Essentials of molecular photochemistry:
Gespeichert in:
| Hauptverfasser: | , |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Oxford [u.a.]
Blackwell Scientific Publ.
1991
|
| Ausgabe: | 1. publ. |
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | XV, 538 S. zahlr. graph. Darst. |
| ISBN: | 0632024291 0632024283 |
Internformat
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Datensatz im Suchindex
| _version_ | 1804122050840756224 |
|---|---|
| adam_text | Essentials of
Molecular
Photochemistry
Andrew Gilbert
The University of Reading
Jim Baggott
Shell International Petroleum Company Ltd
FOREWORDBY
Peter J Wagner
CRC PRESS
BOCARATON • ANNARBOR • BOSTON • LONDON
Contents
Foreword, xi
Preface, xiii
Some Fundamental Physical Constants, xv
1 Molecular Photochemistry, 1
1 1 Introduction, 1
1 2 Thermal vs photochemical reactions, 3
1 3 The energies of photochemical conversions 4
1 4 Electronic states, 6
1 5 Fluorescence, phosphorescence and emission quenching 8
2 The Electronic Structures of Molecules, 11
2 1 Introduction, 11
2 2 The fundamentals of quantum mechanics, 12
221 Wave-particle duality, 12
222 Wavefunctions and the Schrodinger equation, 13
223 Operators, 16
224 The time-dependent Schrodinger equation, 18
225 The Indeterminacy Principle, 19
226 4i 2 as a probability density, 20
2 3 Atomic orbitals, 21
231 Pictures of electron orbitals, 21
232 Orbital energies, 23
233 Orbital angular momentum, 24
234 Electron spin, 27
235 Many-electron atoms, 29
236 Spin multiplicity and spin-orbit coupling, 32
2 4 Molecular orbitals, 32
241 The Born-Oppenheimer approximation, 33
242 The LCAO method, 33
243 Huckel molecular orbital theory, 36
244 Perturbation theory, 41
2 5 Molecular energy levels and state diagrams, 42
251 The electronic states of formaldehyde 42
252 Spin correlation, 43
253 State diagrams, 44
254 Molecular vibrations 45
2 6 Group theory and orbital symmetry 48
V
ViCONTENTS
261 Symmetry elements and operations, 48
262 Point groups, SO
263 Irreducible representations: character tables, 51
264 Orbital symmetry, 54
265 Vanishing integrals, 56
Bibliography, 57
Radiation and Molecular Orbitals, 59
3 1 Light, 59
311 Electromagnetic waves, 59
312 The electromagnetic spectrum, 61
313 Photons, 63
314 Polarization and photon spin, 64
3 2 Electric dipole transitions, 65
321 Molecular dipoles, 65
322 The interaction of molecules with radiation, 66
323 The transition dipole moment, 68
3 3 Selection rules and transition intensities, 71
331 Symmetry-forbidden transitions, 72
332 The Franck-Condon principle, 73
333 Vibronically allowed transitions, 76
334 Spin-forbidden transitions and spin-orbit coupling, 79
3 4 Molecular electronic spectroscopy, 81
341 Visible and near-u v spectroscopy, 81
342 Spectroscopy in condensed phases, 82
343 The Beer-Lambert absorption law, 83
344 Oscillator strengths, 84
345 Types of transition: chromophores, 87
Bibliography, 89
Molecular Photophysics, 91
4 1 The de-excitation of electronically excited molecules, 91
411 Radiative transitions, 91
412 Mirror symmetry, 93
413 Nonradiative transitions, 93
414 Vibrational relaxation, 95
415 The Jablonski diagram, 96
4 2 The kinetics of photophysical processes, 97
421 Radiative lifetimes, 97
422 Measured lifetimes, 99
423 Quantum yields, 100
424 The fluorescence quantum yield, 101
425 The phosphorescence quantum yield, 104
426 E-type delayed fluorescence, 107
4 3 The experimental study of radiative transitions, 109
431 Emission spectroscopy, 109
432 Emission quenching measurements, 111
CONTENTS VM
433 Flash photolysis, 113
434 Time-correlated single photon counting, 114
4 4 The experimental study of nonradiative transitions, 117
441 The experimental measurement of quantum yields, 117
442 The measurement of triplet quantum yields, 118
4421 Quenching methods, 118
4422 Triplet-sensitized isomerization, 121
