Interaction of atoms and molecules with solid surfaces:
Gespeichert in:
| Format: | Buch |
|---|---|
| Sprache: | English |
| Veröffentlicht: |
New York u.a.
Plenum Press
1990
|
| Schriftenreihe: | Physics of solids and liquids
|
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | XX, 679 S. graph. Darst. |
| ISBN: | 0306434245 |
Internformat
MARC
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| 650 | 4 | |a Chimie des surfaces | |
| 650 | 4 | |a Molécules | |
| 650 | 4 | |a Surfaces (Physique) | |
| 650 | 4 | |a Atoms | |
| 650 | 4 | |a Molecules | |
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Datensatz im Suchindex
| _version_ | 1804118507711889408 |
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| adam_text | INTERACTION OF ATOMS AND MOLECULES WITH SOLID SURFACES EDITED BY V.
BORTOLANI UNIVERSITY OF MODENA MODENA, ITALY N. H. MARCH UNIVERSITY OF
OXFORD OXFORD, ENGLAND AND M. P. TOSI INTERNATIONAL CENTER FOR
THEORETICAL PHYSICS TRIESTE, ITALY PLENUM PRESS * NEW YORK AND LONDON
CONTENTS 1. CHEMICAL BONDS OUTSIDE SOLID SURFACES 1 N. H. MARCH 1.1.
INTRODUCTION 1 1.2. PHYSISORPTION ON A PLANAR CONDUCTING SURFACE 2
1.2.1. BOND IN A MOLECULE WITH WEIL-DEFINED CORES 2 1.2.2. APPLICATION
TO COVERAGE DEPENDENCE OF DESORPTION ENERGY OF XE ON PT 3 1.2.3. CASE OF
A H 2 MOLECULE: MODIFICATION OF HEITLER-LONDON THEORY TO INCLUDE IMAGE
EFFECTS 4 1.2.4. INSULATING AND SEMICONDUCTING SURFACES AS WELL AS
METALS . 5 1.3. CHEMISORPTION ON METALLIC SURFACES 6 1.3.1. ELEMENTARY
METAL MODELS 6 1.3.2. RELATION OF LONG-RANGE OSCILLATIONS IN PERTURBED
ELECTRON DENSITY TO LATERAL INTERACTIONS BETWEEN CHEMISORBED SPECIES 7
1.3.3. HYDROGEN CHEMISORBED ON A PT SURFACE 9 1.3.4. LATERAL INTERACTION
BETWEEN TWO CO MOLECULES CHEMISORBED ON PT 9 1.4. MOLECULAR VERSUS
DISSOCIATIVE ADSORPTION ON TRANSITION METAL SURFACES 10 1.4.1.
REACTIVITY OF METAL TOWARD A MOLECULAR ADSORBATE . . . . 11 1.4.2.
BONDING AND VALENCE IN TRANSITION METALS 12 1.4.2.1. RESONATING BONDS 12
1.4.2.2. CALCULATION OF AVERAGE VALENCE 12 1.4.3. ADMOLECULE BONDING TO
A METAL SURFACE 14 1.5. SUMMARY AND SOME FUTURE DIRECTIONS 15 APPENDIXES
16 REFERENCES 23 IX X CONTENTS 2. GAS-SURFACE INTERACTIONS: BASIC
THERMODYNAMICS AND RECENT WORK ON STICKING 25 T. B. GRIMLEY 2.1.
INTRODUCTION 25 2.2. PHYSISORPTION AND CHEMISORPTION 26 2.2.1. GENERAL
26 2.2.2. SURFACE RESIDENCE TIMES 27 2.3. THERMODYNAMICS OF ADSORPTION
28 2.4. STATISTICAL THERMODYNAMICS OF ADSORPTION 30 2.4.1. BASICS 30
2.4.2. LANGMUIR S MODEL 31 2.4.3. TWO-DIMENSIONAL LATTICE GAS 32 2.4.4.
TWO-DIMENSIONAL VAN DER WAALS GAS 33 2.5. RATE OF ADSORPTION 34 2.5.1.
