Stimulating concepts in chemistry:
Gespeichert in:
| Format: | Buch |
|---|---|
| Sprache: | English |
| Veröffentlicht: |
Weinheim [u.a.]
Wiley-VCH
2000
|
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | XVII, 396 S. Ill., graph. Darst. |
| ISBN: | 3527299785 |
Internformat
MARC
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| 245 | 1 | 0 | |a Stimulating concepts in chemistry |c ed.: Fritz Vögtle ... |
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Datensatz im Suchindex
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| adam_text | STIMULATING CONCEPTS IN CHEMISTRY EDITORS: FRITZ VOEGTLE, J. FRAESER
STODDART, MASAKATSU SHIBASAKI WILEY-VCH WEINHEIM * NEW YORK *
CHICHESTER BRISBANE * SINGAPORE * TORONTO TABLE OF CONTENTS NEW TYPES OF
LEWIS ACIDS AS WATER-STABLE CATALYSTS HAVE BEEN DEVELOPED. THESE LEWIS
ACIDS ACTIVATE SUB- STRATES SUCH AS ALDEHYDES EFFICIENTLY IN AQUEOUS
MEDIA. FURTHERMORE, SURFACTANT- AIDED LEWIS ACID CATALYSIS HAS ALSO BEEN
USED FOR REAC- TIONS IN WATER WITHOUT USING ANY ORGANIC SOLVENTS. H 2 Q
FAH OH 2 ,-M N+ ---OH 2 I OH, S. KOBAYASHI, K. MANABE LEWIS ACID
CATALYSIS IN AQUEOUS MEDIA SUPERCRITICAL FLUID (SCF) WITH THE BENEFICIAL
EFFECTS OF BOTH LIQUID- AND GAS-PHASE CHEMISTRY IS AN EMERGING REACTION
MEDIUM FOR MANY SCIENTIFIC AND TECHNICAL REA- SONS. THE REACTION RATE
AND SELCECTIVITY ARE READILY TUN- ABLE BY A SUBTLE CHANGE IN PRESSURE
AND TEMPERATURE. : SOLUTE MOLECULE O : SOLVENT MOLECULE R. NOYORI, T.
IKARIYA SUPERCRITICAL FLUIDS FOR ORGANIC SYNTHESIS 13 METHODS FOR WORKUP
AND PURIFICATION OF ORGANIC REAC- TION MIXTURES ARE BEGINNING TO CHANGE
AS SYNTHESIS AND SEPARATION MERGE FORCES. HIGHLY FLUORINATED, OR FLUOR-
OUS, MOLECULES OFFER A NUM- BER OF ATTRACTIVE FEATURES IN BOTH
TRADITIONAL AND PARALLEL SYNTHESIS VENUES. (FVA+B (F) = HIGHLY
FLUORINATED TAG -C + D WORKUP PHASE PHASE D. P. CURRAN FLUOROUS
TECHNIQUES U (P)_C FOR THE SYNTHESIS OF ORGANIC MOLECULES: A UNIFIED
STRATEGY FOR REACTION AND SEPARA- TION 25 DOMINO REACTIONS PRESENT A
MODERN APPROACH IN ORGANIC SYNTHESIS SINCE THEY ALLOW THE PREPARATION OF
COMPLEX MOLECULES STARTING FROM SIM- PLE SUBSTRATE IN A FEW STEPS AND IN
MANY CASES WITH HIGH STEREOSELECTIVITY. AAOREOVER, AS MULTI-COMPONENT
TRANS- FORMATION THEY ARE HIGHLY SUITABLE FOR COMBINATORIAL CHEMISTRY
AND GIVE ACCESS TO LIBRARIES OF GREAT DIVERSITY. CHO L. F. TIETZE, F.
