Dendritic molecules: concepts, synthesis, perspectives
Gespeichert in:
| Hauptverfasser: | , , |
|---|---|
| Format: | Buch |
| Sprache: | German |
| Veröffentlicht: |
Weinheim [u.a.]
VCH
1996
|
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | XI, 261 S. Ill., zahlr. Darst. |
| ISBN: | 3527293256 |
Internformat
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| 245 | 1 | 0 | |a Dendritic molecules |b concepts, synthesis, perspectives |c G. R. Newkome ; C. N. Moorefield ; F. Vögtle |
| 264 | 1 | |a Weinheim [u.a.] |b VCH |c 1996 | |
| 300 | |a XI, 261 S. |b Ill., zahlr. Darst. | ||
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| 650 | 4 | |a Molecular Structure | |
| 650 | 4 | |a Molecular structure | |
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| 700 | 1 | |a Moorefield, Charles N. |e Verfasser |4 aut | |
| 700 | 1 | |a Vögtle, Fritz |d 1939- |e Verfasser |0 (DE-588)106068520 |4 aut | |
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Datensatz im Suchindex
| _version_ | 1804125328084303872 |
|---|---|
| adam_text | G.R. NEWKOME, C.N. MOOREFIELD, F. VOEGTLE DENDRITIC MOLECULES CONCEPTS *
SYNTHESES * PERSPECTIVES WEINHEIM * NEW YORK * BASEL * CAMBRIDGE * TOKYO
CONTENTS PROLOGUE AND ACKNOWLEDGMENTS V CONTENTS VII 1 MASSES, SIZES,
AND SHAPES OF MACROMOLECULES FROM MULTIFUNCTIONAL MONOMERS 1.1
INTRODUCTION 1 1.2 MOLECULAR MASS AND CHAIN CONNECTIVITY IN
MACROMOLECULES 1 1.2.1 DISTRIBUTION WITH LINEAR CHAINS 1 1.2.2 BRANCHED
STRUCTURES AND GELATION WITH MULTIFUNCTIONAL MONOMERS 2 1.2.3 BRANCHING
WITHOUT NETWORK FORMATION 3 1.3 OVERALL EXTENSION IN SPACE: MOLECULAR
SIZES 4 1.3.1 RADIUS OF GYRATION 4 1.3.1.1 LINEAR CHAINS 5 1.3.1.2
MACROCYCLES 6 1.3.1.3 BRANCHED MACROMOLECULES 6 1.3.2 BREADTH OF THE
DISTRIBUTION FOR THE SQUARED RADIUS OF GYRATION 7 1.4 SHAPE ANALYSIS
FROM THE RADIUS OF GYRATION TENSOR 7 1.4.1 PRINCIPAL MOMENTS 8 1.4.2
ASPHERICITY, ACYLINDRICITY, AND RELATIVE SHAPE ANISOTROPY 9 1.5 APPROACH
TO THE GLOBULAR STATE 9 1.5.1 COLLAPSE OF A LINEAR CHAIN 10 1.5.2 SHAPES
FROM THE SIMULATIONS OF DENDRIMERS 10 1.6 REFERENCES 12 2 FROM THEORY TO
PRACTICE: HISTORICAL PERSPECTIVES 2.1 INTRODUCTION 15 2.2 BRANCHED
ARCHITECTURES 15 2.2.1 EARLY OBSERVATIONS 16 2.2.2 PRELUDE TO PRACTICE
17 2.2.3 INCIPIENT MACROMOLECULAR PROGRESSION 19 2.2.3.1 INITIAL CONCEPT
AND PRACTICE 19 2.2.3.2 IMPLIED DENDRITIC CONSTRUCTION 19 2.2.3.3
ALTERNATIVE ARCHITECTURES 21 2.3 THE FRACTAL GEOMETRY OF MACROMOLECULES
24 2.3.1 INTRODUCTION 24 2.3.2 FRACTAL GEOMETRY 24 2.3.2.1
SELF-SIMILARITY OR SCALE-INVARIANCE 24 2.3.2.2 FRACTAL DIMENSION (D) 24
