High resolution laser photoionization and photoelectron studies:
Gespeichert in:
| Format: | Buch |
|---|---|
| Sprache: | English |
| Veröffentlicht: |
Chichester [u.a.]
Wiley
1995
|
| Schriftenreihe: | Wiley series in ion chemistry and physics
|
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | XVI, 509 S. graph. Darst. |
| ISBN: | 0471941581 |
Internformat
MARC
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| 245 | 1 | 0 | |a High resolution laser photoionization and photoelectron studies |c ed. by Ivan Powis ... |
| 264 | 1 | |a Chichester [u.a.] |b Wiley |c 1995 | |
| 300 | |a XVI, 509 S. |b graph. Darst. | ||
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| 650 | 7 | |a Spectroscopie à haute résolution |2 ram | |
| 650 | 4 | |a High resolution spectroscopy | |
| 650 | 4 | |a Molecular spectroscopy | |
| 650 | 4 | |a Photoelectron spectroscopy | |
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Datensatz im Suchindex
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| adam_text | HIGH RESOLUTION LASER PHOTOIONIZATION AND PHOTOELECTRON STUDIE S WILEY
SERIES IN ION CHEMISTRY AND PHYSICS EDITED BY IVAN POWIS DEPARTMENT OF
CHEMISTRY, UNIVERSITY OF NOTTINGHAM, NOTTINGHAM, ENGLAND, UK TOMAS BAER
DEPARTMENT OF CHEMISTRY, THE UNIVERSITY OF NORTH CAROLINA AT CHAPEL
HILL, CHAPEL HILL, NORTH CAROLINA, USA CHEUK-YIU NG AMES LABORATORY,
USDOE, AND DEPARTMENT OF CHEMISTRY, IOWA STATE UNIVERSITY, AMES , IOWA,
USA LIST OF CONTRIBUTORS XI I I PREFACE XV CHAPTER 1 AN HISTORICAL
INTRODUCTION TO THRESHOLD PHOTOIONIZATION 1 T. BAER AND P-M GUYON 1 .1
INTRODUCTION 1 1 .2 THRESHOLD PHOTOELECTRON SPECTROSCOPY (TPES) 3 1 .2.1
THE SUPPRESSION OF ENERGETIC ELECTRONS BY TOF 8 1 .2.2 THE ROLE OF
AUTOIONIZATION IN TPES 9 1 .2.3 THE MECHANISM FOR THRESHOLD ELECTRON
PRODUCTION 1 1 1 .3 THRESHOLD IONIZATION WITH PULSED LASER SOURCES 1 3 1
.3 .1 THE THIRD SURPRISE 1 5 1 .3 .2 A COMPARISON OF PFI-TPES AND TPES 1
6 1 .4 CONCLUSIONS 1 7 CHAPTER 2 HIGH RESOLUTION SPECTROSCOPY WITH
PHOTOELECTRONS : ZEKE SPECTROSCOPY OF MOLECULAR SYSTEMS 2 1 K.