HAUNERT DOMINO REACTION IN ORGANIC SYNTHESIS. AN APPROACH TO EFFICIENCY,
ELEGANCE, ECOLOGICAL BENEFIT, ECONOMIC ADVANTAGE AND PRESERVATION OF OUR
RESOURCES IN CHEMICAL TRANSFORMATIONS 39 VI TABLE OF CONTENTS
COMBINATORIAL CHEMISTRY HAS PLAYED AN INCREASINGLY IMPORTANT ROLE IN THE
FIELD OF DRUG DISCOVERY FOR IDENTIFICA- TION AND OPTIMIZATION OF DRUG
LEADS. COMBINATORIAL METHODS PROVIDE RAPID ACCESS TO LARGE NUMBERS OF
COMPOUNDS FOR TESTING. SHOWN IS A GENERAL SCHE- MATIC OF A COMBINATORIAL
LIBRARY PREPARED FROM A SMALL SET OF BUILDING BLOCKS. * IH* ++ M O +0
O-O *- * * *-# #-# *-* D +U #-D *-D 4 [4X4 = 16] D* QO D-# OD A. LEE,
J. W. SZEWCZYK, J. A. ELLMAN COMBINATORIAL I FOR DRUG DEVELOPMENT 65
THEORETICAL CATALYTIC ARRAYS CALLED THEOZYMES CAN BE USED TO
QUANTITATE THE EFFECTS OF SPECIFIC NONCOVAL- ENT CATALYST TRANSITION
STATE INTERACTIONS ON REACTION RATES. THIS STRATEGY HAS BEEN USED TO
UNDERSTAND AND PRE- DICT CATALYSIS BY BOTH BIOLOG- ICAL AND SYNTHETIC
CATALYSTS. I- I TRANSITION T STATE MPMM I N WMM , R THEOZYME 1 { M M T
PRODUCT D. J. TANTILLO, K. N. HOUK THEOZYMES AND CATALYST DESIGN 79
STERICALLY AND ELECTRONICAILY UNSYMMETRICAL P,N- IGANDS HAVE BEEN
DESIGNED TO INCORPORATE TWO TYPES OF COORDINATING UNITS, E.G. A
PHOSPHINE GROUP AND A NITROGEN-CONTAINING HETERO- CYCLE. THESE HYBRID
LIGANDS LEAD TO SUPERIOR RESULTS IN VARIOUS METAL-CATALYZED PRO- CESSES
AND ALLOW A SYSTEM- ATIC FINE TUNING OF A GENER- ALIZED STRUCTURE TO
SUIT A SPE- CIFIC PROCESS. A. C. HUMPHRIES, A. PFALTZ ENANTIOSELECTIVE
CATALYSIS USING STERICALLY AND ELECTRONICAILY UNSYMMETRICAL LIGANDS 89
THE SUCCESSFUI DEVEIOPMENT OF THE ASYMMETRIC TWO- CENTER CATALYSIS HAS
OPENED UP A NEW FIELD IN ASYMMET- RIC SYNTHESIS. IT HAS BEE ESPECIALLY
FRUITFUL IN MICHAEL ADDITIONS AND ALDOL REAC- TIONS. M. SHIBASAKI
ASYMMETRIC TWO- CENTER CATALYSIS 105 ~ ;I ^N:LI§!ILP;S ; ASYMMETRIC
PHASE-TRANSFER CATALYSIS USING CHIRAL NONRA- CEMIC ONIUM SALTS OR CROWN
ETHERS HAS NOW GROWN INTO A PRACTICAL METHOD WHEREBY A LARGE NUMBER OF
REACTIONS CAN BE PERFORMED AND SOME OPTICALLY PURE COMPOUNDS CAN BE
PRODUCED EFFECTIVELY ON A LARGE SCALE. (REACTIONJ Y-CH.-Z R-X, Q^X 1
OH, SOLVENT R T. SHIOIRI, Y-CH-Z S. ARAI ASYMMETRIC PHASE TRANSFER
CATALYSIS 123 TABLE OF CONTENTS VII METAL-CATALYZED ENANTIOSE- LECTIVE
REACTIONS ARE USED IN THE SYNTHESIS OF COMPLEX ORGANIC MOLECULES. THESE
TRANSFORMATIONS OFFER COST- EFFECTIVE, HIGHLY SELECTIVE ALTERNATIVES TO