4423 Electron spin resonance, 121
443 Rate coefficients for nonradiative processes, 122
4 5 The theory of nonradiative transitions, 123
451 Fermi s golden rule, 123
452 Selection rules for intersystem crossing, 126
453 Selection rules for internal conversion, 128
454 The Franck-Condon factor, 128
4 6 Stimulated emission and laser action, 131
461 The Einstein coefficients, 132
462 Population inversion, 133
463 Amplification of stimulated emission, 135
464 The optical cavity, 135
465 Dye lasers, 138
466 Q-switching and mode-locking, 139
References, 143
5 Photochemical Reactions, 145
5 1 Excimers, 145
511 Excimer fluorescence, 147
512 The quantum yield for excimer fluorescence, 149
513 Excimer kinetics, 151
514 High-temperature limiting behavior, 153
515 Thermodynamic parameters and excimer structure, 154
516 P-type delayed fluorescence, 155
5:2 Exciplexes, 157
521 Exciplex classification, 157
522 Exciplex thermodynamics, 159
523 Exciplex fluorescence,, 160
524 Exciplex kinetics, 162
525 Exciplex structure and solvent polarity, 164
526 The external heavy atom effect, 167
527 Quenching by molecular oxygen, 168
5 3 Electronic energy transfer, 168
531 Radiative energy transfer, 170
532 Nonradiative energy transfer, 171
533 Long-range Coulombic energy transfer, 172
534 Short-range electron-exchange energy transfer, 175
535 Triplet-triplet energy transfer and sensitization, 176
536 Diffusion-controlled emission quenching, 178
ViijCONTENTS
54 Photoinduced electron transfer, 182
541 The kinetics of electron transfer quenching, 183
542 The thermodynamics of electron transfer, 183
543 Marcus theory, 184
544 The inverted region, 187
5 5 Pericyclic reactions, 188
551 Orbital correlations, 189
552 State correlation diagrams, 191
553 Allowed and forbidden reactions, 193
554 Frontier orbitals, 194
555 Orbital symmetry and stereochemistry, 196
556 The Woodward-Hoffmann rules, 198
557 Orbital symmetry in electrocyclic reactions, 199
558 Orbital symmetry in sigmatropic rearrangements, 203
559A note of caution, 205
5 6 The experimental study of photochemical reactions, 206
561 Product analysis, 206
562 Chemical methods in the study of intermediates, 208
563 Spectroscopic methods, 211
564 Electron spin resonance and CIDNP, 214
565 Rate coefficients for photochemical processes, 221
566 The identification of excited states, 223
References, 227
6 Photochemical Reactions of Ethenes, Polyenes,
and Ethynes, 229
6 1 Introduction, 229
6 2 Geometrical isomerization, 230
6 3 Sigmatropic shifts, 241
6 4 The di-Tt-methane rearrangement, 246
6 5 Reactions of /J,y-enones, 252
6 6 Electrocyclic processes, 256
6 7 Addition reactions, 263
671 Acyclic addition processes, 263
672 Cycloaddition processes, 267
References, 284
7 Photochemical Reactions of the Carbonyl Chromophore, 287
7 1 Introduction, 287
7 2 a-cleavage reactions, 288
7 3 Hydrogen abstraction by the carbonyl group, 302
731 Intermolecular hydrogen abstraction, 302
732 Intramolecular hydrogen abstraction, 310
7 4 Reactions of carboxylic acids and derivatives, 328
7 5 Enone and dienone rearrangements, 330
7 6 Cycloaddition of the carbonyl group to ethenes, dienes, and ethynes, 340
References, 352
CONTENTSiX
8 Aromatic Photochemistry, 355
8 1 Introduction, 3SS
8 2 Ring isomerization reactions, 357
8 3 Photoaddition reactions, 365
831 Acyclic addition to the aromatic ring, 366
832 Cycloadditions to the aromatic ring, 372
8321 Ethenes, 373
8322 1,3-dienes, 381
8323 Ethynes, 383
8324 Additions of C—N multiple bonds, 384
8 4 Substitution, 386
8 5 Cyclization reactions, 391
851 Intramolecular coupling of arenes, 391
852 Cyclization of arene-ethene bichromophoric systems, 394
853 Reactions of aryl 1,2 substituents, 397
854 Cyclodehydrohalogenation, 399
8 6 Dimerization reactions, 401
861 Intermolecular processes, 401
862 Intramolecular processes, 405
8 7 Lateral-nuclear rearrangements, 407
