Metal complexes in aqueous solutions:
Gespeichert in:
| Hauptverfasser: | , |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
New York [u.a.]
Plenum Press
1996
|
| Schriftenreihe: | Modern inorganic chemistry
|
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | X, 253 S: graph. Darst. |
| ISBN: | 0306452480 |
Internformat
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Datensatz im Suchindex
| _version_ | 1804125605354012672 |
|---|---|
| adam_text | METAL COMPLEXES IN AQUEOUS SOLUTIONS ARTHUR E. MARTELL TEXAS A&M
UNIVERSITY COLLEGE STATION, TEXAS ROBERT D. HANCOCK IBC ADVANCED
TECHNOLOGIES AMERICAN FORK, UTAH PLENUM PRESS * NEW YORK AND LONDON
CONTENTS CHAPTER 1 INTRODUCTORY OVERVIEW 1.1 BACKGROUND OF THE STUDY OF
COMPLEX-FORMATION IN AQUEOUS SOLUTION 1 1.2 METAL IONS IN SOLUTION, AND
METAL COMPLEXES 5 1.2.1 METAL IONS IN AQUEOUS SOLUTION 6 1.2.2 TRENDS IN
THE PERIODIC TABLE 9 1.3 STERIC STRAIN IN COMPLEX FORMATION 12 CHAPTER 2
FACTORS GOVERNING THE FORMATION OF COMPLEXES WITH UNIDENTATE LIGANDS IN
AQUEOUS SOLUTION. SOME GENERAL CONSIDERATIONS 2.1 THE ROLE OF THE
SOLVENT 15 2.1.1 PROTONATION REACTIONS IN THE GAS-PHASE 15 2.1.2
COMPLEX-FORMATION REACTIONS OF METAL IONS IN THE GAS-PHASE 21 2.1.3
REACTION RATES IN THE GAS-PHASE 24 2.2 LINEAR FREE ENERGY RELATIONSHIPS
(LFER) 26 2.3 LIGAND FIELD THEORY AND METAL TO LIGAND BONDING 28 2.4
PATTERNS IN LEWIS ACID-BASE BEHAVIOR IN AQUEOUS SOLUTION 34 2.5 THE
COORDINATING TENDENCIES OF DIFFERENT DONOR GROUPS 40 2.5.1 THE NEUTRAL
OXYGEN DONOR 40 2.5.2 THE NEGATIVELY CHARGED OXYGEN DONOR 44 2.5.3 THE
NEUTRAL SATURATED NITROGEN DONOR 49 2.5.4 UNSATURATED NITROGEN DONORS 55
2.5.5 LIGANDS WITH HEAVIER DONOR ATOMS S, SE, P, AS 55 CHAPTER 3
CHELATING LIGANDS 3.1 THE CHELATE EFFECT 63 3.2 THE STANDARD REFERENCE
STATE AND THE CHELATE EFFECT 64 3.3 EQUATIONS FOR PREDICTING THE
STABILITY OF COMPLEXES OF CHELATING LIGANDS 65 3.4 RULE OF AVERAGE
ENVIRONMENT FOR CHELATING LIGANDS 70 3.5 THE SIZE OF THE CHELATE RING
AND COMPLEX STABILITY 73 3.6 THE GEOMETRY OF THE CHELATE RING, AND
PREFERRED METAL ION SIZES 77 3.7 CHELATE RINGS OFOTHER SIZES 82 3.7.1
CHELATE RINGS LARGER THAN SIX MEMBERED 82 3.8 MORE HIGHLY PREORGANIZED
CHELATING LIGANDS 87 3.9 THE EFFECT OF MIXTURES OF CHELATE RINGS OF
DIFFERENT SIZES ON COMPLEX STABILITY 92 3.10 STERIC AND INDUCTIVE
EFFECTS IN CHELATING LIGANDS 93 VII CHAPTER 4 COMPLEXES OF MACROCYCLES
AND OTHER MORE HIGHLY PREORGANIZED LIGANDS 4.1 THE THERMODYNAMICS OF THE
MACROCYCLIC AND CRYPTATE EFFECTS 98 4.2 THE PREFERRED GEOMETRY OF
CHELATE RINGS CONTAINING NEUTRAL OXYGEN AND NITROGEN DONORS 101 4.3 THE
ORIGIN OF THE MACROCYCLIC EFFECT 105 4.4 INDUCTIVE EFFECTS IN COMPLEXES
OF MACROCYCLIC LIGANDS 108 4.5 THE MACROCYCLIC EFFECT IN MIXED DONOR
MACROCYCLES 111 4.6 THE SELECTIVITY OF MACROCYCLIC LIGANDS FOR METAL
IONS 112 4.6.1 THE METAL ION SELECTIVITIES OF THE TETRAAZA MACROCYCLES
113 4.6.2 THE METAL ION SELECTIVITIES OF THE CROWN ETHERS 120 4.6.3 THE
SELECTIVITY PATTERNS OF TRIAZA AND PENTAAZA MACROCYCLES 125 4.7
MACROCYCLES WITH PENDENT DONOR GROUPS 127 4.7.1 TRIAZA MACROCYCLES WITH