2.3.3 APPLIED FRACTAL GEOMETRY 25 2.3.3.1 FRACTALS IN CHEMISTRY 25
2.3.3.2 FRACTALS IN BIOLOGY 27 2.3.3.3 SOLVENT ACCESSIBLE SURFACE AREA
(A S AS) 28 2.3.3.4 DENDRITIC FRACTALITY 30 2.3.4 FRACTAL SUMMATION 34
2.4 REFERENCES 34 3 NOMENCLATURE 3.1 BACKGROUND ONTRIVAL AND TRADITIONAL
NAMES 37 3.2 DEFINITION OF A CASCADE POLYMER 37 3.3 PROPOSED CASCADE
NOMENCLATURE RULES 38 3.4 GENERAL PATTERNS 39 VIII CONTENTS 3.4.1
SIMILAR REPEAT INTERNAL UNITS 39 3.4.2 SIMILAR ARMS WITH DISSIMILAR
INTERNAL UNITS 41 3.4.3 DISSIMILAR ARMS WITH SIMILAR INTERNAL BRANCHES
42 3.4.4 DISSIMILAR ARMS WITH DISSIMILAR INTERNAL BRANCHES OR TERMINAL
GROUPS 42 3.4.5 UNSYMMETRICALLY BRANCHED CASCADES 44 3.5 FRACTAL
NOTATION 45 3.5.1 GENERAL RULES FOR THE PROPOSED FRACTAL NOTATION 45
3.5.2 EXAMPLES USING THE FRACTAL RULES 46 3.6 REFERENCES 46 4 SYNTHETIC
METHODOLOGIES: DIVERGENT PROCEDURES 4.1 GENERAL CONCEPTS 49 4.2 EARLY
PROCEDURES 49 4.3 1 - 2 IV-BRANCHED 52 4.3.1 1 -* 2 N-BRANCHED AND
CONNECTIVITY 52 4.3.2 1 * 2 YV-BRANCHED, AMIDE CONNECTIVITY 56 4.4 1 *
2YLRY/-BRANCHED, AMIDE CONNECTIVITY 61 4.5 1 * » 2ARY/-BRANCHED, ESTER
CONNECTIVITY 62 4.6 1 -» 2 C-BRANCHED 63 4.6.1 1 -* 2 C-BRANCHED,
AMIDE CONNECTIVITY 63 4.6.2 1 * 2 C-BRANCHED AND CONNECTIVITY 64 4.7 1
* 2 C & ARY/-BRANCHED AND CONNECTIVITY 69 4.8 1 * 2^4RV/-BRANCHED,
N-CONNECTIVITY 70 4.9 1 *» 2 ETHANO-BRANCHED, ETHER CONNECTIVITY 70 4.10
1 * 2 57-BRANCHED AND CONNECTIVITY 71 4.11 1 * 2 F-BRANCHED AND
CONNECTIVITY 76 4.12 1 - 3 C-BRANCHED 78 4.12.1 1 * 3 C-BRANCHED,
AMIDE CONNECTIVITY 78 4.12.1.1 1 * 3 C-BRANCHED, AMIDE ( TRIS )
CONNECTIVITY 78 4.12.1.2 1 - 3 (1 -» 2) C-BRANCHED, AMJDE ( TRIS )
CONNECTIVITY 82 4.12.1.3 1 * 3 C-BRANCHED, AMIDE ( BIS/ZOMOTRIS )
CONNECTIVITY 83 4.12.1.4 L-»3 C-BRANCHED, AMWE ( BEHERA S AMINE )
CONNECTIVITY 84 4.12.2 1 - 3 C-BRANCHED AND CONNECTIVITY 88 4.12.3 1 -
3 C-BRANCHED, RAEER CONNECTIVITY 90 4.12.4 1 * » 3 C-BRANCHED, SS/JER &
AMIDE CONNECTIVITY 91 4.13 1 * 3 IV-BRANCHED AND CONNECTIVITY 94 4.14
1 * 3 P-BRANCHED AND CONNECTIVITY 95 4.15 1 * 3 5/-BRANCHED AND
CONNECTIVITY 96 4.16 1 * 3 ADAMANTANE-BRANCHED, ESTER CONNECTIVITY 100
4.17 REFERENCES 101 5 SYNTHETIC METHODOLOGIES: CONVERGENT PROCEDURES 5.1
GENERAL CONCEPTS 107 5.2 1 - 2 C-BRANCHED 108 5.2.1 1 * 2 C-BRANCHED
AND CONNECTIVITY 108 5.2.2 1 * 2 C-BRANCHED, ETHER CONNECTIVITY 110
5.3 1 * 2 ETHANO-BRANCHED, PHOSPHATE CONNECTIVITY 112 5.4 1 -
2,4RY/-BRANCRIED 112 5.4.1 1 * » 2 Y4RY/-BRANCHED AND CONNECTIVITY 112
5.4.2 1 * 2ARY/-BRANCHED, ETHER CONNECTIVITY 118 5.4.3 1 * 2
ARY/-BRANCHED, AMIDE CONNECTIVITY 129 5.4.4 1 * » 2 ARY/-BRANCHED, ETHER
