Molecular catenanes, rotaxanes and knots: a journey through the world of molecular topology
Gespeichert in:
| Format: | Buch |
|---|---|
| Sprache: | English |
| Veröffentlicht: |
Weinheim [u.a.]
Wiley-VCH
1999
|
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | XIV, 368 S. zahlr. Ill., graph. Darst. |
| ISBN: | 3527295720 |
Internformat
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Datensatz im Suchindex
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| adam_text | MOLECULAR CATENANES, ROTAXANES AND KNOTS A JOURNEY THROUGH THE WORLD OF
MOLECULAR TOPOLOGY EDITED BY J.-P. SAUVAGE AND C. DIETRICH-BUCHECKER
WILEY-VCH WEINHEIM * NEW YORK * CHICHESTER BRISBANE * SINGAPORE *
TORONTO CONTENTS 1 CHEMICAL TOPOLOGY - STATISTICAL MUSINGS 1 1.1
CATENANES 1 1.2 OLEFIN METATHESIS 3 1.3 KNOTS 4 REFERENCES 6 2 A KNOT
THEORETIC APPROACH TO MOLECULAR CHIRALITY 7 2.1 TOPOLOGICAL CHIRALITY OF
KNOTS AND LINKS 7 2.2 TOPOLOGICAL CHIRALITY OF EMBEDDED GRAPHS 14 2.3
TOPOLOGICAL CHIRALITY OF MOLECULAR KNOTS AND LINKS 16 2.4 TOPOLOGICAL
CHIRALITY OF MOLECULAR CELL COMPLEXES 18 2.5 MOLECULAR MOEBIUS LADDERS
AND RELATED MOLECULES 21 2.6 USING AUTOMORPHISMS TO PROVE INTRINSIC
CHIRALITY 31 REFERENCES 34 3 SOFT AND HARD MOLECULE-BASED MAGNETS WITH A
FULLY INTERLOCKED THREE-DIMENSIONAL STRUCTURE 37 3.1 INTRODUCTION 37 3.2
MOLECULAR MAGNETISM 37 3.3 MAGNETIC BRICKS 39 3.4 A GAME OF BRICKS AND
PIECES OF MORTAR 40 3.5 STRUCTURE OF MOLECULE-BASED MAGNETS CONTAINING
THREE SPIN CARRIERS, WITH A FULLY INTERLOCKED STRUCTURE 44 3.6 MAGNETIC
PROPERTIES 48 3.6.1 THE TEMPERATURE DEPENDENCE OF MAGNETIC
SUSCEPTIBILITY 48 3.6.2 FIELD DEPENDENCIES OF THE MAGNETIZATION 51 3.7
SOME FURTHER CONSIDERATIONS 53 3.8 A FEW WORDS TO CONCLUDE 54 REFERENCES
55 CONTENTS 4 TRANSITION METAL-INCORPORATING CATENANES 57 4.1
INTRODUCTION 57 4.2 INTERLOCKED COMPOUNDS CONTAINING METALS 58 4.2.1
METAL-CONTAINING ROTAXANES 59 4.2.2 METAL-TEMPLATED SYNTHESIS OF
CATENANES 59 4.2.3 ORGANOMETALLIC CATENANES AND ROTAXANES 60 4.2.4
SELF-ASSEMBLY OF A [2]CATENANE INCORPORATING (EN)PD(H) UNITS .... 62
4.2.4.1 QUANTITATIVE SELF-ASSEMBLY OF A COORDINATION CATENANE 62 4.2.4.2
MECHANISM OF THE RAPID INTERCONVERSION: MOEBIUS STRIP MECHANISM 64
4.2.4.3 IRREVERSIBLE INTERLOCK OF MOLECULAR RINGS 64 4.2.4.4 ELECTRONIC
EFFECTS IN THE SELF-ASSEMBLY OF PD(II)-LINKED CATENANES 66 4.2.5
MADE-TO-ORDER ASSEMBLING OF PD(II)-LINKED CATENANES 68 4.2.5.1
QUANTITATIVE FORMATION OF CATENANES FROM RECTANGULAR MOLECULAR BOXES 68
4.2.5.2 SELECTIVE FORMATION OF CATENANES FROM THREE SPECIES-EIGHT
COMPONENTS 69 4.2.5.3 SCOPE AND LIMITATIONS 71 4.3 CONCLUSION 74
REFERENCES 75 5 CATENANE AND ROTAXANE MOTIFS IN INTERPENETRATING AND
SELF-PENETRATING COORDINATION POLYMERS 77 5.1 INTRODUCTION 77 5.1.1 NETS
