Introduction to surface chemistry and catalysis:
Gespeichert in:
| 1. Verfasser: | |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
New York u.a.
Wiley
1994
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| Schriftenreihe: | A Wiley-Interscience publication
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| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | XXIV, 667 S. Ill., graph. Darst. |
| ISBN: | 0471031925 |
Internformat
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| 245 | 1 | 0 | |a Introduction to surface chemistry and catalysis |c Gabor A. Somorjai |
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| adam_text | INTRODUCTION TO SURFACE CHEMISTRY AND CATALYSIS GABOR A. SOMORJAI
DEPARTMENT OF CHEMISTRY UNIVERSITY OF CALIFORNIA BERKELEY, CALIFORNIA A
WILEY-INTERSCIENCE PUBLICATION JOHN WILEY & SONS, INC. NEW YORK *
CHICHESTER * BRISBANE * TORONTO * SINGAPORE CONTENTS PREFACE XIII
GENERAL INTRODUCTION XV LISTS OF CONSTANTS XVII LIST OF SYMBOLS XIX 1
SURFACES * AN INTRODUCTION 1 1.1 HISTORICAL PERSPECTIVE, 1 1.2 SURFACES
AND INTERFACES*CLASSIFICATION OF PROPERTIES, 3 1.3 EXTERNAL SURFACES, 5
1.3.1 SURFACE CONCENTRATION, 5 1.3.1.1 CLUSTERS AND SMALL PARTICLES, 6
1.3.1.2 THIN FILMS, 8 1.3.2 INTERNAL SURFACES*MICROPOROUS SOLIDS, 10 1.4
CLEAN SURFACES, 12 1.5 INTERFACES, 13 1.5.1 ADSORPTION, 13 1.5.2
THICKNESS OF SURFACE LAYERS, 15 1.6 THE TECHNIQUES OF SURFACE SCIENCE,
15 1.7 SUMMARY AND CONCEPTS, 17 1.8 PROBLEMS, 17 REFERENCES, 18 2 THE
STRUCTURE OF SURFACES 36 2.1 INTRODUCTION, 36 2.2 SURFACE DIFFRACTION,
42 2.3 NOTATION OF SURFACE STRUCTURES, 43 2.3.1 ABBREVIATED NOTATION OF
SIMPLE SURFACE STRUCTURES, 45 2.3.2 NOTATION OF HIGH-MILLER-INDEX,
STEPPED SURFACES, 47 VII VIII CONTENTS 2.4 THE STRUCTURE OF CLEAN
SURFACES, 48 2.4.1 BOND-LENGTH CONTRACTION OR RELAXATION, 48 2.5
RECONSTRUCTION, 50 2.5.1 ATOMIC STEPS AND KINKS, 52 2.6 THE STRUCTURE OF
ADSORBED MONOLAYERS, 54 2.6.1 ORDERED MONOLAYERS AND THE REASONS FOR
ORDERING, 54 2.6.2 ADSORBATE-INDUCED RESTRUCTURING, 55 2.6.3 ATOMIC
ADSORPTION AND PENETRATION INTO SUBSTRATES, 58 2.6.4 METALS ON METALS:
EPITAXIAL GROWTH, 60 2.6.5 GROWTH MODES AT METAL SURFACES, 60 2.6.6
MOLECULAR ADSORPTION, 60 2.6.6.1 ETHYLENE, 62 2.6.6.2 BENZENE, 66 2.6.7
COADSORBED MONOLAYERS, 67 2.6.8 PHYSISORBED MONOLAYERS, 72 2.7 SUMMARY
AND CONCEPTS, 74 2.8 PROBLEMS, 74 REFERENCES, 75 3 THERMODYNAMICS OF
SURFACES 271 3.1 INTRODUCTION, 271 3.2 DEFINITION OF SURFACE
THERMODYNAMIC FUNCTIONS, 272 3.3 WORK NEEDED TO CREATE A SURFACE OF A
ONE-COMPONENT SYSTEM: SURFACE TENSION, 273 3.3.1 THE SURFACE FREE ENERGY
IS AIWAYS POSITIVE, 275 3.3.2 TEMPERATURE DEPENDENCE OF THE SPECIFIC
SURFACE FREE ENERGY, 277 3.3.3 SURFACE HEAT CAPACITY, 277 3.3.3.1
EXPERIMENTAL ESTIMATES, 277 3.3.3.2 THEORETICAL ESTIMATES, 278 3.4 THE
SURFACE ENERGY AND SURFACE COMPOSITION OF TWO- COMPONENT SYSTEMS, 282
3.4.1 THE WAGNER EXPERIMENT, 284 3.4.2 SURFACE SEGREGATION IN BINARY