AND AMIDE CONNECTIVITY 131 5.4.5 1 * 2Y4RY/-BRANCHED, ETHER AND
URETHANE CONNECTIVITY 136 5.4.6 1 * » 2ARY/-BRANCHED, &TER CONNECTIVITY
138 5.4.7 1 * 2/4RY/-BRANCHED, II^ER AND ESTER CONNECTIVITY 143 5.4.8
1 * 2 ARY /-BRANCHED, ETHER AND KETONE CONNECTIVITY 145 CONTENTS IX
5.4.9 1 * » 2/LRY/-BRANCHED, ETHYNE CONNECTIVITY 145 5.5 1 - 2
N-BRANCHED 157 5.5.1 1 * 2 A -BRANCHED, AMIDE CONNECTIVITY 157 5.6 1
- 2 C- & N-BRANCHED, FCTER CONNECTIVITY 159 5.7 1 *» * 2 SZ -BRANCHED,
SILYLOXY CONNECTIVITY 159 5.8 REFERENCES 161 6 SYNTHETIC METHODOLOGIES:
ONE-STEP (HYPERBRANCHED) PROCEDURES 6.1 GENERAL CONCEPTS 165 6.2 1 - 2
ARY/-BRANCHED 165 6.2.1 1 * 2^4RY/-BRANCHED AND CONNECTIVITY 165 6.2.2
1 * * 2 ARY/-BRANCHED, ESTER CONNECTIVITY 167 6.2.3 1 *
2/LRY/-BRANCHED, ETHER CONNECTIVITY 169 6.2.4 1 *» 2/LRY/-BRANCHED,
/ZER AND KETONE CONNECTIVITY 169 6.2.5 1 * 2/LRY/-BRANCHED, AMIDE
CONNECTIVITY 169 6.2.6 1 -» 2 ARY/-BRANCHED, CARBAMATE CONNECTIVITY 172
6.2.7 1 * 2 ARY/-BRANCHED, URETHANE CONNECTIVITY 174 6.2.8 1 *
2ARY/-BRANCHED, ETHER AND ESTER CONNECTIVITY 174 6.3 1 - 2 C-BRANCHED
175 6.3.1 1 * 2 C-BRANCHED, ESTER CONNECTIVITY 175 6.3.2 1 * 2
C-BRANCHED, T/W CONNECTIVITY 177 6.3.3 1 * 2 C-BRANCHED, AMIDE
CONNECTIVITY 178 6.3.4 1 - 2 ARY/-BRANCHED, C-CONNECTIVITY 179 6.3.5 1
*» 2 A -BRANCHED AND CONNECTIVITY 179 6.4 1 *» 3 GE-BRANCHED AND
CONNECTIVITY 179 6.5 1 -» 3 (2)SI-BRANCHED AND CONNECTIVITY 180 6.6
REFERENCES 181 7 CHIRAL DENDRITIC MACROMOLECULES 7.1 DIVERGENT
PROCEDURES TO CHIRAL DENDRIMERSS 182 7.1.1 1 -» 3 C-BRANCHED, ETHER AND
AMIDE CONNECTIVITY 183 7.1.2 1 -» 2 C-BRANCHED 183 7.1.3 1 *
2Y4RY/-BRANCHED, ESTER AND AMIDE CONNECTIVITY 187 7.1.4 1 * » 2
ARY/-BRANCHED, ETHER AND ESTER CONNECTIVITY 187 7.1.5 1 -» 2 N-BRANCHED
AND CONNECTIVITY 187 7.1.6 1 * 2 N-BRANCHED, AMZUEFE-CONNECTIVITY 188
7.2 CONVERGENT PROCEDURES TO CHIRAL DENDRIMERS 192 7.2.1 1 - 2
ARY/-BRANCHED, ETHER CONNECTIVITY 192 7.2.2 1 *» 2 C-BRANCHED, AMIDE
CONNECTIVITY 192 7.2.3 1 - 2ARY/-BRANCHED, EZTZER CONNECTIVITY 196
7.2.4 1 -» 3 P- ANDARY/-BRANCHED, P- AND Z7ZER-CONNECTIVITY 198 7.3
REFERENCES 199 8 DENDRIMERS CONTAINING METAL SITES 8.1 METALS AS
BRANCHING CENTERS 201 8.2 METALS AS BUILDING BLOCK CONNECTORS 204 8.3
METAL CENTERS AS TERMINATION GROUPS (SURFACE FUNCTIONALIZATION) 209 8.4
METALS AS TRANSFORMATION AUXILIARIES 219 8.4.1 SITE-SPECIFIC METAL
INCLUSION 219 8.4.2 RANDOM METAL INCLUSION 219 8.5 REFERENCES 221 X
CONTENTS 9 DENDRITIC NETWORKS 9.1 INTRODUCTION: DENDRITIC ASSEMBLIES 223
9.2 NETWORK FORMATION AND CLASSIFICATION 225 9.2.1 ORDERED VERSUS RANDOM