References, 409
9 Photochemical Reactions of Nitrogen-containing
Chromophores, 411
9 1 Amines, 411
9 2 JTC=N—R chromophores, 412
9 3 N-oxides and related nitrogen chromophores, 425
9 4 Nitriles, 432
9 5 Nitrites, 433
9 6 Nitro compounds, 436
9 7 Azo compounds, 442
9 8 Diazo compounds, azides and diazonium salts, 450
References, 455
10 The Photochemistry of Other Organic
Chromophores, 457
10 1 Alkanes and cycloalkanes, 457
10 2 Alkyl halides, 462
10 3 Alcohols, ethers, and peroxides, 468
10 4 Hypohalites, 475
10 5 Sulfur-containing chromophores, 477
10 5 1 Thiols, sulfides and disulfides, 477
10 5 2 Thiocarbonyl compounds (thiones), 479
10 5 3 Sulfoxides, 490
10 5 4 Sulfones, 493
10 5 5 Sulfonic acid derivatives, 495
References, 498
XCONTENTS
11 Photo-oxygenation Reactions, 501
11 1 Introduction, SO 1
11 2 Electronic states of molecular oxygen, SOI
11 3 Reactions involving photogenerated radicals and radical ions, S03
11 3 1 Radical chain processes, S03
11 3 2 Radical ions—electron-transfer-sensitized photo-oxygenations, 505
11 4 Photo-oxygenation involving singlet oxygen, 511
11 4 1 Ene reaction, 512
11 4 2 Formation of dioxetanes by 02 cycloaddition to ethenes, 516
11 4 3 Photo-oxygenation of thiocarbonyl compounds, 518
11 4 4 (27t + 47r) addition of 02 to 1,3-dienes, 520
References, 525
Index, 527
|
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| language | English |
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| spelling | Gilbert, Andrew Verfasser aut Essentials of molecular photochemistry Andrew Gilbert ; Jim Baggott 1. publ. Oxford [u.a.] Blackwell Scientific Publ. 1991 XV, 538 S. zahlr. graph. Darst. txt rdacontent n rdamedia nc rdacarrier Chromoforen gtt Elektromagnetische straling gtt Elektronenbanen gtt Elektronenstructuur gtt Fotochemie gtt Fotofysische eigenschappen gtt Photochimie Photochimie ram Photochemistry Fotochemie (DE-588)4045873-8 gnd rswk-swf Selbstreplikation (DE-588)4481488-4 gnd rswk-swf Organische Chemie (DE-588)4043793-0 gnd rswk-swf Fotochemie (DE-588)4045873-8 s Organische Chemie (DE-588)4043793-0 s DE-604 Selbstreplikation (DE-588)4481488-4 s Baggott, Jim 1957- Verfasser (DE-588)132721600 aut HEBIS Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=005047955&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Gilbert, Andrew Baggott, Jim 1957- Essentials of molecular photochemistry Chromoforen gtt Elektromagnetische straling gtt Elektronenbanen gtt Elektronenstructuur gtt Fotochemie gtt Fotofysische eigenschappen gtt Photochimie Photochimie ram Photochemistry Fotochemie (DE-588)4045873-8 gnd Selbstreplikation (DE-588)4481488-4 gnd Organische Chemie (DE-588)4043793-0 gnd |
| subject_GND | (DE-588)4045873-8 (DE-588)4481488-4 (DE-588)4043793-0 |
| title | Essentials of molecular photochemistry |
| title_auth | Essentials of molecular photochemistry |
| title_exact_search | Essentials of molecular photochemistry |
| title_full | Essentials of molecular photochemistry Andrew Gilbert ; Jim Baggott |
| title_fullStr | Essentials of molecular photochemistry Andrew Gilbert ; Jim Baggott |
| title_full_unstemmed | Essentials of molecular photochemistry Andrew Gilbert ; Jim Baggott |
| title_short | Essentials of molecular photochemistry |
| title_sort | essentials of molecular photochemistry |
| topic | Chromoforen gtt Elektromagnetische straling gtt Elektronenbanen gtt Elektronenstructuur gtt Fotochemie gtt Fotofysische eigenschappen gtt Photochimie Photochimie ram Photochemistry Fotochemie (DE-588)4045873-8 gnd Selbstreplikation (DE-588)4481488-4 gnd Organische Chemie (DE-588)4043793-0 gnd |
| topic_facet | Chromoforen Elektromagnetische straling Elektronenbanen Elektronenstructuur Fotochemie Fotofysische eigenschappen Photochimie Photochemistry Selbstreplikation Organische Chemie |
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