Optical properties of metal clusters:
Gespeichert in:
| Hauptverfasser: | , |
|---|---|
| Format: | Buch |
| Sprache: | German |
| Veröffentlicht: |
Berlin u.a.
Springer
1995
|
| Schriftenreihe: | Springer series in materials science
25 |
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | Hier auch später erschienene, unveränderte Nachdrucke |
| Beschreibung: | XX, 532 S. Ill., graph. Darst. |
| ISBN: | 3540578366 0387578366 9783642081910 |
Internformat
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| 100 | 1 | |a Kreibig, Uwe |e Verfasser |4 aut | |
| 245 | 1 | 0 | |a Optical properties of metal clusters |c Uwe Kreibig ; Michael Vollmer |
| 264 | 1 | |a Berlin u.a. |b Springer |c 1995 | |
| 300 | |a XX, 532 S. |b Ill., graph. Darst. | ||
| 336 | |b txt |2 rdacontent | ||
| 337 | |b n |2 rdamedia | ||
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| 490 | 1 | |a Springer series in materials science |v 25 | |
| 500 | |a Hier auch später erschienene, unveränderte Nachdrucke | ||
| 650 | 4 | |a Electronic structure | |
| 650 | 4 | |a Metal clusters |x Optical properties | |
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| 689 | 0 | 1 | |a Optische Eigenschaft |0 (DE-588)4123887-4 |D s |
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| 700 | 1 | |a Vollmer, Michael |e Verfasser |4 aut | |
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Datensatz im Suchindex
| _version_ | 1804124262191071232 |
|---|---|
| adam_text | UWE KREIBIG MICHAEL VOLLMER OPTICAL PROPERTIES OF METAL CLUSTERS WITH
236 FIGURES SPRINGER TABLE OF CONTENTS 1. INTRODUCTION 1 2. THEORETICAL
CONSIDERATIONS 13 2.1 SINGLE CLUSTERS: EXTRINSIC SIZE EFFECTS OF THE
OPTICAL PROPERTIES . 14 2.1.1 OPTICAL MATERIAL FUNCTIONS OF BULK METALS
14 (A) FREE ELECTRON OPTICAL RESPONSE 14 (B) INTERBAND TRANSITIONS AND
CORE EFFECTS IN REALISTIC METALS 16 (C) FUNDAMENTAL PROPERTIES OF THE
DIELECTRIC FUNCTION ... 19 (D) PENETRATION DEPTH OF ELECTROMAGNETIC
WAVES IN METALS 21 2.1.2 QUASISTATIC RESPONSE OF A SMALL METAL SPHERE TO
AN ELECTRIC FIELD 23 2.1.3 EXACT ELECTRODYNAMIC CALCULATION OF SPHERICAL
METAL CLUSTERS (MIE THEORY) 26 (A) RESPONSE OF METAL SPHERES 28 (B)
POSITIONS AND SHAPES OF PLASMA RESONANCES 30 (C) RESONANCES OF SPECIAL
METALS 35 (D) EXTRINSIC CLUSTER SIZE EFFECTS 41 2.1.4 EXTENSIONS OF THE
MIE THEORY 53 (A) NONSPHERICAL CLUSTER SHAPES 54 (B) CORE-SHELL
PARTICLES (SPHERICAL HETERO-SYSTEMS) 58 (C) SUBSTRATE EFFECTS 61 (D)
NEAR FIELDS AND SURFACE ENHANCED RAMAN SCATTERING 63 (E) NONLINEAR
OPTICAL EFFECTS 69 (F) NONLOCAL RESPONSE AND ADDITIONAL SURFACE
ABSORPTION 72 (G) LONGITUDINAL PLASMONS 75 2.2 SINGLE CLUSTERS:
INTRINSIC SIZE EFFECTS OF THE OPTICAL PROPERTIES . 76 2.2.1
SIZE-DEPENDENT OPTICAL MATERIAL FUNCTIONS OF METAL CLUSTERS 78 (A)