MUELLER-DETHLEFS 2.1 INTRODUCTION 2 2 2 .1 .1 DEVELOPMENT OF
PHOTOIONIZATION EXPERIMENTS 2 8 2.2 FROM PHOTOELECTRON TO ZEKE
SPECTROSCOPY 3 1 2 .2.1 PRINCIPLE OF ZEKE DETECTION 3 1 2 .2.2 THE
DELAYED PULSED FIELD IONIZATION OF RYDBERG STATES 3 4 2.3 DETAILS OF THE
ZEKE EXPERIMENT : TOWARD HIGHEST RESOLUTION 3 7 2.4 ROTATIONALLY
RESOLVED ZEKE SPECTROSCOPY OF MOLECULES 4 3 2.4.1 NO 4 3 2.4.2 BENZENE 4
7 2.4.3 H2O AND H2 S 5 8 2.5 VIBRATIONALLY RESOLVED ZEKE SPECTROSCOPY OF
MOLECULAR CLUSTERS 60 2 .5.1 AR-NO 60 2 .5.2 THE NO DIMER 60 2 .5.3
HYDROGEN-BONDED COMPLEXES 6 1 2 .5.4 COMPARISON BETWEEN THE DIFFERENT
HYDROGEN-BONDE D PHENOL-X COMPLEXES 69 2.6 PERSPECTIVES AND CONCLUSIONS
70 CHAPTER 3 STATE-RESOLVED PHOTOIONIZATION DYNAMICS OF SMALL MOLECULES
USING COHERENT VUV RADIATION 7 9 R.T. REDMAN AND MG. WHITE 3.1
INTRODUCTION 80 3.2 PHOTOIONIZATION DYNAMICS 84 3.3 EXPERIMENT 87 3 .3.1
COHERENT VUV HARMONIC GENERATION 89 3 .3.2 ZEKE-PFI TECHNIQUES 9 2 3.4
ROTATIONALLY RESOLVED PHOTOIONIZATION OF MOLECULES: SELECTED EXAMPLES 9
6 3.4.1 DIATOMIC MOLECULES 9 6 3.4.2 NONLINEAR POLYATOMIC MOLECULES 10 4
3 .5 SUMMARY 11 2 CHAPTER 4 VUV-ZEKE PHOTOELECTRON SPECTROSCOPY :
FINAL-STATE INTERACTIONS IN SMALL MOLECULAR SYSTEMS 119 F . MERKT AND
T.P. SOFILEY 4.1 EXPERIMENTAL TECHNIQUES 120 4 .1.1 INTRODUCTION : THE
ADVANTAGES OF SINGLE-PHOTON IONIZATION 12 0 4 .1.2 VACUUM ULTRAVIOLET
AND EXTREME ULTRAVIOLET RADIATION SOURCES 12 1 4 .1.3 EXPERIMENTAL ZEKE
PHOTOELECTRON SPECTROSCOPY 12 6 4.2 INTENSITY PERTURBATIONS IN
ROTATIONALLY RESOLVED SPECTRA 12 8 4.2.1 INTENSITIES IN CONVENTIONAL,
THRESHOLD AND ZEKE PHOTOELECTRON SPECTROSCOPY 12 8 4.2.2 THE HYDROGEN
MOLECULE 13 1 4.2.3 THE NITROGEN MOLECULE 13 4 4.2.4 THE OXYGEN MOLECULE
13 6 4 .2.5 THE CARBON DIOXIDE MOLECULE 13 8 4 .2.6 OTHER EXAMPLES OF
FINAL-STATE INTERACTIONS 14 0 4 .2.7 CONCLUSIONS 14 1 4.3 REVIEW OF
FACTORS AFFECTING HIGH RYDBERG STATE LIFETIMES 14 3 4 .3.1 LIFETIMES OF
THE STATES DETECTED IN ZEKE-PFI EXPERIMENTS 14 3 4 .3.2 THE NATURE AND
THE FORMATION OF THE ZEKE STATES 14 5 4 .3.3 EFFECTS OF ELECTRIC FIELDS
147 4.4 THEORETICAL MODELS 149 4 .4.1 ROTATIONAL AUTOIONIZATION 149 4
.4.2 ELECTRIC FIELD EFFECTS 15 5 4 .4.3 COMPLEX RESONANCES IN
VIBRATIONAL AND ELECTRONI C AUTOIONIZATION 164 CHAPTER 5 ROTATIONALLY
RESOLVED AUTOIONIZATION OF MOLECULAR RYDBERG STATES 17 1 H.