77 5.1.2 INTERPENETRATION OF NETS 79 5.2 INTERPENETRATING 1D POLYMERS 80
5.3 INTERPENETRATING 2D NETWORKS 83 5.3.1 PARALLEL INTERPENETRATION OF
2D FRAMEWORKS 83 5.3.1.1 INTERPENETRATING PAIRS OF SHEETS 83 5.3.1.2
PARALLEL INTERPENETRATION OF MORE THAN TWO SHEETS 87 5.3.1.3 PARALLEL
INTERPENETRATION OF SHEETS OTHER THAN (6,3) AND (4,4) 87 5.3.1.4
PARALLEL INTERPENETRATION OF 2D NETS TO GIVE A 3D INTERLOCKED COMPOSITE
87 5.3.2 INCLINED INTERPENETRATION OF 2D FRAMEWORKS 88 5.3.2.1 MORE THAN
ONE SHEET PASSING THROUGH ANY RING 89 5.4 INTERPENETRATING 3D NETWORKS
91 5.4.1 INTERPENETRATING 3-CONNECTED 3D NETS 91 5.4.1.1
INTERPENETRATING (10,3)-A NETS 92 5.4.1.2 INTERPENETRATING (10,3)-B NETS
93 5.4.1.3 INTERPENETRATING (8,3)-C NETS 94 5.4.2 INTERPENETRATING
4-CONNECTED 3D NETS 94 5.4.2.1 INTERPENETRATING DIAMOND-LIKE NETS 94
5.4.2.2 INTERPENETRATING QUARTZ-LIKE NETS 95 5.4.2.3 INTERPENETRATING
PTS-LIKE NETS 95 CONTENTS IX 5.4.3 INTERPENETRATING 6-CONNECTED 3D NETS
95 5.4.3.1 INTERPENETRATING A-PO-LIKE NETS 95 5.4.3.2 INTERPENETRATING
6-CONNECTED NETS UNRELATED TO A-PO 98 5.4.4 INTERPENETRATING 3D NETS
EACH CONTAINING TWO TYPES OF NODES WITH DIFFERENT CONNECTIVITIES 99
5.4.5 INTERPENETRATING 3D NETS WITH DIFFERENT CHEMICAL COMPOSITIONS ...
101 5.4.5.1 INTERPENETRATING NETS OF THE SAME TOPOLOGY BUT DIFFERENT
CHEMICAL COMPOSITION 101 5.4.5.2 INTERPENETRATING 3D NETS OF DIFFERENT
TOPOLOGY 102 5.5 SELF-PENETRATING AND SELF-CATENATING NETWORKS 103 5.6
CLOSING COMMENTS - PROPERTIES AND APPLICATIONS 104 REFERENCES 105 6
MOLECULAR KNOTS - FROM EARLY ATTEMPTS TO HIGH-YIELD TEMPLATE SYNTHESES
107 6.1 INTRODUCTION 107 6.1.1 TOPOLOGY - FROM ARTS TO MATHEMATICS 107
6.1.2 BIOLOGICAL TOPOLOGY - DNA AND PROTEINS 109 6.1.3 HISTORICAL
PERSPECTIVES - CATENANES AND CHEMICAL KNOTS 111 6.1.4 THE VARIOUS ROUTES
TOWARDS A MOLECULAR KNOT - EARLY ATTEMPTS 112 6.1.4.1 APPROACHES
INVOLVING RANDOMNESS 112 6.1.4.2 ATTEMPTS USING DIRECTED SYNTHESES 114
6.1.4.3 ATTEMPTS BASED ON TEMPLATED SYNTHESIS 115 6.2 FIRST SYNTHESIS
116 6.2.1 STRATEGY 116 6.2.2 A SYNTHETIC MOLECULAR TREFOIL KNOT - FIRST
RESULTS 119 6.3 GENERALIZATION AND IMPROVEMENTS 123 6.3.1 FORMATION OF
DOUBLE-STRANDED HELICAL PRECURSORS WITH POLYMETHYLENE LINKERS 123 6.3.2
A DRAMATIC IMPROVEMENT - USE OF 1,3-PHENYLENE SPACER BETWEEN THE
COORDINATING UNITS 125 6.3.3 HIGH-YIELD SYNTHESIS OF A DICOPPER(I)
TREFOIL KNOT USING RING-CLOSING METATHESIS METHODOLOGY 126 6.4 TREFOIL
KNOTS AS TRANSITION METAL LIGANDS - SPECIFIC KINETIC, ELECTROCHEMICAL,
AND PHOTOCHEMICAL PROPERTIES 129 6.4.1 TOPOLOGICAL EFFECT - THE
POLYMETHYLENE BRIDGED COMPLEXES 129 6.4.2 STRUCTURAL EFFECT - THE
PHENYLENE BRIDGED TREFOIL KNOT CU 2 (K-84)P + 132 6.5 RESOLUTION OF A
MOLECULAR KNOT INTO ITS ENANTIOMERS 135 6.5.1 STRATEGY AND ACHIEVEMENTS
