Streuung leichter Moleküle an Einkristallmetalloberflächen:
Gespeichert in:
| 1. Verfasser: | |
|---|---|
| Format: | Buch |
| Sprache: | German |
| Veröffentlicht: |
Göttingen
Max-Planck-Inst. für Strömungsforschung
1996
|
| Schriftenreihe: | Max-Planck-Institut für Strömungsforschung <Göttingen>: Berichte
1996,11 |
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | Zugl.: Göttingen, Univ., Diss. |
| Beschreibung: | X, 181 S. graph. Darst. |
Internformat
MARC
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| 084 | |a CHE 180d |2 stub | ||
| 100 | 1 | |a Bertino, Massimo |e Verfasser |4 aut | |
| 245 | 1 | 0 | |a Streuung leichter Moleküle an Einkristallmetalloberflächen |c Massimo Bertino |
| 264 | 1 | |a Göttingen |b Max-Planck-Inst. für Strömungsforschung |c 1996 | |
| 300 | |a X, 181 S. |b graph. Darst. | ||
| 336 | |b txt |2 rdacontent | ||
| 337 | |b n |2 rdamedia | ||
| 338 | |b nc |2 rdacarrier | ||
| 490 | 1 | |a Max-Planck-Institut für Strömungsforschung <Göttingen>: Berichte |v 1996,11 | |
| 500 | |a Zugl.: Göttingen, Univ., Diss. | ||
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| 650 | 0 | 7 | |a Molekularstrahl |0 (DE-588)4170381-9 |2 gnd |9 rswk-swf |
| 655 | 7 | |0 (DE-588)4113937-9 |a Hochschulschrift |2 gnd-content | |
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| 830 | 0 | |a Max-Planck-Institut für Strömungsforschung <Göttingen>: Berichte |v 1996,11 |w (DE-604)BV000895025 |9 1996,11 | |
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Datensatz im Suchindex
| _version_ | 1808046301263167488 |
|---|---|
| adam_text |
CONTENTS
1
INTRODUCTION
1
2
EXPERIMENTAL
METHOD
4
2.1
THE
HE
SCATTERING
APPARATUS
"
HUGO
II
"
.
4
2.1.1
WHY
D
2
BEAMS?
.
5
2.1.2
THE
RECYCLING
SYSTEM
.
8
2.2
CONVENTIONAL
SOURCE
.
10
2.3
HOT
SOURCE
.
11
2.3.1
CONSTRUCTION
OF
THE
HOT
SOURCE
.
11
2.3.2
OPERATION
OF
THE
HOT
SOURCE
.
14
2.4
BEAM
ROTATIONAL
AND
VIBRATIONAL
POPULATIONS
.
16
2.4.1
ROTATIONS
.
16
2.4.2
VIBRATIONS
.
19
3
THEORY
20
3.1
SCATTERING
OF
NOBLE
GAS
ATOMS
FROM
SURFACES
.
21
3.2
MOLECULE-SURFACE
INTERACTION
.
23
3.2.1
ONE
AND
TWO-DIMENSIONAL
POTENTIAL
ENERGY
SURFACE
.
.
25
VIII
3.2.2
MULTIDIMENSIONAL
POTENTIAL
ENERGY
SURFACE
.
28
3.3
KINEMATICS
OF
SCATTERING
.
30
3.4
DEBYE-WALLER
EXPONENT
.
33
3.5
EIKONAL
APPROXIMATION
.
34
3.6
DETERMINATION
OF
DIFFRACTION
REFLECTIVITIES
.
37
4
DIFFRACTION
MEASUREMENTS
FROM
CU(001)
40
4.1
INTRODUCTION
.
40
4.2
EXPERIMENTAL
.
41
4.3
EXPERIMENTAL
RESULTS
.
43
,4.3.1
MEASURED
ANGULAR
DISTRIBUTIONS
.
43
4.3.2
DIFFRACTION
REFLECTIVITIES
.
45
4.3.3
ROTATIONAL
EXCITATION
AND
DIFFRACTION
PROBABILITIES
.
58
4.3.4
TOF
MEASUREMENTS
.
62
4.4
DISCUSSION
.
66
4.4.1
COMPARISON
WITH
PREVIOUS
MEASUREMENTS
.
66
4.4.2
EIKONAL
APPROXIMATION
.