LEFEBVRE-BRION 5 .1 INTRODUCTION 17 2 5.2 THEORETICAL TREATMENT OF HIGH
RYDBERG STATES 17 2 5 .2.1 GENERALITIES ON DIFFERENT HUND S COUPLING
CASES 17 2 5 .2.2 RYDBERG STATES HAVING A E ION CORE 17 3 5 .2.3 RYDBERG
STATES HAVING A 2N ION CORE 17 4 5 .2.4 EXAMPLES OF RYDBERG COMPLEXES 17
5 5.3 ROTATIONAL AUTOIONIZATION 18 4 5 .3.1 ROTATIONAL AUTOIONIZATION
FOR A E ION CORE 18 4 5 .3.2 ROTATIONAL AUTOIONIZATION FOR A 2II ION
CORE 18 8 5.4 CONCLUSION 19 0 CHAPTER 6 ROTATIONALLY RESOLVED
RESONANCE-ENHANCED MULTIPHOTON IONIZATION PHOTOELECTRON SPECTROSCOPY OF
DIATOMI C HYDRIDES 19 5 C.A. DE LANGE 6.1 INTRODUCTION 19 6 6.2
EXPERIMENTAL TECHNIQUES 19 9 6.2 .1 `MAGNETIC BOTTLE ELECTRON
SPECTROMETER 19 9 6.2.2 TIME-OF-FLIGHT TO ENERGY CONVERSION AND
CALIBRATION 202 6.2.3 WAVELENGTH SPECTRA AND PHOTOELECTRON SPECTRA 204
6.2.4 MASS-RESOLVED ION DETECTION 20 5 6.2.5 ZEKE-PFI 20 5 6.2.6
NANOSECOND LASER SYSTEM 20 6 6.3 THEORY 207 6.4 DIATOMIC HYDRIDES 21 1
6.4.1 THE OH RADICAL 21 1 6.4.2 THE NH RADICAL 220 6.4.3 THE HC1
MOLECULE 232 6.5 CONCLUSIONS 242 CHAPTER 7 EXPLOITING POLARIZATION IN
THE STUDY OF MOLECULA R PHOTOIONIZATION DYNAMICS 247 K.L. REID AND D.J.
LEAHY 7.1 INTRODUCTION 248 7.2 TWO-PHOTON IONIZATION 254 7.2.1
ADVANTAGES 254 7.2.2 FORMALISM 259 7.3 APPLICATIONS 265 7 .3.1 THE FIRST
`COMPLETE MOLECULAR PHOTOIONIZATION EXPERIMENT: NO(A ZE +) 26 5 7 .3.2
FURTHER EXPERIMENTS 274 7 .3.3 DETERMINATION OF ALIGNMENT 27 5 7 .3.4
EXTENSION TO OTHER SYSTEMS 276 7.4 CONCLUSIONS 277 CHAPTER 8
ROTATIONALLY RESOLVED PHOTOELECTRON SPECTRA A T NEAR-THRESHOLD KINETIC
ENERGIES 28 1 K. WANG AND V . MCKOY 8.1 INTRODUCTION 28 2 8.2 THEORY AND
FORMULATION 284 8 .2 .1 (N + 1 ) REMPI FOR LINEAR MOLECULES 284 8 .2.2
(N + 1 ) REMPI FOR ASYMMETRIC TOPS 29 1 8 .2 .3 (N + 1 ) REMPI FOR
SYMMETRIC TOPS 29 5 8 .2.4 COMPUTATIONAL PROCEDURES 296 8.3 RESULTS AND
DISCUSSION 297 8 .3 .1 REMPI VIA RYDBERG STATES OF LINEAR MOLECULES 297
8 .3 .2 ZEKE-PFI OF LINEAR MOLECULES 31 2 8 .3 .3 ZEKE-PFI OF NONLINEAR
MOLECULES 31 9 CHAPTER 9 LOW-FREQUENCY TORSIONAL AND VIBRATIONAL MOTIONS
I N TOLUENE +, PHENYLSILANE + , AND BENZYL + : EXPERIMENTS AND AB INITIO
CALCULATIONS 33 1 K.-T. LU, G.C EIDEN, J.K. BADENHOOP, F .A . WEINHOLD,
AND JC WEISSHAAR 9 .1 INTRODUCTION 33 2 9.2 EXPERIMENTAL TECHNIQUE 33 3
9.3 , INTERNAL ROTATION IN TOLUENE AND PHENYLSILANE NEUTRAL S AND
CATIONS 334 9 .3.1 INTRODUCTION TO INTERNAL ROTATION BARRIERS 334 9 .3.2
ROTOR STATES 33 6 9 .3 .3 S 1-SO SELECTION RULES 337 9 .3.4 PFI
SELECTION RULES 33 8 9 .3.5 S 1-SO SPECTRA AND ASSIGNMENTS 340 9 .3 .6