THE MORE CLASSICAL METHODS. ADDITIONAL LEVELS OF EFFICIENCY ARE ACHIEVED
WHEN VARIOUS CATA- LYTIC REACTIONS ARE USED SUCCESSIVELY. 20MOL% CHIRAL
CATALYST 1 COV^COV 10MOL% CATALYST 2 0 HO» CT A-Q3 V-F0H WODESNTOL 2MOL%
CATALYST 3 A. H. HOVEYDA ASYMMETRIE CATALYSIS IN TARGET-ORIENTED
SYNTHESIS 145 THE HYPOTHETICAL FULLERENE - ACETYLENE HYBRID AT RIGHT
SYMBOLIZES THE EXCITING PROSPECTS THAT HAVE ARISEN FROM THE DISCOVERY OF
FULLER- ENES, AND THE PROFOUND CHANGES THEY HAVE INDUCED IN OUR VIEW OF
ACETYLENE AND CARBON ALLOTROPE CHEMISTRY. THE PREPARATION OF MOLECU- LAR
AND POLYMERIC ACETYLENIC CARBON ALLOTROPES, AS WELL AS CARBON-RICH
NANOMETER-SIZED STRUETURES, HAS OPENED UP NEW AVENUES IN FUNDAMEN- TAL
AND TECHNOLOGICAL RESEARCH AT THE INTERFACE OF CHEMISTRY WITH MATERIALS
SCIENCE. Y. RUBIN, F. DIEDERICH FROM FULLERENES TO NOVEL CARBON
ALLOTROPES: EXCITING PROSPECTS FOR ORGANIC SYNTHESIS 163 IN DENDRIMER
CHEMISTRY THERE ARE DIFFERENT WAYS TO DISPLAY FUNCTIONALITIES. ON THE
ONE HAND, A CENTRAL FUNCTIONAL UNIT CAN BE DEN- DRYLATED TO CHANGE SOME
OF ITS PROPERTIES. ON THE OTHER HAND, IT IS POSSIBLE TO ATTACH
FUNCTIONAL GROUPS TO THE PERIPHERY OF A DENDRIMER SKELETON, I.E., THE
FUNCTIONAL- ITY CAN BE MULTIPLIED. S = FUNCTIONAL UNIT S. GESTERMANN, R.
HESSE, B. WINDISCH, F. VOEGTLE DENDRITIC ARCHITECTURES 187
SELF-ASSEMBLING CAPSULES ARE ABOUT TO LEAVE THE PLAY- GROUND OF BASIC
RESEARCH AND BEGIN THEIR CAREER IN MATERIALS SCIENCES. THE LONG WAY FROM
THE PRINCIPLES OF SELF-ORGANIZATION THROUGH NONCOVALENT INTERACTIONS AND
THE FILLING OF SPACE INSIDE HOST MOLECULES VIA CHIRAL RECOGNITION AND
CATAL- YSIS IN REACTION VESSELS TO HYDROGEN-BONDED LIQUID CRYSTALS AND
FIBERS FORMS THE BACKBONE OF THIS REVIEW. C. A. SCHALLEY, J. REBEK
CHEMICAL ENCAPSULATION IN SELF-ASSEMBLING CAPSULES 199 VIII TABLE OF
CONTENTS KINETICALLY STABLE SUPER- ARCHITECTURES CAN BE ASSEM- BLED BY
RELYING UPON BOTH NONCOVALENT BONDS AND MECHANICAL COERCION. THUS, AT
ELEVATED TEMPERATURES, ROTAXANE-LIKE COMPLEXES (A) ARE GENERATED WHEN
MACRO- CYCLES SLIP OVER THE STOPPERS OF CHEMICAL DUMBBELLS, WHILE
HEMICARCEPLEXES (B) ARE CREATED WHEN GUESTS SQUEEZE THROUGH THE PORTALS
OF HEMICARCERANDS. M. C. T. FYFE, F. M. RAYMO, J. F. STODDART
SLIPPAGE AND CONSTRICTIVE BINDING 211 SOFT AND TOPOLOGICALLY ADAPTABLE
SUPRAMOLECULAR MODULES THAT ALLOW HOST LAT- TICES TO ACHIEVE DENSE PACK-
ING THROUGH LOW-ENERGY DEFORMATIONS, WHILE RETAIN- ING THEIR INHERENT