225 9.2.1.1 METHODS OF FORMATION 225 9.2.1.2 COVALENT AND NON-COVALENT
POSITIONING 227 9.3 RANDOM CONNECTIVITY 227 9.3.1 RANDOM,
COVALENTLY-LINKED DENDRIMER NETWORKS 227 9.3.2 COUPLING VIA
SURFACE-TO-SURFACE INTERACTION 228 9.3.3 COUPLING VIA SURFACE-TO-SURFACE
BRIDGING UNITS 229 9.4 ORDERED DENDRITIC NETWORKS 229 9.4.1 MULTILAYER
CONSTRUCTION 229 9.4.2 DIRECTED NETWORK CONSTRUCTION 229 9.4.2.1
COVALENT, METAL-BASED ASSEMBLY 229 9.4.2.2 HYPERBRANCHED-TYPE,
METAL-BASED ASSEMBLY 230 9.4.2.3 HYDROGEN-BONDING ASSEMBLY 231 9.4.2.4
COVALENT ASSEMBLY 236 9.5 REFERENCES 237 10 UTILITARIAN ASPECTS 10.1
GENERAL APPLICATIONS 241 10.2 CHROMATOGRAPHY 241 10.2.1 ION EXCHANGE
PROCESS 241 10.2.2 ELEKTROKINETIC CAPILLARY CHROMATOGRAPHY 241 10.2.3
SIZE EXCLUSION CHROMATOGRAPHY 242 10.2.4 GAS SEPARATION MEMBRANES 242
10.3 ELECTRONIC PROPERTIES 242 10.3.1 SEMICONDUCTION 242 10.3.2
PHOTOCHEMICAL MOLECULAR DEVICES 242 10.4 PHYSICAL PROPERTIES 243 10.4.1
SOLUBILIZATION/DRUG DELIVERY 243 10.4.2 SIZE CALIBRATION/PORE CREATION
244 10.4.3 ANTIOXIDANTS 244 10.4.4 INKS AND TONERS 244 10.4.5 LIQUID
CRYSTALS 245 10.4.6 CHEMICAL SENSITIVITY 245 10.5 CATALYSIS 245 10.6
BIOCHEMICAL/PHARMACEUTICAL 245 10.6.1 SUCROSE MIMETIC 245 10.6.2
MAP/ANTIGEN 245 10.6.3 ANTIBODY CONJUGATES/LABELING 246 10.6.4 NUCLEIC
ACIDS 246 10.6.5 GENE THERAPY 247 10.6.6 PHARMACEUTICAL COMPLEXES/BORON
NEUTRON CAPTURE THERAPY 247 10.6.7 SPECIFIC RECEPTORS 248 10.7 SYNTHETIC
ASPECTS 248 10.7.1 BUILDING BLOCK PREPARATION (PATENTS) 248 10.7.2
DENDRIMER PREPARATION (PATENTS) 249 11 APPENDICES 11.1 KEY REVIEWS AND
HIGHLIGHTS 251 11.1.1 1996 REVIEWS 251 11.1.2 1995 REVIEWS 251 11.1.3
1994 REVIEWS 251 CONTENTS XI 11.1.4 1993 REVIEWS 253 11.1.5 1992 REVIEWS
253 11.1.6 1991 REVIEWS 254 11.1.7 1990 REVIEWS 255 11.1.8 1989 REVIEWS
255 11.1.9 1988 REVIEWS 255 11.1.10 1987 REVIEWS 256 11.1.11 1986 AND
EARLIER REVIEWS 256 11.2 ADVANCES SERIES 256 11.3 GLOSSARY OF TERMS 257
INDEX 259
|
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| id | DE-604.BV010840100 |
| illustrated | Illustrated |
| indexdate | 2024-07-09T17:59:48Z |
| institution | BVB |
| isbn | 3527293256 |
| language | German |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-007246411 |
| oclc_num | 35043449 |
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| owner | DE-355 DE-BY-UBR DE-703 DE-29T DE-91G DE-BY-TUM DE-19 DE-BY-UBM DE-83 DE-11 DE-188 |
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| physical | XI, 261 S. Ill., zahlr. Darst. |
| publishDate | 1996 |
| publishDateSearch | 1996 |
| publishDateSort | 1996 |
| publisher | VCH |