GENERAL 34 2.5.2. THEORETICAL DESCRIPTION OF STICKING 35 2.5.2.1.
GENERAL 35 2.5.2.2. STICKING ON A COLD SOLID 35 2.5.2.3. THE HAMILTONIAN
40 2.5.2.4. STICKING ON A SOLID AT FINITE TEMPERATURE . . . . 42
2.5.2.5. LOSS TO ELECTRONS 43 2.5.2.6. LOSS TO PHONONS 45 2.5.2.7. THE
SEMICLASSICAL METHOD (TRAJECTORY APPROXIMATION) 47 APPENDIXES 51
REFERENCES 52 3. THEORY OF ATOM-SURFACE COLLISIONS 53 W. KOHN 3.1.
INTRODUCTION 53 3.2. PART 1: THE RIGID TARGET MODEL 54 3.2.1. THE
ATOMIC-SURFACE INTERACTION POTENTIAL* A PRIORI CALCULATIONS 54 3.2.1.1.
LONG-RANGE POLARIZATION (VAN DER WAALS) ATTRACTION . 54 3.2.1.2. THE
POTENTIAL AT SHORTER DISTANCES 55 3.2.2. CALCULATIONS OF ATOM-SURFACE
SCATTERING 60 3.2.3. THE ATOM-SURFACE INTERACTION POTENTIAL FROM
EMPIRICAL DATA 61 3.2.3.1. BOUND STATE LEVELS; V 0 (R) 62 3.2.3.2.
ELASTIC DIFFRACTION SCATTERING; V G (Z) 62 3.2.3.3. DEBYE-WALLER
REDUCTION OF ELASTIC SCATTERING PROCESSES 63 CONTENTS XI 3.3. PART 2:
DYNAMICS OF INTERACTING INCIDON AND TARGET ATOMS . . . 63 3.3.1.
FORMULATION 63 3.3.2. REGIMES 65 3.3.3. CLASSICAL REGIME 65 3.3.4.
QUANTUM EFFECTS 65 3.3.4.1. THE EXTREME QUANTUM REGIME 66 3.3.4.2.
QUANTUM CORRECTIONS IN NEARLY CLASSICAL REGIMES . 67 REFERENCES 69 4.
BASIC VIBRATIONAL PROPERTIES OF SURFACES 71 F. GARCIA-MOLINER 4.1.
GENERALITIES ON LATTICE DYNAMICS 71 4.2. EQUATIONS OF MOTION AND FORCE
CONSTANTS 73 4.3. DYNAMICAL MATRIX AND EIGENVECTORS 75 4.4. SOME
PRACTICAL EXAMPLES 77 4.5. THE LAYER DESCRIPTION OF LATTICE DYNAMICS 80
4.6. SURFACE WAVES: A SUMMARY OF THE LONG-WAVE LIMIT 82 4.7. SURFACE
PHONON CALCULATIONS 87 4.8. LATTICE DYNAMICS IN TERMS OF GREEN
FUNCTIONS 89 4.9. SURFACE DYNAMICS IN TERMS OF GREEN FUNCTIONS 91 4.10.
EXAMPLES OF APPLICATION 94 4.11. SURFACE PHONON SPECTRA AND INELASTIC
ATOM-SURFACE SCATTERING DATA 103 APPENDIXES 108 BIBLIOGRAPHY 114
REFERENCES 115 5. ELECTRONIC STRUCTURE OF METAL SURFACES 117 J. E.
INGLESFIELD 5.1. INTRODUCTION 117 5.2. SURFACE PERIODICITY AND THE
TWO-DIMENSIONAL BLOCH PROPERTY . . 118 5.3. BULK STATES AT THE SURFACE
122 5.3.1. LOCAL DENSITY OF STATES 125 5.3.2. BAND NARROWING AT THE
SURFACE 126 5.4. SURFACE STATES 131 5.4.1. SHOCKLEY STATES 131 5.4.2.