DIMEN- SIONALITY AND SUPRAMOLECULAR CONNECTIVITY, CAN FACILITATE THE
SYSTEMATIC DESIGN OF MOLECULAR INCLUSION COM- POUNDS. THIS IS DEMON-
STRATED BY THE ABILITY TO PRE- DICT AND MAINTAIN ARCHITEC- TURAL CONTROL
IN A SERIES OF LAMELLAR HOST FRAMEWORKS. K. T. HOLMAN, M. D. WARD
CRYSTAL ENGINEERING WITH SOFT AND TOPOLOGICALLY ADAPTABLE MOLECULAR HOST
FRAMEWORKS 221 SYNTHETIC ROUTES TO PRECISELY DEFINED MOLECULAR WIRES AND
DEVICES ARE DESCRIBED ALONG WITH PROCEDURES FOR TESTING THEIR ELECTRONIC
PROPERTIES. 0 2 N^ NH 2 J. M. TOUR MOLECULAR WIRES AND DEVICES 237 THE
EXTENSION OF THE CON- CEPTS OF DEVICE AND MACHINE TO THE MOLECULAR LEVEL
IS OF GREAT SCIENTIFIC INTEREST SINCE IT INTRODUCES NEW IDEAS INTO THE
FIELD OF CHEMISTRY AND STIMULATES THE INGENUITY OF RESEARCHERS ENGAGED
IN THE EMERGING FIELDS OF NANOSCI- ENCE AND NANOTECHNOLOGY. MOLECULAR
COMPONENTS 1 * SIMPLE ACSS SUPRAMOLECULAR SYSTEM ^ & Q O ^ V.
BALZANI, A. CREDI, M. VENTURI MOLECULAR-LEVEL DEVICES AND MACHINES 255
CORNPIEX FUNCIION TABLE OF CONTENTS IX LONG-RANGE ELECTRON AND ENERGY
TRANSFER MAY TAKE PLACE OVER LARGE DISTANCES BY A THROUGH-BOND OR
SUPEREX- CHANGE MECHANISM, IN WHICH THE ELECTRON TUNNELS THROUGH THE
INTERVENING MEDIUM. EXAMPLES INCLUDE ELECTRON TRANSFER THROUGH SATURED
HYDROCARBON BRIDGES THROUGH SOLVENT MOLECULES AND THROUGH N-STACKS OF
BASE PAIRS IN DNA. E ET OVER 13.5 A *MEO MEO DMN DCV CN ~CN ELECTRON
MOVES THROUGH C* BONDS DMN T7T ., DCV A AND A BONDS, M. N. PADDON-ROW
ELECTRON AND ENERGY TRANSFER 267 THE SUPRAMOLECULAR SYNTHON IS THE
SUPRAMOLECULAR EQUI- VALENT OF THE FUNCTIONAL GROUP AND IS AS USEFUL IN
SUPRA- MOLECULAR CHEMISTRY AS IS THE FUNCTIONAL GROUP IN MOLECU- LAR
CHEMISTRY. SYNTHONS ARE SMALL REPETITIVE UNITS THAT ECONOMICALLY, YET
FULLY, CAP- TURE THE ESSENCE OF A CRYSTAL STRUCTURE. ^ ; SYNTHOI G. R.
DESIRAJU THE SUPRAMOLECULAR SYNTHON IN CRYSTAL ENGINEERING 293
CONNECTING LUMOPHORES AND RECEPTORS WITH SPACERS PER- MITS THE BUILD-UP
OF MODULAR SYSTEMS OF INCREASING LOGICAL COMPLEXITY. EVEN THE SIM- PLEST
OF THESE SYSTEMS CAN BE POWERFUL MOLECULAR SENSORS. LIGHT POWER LIGHT
OUTPUT CHEMICAI INPUT A. P. DE SILVA, D. B. FOX, T. S. MOODY LUMINESCENT
LOGIC AND SENSING 307 NANOCHEMISTRY CREATE S NEW OPPORTUNITIES FOR
CHEMISTRY, SINCE MOLECULAR CHARACTERIS- TICS ARE OBTAINED WHICH NO
LONGER RESEMBLE AN ENSEMBLE AVERAGE. THE TASK OF NANO- CHEMISTRY IS TO
PROVIDE AN INSIGHT INTO STRUCTURE AND FUNCTION AT A MOLECULAR LEVEL. S.
