Relaxation dynamics in molecular crystals:
Gespeichert in:
| 1. Verfasser: | |
|---|---|
| Format: | Abschlussarbeit Buch |
| Sprache: | German |
| Veröffentlicht: |
Berlin
Köster
1994
|
| Ausgabe: | 1. Aufl. |
| Schriftenreihe: | Wissenschaftliche Schriftenreihe Physik
12 |
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | 173 S. graph. Darst. |
| ISBN: | 3929937433 |
Internformat
MARC
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| 250 | |a 1. Aufl. | ||
| 264 | 1 | |a Berlin |b Köster |c 1994 | |
| 300 | |a 173 S. |b graph. Darst. | ||
| 336 | |b txt |2 rdacontent | ||
| 337 | |b n |2 rdamedia | ||
| 338 | |b nc |2 rdacarrier | ||
| 490 | 1 | |a Wissenschaftliche Schriftenreihe Physik |v 12 | |
| 502 | |a Zugl.: Düsseldorf, Univ., Habil.-Schr., 1994 | ||
| 650 | 4 | |a Molecular crystals | |
| 650 | 4 | |a Molecular relaxation | |
| 650 | 4 | |a Proton transfer reactions | |
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Datensatz im Suchindex
| _version_ | 1807502994384617472 |
|---|---|
| adam_text |
TABLE
OF
CONTENTS
I
INTRODUCTION
4
II
MOLECULAR
SYSTEMS
8
A
HOST
MATRIX
.
8
A.L
P-TERPHENYL
.
8
A.
1.1
CRYSTAL
STRUCTURE
.
8
A.
1.2
ELECTRONIC
STATES
AND
SPECTRA
.
11
A.
2
BENZOIC
ACID
.
12
A.
2.1
CRYSTAL
STRUCTURE
.
12
A.2.2
ELECTRONIC
STATES
AND
SPECTRA
.
15
B
GUEST
PROBE
MOLECULES:
TETRACENE
AND
PENTACENE
.
17
B.L
MOLECULAR
STRUCTURE
.
17
B.2
ELECTRONIC
STATES
AND
SPECTRA
.
18
C
GUEST-HOST
SYSTEMS
.
20
C.L
P-TERPHENYL
DOPED
WITH
TETRACENE
OR
PENTACENE
.
20
C.2
BENZOIC
ACID
DOPED
WITH
PENTACENE
.
20
III
EXPERIMENTAL
22
A
SAMPLE
PREPARATION
.
22
B
STATIONARY
SPECTROSCOPY
.
23
B.L
ABSORPTION
SPECTRA
.
23
B.2
FLUORESCENCE
AND
PHOSHORESCENCE
SPECTRA
.
24
1
TABLE
OF
CONTENTS
B.3
FLUORESCENCE
EXCITATION
SPECTRA
.
26
C
DYNAMIC
SPECTROSCOPY
.
27
C.L
FLUORESCENCE
LIFETIME
MEASUREMENT
.
27
C.2
TRANSIENT
GRATING
TECHNIQUE
.
28
IV
RESULTS
AND
DISCUSSION
30
A
PURE
CRYSTALS
(HOST
MATRICES)
.
30
A.L
P-TERPHENYL
.
30
A.
1.1
FLUORESCENCE
SPECTRUM
.
30
A.
1.1.
A
VIBRATIONAL
ANALYSIS
.
32
A.L.L.B
TEMPERATURE
DEPENDENCE
.
41
A.2
BENZOIC
ACID
.
42
A.2.1
FLUORESCENCE
AND
PHOSPHORESCENCE
SPECTRA
.
42
A.2.1.A
TEMPERATURE
DEPENDENCE
OF
THE
FLUORESCENCE
.
45
A.2.1.B
TEMPERATURE
DEPENDENCE
OF
THE
PHOSPHORESCENCE
.
49
B
DOPED
CRYSTALS
(GUEST-HOST
SYSTEM)
.
52
B.L
STATIONARY
GUEST
SPECTRA
.
52
B.L.L
P~TERPHENYL:TETRACENE
.
52
B.1.2
P-TERPHENYL:PENTACENE
.
55
B.1.3
BENZOIC
ACID:PENTACENE
.