TAMM STATES 134 5.4.3. IMAGE POTENTIAL STATES 138 X)! CONTENTS 5.5. THE
SURFACE OF JELLIUM 141 5.6. CALCULATING SURFACE ELECTRONIC STRUCTURE 145
5.7. PLASMONS AND MANY-BODY EFFECTS 148 REFERENCES 152 6. BASIC
STRUCTURAL AND ELECTRONIC PROPERTIES OF SEMICONDUCTOR SURFACES 155 C. M.
BERTONI 6.1. INTRODUCTION 155 6.2. ELECTRONIC SURFACE STATES: SIMPLE
MODELS 156 6.2.1. ONE-DIMENSIONAL CHAIN OF ATOMS 156 6.2.2. EVANESCENT
WAVE FUNCTIONS, TRUNCATED CHAIN, AND SURFACE STATES 158 6.2.3. COMPLEX-^
ENERGY DISPERSION AND MATCHING CONDITIONS . 159 6.2.4. TIGHT-BINDING
MODEL FOR THE LINEAR CHAIN 160 6.2.5. CLASSIFICATION OF SURFACE STATES
163 6.3. SURFACES IN THREE DIMENSIONS 164 6.3.1. SURFACE PERIODICITY:
IDEAL, RELAXED, AND RECONSTRUCTED SURFACES 164 6.3.2. OBSERVATION OF THE
ELECTRONIC STRUCTURE OF SURFACES . . . . 166 6.3.3. REMAPPING OF THE
BULK STATES: THE PROJECTED BULK BAND STRUCTURE 167 6.3.4. FINITE-SLAB
CALCULATIONS. SURFACE BANDS AND LOCAL DENSITY OF STATES 170 6.3.5.
SURFACE STATES IN THE GAP OF SEMICONDUCTORS, BAND BENDING, AND
FERMI-LEVEL PINNING 173 6.3.6. THE EMPIRICAL TIGHT-BINDING METHOD 175
6.3.7. APPLICATION TO THE CLEAVAGE SURFACES OF III-V COMPOUNDS 176 6.4.
FIRST-PRINCIPLES DESCRIPTION OF THE SURFACE ELECTRONIC STRUCTURE AS A
FUNCTION OF THE ATOMIC CONFIGURATION 179 6.4.1. DENSITY FUNCTIONAL
THEORY AND THE LOCAL DENSITY APPROXIMATION 179 6.4.2. THE
SELF-CONSISTENT POTENTIAL IN A REPEATED-SLAB CALCULATION 181 6.4.3.
LIMITS OF THE LOCAL DENSITY APPROXIMATION AND OF THE DENSITY FUNCTIONAL
THEORY 186 6.5. THE ELECTRONIC STATES AND THE STRUCTURE OF SEMICONDUCTOR
SURFACES 187 6.5.1. THE SI(LLL) (2 X 1) SURFACE 187 6.5.2. THE SI(L 11)
(7X7) SURFACE 192 6.5.3. OTHER SURFACES OF COVALENT SEMICONDUCTORS 195
6.5.4. POLAR SURFACES OF IONIC SEMICONDUCTORS 196 6.5.5. OVERLAYERS AND
INTERFACES 196 6.6. CONCLUSIONS 198 REFERENCES 199 CONTENTS XIII 7.