135 6.5.2 OPTICAL PROPERTIES AND PERSPECTIVES 137 6.6 CONCLUSION 138
REFERENCES 139 X CONTENTS 7 ORGANIC TEMPLATE-DIRECTED SYNTHESES OF
CATENANES, ROTAXANES, AND KNOTS 143 7.1 BRIEF HISTORY AND BACKGROUND 143
7.2 PSEUDOROTAXANES AND ROTAXANES INCORPORATING MACROCYCLIC POLYETHERS
AND SECONDARY DIALKYLAMMONIUM SALTS AS THEIR COMPONENTS 146 7.3
PSEUDOROTAXANES, CATENANES, ROTAXANES, AND KNOTS INCORPORATING
TT-ELECTRON-RICH AND DEFICIENT COMPONENTS 153 7.4 CATENANES AND
ROTAXANES INCORPORATING AMIDE RECOGNITION SITES IN THEIR COMPONENTS 163
7.5 CATENANES AND ROTAXANES INCORPORATING CYCLODEXTRINS AS THEIR
MACROCYCLIC COMPONENTS 166 7.6 REFLECTIONS AND OPPORTUNITIES 169
REFERENCES 170 8 AMIDE-BASED CATENANES, ROTAXANES AND PRETZELANES 177
8.1 INTRODUCTION 177 8.2 AMIDE-BASED CATENANES 178 8.3 AMIDE-BASED
ROTAXANES 189 8.3.1 CLIPPING 190 8.3.2 THREADING 191 8.3.3 SLIPPING 203
8.4 CHEMISTRY WITH AMIDE-BASED CATENANES AND ROTAXANES 205 8.5
STEREOCHEMISTRY OF AMIDE-BASED CATENANES AND ROTAXANES 211 8.6
CONCLUSION AND OUTLOOK 216 8.7 ADDENDUM 217 REFERENCES 219 9 POLYMER
CHAINS IN CONSTRAINING ENVIRONMENTS 223 SYNOPSIS 223 9.1 INTRODUCTION
224 9.2 CHAINS CONSTRAINED IN HOMOGENEOUS (ONE-PHASE) SYSTEMS 225 9.2.1
INTER-CHAIN ENTANGLEMENTS 225 9.2.2 CHAIN-JUNCTION ENTANGLEMENTS AND
CONSTRAINED-JUNCTION THEORY . 225 9.2.3 CONSTRAINED-CHAIN THEORY 227
9.2.4 DIFFUSED CONSTRAINTS THEORY 227 9.2.5 SLIP-LINK THEORY 228
9.2.6 SOME RELEVANT EXPERIMENTS 228 9.3 SORPTION AND EXTRACTION 229
9.3.1 GENERAL APPROACH 229 9.3.2 LINEAR DILUENTS 230 9.3.3 CYCLIC
DILUENTS 231 9.4 TRAPPING OF CYCLICS 231 CONTENTS XI 9.4.1 EXPERIMENTAL
RESULTS 231 9.4.2 THEORETICAL INTERPRETATION 232 9.4.3 OLYMPIC
NETWORKS 233 9.5 CHAINS CONSTRAINED WITHIN SECOND PHASES OR AT
INTERFACES 233 9.5.1 ESSENTIALLY ONE-DIMENSIONAL SYSTEMS 233 9.5.1.1
ZEOLITES AS ILLUSTRATIVE SYSTEMS 233 9.5.1.2 SIMPLE MIXING OF A POLYMER
AND A ZEOLITE 234 9.5.1.3 POLYMERIZING MONOMER WITHIN ZEOLITE CAVITIES
234 9.5.2 ESSENTIALLY TWO-DIMENSIONAL SYSTEMS 236 9.5.2.1 SOME IMPORTANT
EXAMPLES 236 9.5.2.2 POLYMERS BETWEEN TWO SURFACES 236 9.5.2.3 POLYMERIC
COATINGS 237 9.5.2.4 ELASTOMERS BOUND TO REINFORCING FILIER PARTICLES
238 9.5.3 ESSENTIALLY THREE-DIMENSIONAL SYSTEMS 238 9.5.3.1 GENERAL
FEATURES 238 9.5.3.2 TUBULES 238 9.5.3.3 MESOPOROUS SILICA 238 9.5.3.4
VYCOR GLASS 239 9.5.3.5 THERMOPORIMETRY 239 REFERENCES 240 10
POLYCATENANES, POLY[2]CATENANES, AND POLYMERIC CATENANES . . . 247 10.1
INTRODUCTION 247 10.2 POLYCATENANES LINKED BY TOPOLOGICAL BONDS 250 10.3
POLY[2]CATENANES LINKED BY ALTERNATING TOPOLOGICAL AND COVALENT BONDS
256 10.4 CATENATED CYCLIC POLYMERS 268 10.5 CONCLUSIONS AND PERSPECTIVE
272 REFERENCES 274 11 POLYROTAXANES - SYNTHESES AND PROPERTIES . 277