ALLOY SYSTEMS, 285 3.4.3 SURFACE COMPOSITION OF ALLOYS FROM MODEL
CALCULATIONS, 289 3.5 SURFACES WHEN NO BULK PHASE EXISTS:
TWO-DIMENSIONAL PHASES, 291 3.5.1 MONOMOLECULAR FILMS, 291 3.6
METASTABLE SURFACE PHASES, 292 3.7 CURVED SURFACES, 293 3.7.1 CAPILLARY
RISE, 294 3.7.2 THE VAPOR PRESSURE OF CURVED SURFACES, 295 3.7.3 THE
CONTACT ANGLE AND ADHESION, 296 3.7.4 NUCLEATION, 298 3.8 THERMODYNAMICS
OF ADSORBED MONOLAYERS, 301 3.8.1 HEAT OF ADSORPTION, 301 3.8.2
TWO-DIMENSIONAL PHASE APPROXIMATION, 302 3.8.3 ADSORPTION ISOTHERMS, 302
CONTENTS IX 3.8.4 INTEGRAL AND DIFFERENTIAL HEATS OF ADSORPTION, 307
3.8.5 MOLECULAR AND DISSOCIATIVE ADSORPTION, 308 3.9 SUMMARY AND
CONCEPTS, 313 3.10 PROBLEMS, 314 REFERENCES, 315 4 DYNAMICS AT SURFACES
319 4.1 INTRODUCTION, 319 4.2 SURFACE ATOM VIBRATIONS, 319 4.2.1 THE
HARMONIE OSCILLATOR MODEL, 319 4.2.2 VIBRATIONAL MODES OF SURFACE ATOMS,
322 4.2.3 SURFACE MEAN-SQUARE DISPLACEMENTS, 322 4.2.4 VIBRATIONS OF
ADSORBED ATOMS AND MOLECULES, 324 4.3 ELEMENTARY PROCESSES OF
GAS-SURFACE INTERACTION, 329 4.3.1 ADSORPTION. ENERGY ACCOMMODATION
COEFFICIENTS, 331 4.3.2 STICKING PROBABILITY, 333 4.3.3 MODELS OF ENERGY
TRANSFER AND ADSORPTION, 336 4.3.4 SURFACE DIFFUSION, 340 4.3.5
MECHANISMS OF SURFACE DIFFUSION, 343 4.3.6 DESORPTION, 347 4.3.7
SURFACE-STRUCTURE SENSITIVITY OF THERMAL DESORPTION, 349 4.3.8
COLLISION-INDUCED DESORPTION, 350 4.3.9 ELECTRON-BEAM-INDUCED
DESORPTION, 351 4.3.10 PHOTON-STIMULATED DESORPTION, 351 4.3.11
ION-BEAM-INDUCED DESORPTION AND SPUTTERING, 351 4.4 SUMMARY AND
CONCEPTS, 352 4.5 PROBLEMS, 352 REFERENCES, 354 5 ELECTRICA! PROPERTIES
OF SURFACES 362 5.1 THE SURFACE ELECTRON POTENTIAL, 362 5.2 THE SURFACE
SPACE CHARGE, 363 5.2.1 THE SURFACE SPACE CHARGE AT THE SOLID-VACUUM
INTERFACE, 363 5.2.2 SURFACE SPACE CHARGE AT THE SOLID-LIQUID INTERFACE,
365 5.3 THE WORK FUNCTION, 366 5.3.1 EFFECT OF SURFACE ROUGHNESS ON WORK
FUNCTION, 367 5.3.2 CHANGE OF WORK FUNCTION WITH PARTICLE SIZE, 367 5.4
ADSORPTION-INDUCED CHARGE TRANSFER AT SURFACES: METALS AND INSULATORS,
369 5.4.1 CHARGE TRANSFER AT THE SOLID-SOLID INTERFACE, 375 5.4.2
GAS-PHASE ION PRODUCTION BY SURFACE IONIZATION: EMISSION OF POSITIVE AND
NEGATIVE IONS, 376 5.5 SURFACE ELECTRON DENSITY OF STATES, 378 5.6
ELECTRON EXCITATION AT SURFACES, 379 5.6.1 THERMAL EMISSION OF ELECTRONS
FROM SURFACES, 380 5.7 ELECTRON EMISSION FROM SURFACES BY INCIDENT
ELECTRON OR PHOTON BEAMS, 382 X CONTENTS 5.7.1 HIGH-RESOLUTION
ELECTRON-ENERGY-LOSS SPECTROSCOPY (HREELS), 384 5.7.2 X-RAY
PHOTOELECTRON SPECTROSCOPY (XPS), 386 5.7.3 AUGER ELECTRON SPECTROSCOPY
(AES), 389 5.8 FIELD ELECTRON EMISSION, 390 5.9 FIELD IONIZATION, 391
5.10 ELECTRON TUNNELING, 392 5.10.1 THE SCANNING TUNNELING MICROSCOPE
(STM), 392 5.11 SUMMARY AND CONCEPTS, 394 5.12 PROBLEMS, 394 REFERENCES,
395 6 THE SURFACE CHEMICAL BOND 400 6.1 INTRODUCTION, 400 6.2 BONDING
TRENDS ACROSS THE PERIODIC TABLE, 401 6.3 CLUSTER-LIKE BONDING OF