CATION ROTOR STATES : PFI SPECTRA OF TOLUENE+ AND PHENYLSILANE + 34 1 9
.3 .7 BOND ENERGIES FROM ADIABATIC IONIZATION POTENTIALS 347 9 .3 .8 AB
INITIO EQUILIBRIUM GEOMETRIES AND TORSIONAL BARRIERS 348 9 .3 .9
VIBRONIC COUPLING IN PHENYLSILANE + AND TOLUENE+ 35 1 9 .3 .10
DONOR-ACCEPTOR MODEL OF CH3 AND SIH3 TORSIONAL POTENTIALS 354 9.4
R2PI-PFI STUDIES OF THE BENZYL RADICAL 359 9.4.1 R2PI AND PFI SPECTRA
359 9.4.2 ASSIGNMENT OF BENZYL+ VIBRATIONAL BANDS 360 9.4.3 VIBRONIC
COUPLING MECHANISM 364 9.4.4 NATURE OF EXOCYCLIC C-C BOND IN BENZYL AND
BENZYL+ 364 CHAPTER 10 ZEKE STUDIES WITH PICOSECOND LASERS 369 J.L. KNEE
10 .1 INTRODUCTION 370 10.2 BACKGROUND 37 1 10 .2.1 FORMULATION OF THE
MOLECULAR PROBLEM 37 1 10 .2.2 AVAILABLE EXPERIMENTAL TECHNIQUES 37 5
10.3 PHOTOELECTRON PROBING OF MOLECULAR DYNAMICS 37 9 10 .3.1 LASER
TIME-OF-FLIGHT PHOTOELECTRON SPECTROSCOPY 380 10 .3.2 METHODOLOGY FOR
DYNAMICS STUDIES USING ZEKE PES 383 10.4 APPLICATIONS OF TIME-RESOLVED
ZEKE 38 9 10 .4.1 ZEKE STUDIES OF IVR 389 10 .4.2 VAN DER WAALS MOLECULE
IVR AND VIBRATIONAL PREDISSOCIATION 39 3 10 .4.3 ELECTRONIC STATE
NONRADIATIVE TRANSITIONS 39 8 10.5 FUTURE DIRECTIONS 40 0 CHAPTER 11 ON
THE CONTROL OF MOLECULAR PHOTOIONIZATION : EFFECTS OF MODE SPECIFICITY
IN DISCRETE-CONTINUUM COUPLING ON THE DYNAMICS OF NEAR-THRESHOLD
ELECTRON EJECTIO N IN NO2 40 7 E.R. GRAN T 11 .1 INTRODUCTION 40 8 11 .1
.1 VIBRATIONAL AUTOIONIZATION 40 8 11 .1.2 NORMAL COORDINATE DEPENDENCE
OF VIBRATIONA L AUTOIONIZATION 409 11 .1 .3 ELECTRONIC STRUCTURE OF THE
HIGHER EXCITED STATES OF NO 2 410 11.2 PHOTOSELECTION AND THE
PREPARATION OF EXCITED STATES OF NO 2 41 1 11.3 TRIPLE RESONANCE AND THE
MODE-SELECTED VIBRATIONAL AUTOIONIZATION OF NO 2 41 3 11.4
TRIPLE-RESONANT THRESHOLD PHOTOIONIZATION OF NO 2: THE EFFECT OF MODE
SELECTIVITY IN DISCRETE-CONTINUUM INTERACTIONS ON THRESHOLD
PHOTOIONIZATION INTENSITIES 419 11 .4.1 METHOD FOR HIGH-RESOLUTION
THRESHOLD PHOTOIONIZATIO N SPECTROSCOPY 419 11 .4.2 VIBRATIONAL
STRUCTURE 420 11.4.3 ROTATIONAL STRUCTURE IN THE VIBRATIONAL GROUND
STATE O F NO2+ 42 3 11 .4.4 ROTATIONAL INTENSITIES FOR THRESHOLD
PHOTOIONIZATION TO FORM VIBRATIONALLY EXCITED STATES OF NO 2 + 42 9 11
.5 CONCLUSIONS 43 2 CHAPTER 12 PHYSICS OF NEAR-THRESHOLD STATES IN
MOLECULA R HYDROGEN 43 7 E.E. EYLER 12 .1 INTRODUCTION 43 8 12.2 GENERAL
BEHAVIOR OF NEAR-THRESHOLD LEVELS 43 9 12.2.1 LONG-RANGE POTENTIALS :
RYDBERG STATES IN THE COULOMB POTENTIAL 43 9 12.2.2 SHORT-RANGE
POTENTIALS 44 1 12.3 ATOM-LIKE MOLECULES: NONPENETRATING RYDBERG STATES
44 5 12.3.1 OVERALL STRUCTURE OF RYDBERG STATES WITH HIGH N AND 1 44 5