LOW-ENERGY ELECTRON DIFFRACTION 201 J. *. PENARY 7.1. LOW-ENERGY
ELECTRON DIFFRACTION EXPERIMENTS 201 7.2. TYPICAL EXPERIMENTAL DATA 202
7.3. THEORETICAL PROBLEMS 203 7.4. KINEMATIC THEORY 204 7.5. MULTIPLE
SCATTERING 208 REFERENCES 211 8. THEORETICAL ASPECTS OF ADSORPTION 213
B. I. LUNDQVIST 8.1. INTRODUCTION 213 8.2. QUESTIONS POSED BY
EXPERIMENTS 215 8.2.1. STATIC EXPERIMENTS 215 8.2.2. MOLECULAR
VIBRATIONS AND ROTATIONS AT SURFACES 216 8.2.3. CATALYTIC REACTIONS 217
8.2.3.1. AMMONIA SYNTHESIS 217 8.2.3.2. METHANATION 218 8.2.3.3.
POTENTIAL-ENERGY FEATURES TO BE EXPLAINED . . . . 218 8.3. MAKING BONDS
AT A SURFACE 219 8.3.1. SEPARATED ADSORBATE AND SUBSTRATE 219 8.3.1.1.
NEUTRAL ADSORBATE 219 8.3.1.2. CHARGED ADSORBATE 220 8.3.1.3. CHARGE
TRANSFER 220 8.3.2. PAULI REPULSION 220 8.3.3. PHYSISORPTION 221
8.3.3.1. INERT ATOMS AND MOLECULES 221 8.3.3.2. REACTIVE SPECIES WITH
FROZEN ELECTRON CONFIGURATIONS 222 8.3.4. REACTIVE ADSORBATES 222
8.3.4.1. CHEMISORPTION 222 8.3.4.2. SOME CHEMISORPTION CALCULATIONS 226
8.3.4.3. SYSTEMATICS 230 8.4. BREAKING MOLECULAR BONDS AT SURFACES 238
8.4.1. APPLICATION OF SIMPLE RULES 238 8.4.2. HYDROGEN ADSORPTION ON AN
MG SURFACE 239 8.4.3. CONCEPTUAL PICTURE OF DISSOCIATIVE ADSORPTION 240
8.5. APPLICATIONS 243 8.5.1. MODIFICATION OF POTENTIAL-ENERGY SURFACES
244 8.5.1.1. CHANGE OF SUBSTRATE OR SURFACE . 244 8.5.1.2. CHANGE OF
SITE AND OVERLAP 244 XIV CONTENTS 8.5.1.3. APPLICATION OF ELECTRIC FIELD
245 8.5.1.4. CHANGE OF WORK FUNCTION 245 8.5.1.5. CHANGE OF
ELECTROSTATIC POTENTIAL 245 8.5.2. EQUILIBRIUM PROPERTIES 246 8.5.3.
MOLECULAR VIBRATIONS AND ROTATIONS AT SURFACES 246 8.5.4. ELECTRONIC
FACTOR IN CATALYSIS 247 8.5.4.1. ROLE OF TRANSITION METALS 247 8.5.4.2.
POISONS AND PROMOTERS 248 8.6. CONCLUDING REMARKS 249 REFERENCES 250 9.
ELECTRONIC THEORY OF CHEMISORPTION 255 D. SPANJAARD AND M. C.
DESJONQUERES 9.1. INTRODUCTION 255 9.2. OUTLINE OF THE PROBLEM 259
9.2.1. IONIZATION LEVEL 260 9.2.2. AFFINITY LEVEL 260 9.3. THE
ANDERSON-GRIMLEY-NEWNS HAMILTONIAN 261 9.3.1. HARTREE-FOCK TREATMENT 262
9.3.1.1. LOCAL DENSITY OF STATES ON THE ADSORBATE 263 9.3.1.2. BINDING
ENERGY 271 9.3.1.3. DISCUSSION 275 9.3.2. BEYOND THE HARTREE-FOCK
TREATMENT 276 9.4. A SIMPLE CHEMISORPTION MODEL FOR TIGHT-BINDING
SYSTEMS . . . 278 9.4.1. MODELS 279 9.4.1.1. GENERAL CHARACTERISTICS 279
9.4.1.2. ANALYTICAL MODELS 280 9.4.1.3. IMPROVED MODELS 285 9.4.2.
ADSORPTION OF SIMPLE ELEMENTS ON BCC TRANSITION METAL SURFACES 288
9.4.2.1. LOW-INDEX FACES 289 9.4.2.2. STEPPED SURFACES 297 9.5. BRIEF
SUMMARY OF OTHER METHODS 301 9.5.1. EFFECTIVE MEDIUM THEORY 301 9.5.2.