MOLECULAR ADSORBATES, 402 6.4 THE CARBON MONOXIDE CHEMISORPTION BOND,
409 6.5 ADSORBATE-INDUCED RESTRUCTURING. THE FLEXIBLE SURFACE, 412 6.6
THERMAL ACTIVATION OF BOND BREAKING, 417 6.7 SURFACE-STRUCTURE
SENSITIVITY OF BOND BREAKING, 419 6.8 COVERAGE DEPENDENCE OF BONDING AND
COADSORPTION, 425 6.8.1 COADSORPTION, 426 6.9 WEAK SURFACE BONDS, 430
6.9.1 PHASE TRANSFORMATIONS IN THE WEAKLY ADSORBED LAYER, 433 6.10
SUMMARY AND CONCEPTS, 436 6.11 PROBLEMS, 436 REFERENCES, 438 7 CATALYSIS
BY SURFACES 442 7.1 INTRODUCTION, 443 7.1.1 BRIEF HISTORY OF SURFACE
CATALYSIS, 444 7.2 CATALYTIC ACTION, 445 7.2.1 KINETIC EXPRESSIONS, 446
7.2.2 SELECTIVE CATALYSIS, 448 7.2.3 TABULATED KINETIC PARAMETERS FOR
CATALYTIC REACTIONS, 449 7.3 CATALYST PREPARATION, DEACTIVATION, AND
REGENERATION, 450 7.3.1 CATALYST PREPARATION, 450 7.3.2 CATALYST
DEACTIVATION, 451 7.3.3 CATALYST REGENERATION, 452 7.4 METAL CATALYSIS,
452 7.4.1 TRENDS ACROSS THE PERIODIC TABLE, 452 7.4.2 SOME FREQUENTLY
USED CONCEPTS OF METAL CATALYSIS, 454 7.5 CATALYSIS BY IONS AT SURFACES.
ACID-BASE CATALYSIS, 456 7.5.1 ACID CATALYSIS IN SOLUTIONS, 457 7.5.2
SOLID ACIDS, 458 7.5.3 CARBENIUM ION REACTIONS, 459 MOST FREQUENTLY USED
CATALYST MATENALS, 459 SURFACE-SCIENCE APPROACH TO CATALYTIC CHEMISTRY,
461 7.7.1 TECHNIQUES TO CHARACTERIZE AND STUDY THE REACTIVITY OF
SMALL-AREA CATALYST SURFACES, 463 7.7.1.1 HIGH-PRESSURE REACTORS, 463
7.7.1.2 COMPARISON OF THE REACTIVITIES OF SMALL- AND LARGE-SURFACE-AREA
CATALYSTS, 464 CASE HISTORIES OF SURFACE CATALYSTS, 465 7.8.1 AMMONIA
SYNTHESIS, 465 7.8.1.1 THERMODYNAMICS AND KINETICS, 465 7.8.1.1.1
KINETICS, 466 7.8.1.2 CATALYST PREPARATION, 466 7.8.1.3 ACTIVITY FOR
AMMONIA SYNTHESIS USING TRANSITION METALS ACROSS THE PERIODIC TABLE, 467
7.8.1.4 SURFACE SCIENCE OF AMMONIA SYNTHESIS, 467 7.8.1.4.1 STRUCTURE
SENSITIVITY OF AMMONIA SYNTHESIS, 467 7.8.1.4.2 KINETICS OF DISSOCIATIVE
NITROGEN ADSORPTION, 470 7.8.1.4.3 EFFECTS OF ALUMINUM OXIDE IN
RESTRUCTURING IRON SINGLE-CRYSTAL SURFACES FOR AMMONIA SYNTHESIS, 471
7.8.1.4.4 CHARACTERIZATION OF THE RESTRUCTURED SURFACES, 472 7.8.1.4.5
EFFECT OF POTASSIUM ON THE DISSOCIATIVE CHEMISORPTION OF NITROGEN ON
IRON SINGLE-CRYSTAL SURFACES IN UHV, 475 7.8.1.4.6
TEMPERATURE-PROGRAMMED DESORPTION STUDIES OF AMMONIA FROM IRON SURFACES
IN THE PRESENCE OF POTASSIUM, 477 7.8.1.4.7 EFFECTS OF POTASSIUM ON
AMMONIA SYNTHESIS KINETICS, 478 7.8.1.4.8 EFFECTS OF POTASSIUM ON THE
ADSORPTION OF AMMONIA ON IRON UNDER AMMONIA SYNTHESIS CONDITIONS, 480
7.8.1.5 MECHANISM AND KINETICS OF AMMONIA SYNTHESIS, 482 7.8.2
HYDROGENATION OF CARBON MONOXIDE, 483 7.8.2.1 THERMODYNAMICS, 483
7.8.2.2 CATALYST PREPARATION, 488 7.8.2.3 METHANATION. KINETICS, SURFACE
SCIENCE, MECHANISMS, 489 7.8.2.4 PROMOTION OF THE RATES OF C*O BOND
HYDROGENATION BY THE OXIDE-METAL INTERFACE, 491 7.8.2.5 METHANOL
PRODUCTION. KINETICS, SURFACE SCIENCE, AND MECHANISMS, 494 7.8.2.6