GENERAL REMARKS 78 (B) CLASSICAL MODELS FOR E(W, R) 79 (C)
QUANTUM-MECHANICAL MODELS FOR E(U , R) 88 2.2.2 DIRECT
QUANTUM-MECHANICAL CALCULATIONS OF THE OPTICAL RESPONSE 99 X TABLE OF
CONTENTS (A) JELLIUM APPROXIMATION METHODS 101 (B) QUANTUM CHEMICAL
METHODS 108 (C) WIDTHS AND SHAPES OF THE RESONANCES 114 2.2.3 EFFECTS OF
LOWER-LYING ELECTRONS 118 2.3 CLUSTER MATTER 123 2.3.1 CLASSIFICATION OF
CLUSTER MATTER 124 (A) TOPOLOGICAL AND OPTICAL CHARACTERISTICS OF
CLUSTER MATTER 124 (B) THE EFFECTIVE FIELD 133 2.3.2 STATISTICALLY
DISTRIBUTED SINGLE CLUSTERS: EFFECTIVE MEDIUM THEORIES 135 (A) SURVEY OF
EFFECTIVE MEDIUM CONCEPTS 137 (B) DERIVATION OF THE GENZEL E E FF 147
(C) BOUNDS OF E FF 150 (D) CLUSTER SIZE LIMITATIONS 152 (E) EFFECTIVE
MEDIA WITH OPTICALLY NONLINEAR CLUSTERS OR MATRICES 152 2.3.3 SEPARATED
CLUSTER AGGREGATES: QUASI-STATIC AND ELECTRODYNAMIC CALCULATIONS 155 (A)
QUASI-STATIC APPROXIMATION 157 (B) THE CLUSTER PAIR 158 (C) THE LINEAR
CLUSTER TRIPLET AND LINEAR CLUSTER CHAINS 160 (D) DIPOLE COUPLING IN
SINGLE EXTENDED CLUSTER ARRAYS . . 161 (E) THE GENERAL CASE: GENERALIZED
MIE THEORY (GMT) . . 164 2.3.4 DENSELY PACKED MIXTURES OF CLUSTERS AND
AGGREGATES .... 171 (A) COMBINATION OF SEPARATED SINGLE CLUSTERS AND
AGGREGATES 172 (B) OTHER STATISTICAL CONCEPTS 174 (C) THE BERGMAN
EFFECTIVE DIELECTRIC FUNCTION 177 2.3.5 NANOSTRUCTURED MATTER 184 2.4
SUMMARY AND DISCUSSION 187 2.4.1 LARGE CLUSTERS: SURFACE PLASMONS 187
2.4.2 SMALL AND VERY SMALL CLUSTERS: WHAT IS A PLASMON? .... 193 3.
EXPERIMENTAL METHODS 203 3.1 GENERAL REMARKS 203 3.2 PREPARATION OF
METAL CLUSTERS 207 3.2.1 GENERAL REMARKS 208 3.2.2 FREE CLUSTERS 212
3.2.3 CLUSTERS ON SURFACES 214 3.2.4 CLUSTERS IN SOLIDS 216 (A) MATRIX
ISOLATION, COLOR CENTERS, PHOTOGRAPHIC MATERIALS 216 (B) GLASSES AND
POLYMERS 218 TABLE OF CONTENTS XI (C) OTHER METHODS 219 3.2.5 CLUSTERS
IN LIQUIDS 220 3.2.6 LIGAND STABILIZED CLUSTERS 226 3.2.7 CLUSTER
AGGREGATES 231 (A) COAGULATION AGGREGATES 231 (B) COALESCENCE AGGREGATES
232 3.2.8 DENSE CLUSTER MATTER 233 3.3 CHARACTERIZATION OF METAL
CLUSTERS 234 3.3.1 GENERAL REMARKS 235 3.3.2 CLUSTERS IN BEAMS 236 3.3.3
CLUSTERS ON SUPPORTS, IN MATRICES ETC 238 (A) TRANSMISSION ELECTRON
MICROSCOPY 238 (B) ELECTRON DIFFRACTION 245 (C) OTHER METHODS 246 (D)
CLUSTER MATTER 250 3.4 NONDESTRUCTIVE SPECTROSCOPIES 255 3.4.1 COMMON
METHODS 255 3.4.2 OTHER TECHNIQUES 259 3.4.3 EXPERIMENTAL MEASURES FOR
ABSORPTION, SCATTERING, AND EXTINCTION 260 3.4.4 ADVANTAGES AND
DRAWBACKS 265 3.5 DESTRUCTIVE SPECTROSCOPIES 266 3.5.1 TWO PHOTON
IONIZATION 267 3.5.2 BEAM DEPLETION SPECTROSCOPY 270 3.5.3 DISSOCIATION
SPECTROSCOPY OF SUPPORTED CLUSTERS 272 3.5.4 ADVANTAGES AND DRAWBACKS
273 4. EXPERIMENTAL RESULTS AND DISCUSSION 275 4.1 LARGE CLUSTERS 278