BECKER, K. MUELLEN NANOCHEMISTRY - ARCHITECTURE AT THE MESOSCALE 317 THIS
CHAPTER FOCUSES ON MIMICS BASED ON NATURAL ENZYMES AND OTHER BIOPOLY-
MERS, SYNTHETIC MACROMOLE- CULES AND SMALL-MOLECULE HOST-GUEST
INTERACTIONS. NIMM PU-PYHM FF I I *HPYU AR 1 R G G C C T A J G CTA C
5 -RIBO 3 -DEOXYRIBO A. J. KIRBY ENZYME MIMICS 341 RECENT DEVELOPMENTS
IN ENZYME INHIBITOR DESIGN ARE REVIEWED, WITH PARTICULAR EMPHASIS ON THE
DISTAL BINDING ANALOG APPROACH. DISTAL BINDING SITE I ENZYME ACTIVE
SITE * ENZYME-INHIBITOR COMPLEX K. D. KREUTTER, C.-H. WONG ASYMMETRIE
TWO-ENZYME INHIBITORS 355 X TABLE OF CONTENTS THIS CHAPTER HIGHLIGHTS
THE INTERPLAY BETWEEN ORGANIC SYNTHESIS, BIOPHYSICS AND CELL BIOLOGY IN
THE STUDY OF PROTEIN LIPIDATION AND ITS REL- EVANCE TO TARGETING
PROTEINS TOWARDS THE PLASMA MEM- BRANE OF CELLS IN PRECISE MOLECULAR
DETAIL. D. KADEREIT, J. KUHLMANN, H. WALDMANN ORGANIC SYNTHESIS AND CELL
BIOLOGY 369 BIOPBYSICAL CHEMISUY MOLECULAR BIOLOGV
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| genre_facet | Aufsatzsammlung |
| id | DE-604.BV013431222 |
| illustrated | Illustrated |
| indexdate | 2024-07-09T18:45:48Z |
| institution | BVB |
| isbn | 3527299785 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-009166941 |
| oclc_num | 247824277 |
| open_access_boolean | |
| owner | DE-20 DE-29T DE-703 DE-355 DE-BY-UBR DE-19 DE-BY-UBM DE-1046 DE-526 DE-634 DE-11 DE-188 |
| owner_facet | DE-20 DE-29T DE-703 DE-355 DE-BY-UBR DE-19 DE-BY-UBM DE-1046 DE-526 DE-634 DE-11 DE-188 |
| physical | XVII, 396 S. Ill., graph. Darst. |
| publishDate | 2000 |
| publishDateSearch | 2000 |
| publishDateSort | 2000 |
| publisher | Wiley-VCH |
| record_format | marc |
| spelling | Stimulating concepts in chemistry ed.: Fritz Vögtle ... Weinheim [u.a.] Wiley-VCH 2000 XVII, 396 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Chemie - Aufsatzsammlung Chemie Chemistry Chemie (DE-588)4009816-3 gnd rswk-swf (DE-588)4143413-4 Aufsatzsammlung gnd-content Chemie (DE-588)4009816-3 s DE-604 Vögtle, Fritz 1939- Sonstige (DE-588)106068520 oth GBV Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=009166941&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Stimulating concepts in chemistry Chemie - Aufsatzsammlung Chemie Chemistry Chemie (DE-588)4009816-3 gnd |
| subject_GND | (DE-588)4009816-3 (DE-588)4143413-4 |
| title | Stimulating concepts in chemistry |
| title_auth | Stimulating concepts in chemistry |
| title_exact_search | Stimulating concepts in chemistry |
| title_full | Stimulating concepts in chemistry ed.: Fritz Vögtle ... |
| title_fullStr | Stimulating concepts in chemistry ed.: Fritz Vögtle ... |
| title_full_unstemmed | Stimulating concepts in chemistry ed.: Fritz Vögtle ... |
| title_short | Stimulating concepts in chemistry |
| title_sort | stimulating concepts in chemistry |
| topic | Chemie - Aufsatzsammlung Chemie Chemistry Chemie (DE-588)4009816-3 gnd |
| topic_facet | Chemie - Aufsatzsammlung Chemie Chemistry Aufsatzsammlung |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=009166941&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT vogtlefritz stimulatingconceptsinchemistry |