12 .3 .2 AUTOIONIZATION AND PREDISSOCIATION 44 8 12 .3 .3 EFFECTS OF
EXTERNAL ELECTRIC FIELDS 44 8 12.4 RYDBERG NP STATES OF MOLECULAR
HYDROGEN 45 0 12.4 .1 UNDERSTANDING STRONG INTERCHANNEL PERTURBATIONS :
TWO-CHANNEL QUANTUM-DEFECT THEORY 45 1 12.4.2 HIGH-PRECISION ENERGY
LEVEL MEASUREMENTS 45 3 12 .4.3 DETERMINATION OF THE IONIZATION
POTENTIAL 45 5 12.4.4 DYNAMICS OF THE NP STATES 45 9 12.5 HIGH
VIBRATIONAL LEVELS NEAR THE SECOND DISSOCIATION LIMIT 46 1 12 .5 .1
GENERAL STRUCTURE 46 1 12 .5 .2 PERTURBATIONS, INCLUDING GERADE-UNGERADE
MIXING 464 12.5.3 RELATION TO LONG-RANGE ATOMIC COLLISIONS AND TRAP
PHYSICS 46 7 12.6 NEAR-THRESHOLD DISSOCIATION TO H(LS) + H(2S OR 2P) 46
9 12.6.1 GENERAL OBSERVATIONS AND CALCULATED CROSS-SECTIONS 46 9 12.6.2
HIGH-RESOLUTION MEASUREMENTS OF CONTINUUM STRUCTURE , INCLUDING ATOMIC
2S : 2P BRANCHING RATIOS 47 0 12.6.3 DETERMINATION OF THE DISSOCIATION
LIMIT 474 12.6.4 SHAPE RESONANCES ABOVE THE THRESHOLD 47 5 12 .6.5
PROSPECTS FOR OBSERVING VIBRATIONAL RYDBERG STATES OF A N ION PAIR 47 7
12.7 SUMMARY AND CONCLUSIONS 47 8 AUTHOR INDEX 48 3 SUBJECT INDEX 503
|
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| id | DE-604.BV012867813 |
| illustrated | Illustrated |
| indexdate | 2024-07-09T18:35:08Z |
| institution | BVB |
| isbn | 0471941581 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-008757113 |
| oclc_num | 31132601 |
| open_access_boolean | |
| owner | DE-91G DE-BY-TUM DE-703 DE-11 DE-188 |
| owner_facet | DE-91G DE-BY-TUM DE-703 DE-11 DE-188 |
| physical | XVI, 509 S. graph. Darst. |
| publishDate | 1995 |
| publishDateSearch | 1995 |
| publishDateSort | 1995 |
| publisher | Wiley |
| record_format | marc |
| series2 | Wiley series in ion chemistry and physics |
| spelling | High resolution laser photoionization and photoelectron studies ed. by Ivan Powis ... Chichester [u.a.] Wiley 1995 XVI, 509 S. graph. Darst. txt rdacontent n rdamedia nc rdacarrier Wiley series in ion chemistry and physics Eletricidade e eletronica (fisica) larpcal Espectroscopia larpcal Estrutura molecular (quimica teorica) larpcal Ionisation multiphotonique Molécule Photoionisation Photoionisation ram Spectre photoélectronique Spectroscopie laser Spectroscopie laser ram Spectroscopie moléculaire ram Spectroscopie photoélectrique ram Spectroscopie à haute résolution Spectroscopie à haute résolution ram High resolution spectroscopy Molecular spectroscopy Photoelectron spectroscopy Photoionization ZEKE-Spektroskopie (DE-588)4509853-0 gnd rswk-swf ZEKE-Spektroskopie (DE-588)4509853-0 s DE-604 Powis, Ivan Sonstige oth