4.1.1 LARGE CLUSTERS IN BEAMS AND SMOKE 278 (A) SMOKES 278 (B) BEAMS 281
(C) INCANDESCENT RADIATION FROM CLUSTERS 284 4.1.2 SEPARATED LARGE
CLUSTERS IN MATRICES 285 (A) GENERAL REMARKS 285 (B) EXPERIMENTAL
VERIFICATION OF MIE S THEORY 286 (C) MIE DIPOLE RESONANCE: POSITION,
WIDTH, THE 1/FI-EFFECT, AND CHEMICAL INTERFACE DAMPING (CID) 294 (D)
SPHERICAL CLUSTERS IN VARIOUS MATRICES 302 (E) ELLIPSOIDAL CLUSTERS 305
(F) THE DIELECTRIC FUNCTION OF CLUSTER MATERIAL AND STRUCTURAL PHASE
TRANSITIONS 307 XII TABLE OF CONTENTS (G) SIZE EFFECTS IN THE
TEMPERATURE DEPENDENCE OF THE CLUSTER ABSORPTION 317 4.1.3 LARGE
CLUSTERS ON SUPPORTS 321 (A) THIN FILMS 322 (B) VERIFICATION OF
THEORETICAL APPROACHES 323 (C) SHAPE AND SUBSTRATE EFFECTS 324 (D)
SURFACE PLASMON INDUCED DESORPTION 328 4.2 SMALL AND VERY SMALL CLUSTERS
333 4.2.1 SMALL AND VERY SMALL FREE CLUSTERS IN BEAMS 333 (A) TRIMERS
333 (B) VERY SMALL CLUSTERS 334 (C) BETWEEN SMALL AND LARGE CLUSTERS 342
(D) PICO- AND FEMTOSECOND SPECTROSCOPY 349 4.2.2 SMALL AND VERY SMALL
CLUSTERS IN MATRICES 351 (A) EXPERIMENTS CONCERNING PHOTOGRAPHY 352 (B)
CHEMICALLY PREPARED LIGAND STABILIZED CLUSTERS 353 (C) PHYSICALLY
PREPARED CLUSTERS 358 4.2.3 SMALL AND VERY SMALL CLUSTERS ON SURFACES
364 (A) ISLAND FILMS 364 (B) FROM VERY SMALL TO SMALL SPHERES AND
ELLIPSOIDS.... 364 4.3 SPECIAL EXPERIMENTS 366 4.3.1 FROM MOLECULAR TO
METALLIC CLUSTERS: COVERING ALL SIZE RANGES 366 4.3.2 HETEROGENEOUS
CLUSTERS 371 (A) BINARY AG/AU SYSTEMS: NUCLEUS/SHELL AND HOMOGENEOUS
ALLOY CLUSTERS 372 (B) DIELECTRIC CORE CLUSTERS 374 (C) OTHER SHELL
CLUSTERS 375 4.3.3 SERS FROM CLUSTER SAMPLES 376 4.3.4 CHEMICAL
REACTIONS 380 (A) GENERAL REMARKS 380 (B) EXPERIMENTS 382 (C)
CONCLUSIONS 386 4.3.5 NONLINEAR OPTICAL EFFECTS OF CLUSTERS 387 (A)
SECOND ORDER PROCESSES 387 (B) THIRD ORDER PROCESSES 388 4.3.6 LIGHT
EMISSION BY NONOPTICAL EXCITATION 389 (A) ELECTROLUMINESCENCE 391 (B)
EXCITATION WITH FAST ELECTRONS 393 (C) EXCITATION WITH TUNNELING
ELECTRONS 393 4.4 CLUSTER MATTER 395 4.4.1 INTERACTING SINGLE CLUSTERS
AND AGGREGATES 397 (A) COMPARISON TO EFFECTIVE MEDIUM THEORIES 397 (B)
HIGHER ORDER EXTINCTION PROCESSES 403 TABLE OF CONTENTS XIII (C)
COAGULATION EFFECTS 407 (D) QUANTITATIVE COMPARISON TO DIRECT
ELECTRODYNAMIC CALCULATIONS 413 (E) LIGHT-INDUCED AGGREGATION 418 4.4.2
COALESCENCE EFFECTS 420 4.4.3 DENSE CLUSTER MATTER 425 (A) THE OSEEN
TRANSITION 425 (B) TRANSITION TO COMPACT THIN FILMS 432 APPENDIX 437 A.L
TABLES: OPTICAL SPECTROSCOPY EXPERIMENTS WITH METAL CLUSTERS 437 A.2
SURVEY OF OPTICAL SPECTRA OF ELEMENTAL METAL CLUSTERS AND
CHAIN-AGGREGATES 451 A.3 MIE COMPUTER PROGRAM 473 REFERENCES J 483
SUBJECT INDEX 527
|
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| author | Kreibig, Uwe Vollmer, Michael |