58
B.2
INTRAMOLECULAR
RADIATIONLESS
PROCESSES
.
60
B.2.1
INTERSYSTEM
CROSSING
.
60
B.2.1.A
P-TERPHENYL:PENTACENE
.
60
B.2.1.A.L
THEORETICAL
MODEL
AND
CALCULATIONS
.
62
B.2.1.B
BENZOIC
ACID:PENTACENE-AI^
.
72
B.2.1.C
BENZOIC
ACID-D:PENTACENE- FO,I,S,3,^,5,6
.
74
B.2.1.C.L
DIRECT
FLUORESCENCE
LIFETIME
MEASUREMENTS
.
79
B.2.1.C.2
THEORETICAL
ANALYSIS
IN
TERMS
OF
THE
SHARF-SILBEY
MODEL
.
82
2
TABLE
OF
CONTENTS
B.3
INTERMOLECULAR
RADIATIONLESS
PROCESSES
.
87
B.3.1
SINGLET
EXCITATION
ENERGY
TRANSFER
VIA
HOST
BAND
.
87
B.3.1.A
P-TERPHENYL:TETRACENE
.
87
B.3.1.B
P-TERPHENYL:
PENT
ACENE
.
98
B.3.
2
SINGLET
EXCITATION
ENERGY
TRANSFER
VIA
GUEST
BAND
.
102
B.3.
3
ELECTRON-PHONON
INTERACTIONS
.
112
B.3.3.A
P-TERPHENYL:TETRACENE
.
112
B.3.3.A.L
FLUORESCENCE
AND
EXCITATION
SPECTRA
.
112
B.3.3.A.2
THEORETICAL
MODEL
AND
COMPUTATIONAL
SIMULATIONS
.
116
B.3.3.A.3
NATURE
OF
THE
PSEUDOLOCAL
PHONON
.
117
B.3.3.A.4
CALCULATION
OF
THE
INTENSITY
DISTRIBUTION
IN
THE
PHONON
SIDEBAND
118
B.3.3.A.5
TWO-DIMENSIONAL
MODEL
FOR
THE
SITE
REORIENTATION
PROCESS
.
.
.
121
B.3.3.B
P-TERPHENYL:PENTACENE
.
124
B.3.3.B.L
FLUORESCENCE
AND
EXCITATION
SPECTRA
.
125
B.3.3.B.2
THE
STRUCTURAL
NATURE
OF
THE
PHONON
SIDEBANDS
.
129
B.
3.3.B.3
CALCULATION
OF
THE
PSEUDOLOCAL
PHONONS
.
132
V
CONCLUSION
AND
SUMMARY
137
APPENDIX
A.
1
141
APPENDIX
A.
2
142
APPENDIX
A.
3
148
APPENDIX
A.
4
149
APPENDIX
A.5
152
APPENDIX
A.6
153
3 |
| any_adam_object | 1 |
| author | Kryschi, Carola 1957- |
| author_GND | (DE-588)112092241 |
| author_facet | Kryschi, Carola 1957- |
| author_role | aut |
| author_sort | Kryschi, Carola 1957- |
| author_variant | c k ck |
| building | Verbundindex |
| bvnumber | BV008837693 |
| callnumber-first | Q - Science |
| callnumber-label | QD921 |
| callnumber-raw | QD921 |
| callnumber-search | QD921 |
| callnumber-sort | QD 3921 |
| callnumber-subject | QD - Chemistry |
| classification_rvk | UM 4000 |
| ctrlnum | (OCoLC)30820058 (DE-599)BVBBV008837693 |
| dewey-full | 548.9 |
| dewey-hundreds | 500 - Natural sciences and mathematics |
| dewey-ones | 548 - Crystallography |
| dewey-raw | 548.9 |
| dewey-search | 548.9 |
| dewey-sort | 3548.9 |
| dewey-tens | 540 - Chemistry and allied sciences |
| discipline | Chemie / Pharmazie Physik |
| edition | 1. Aufl. |
| format | Thesis Book |
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| genre | (DE-588)4113937-9 Hochschulschrift gnd-content |
| genre_facet | Hochschulschrift |
| id | DE-604.BV008837693 |
| illustrated | Illustrated |
| indexdate | 2024-08-16T00:46:22Z |
| institution | BVB |
| isbn | 3929937433 |
| language | German |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-005843600 |
| oclc_num | 30820058 |
| open_access_boolean | |
| owner | DE-355 DE-BY-UBR DE-384 DE-634 DE-188 |
| owner_facet | DE-355 DE-BY-UBR DE-384 DE-634 DE-188 |
| physical | 173 S. graph. Darst. |
| publishDate | 1994 |
| publishDateSearch | 1994 |
| publishDateSort | 1994 |
| publisher | Köster |
| record_format | marc |