| record_format | marc |
| spelling | Newkome, George R. 1938- Verfasser (DE-588)1234616327 aut Dendritic molecules concepts, synthesis, perspectives G. R. Newkome ; C. N. Moorefield ; F. Vögtle Weinheim [u.a.] VCH 1996 XI, 261 S. Ill., zahlr. Darst. txt rdacontent n rdamedia nc rdacarrier Dendrimeren gtt Macromoleculen gtt Structuur-activiteit-relatie gtt Synthese (chemie) gtt Macromolecular Substances Macromolecules Molecular Structure Molecular structure Sternpolymere (DE-588)4245705-1 gnd rswk-swf Sternpolymere (DE-588)4245705-1 s DE-604 Moorefield, Charles N. Verfasser aut Vögtle, Fritz 1939- Verfasser (DE-588)106068520 aut GBV Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=007246411&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Newkome, George R. 1938- Moorefield, Charles N. Vögtle, Fritz 1939- Dendritic molecules concepts, synthesis, perspectives Dendrimeren gtt Macromoleculen gtt Structuur-activiteit-relatie gtt Synthese (chemie) gtt Macromolecular Substances Macromolecules Molecular Structure Molecular structure Sternpolymere (DE-588)4245705-1 gnd |
| subject_GND | (DE-588)4245705-1 |
| title | Dendritic molecules concepts, synthesis, perspectives |
| title_auth | Dendritic molecules concepts, synthesis, perspectives |
| title_exact_search | Dendritic molecules concepts, synthesis, perspectives |
| title_full | Dendritic molecules concepts, synthesis, perspectives G. R. Newkome ; C. N. Moorefield ; F. Vögtle |
| title_fullStr | Dendritic molecules concepts, synthesis, perspectives G. R. Newkome ; C. N. Moorefield ; F. Vögtle |
| title_full_unstemmed | Dendritic molecules concepts, synthesis, perspectives G. R. Newkome ; C. N. Moorefield ; F. Vögtle |
| title_short | Dendritic molecules |
| title_sort | dendritic molecules concepts synthesis perspectives |
| title_sub | concepts, synthesis, perspectives |
| topic | Dendrimeren gtt Macromoleculen gtt Structuur-activiteit-relatie gtt Synthese (chemie) gtt Macromolecular Substances Macromolecules Molecular Structure Molecular structure Sternpolymere (DE-588)4245705-1 gnd |
| topic_facet | Dendrimeren Macromoleculen Structuur-activiteit-relatie Synthese (chemie) Macromolecular Substances Macromolecules Molecular Structure Molecular structure Sternpolymere |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=007246411&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT newkomegeorger dendriticmoleculesconceptssynthesisperspectives AT moorefieldcharlesn dendriticmoleculesconceptssynthesisperspectives AT vogtlefritz dendriticmoleculesconceptssynthesisperspectives |