11.1 INTRODUCTION 277 11.2 GENERAL PRINCIPLES OF POLYROTAXANE SYNTHESES
278 11.2.1 NOMENCLATURE 278 11.2.2 STRUCTURAL REQUIREMENTS - SIZE OF THE
CYCLIC SPECIES AND BLOCKING GROUPS 280 11.2.3 DRIVING FORCES FOR
THREADING 280 11.2.3.1 STATISTICAL THREADING AND CHEMICAL CONVERSION 281
11.2.3.2 THREADING DRIVEN BY ENTHALPY 281 11.3 SYNTHESES OF
POLYROTAXANES 285 11.3.1 STATISTICAL APPROACHES 285 11.3.2
HYDROPHILIC-HYDROPHOBIC INTERACTIONS 288 11.3.3 HYDROGEN BONDING 294
11.3.4 METAL TEMPLATES 303 XU CONTENTS 11.3.5 SELF-ASSEMBLY - N-N
STACKING AND CHARGE TRANSFER 304 11.3.6 OTHER COMPLEXES 307 11.4
CHARACTERIZATION 309 11.5 PROPERTIES AND POTENTIAL APPLICATIONS 311
11.5.1 PHASE BEHAVIOR - GLASS TRANSITIONS AND MELTING TEMPERATURES ....
312 11.5.2 ELECTRONIC PROPERTIES 313 11.5.3 SOLUBILITY 313 11.5.4
SOLUTION VISCOSITY AND MELT VISCOSITY 315 11.5.5 MECHANICAL PROPERTIES
315 11.6 CONCLUSIONS AND SOME PERSPECTIVES 316 REFERENCES 318 12
SYNTHETIC DNA TOPOLOGY 323 12.1 INTRODUCTION 323 12.1.1 DNA HELICITY
LEADS TO LINKED TOPOLOGICAL SPECIES 323 12.1.2 DNA BRANDUNG TOPOLOGY 325
12.1.3 DNA AS A SYNTHETIC MATERIAL 326 12.2 POLYHEDRAL CATENANES 328
12.2.1 A DNA CUBE 328 12.2.2 A SOLID-SUPPORT METHODOLOGY 329 12.2.3 A
TRUNCATED OCTAHEDRON 331 12.3 KNOTS 331 12.3.1 KNOTS, CATENANES AND
NODES 331 12.3.2 DNA KNOTS 334 12.3.3 TOPOISOMERIZATION OF DNA KNOTS 335
12.3.4 AN RNATOPOISOMERASE 335 12.4 JUNCTIONS, ANTIJUNCTIONS, AND
MESOJUNCTIONS 337 12.5 BORROMEAN RINGS 339 12.6 TOPOLOGICAL PROTECTION
341 12.7 DNA DOUBLE-CROSSOVER MOLECULES 341 12.7.1 MOTIFS AND PROPERTIES
341 12.7.2 CROSSOVER TOPOLOGY 344 12.7.3 LIGATION OF DOUBLE CROSSOVER
MOLECULES 344 12.7.4 DOUBLE-CROSSOVER MOLECULES AS A ROUTE TO LINEAR
CATENANES AND ROTAXANES *. 348 12.7.5 TWO-DIMENSIONAL ARRAYS OF
DOUBLE-CROSSOVER MOLECULES 349 12.8 CONCLUDING COMMENTS 351 12.8.1
APPLICATIONS OF SYNTHETIC DNA TOPOLOGY 351 12.8.2 SYNTHETIC DNA TOPOLOGY
LEADS TO DNA NANOTECHNOLOGY 353 REFERENCES 354 INDEX 357
|
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| id | DE-604.BV012527509 |
| illustrated | Illustrated |
| indexdate | 2024-07-09T18:29:08Z |
| institution | BVB |
| isbn | 3527295720 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-008505225 |
| oclc_num | 41017890 |
| open_access_boolean | |
| owner | DE-703 DE-20 DE-29T DE-Aug4 DE-355 DE-BY-UBR DE-19 DE-BY-UBM DE-11 |
| owner_facet | DE-703 DE-20 DE-29T DE-Aug4 DE-355 DE-BY-UBR DE-19 DE-BY-UBM DE-11 |
| physical | XIV, 368 S. zahlr. Ill., graph. Darst. |
| publishDate | 1999 |
| publishDateSearch | 1999 |
| publishDateSort | 1999 |
| publisher | Wiley-VCH |
| record_format | marc |