| series | Wissenschaftliche Schriftenreihe Physik |
| series2 | Wissenschaftliche Schriftenreihe Physik |
| spelling | Kryschi, Carola 1957- Verfasser (DE-588)112092241 aut Relaxation dynamics in molecular crystals Carola Kryschi 1. Aufl. Berlin Köster 1994 173 S. graph. Darst. txt rdacontent n rdamedia nc rdacarrier Wissenschaftliche Schriftenreihe Physik 12 Zugl.: Düsseldorf, Univ., Habil.-Schr., 1994 Molecular crystals Molecular relaxation Proton transfer reactions Molekülkristall (DE-588)4133483-8 gnd rswk-swf Relaxationsspektroskopie (DE-588)4177696-3 gnd rswk-swf Relaxation (DE-588)4049365-9 gnd rswk-swf Terphenyle (DE-588)4184784-2 gnd rswk-swf Benzoesäure (DE-588)4144531-4 gnd rswk-swf Optische Spektroskopie (DE-588)4043680-9 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Benzoesäure (DE-588)4144531-4 s Molekülkristall (DE-588)4133483-8 s Relaxationsspektroskopie (DE-588)4177696-3 s DE-604 Terphenyle (DE-588)4184784-2 s Relaxation (DE-588)4049365-9 s Optische Spektroskopie (DE-588)4043680-9 s Wissenschaftliche Schriftenreihe Physik 12 (DE-604)BV009162695 12 DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=005843600&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Kryschi, Carola 1957- Relaxation dynamics in molecular crystals Wissenschaftliche Schriftenreihe Physik Molecular crystals Molecular relaxation Proton transfer reactions Molekülkristall (DE-588)4133483-8 gnd Relaxationsspektroskopie (DE-588)4177696-3 gnd Relaxation (DE-588)4049365-9 gnd Terphenyle (DE-588)4184784-2 gnd Benzoesäure (DE-588)4144531-4 gnd Optische Spektroskopie (DE-588)4043680-9 gnd |
| subject_GND | (DE-588)4133483-8 (DE-588)4177696-3 (DE-588)4049365-9 (DE-588)4184784-2 (DE-588)4144531-4 (DE-588)4043680-9 (DE-588)4113937-9 |
| title | Relaxation dynamics in molecular crystals |
| title_auth | Relaxation dynamics in molecular crystals |
| title_exact_search | Relaxation dynamics in molecular crystals |
| title_full | Relaxation dynamics in molecular crystals Carola Kryschi |
| title_fullStr | Relaxation dynamics in molecular crystals Carola Kryschi |
| title_full_unstemmed | Relaxation dynamics in molecular crystals Carola Kryschi |
| title_short | Relaxation dynamics in molecular crystals |
| title_sort | relaxation dynamics in molecular crystals |
| topic | Molecular crystals Molecular relaxation Proton transfer reactions Molekülkristall (DE-588)4133483-8 gnd Relaxationsspektroskopie (DE-588)4177696-3 gnd Relaxation (DE-588)4049365-9 gnd Terphenyle (DE-588)4184784-2 gnd Benzoesäure (DE-588)4144531-4 gnd Optische Spektroskopie (DE-588)4043680-9 gnd |
| topic_facet | Molecular crystals Molecular relaxation Proton transfer reactions Molekülkristall Relaxationsspektroskopie Relaxation Terphenyle Benzoesäure Optische Spektroskopie Hochschulschrift |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=005843600&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| volume_link | (DE-604)BV009162695 |
| work_keys_str_mv | AT kryschicarola relaxationdynamicsinmolecularcrystals |