QUANTUM CHEMISTRY METHODS 302 9.6. ADSORPTION OF HOMONUCLEAR DIATOMIC
MOLECULES ON METALS . . . 303 9.6.1. OUTLINE OF THE PROBLEM 303 9.6.2.
ADIABATIC POTENTIAL-ENERGY SURFACES FOR DIATOMIC MOLECULES ON TRANSITION
METAL SURFACES 305 9.7. CONCLUSIONS 314 APPENDIXES 314 REFERENCES 321
CONTENTS XV 10. SURFACE VIBRATION SPECTROSCOPY 325 H. IBACH 10.1.
INTRODUCTION 325 10.2. EXPERIMENTAL TECHNIQUES FOR SURFACE VIBRATION
SPECTROSCOPY . . 326 10.2.1. OVERVIEW 326 10.2.2. INFRARED REFLECTION
ABSORPTION SPECTROSCOPY 326 10.2.3. INELASTIC HELIUM SCATTERING 328
10.3. ELECTRON ENERGY LOSS SPECTROSCOPY 332 10.3.1. GENERAL
CONSIDERATIONS 332 10.3.2. CATHODE SYSTEM 333 10.3.3. CYLINDRICAL
DEFLECTORS 333 10.3.4. LENS SYSTEMS AND PERFORMANCE OF SPECTROMETERS . .
. . 336 10.4. ELECTRON-SOLID INTERACTION 338 10.4.1. DIPOLE
SCATTERING*DIELECTRIC THEORY 338 10.4.2. ELECTRON-ION CORE SCATTERING
(INELASTIC ELECTRON DIFFRACTION) 342 10.4.3. RESONANCE SCATTERING 344
10.5. LOCALIZED VIBRATIONS AT SURFACES 346 10.5.1. VIBRATIONS AND THE
CHEMICAL BOND 346 10.5.2. SELECTION RULES AND LOCAL SYMMETRY 348 10.6.
SURFACE PHONONS: FORCE CONSTANT MODELS 349 10.7. EPITAXIAL METAL
OVERLAYERS 351 10.7.1. GENERAL REMARKS 351 10.7.2. EPITAXIALLY GROWN
IRON OVERLAYERS ON CU(100) 353 REFERENCES 356 11. SCANNING TUNNELING
MICROSCOPY 357 R. M. FEENSTRA 11.1. INTRODUCTION 357 11.2. BASIC
PRINCIPLES 358 11.3. THEORY 361 11.4. EXAMPLE: THE SI(L 11)2 X 1 SURFACE
366 11.4.1. MICROSCOPY 366 11.4.2. SPECTROSCOPY 375 11.5. SUMMARY 379
REFERENCES 379 12. DEFECT STRUCTURES AT SURFACES 381 J. LAPUJOULADE
12.1. INTRODUCTION TO SURFACE DEFECTS 381 XVI CONTENTS 12.2.
EXPERIMENTAL CHARACTERIZATION OF SURFACE DEFECTS 382 12.2.1. SURFACE
MICROSCOPY 383 12.2.2. DIFFRACTION TECHNIQUES 383 12.2.3. THERMAL ENERGY
ATOM SCATTERING (TEAS) 384 12.3. PHYSICS OF AN ISOLATED DEFECT 386
12.3.1. ENERGY ASSOCIATED WITH THE CREATION OF A DEFECT . . . . 386
12.3.2. ENTROPY FORMATION OF A DEFECT 387 12.3.3. RELAXATION EFFECTS 387
12.4. INTERACTION BETWEEN DEFECTS 388 12.4.1. SHORT-RANGE INTERACTION
388 12.4.2. LONG-RANGE INTERACTION 389 12.5. STATISTICS OF DEFECTS: THE
ROUGHENING TRANSITION 389 12.5.1. THE BCF ARGUMENT 390 12.5.2. A
RENORMALIZATION APPROACH 391 12.5.3. APPLICATION TO DISCRETE MODELS:
SOS, DGSOS, BCSOS . 393 12.5.4. CONSEQUENCES OF THE ROUGHENING
TRANSITION FOR CRYSTAL SHAPES 395 12.6. THE ROUGHENING TRANSITION ON
VICINAL SURFACES 395 12.6.1. STATISTICAL EQUILIBRIUM OF AN ISOLATED STEP
396 12.6.2. STATISTICS OF A VICINAL SURFACE 397 12.6.2.1.