67
4.4.3
INFLUENCE
OF
DISSOCIATIVE
CHEMISORPTION
.
70
5
DIFFRACTION
MEASUREMENTS
FROM
NI(110)
77
5.1
INTRODUCTION
.
77
5.2
EXPERIMENTAL
.
78
5.3
EXPERIMENTAL
RESULTS
.
80
5.3.1
MEASURED
ANGULAR
DISTRIBUTIONS
.
80
5.3.2
DIFFRACTION
REFLECTIVITIES
.
82
5.3.3
DEBYE-WALLER
ANALYSIS
.
90
IX
5.4
DISCUSSION
.
93
5.4.1
EIKONAL
APPROXIMATION
.
93
5.4.2
RID
INTENSITIES
.
94
5.4.3
INFLUENCE
OF
DISSOCIATIVE
CHEMISORPTION
ON
THE
SCATTE
RING
PROCESS
.
96
6
COMPARISON
OF
D2
DIFFRACTION
FROM
CU(001)
AND
NI(110)
100
6.1
INTRODUCTION
.
100
6.2
ROLE
OF
THE
PHYSISORPTION
POTENTIAL
.
101
6.3
ROTATIONAL
EXCITATION
.
101
6.4
THE
SURFACE
AS
EMMENTHAL
CHEESE
.
103
6.5
STICKING
AND
SCATTERING
.
105
7
COMPARISON
BETWEEN
HE
AND
D
2
SCATTERING
FROM
CU(001)
AT
HIGH
INCIDENT
ENERGIES
111
7.1
INTRODUCTION
.
111
7.2
THEORY
.
112
7.3
EXPERIMENTAL
.
115
7.4
EXPERIMENTAL
RESULTS
.
116
7.5
DISCUSSION
.
124
7.5.1
ENERGY
DEPENDENCE
.
124
7.5.2
TEMPERATURE
DEPENDENCE
.
129
7.5.3
FWHM
OF
THE
TOF
SPECTRA
.
130
8
MEASUREMENT
OF
THE
REACTION
TIME
IN
THE
HYDROGEN
MOLE
CULE
EXCHANGE
REACTION
ON
NI(110)
133
8.1
INTRODUCTION
.
133
X
8.2
EXPERIMENTAL
.
135
8.3
EXPERIMENTAL
RESULTS
.
139
8.3.1
ANGULAR
DISTRIBUTIONS
.
139
8.3.2
TOF
MEASUREMENTS
WITH
CHOPPER
2
.
141
8.3.3
TOF
MEASUREMENTS
WITH
CHOPPER
1
.
144
8.4
DISCUSSION
.
151
8.4.1
ANGULAR
DEPENDENCE
OF
THE
DESORPTION
TEMPERATURE
.
.
152
8.4.2
MEAN
REACTION
TIME
.
154
9
CONCLUSIONS
158
A
APPENDIX
162
A.L
INTERNAL
DEGREES
OF
FREEDOM
OF
DIATOMIC
MOLECULES
.
162
A.1.1
ROTATIONS
.
162
A.L.
2
VIBRATIONS
.
164
A.2
DETERMINATION
OF
BEAM
INTENSITIES
.
164
A.3
MATHEMATICAL
PROCEDURE
FOR
THE
ANALYSIS
OF
THE
TOF
SPECTRA
OF
THE
REACTION
TIME
EXPERIMENT
.