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| illustrated | Illustrated |
| indexdate | 2024-07-09T17:42:52Z |
| institution | BVB |
| isbn | 3540578366 0387578366 9783642081910 |
| language | German |
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| owner_facet | DE-355 DE-BY-UBR DE-384 DE-703 DE-20 DE-91G DE-BY-TUM DE-19 DE-BY-UBM DE-83 DE-188 DE-29T |
| physical | XX, 532 S. Ill., graph. Darst. |
| publishDate | 1995 |
| publishDateSearch | 1995 |
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| publisher | Springer |
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| series | Springer series in materials science |
| series2 | Springer series in materials science |
| spelling | Kreibig, Uwe Verfasser aut Optical properties of metal clusters Uwe Kreibig ; Michael Vollmer Berlin u.a. Springer 1995 XX, 532 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Springer series in materials science 25 Hier auch später erschienene, unveränderte Nachdrucke Electronic structure Metal clusters Optical properties Optische Eigenschaft (DE-588)4123887-4 gnd rswk-swf Metallcluster (DE-588)4128942-0 gnd rswk-swf Metallcluster (DE-588)4128942-0 s Optische Eigenschaft (DE-588)4123887-4 s DE-604 Vollmer, Michael Verfasser aut Springer series in materials science 25 (DE-604)BV000683335 25 GBV Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=006557118&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Kreibig, Uwe Vollmer, Michael Optical properties of metal clusters Springer series in materials science Electronic structure Metal clusters Optical properties Optische Eigenschaft (DE-588)4123887-4 gnd Metallcluster (DE-588)4128942-0 gnd |
| subject_GND | (DE-588)4123887-4 (DE-588)4128942-0 |
| title | Optical properties of metal clusters |
| title_auth | Optical properties of metal clusters |
| title_exact_search | Optical properties of metal clusters |
| title_full | Optical properties of metal clusters Uwe Kreibig ; Michael Vollmer |
| title_fullStr | Optical properties of metal clusters Uwe Kreibig ; Michael Vollmer |
| title_full_unstemmed | Optical properties of metal clusters Uwe Kreibig ; Michael Vollmer |
| title_short | Optical properties of metal clusters |
| title_sort | optical properties of metal clusters |
| topic | Electronic structure Metal clusters Optical properties Optische Eigenschaft (DE-588)4123887-4 gnd Metallcluster (DE-588)4128942-0 gnd |
| topic_facet | Electronic structure Metal clusters Optical properties Optische Eigenschaft Metallcluster |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=006557118&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
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| work_keys_str_mv | AT kreibiguwe opticalpropertiesofmetalclusters AT vollmermichael opticalpropertiesofmetalclusters |