PENDENT DONOR GROUPS 127 4.7.2 LIGANDS BASED ON CYCLEN, THAT HAVE
PENDENT DONORS 131 4.7.3 LIGANDS BASED ON HEXADENTATE MACROCYCLES, THAT
HAVE PENDENT DONOR GROUPS 132 4.8 THECRYPTANDS 134 4.9 MACROCYCLES WITH
PENDENT DONOR GROUPS ATTACHED VIA THE CARBON ATOMS OF THE BRIDGING
GROUPS 137 4.10 MORE HIGHLY PREORGANIZED MACROCYCLES 138 4.11
BINUCLEATING MACROCYCLES 140 4.12 CONCLUSIONS 142 CHAPTER 5 MEDICAL
APPLICATIONS OF METAL COMPLEXES 5.1 APPLICATIONS OF LIGAND DESIGN
PRINCIPLES 151 5.1.1 HARD METAL IONS OF BIOMEDICAL INTEREST (LI + , RB+,
SR 2+ , Y 3+ , SM 3+ , GD 3+ , DY 3 +, HO 3+ , YB 3+ , FE 3+ , PU 4+ ,
AL 3 +, GA 3+ ) 151 5.1.2 METAL IONS OF BIOMEDICAL INTEREST, THAT ARE
INTERMEDIATE IN HSAB (NI 2+ , CU 2+ , IN 3+ , PB 2+ , BI 2+ ) 154 5.1.3
SOFT METAL IONS OF BIOMEDICAL INTEREST (CD(II), HG(II), T1(I), PT(LL),
AU(I), AU(III), AND POSSIBLY TC IN ITS +1 TO +7 OXIDATION STATES)....154
5.2 IRAN OVERLOAD 155 5.2.1 THE HYDROXYPYRIDINONES 159 5.3 ALUMINUM 160
5.4 NICKEL 160 5.5 COPPER 161 5.6 PLUTONIUM AND THE ACTINIDES 161 5.7
URANIUM 162 5.8 TOXIC HEAVY METAL IONS 163 5.9 CADMIUM 163 5.10 LEAD 164
5.11 ARSENIC 165 5.12 MERCURY 165 5.13 GENERAL SUMMARY 165 5.14
DIAGNOSTIC RADIOPHARMACEUTICALS BASED ON GA(III) AND IN(III) COMPLEXES
166 5.14.1 SYNTHESIS AND EVALUATION OF NEW LOW MOLECULAR WEIGHT LIGANDS
168 5.14.2 HYDROXYPYRIDINONES 174 5.14.3 BIFUNCTIONAL CHELATES OF
GA(III) AND IN(III) 175 5.15 TECHNETIUM 177 5.15.1 TECHNETIUM(VII) 178
5.15.2 TECHNETIUM(VI) 178 5.15.3 TECHNETIUM(V) 180 5.15.4 TECHNETIUM(IV)
181 5.15.5 TECHNETIUM(III) 182 5.15.6 TECHNETIUM(II) 184 5.15.7
TECHNETIUM(I) 184 5.16 RHENIUM 185 5.16.1 DEVELOPMENT OF
RHENIUM-RADIOPHARMACEUTICALS OF THERAPEUTIC VALUE 185 5.17 MAGNETIC
RESONANCE IMAGING (MRI) 186 5.17.1 FACTORS INFLUENCING THE
WATER-RELAXATION ABILITY OF PARAMAGNETIC COMPLEXES 187 5.17.2
CONCENTRATION OF THE PARAMAGNETIC COMPLEX 188 5.17.3 MAGNETIC MOMENTOF
THE PARAMAGNETIC COMPLEX 188 5.17.4 MODULATION OF MAGNETIC INTERACTIONS
BETWEEN UNPAIRED ELECTRONS AND NUCLEI 188 5.17.5 NUMBER OF COORDINATED
WATER MOLECULES 188 5.17.6 RATE OF WATER EXCHANGE 188 5.17.7
METAL-TO-NUCLEUS DISTANCE 189 5.17.8 METAL CHELATES RECENTLY
INVESTIGATED FOR MAGNETIC RESONANCE IMAGING 189 5.17.9 HEPATOBILIARY MRI
CONTRAST AGENTS 191 5.17.10 NEW MRI CONTRAST AGENTS 191 CHAPTER 6 THE
SELECTIVITY OF LIGANDS OF BIOLOGICAL INTEREST FOR METAL IONS IN AQUEOUS
SOLUTION. SOME IMPLICATIONS FOR BIOLOGY 6.1 SIGNIFICANCE OF HSAB IDEAS
FOR ZINC-CONTAINING METALLOENZYMES 199 6.2 CHELATE RING SIZE AND METAL
ION SELECTIVITY 203 6.3 THE NEUTRAL OXYGEN DONOR 207 6.4 THE NEGATIVE
OXYGEN DONOR 210 6.5 THE NEUTRAL NITROGEN DONOR 212 6.6 SULFURDONORS 213
IX CHAPTER 7 STABILITY CONSTANTS AND THEIR MEASUREMENT 7.1 INTRODUCTION
217 7.2 EARLY WORK 217 7.3 RECENTWORK 218 7.4 THE STABILITY CONSTANT 220
7.5 PHANDP[H] 222 7.6 CA(II)-EDTA COMPLEXES 223 7.6.1 STABILITY
CONSTANTS FOR CA(II)-EDTA 223 7.7 SPECIES DISTRIBUTION DIAGRAMS 225 7.8
EXPERIMENTAL METHODS FOR MEASURING COMPLEX EQUILIBRIA 226 7.8.1
ABSORBANCE METHODS 228 7.9 SPECIFIC METAL ION ELECTRODES 229 7.10
POLAROGRAPHY ANDTHE STUDY OF SOLUTION EQUILIBRIA 231 7.11 OTHER METHODS