167
BIBLIOGRAFY
171
ACKNOWLEDGEMENTS
183 |
| any_adam_object | 1 |
| author | Bertino, Massimo |
| author_facet | Bertino, Massimo |
| author_role | aut |
| author_sort | Bertino, Massimo |
| author_variant | m b mb |
| building | Verbundindex |
| bvnumber | BV011197318 |
| classification_tum | PHY 611d PHY 321d CHE 180d |
| ctrlnum | (OCoLC)45584341 (DE-599)BVBBV011197318 |
| discipline | Physik Chemie |
| format | Book |
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| genre | (DE-588)4113937-9 Hochschulschrift gnd-content |
| genre_facet | Hochschulschrift |
| id | DE-604.BV011197318 |
| illustrated | Illustrated |
| indexdate | 2024-08-22T00:41:59Z |
| institution | BVB |
| language | German |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-007510448 |
| oclc_num | 45584341 |
| open_access_boolean | |
| owner | DE-91 DE-BY-TUM DE-355 DE-BY-UBR DE-83 |
| owner_facet | DE-91 DE-BY-TUM DE-355 DE-BY-UBR DE-83 |
| physical | X, 181 S. graph. Darst. |
| publishDate | 1996 |
| publishDateSearch | 1996 |
| publishDateSort | 1996 |
| publisher | Max-Planck-Inst. für Strömungsforschung |
| record_format | marc |
| series | Max-Planck-Institut für Strömungsforschung <Göttingen>: Berichte |
| series2 | Max-Planck-Institut für Strömungsforschung <Göttingen>: Berichte |
| spelling | Bertino, Massimo Verfasser aut Streuung leichter Moleküle an Einkristallmetalloberflächen Massimo Bertino Göttingen Max-Planck-Inst. für Strömungsforschung 1996 X, 181 S. graph. Darst. txt rdacontent n rdamedia nc rdacarrier Max-Planck-Institut für Strömungsforschung <Göttingen>: Berichte 1996,11 Zugl.: Göttingen, Univ., Diss. Nickel (DE-588)4042133-8 gnd rswk-swf Wasserstoffisotop (DE-588)4189274-4 gnd rswk-swf Kristallfläche (DE-588)4151344-7 gnd rswk-swf Kupfer (DE-588)4033734-0 gnd rswk-swf Streuung (DE-588)4058056-8 gnd rswk-swf Potenzialhyperfläche (DE-588)4267440-2 gnd rswk-swf Molekularstrahl (DE-588)4170381-9 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Kupfer (DE-588)4033734-0 s Kristallfläche (DE-588)4151344-7 s Molekularstrahl (DE-588)4170381-9 s Wasserstoffisotop (DE-588)4189274-4 s Streuung (DE-588)4058056-8 s Potenzialhyperfläche (DE-588)4267440-2 s DE-604 Nickel (DE-588)4042133-8 s Max-Planck-Institut für Strömungsforschung <Göttingen>: Berichte 1996,11 (DE-604)BV000895025 1996,11 DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=007510448&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Bertino, Massimo Streuung leichter Moleküle an Einkristallmetalloberflächen Max-Planck-Institut für Strömungsforschung <Göttingen>: Berichte Nickel (DE-588)4042133-8 gnd Wasserstoffisotop (DE-588)4189274-4 gnd Kristallfläche (DE-588)4151344-7 gnd Kupfer (DE-588)4033734-0 gnd Streuung (DE-588)4058056-8 gnd Potenzialhyperfläche (DE-588)4267440-2 gnd Molekularstrahl (DE-588)4170381-9 gnd |
| subject_GND | (DE-588)4042133-8 (DE-588)4189274-4 (DE-588)4151344-7 (DE-588)4033734-0 (DE-588)4058056-8 (DE-588)4267440-2 (DE-588)4170381-9 (DE-588)4113937-9 |
| title | Streuung leichter Moleküle an Einkristallmetalloberflächen |
| title_auth | Streuung leichter Moleküle an Einkristallmetalloberflächen |
| title_exact_search | Streuung leichter Moleküle an Einkristallmetalloberflächen |
| title_full | Streuung leichter Moleküle an Einkristallmetalloberflächen Massimo Bertino |
| title_fullStr | Streuung leichter Moleküle an Einkristallmetalloberflächen Massimo Bertino |
| title_full_unstemmed | Streuung leichter Moleküle an Einkristallmetalloberflächen Massimo Bertino |
| title_short | Streuung leichter Moleküle an Einkristallmetalloberflächen |
| title_sort | streuung leichter molekule an einkristallmetalloberflachen |
| topic | Nickel (DE-588)4042133-8 gnd Wasserstoffisotop (DE-588)4189274-4 gnd Kristallfläche (DE-588)4151344-7 gnd Kupfer (DE-588)4033734-0 gnd Streuung (DE-588)4058056-8 gnd Potenzialhyperfläche (DE-588)4267440-2 gnd Molekularstrahl (DE-588)4170381-9 gnd |
| topic_facet | Nickel Wasserstoffisotop Kristallfläche Kupfer Streuung Potenzialhyperfläche Molekularstrahl Hochschulschrift |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=007510448&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| volume_link | (DE-604)BV000895025 |
| work_keys_str_mv | AT bertinomassimo streuungleichtermolekuleaneinkristallmetalloberflachen |