| spelling | Molecular catenanes, rotaxanes and knots a journey through the world of molecular topology ed. by J.-P. Sauvage ... Weinheim [u.a.] Wiley-VCH 1999 XIV, 368 S. zahlr. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Alkenen gtt Catenanen gtt Chiraliteit gtt DNA-topoisomerase gtt Metathese (chemie) gtt Rotaxanen gtt Verknopingen gtt Catenanes Knot theory Rotaxanes Knoten Chemie (DE-588)4164313-6 gnd rswk-swf Rotaxane (DE-588)4178513-7 gnd rswk-swf Catenane (DE-588)4147390-5 gnd rswk-swf Catenane (DE-588)4147390-5 s DE-604 Rotaxane (DE-588)4178513-7 s Knoten Chemie (DE-588)4164313-6 s Sauvage, Jean-Pierre 1944- Sonstige (DE-588)120961121 oth HEBIS Datenaustausch Darmstadt application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=008505225&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Molecular catenanes, rotaxanes and knots a journey through the world of molecular topology Alkenen gtt Catenanen gtt Chiraliteit gtt DNA-topoisomerase gtt Metathese (chemie) gtt Rotaxanen gtt Verknopingen gtt Catenanes Knot theory Rotaxanes Knoten Chemie (DE-588)4164313-6 gnd Rotaxane (DE-588)4178513-7 gnd Catenane (DE-588)4147390-5 gnd |
| subject_GND | (DE-588)4164313-6 (DE-588)4178513-7 (DE-588)4147390-5 |
| title | Molecular catenanes, rotaxanes and knots a journey through the world of molecular topology |
| title_auth | Molecular catenanes, rotaxanes and knots a journey through the world of molecular topology |
| title_exact_search | Molecular catenanes, rotaxanes and knots a journey through the world of molecular topology |
| title_full | Molecular catenanes, rotaxanes and knots a journey through the world of molecular topology ed. by J.-P. Sauvage ... |
| title_fullStr | Molecular catenanes, rotaxanes and knots a journey through the world of molecular topology ed. by J.-P. Sauvage ... |
| title_full_unstemmed | Molecular catenanes, rotaxanes and knots a journey through the world of molecular topology ed. by J.-P. Sauvage ... |
| title_short | Molecular catenanes, rotaxanes and knots |
| title_sort | molecular catenanes rotaxanes and knots a journey through the world of molecular topology |
| title_sub | a journey through the world of molecular topology |
| topic | Alkenen gtt Catenanen gtt Chiraliteit gtt DNA-topoisomerase gtt Metathese (chemie) gtt Rotaxanen gtt Verknopingen gtt Catenanes Knot theory Rotaxanes Knoten Chemie (DE-588)4164313-6 gnd Rotaxane (DE-588)4178513-7 gnd Catenane (DE-588)4147390-5 gnd |
| topic_facet | Alkenen Catenanen Chiraliteit DNA-topoisomerase Metathese (chemie) Rotaxanen Verknopingen Catenanes Knot theory Rotaxanes Knoten Chemie Rotaxane Catenane |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=008505225&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT sauvagejeanpierre molecularcatenanesrotaxanesandknotsajourneythroughtheworldofmoleculartopology |