236 7.12 COMPETITION METHODS 236 7.12.1 LIGAND-LIGAND COMPETITION BY
POTENTIOMETRIE METHODS 236 7.12.2 SPECTROPHOTOMETRIC DETERMINATIONS OF
COMPETITION CONSTANTS 237 7.13 AMPHOTERIC METAL IONS 238 7.14 CRITICAL
STABILITY CONSTANTS AND THEIR SELECTION 238 7.14.1 MINIMUM REQUIREMENTS
FOR EQUILIBRIUM DATA 239 7.15 DEVELOPMENT OF A COMPLETE METAL COMPLEX
DATABASE 240 INDEX 245 X
|
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| indexdate | 2024-07-09T18:04:13Z |
| institution | BVB |
| isbn | 0306452480 |
| language | English |
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| spelling | Martell, Arthur E. Verfasser aut Metal complexes in aqueous solutions Arthur E. Martell ; Robert D. Hancock New York [u.a.] Plenum Press 1996 X, 253 S: graph. Darst. txt rdacontent n rdamedia nc rdacarrier Modern inorganic chemistry Chelaten gtt Coördinatieverbindingen gtt EDTA gtt Macrocyclische verbindingen gtt Metais e seus compostos (quimica) larpcal Overgangsmetaalcomplexen gtt Solucoes (fisico-quimica) larpcal Water gtt Metal complexes Solution (Chemistry) Metallkomplexe (DE-588)4038898-0 gnd rswk-swf Wässrige Lösung (DE-588)4124928-8 gnd rswk-swf Metallkomplexe (DE-588)4038898-0 s Wässrige Lösung (DE-588)4124928-8 s DE-604 Hancock, Robert D. Verfasser aut GBV Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=007446612&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Martell, Arthur E. Hancock, Robert D. Metal complexes in aqueous solutions Chelaten gtt Coördinatieverbindingen gtt EDTA gtt Macrocyclische verbindingen gtt Metais e seus compostos (quimica) larpcal Overgangsmetaalcomplexen gtt Solucoes (fisico-quimica) larpcal Water gtt Metal complexes Solution (Chemistry) Metallkomplexe (DE-588)4038898-0 gnd Wässrige Lösung (DE-588)4124928-8 gnd |
| subject_GND | (DE-588)4038898-0 (DE-588)4124928-8 |
| title | Metal complexes in aqueous solutions |
| title_auth | Metal complexes in aqueous solutions |
| title_exact_search | Metal complexes in aqueous solutions |
| title_full | Metal complexes in aqueous solutions Arthur E. Martell ; Robert D. Hancock |
| title_fullStr | Metal complexes in aqueous solutions Arthur E. Martell ; Robert D. Hancock |
| title_full_unstemmed | Metal complexes in aqueous solutions Arthur E. Martell ; Robert D. Hancock |
| title_short | Metal complexes in aqueous solutions |
| title_sort | metal complexes in aqueous solutions |
| topic | Chelaten gtt Coördinatieverbindingen gtt EDTA gtt Macrocyclische verbindingen gtt Metais e seus compostos (quimica) larpcal Overgangsmetaalcomplexen gtt Solucoes (fisico-quimica) larpcal Water gtt Metal complexes Solution (Chemistry) Metallkomplexe (DE-588)4038898-0 gnd Wässrige Lösung (DE-588)4124928-8 gnd |
| topic_facet | Chelaten Coördinatieverbindingen EDTA Macrocyclische verbindingen Metais e seus compostos (quimica) Overgangsmetaalcomplexen Solucoes (fisico-quimica) Water Metal complexes Solution (Chemistry) Metallkomplexe Wässrige Lösung |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=007446612&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
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