PRODUCTION OF HIGHER-MOLECULAR-WEIGHT HYDROCARBONS. KINETICS, SURFACE
SCIENCE, AND MECHANISMS, 495 XII CONTENTS 7.8.2.7 FORMATION OF
OXYGENATED HYDROCARBONS FROM CO AND H 2 AND ORGANIC MOLECULES, 500 7.8.3
HYDROCARBON CONVERSION ON PLATINUM, 500 7.8.3.1 INTRODUCTION, 500
7.8.3.2 STRUCTURE SENSITIVITY OF HYDROCARBON CONVERSION REACTIONS ON
PLATINUM SURFACES, 503 7.8.3.3 CARBONACEOUS OVERLAYERS, 505 7.8.3.4
CATALYSIS IN THE PRESENCE OF A STRONGLY ADSORBED OVERLAYER, 507 7.8.3.5
STRUCTURE MODIFIERS, 509 7.8.3.5.1 SITE BLOCKING BY SULFUR, 509
7.8.3.5.2 ENSEMBLE EFFECT IN ALLOY CATALYSIS AND THE CREATION OF NEW
SITES BY ALLOYS, 510 7.8.3.6 THE BUILDING OF IMPROVED PLATINUM AND OTHER
METAL CATALYSTS, 512 7.9 SUMMARY AND CONCEPTS, 513 7.10 PROBLEMS, 513
REFERENCES, 515 8 MECHANICAL PROPERTIES OF SURFACES 596 8.1
INTRODUCTION, 596 8.2 HISTORICAL PERSPECTIVE, 597 8.3 HARDNESS, 597 8.4
MECHANICAL FORCES REQUIRED TO BREAK A CHEMICAL BOND, 600 8.5 ADHESION,
602 8.6 SURFACES IN RELATIVE MOTION. TRIBOLOGY, 603 8.6.1 FRICTION AND
SLIDING, 603 8.6.2 HEATING BY FRICTION, 605 8.6.3 APPLICATIONS OF
FRICTION, 605 8.6.4 LUBRICATION, 606 8.7 SOLID LUBRICANTS. COATINGS, 609
8.7.1 COATINGS: MECHANICAL PROTECTION, 610 8.7.2 COATINGS: CHEMICAL
PROTECTION, 611 8.8 CRACK FORMATION AND PROPAGATION. FRACTURE, 611 8.9
SUMMARY AND CONCEPTS, 613 8.10 PROBLEMS, 613 REFERENCES, 614 ANSWERS TO
THE PROBLEMS 619 INDEX 643
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| spelling | Somorjai, Gabor A. Verfasser aut Introduction to surface chemistry and catalysis Gabor A. Somorjai New York u.a. Wiley 1994 XXIV, 667 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier A Wiley-Interscience publication Katalyse (DE-588)4029921-1 gnd rswk-swf Oberflächenchemie (DE-588)4126166-5 gnd rswk-swf Oberflächenchemie (DE-588)4126166-5 s Katalyse (DE-588)4029921-1 s DE-604 GBV Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=006470249&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Somorjai, Gabor A. Introduction to surface chemistry and catalysis Katalyse (DE-588)4029921-1 gnd Oberflächenchemie (DE-588)4126166-5 gnd |
| subject_GND | (DE-588)4029921-1 (DE-588)4126166-5 |
| title | Introduction to surface chemistry and catalysis |
| title_auth | Introduction to surface chemistry and catalysis |
| title_exact_search | Introduction to surface chemistry and catalysis |
| title_full | Introduction to surface chemistry and catalysis Gabor A. Somorjai |
| title_fullStr | Introduction to surface chemistry and catalysis Gabor A. Somorjai |
| title_full_unstemmed | Introduction to surface chemistry and catalysis Gabor A. Somorjai |
| title_short | Introduction to surface chemistry and catalysis |
| title_sort | introduction to surface chemistry and catalysis |
| topic | Katalyse (DE-588)4029921-1 gnd Oberflächenchemie (DE-588)4126166-5 gnd |
| topic_facet | Katalyse Oberflächenchemie |
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