GBV Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=008757113&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | High resolution laser photoionization and photoelectron studies Eletricidade e eletronica (fisica) larpcal Espectroscopia larpcal Estrutura molecular (quimica teorica) larpcal Ionisation multiphotonique Molécule Photoionisation Photoionisation ram Spectre photoélectronique Spectroscopie laser Spectroscopie laser ram Spectroscopie moléculaire ram Spectroscopie photoélectrique ram Spectroscopie à haute résolution Spectroscopie à haute résolution ram High resolution spectroscopy Molecular spectroscopy Photoelectron spectroscopy Photoionization ZEKE-Spektroskopie (DE-588)4509853-0 gnd |
| subject_GND | (DE-588)4509853-0 |
| title | High resolution laser photoionization and photoelectron studies |
| title_auth | High resolution laser photoionization and photoelectron studies |
| title_exact_search | High resolution laser photoionization and photoelectron studies |
| title_full | High resolution laser photoionization and photoelectron studies ed. by Ivan Powis ... |
| title_fullStr | High resolution laser photoionization and photoelectron studies ed. by Ivan Powis ... |
| title_full_unstemmed | High resolution laser photoionization and photoelectron studies ed. by Ivan Powis ... |
| title_short | High resolution laser photoionization and photoelectron studies |
| title_sort | high resolution laser photoionization and photoelectron studies |
| topic | Eletricidade e eletronica (fisica) larpcal Espectroscopia larpcal Estrutura molecular (quimica teorica) larpcal Ionisation multiphotonique Molécule Photoionisation Photoionisation ram Spectre photoélectronique Spectroscopie laser Spectroscopie laser ram Spectroscopie moléculaire ram Spectroscopie photoélectrique ram Spectroscopie à haute résolution Spectroscopie à haute résolution ram High resolution spectroscopy Molecular spectroscopy Photoelectron spectroscopy Photoionization ZEKE-Spektroskopie (DE-588)4509853-0 gnd |
| topic_facet | Eletricidade e eletronica (fisica) Espectroscopia Estrutura molecular (quimica teorica) Ionisation multiphotonique Molécule Photoionisation Spectre photoélectronique Spectroscopie laser Spectroscopie moléculaire Spectroscopie photoélectrique Spectroscopie à haute résolution High resolution spectroscopy Molecular spectroscopy Photoelectron spectroscopy Photoionization ZEKE-Spektroskopie |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=008757113&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT powisivan highresolutionlaserphotoionizationandphotoelectronstudies |