_unstemmed | Chemistry for the 21st century ed. by Ehud Keinan ... |
| title_short | Chemistry for the 21st century |
| title_sort | chemistry for the 21st century |
| topic | Chemie Chemistry Chemistry trends Chemie (DE-588)4009816-3 gnd |
| topic_facet | Chemie Chemistry Chemistry trends Aufsatzsammlung |
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