RENORMALIZATION APPROACH 397 12.6.2.2. DISCRETE MODEL 398 12.6.3.
EXPERIMENTAL RESULTS 399 12.7. MOBILITY OF DEFECTS 402 12.8. CONCLUSION
403 REFERENCES . 404 13. MOLECULAR SCATTERING FROM SURFACES (THEORY) 407
A. E. DEPRISTO 13.1. INTRODUCTION AND SCATTERING FROM RIGID SURFACES 407
13.2. LOW-ENERGY EXCITATIONS: PHONONS AND ELECTRON-HOLE PAIRS . . . 413
13.3. SCATTERING FROM NONRIGID SURFACES 423 13.4. DISSOCIATIVE
CHEMISORPTION: THE MODEL 430 13.5. DISSOCIATIVE CHEMISORPTION: RESULTS
438 REFERENCES 457 14. THE STRUCTURE OF MOLECULES ON SURFACES AS
DETERMINED USING ELECTRON- STIMULATED DESORPTION 459 T. E. MADEY, S. A.
JOYCE, AND A. L. JOHNSON 14.1. INTRODUCTION 459 14.2. GENERAL
EXPERIMENTAL OBSERVATIONS 461 CONTENTS XVII 14.3. MECHANISMS OF ESD AND
PSD 462 14.4. EXPERIMENTAL PROCEDURES 464 14.5. EXAMPLES OF THE USE OF
ESDIAD 467 14.5.1. ESDIAD OF POSITIVE IONS 467 14.5.1.1. NH 3 ON METALS
467 14.5.1.2. H 2 0, NH 3 , AND HF ON SI(100) 471 14.5.2. ESDIAD OF
NEGATIVE IONS 473 14.6. SUMMARY AND CONCLUSIONS 474 REFERENCES 475 15.
PHOTOEMISSION FROM ADSORBATES 477 A. M. BRADSHAW 15.1. GENERAL
CONSIDERATIONS 477 15.1.1. INTRODUCTION 477 15.1.2. PHOTOELECTRON
SPECTROSCOPY OF FREE MOLECULES 478 15.1.3. THE SURFACE CASE 483 15.1.4.
EXPERIMENTAL ASPECTS 487 15.2. VALENCE-LEVEL PHOTOEMISSION FROM ADSORBED
MOLECULES . . . . 489 15.2.1. SELECTION RULES 489 15.2.2. CO ADSORPTION
492 15.2.3. BENZENE ADSORPTION 495 15.2.4. THE SURFACE FORMATE SPECIES
497 15.3. ADSORBATE-INDUCED SURFACE BAND STRUCTURES 500 15.3.1. GENERAL
REMARKS 500 15.3.2. PHYSISORPTION OF RARE GASES 503 15.3.3. CHALCOGEN
ADSORPTION 504 15.3.4. BAND FORMATION IN CO LAYERS 508 15.4. CORE-LEVEL
PHOTOEMISSION FROM ADSORBATES 511 15.4.1. INTRODUCTION 511 15.4.2.
FINGERPRINTING: CO, NO, AND N 2 ADSORPTION 513 15.4.3. SURFACE AND
INTERFACE REACTIONS 518 15.4.4. PHOTOELECTRON DIFFRACTION 521 REFERENCES
526 16. RATE EQUATIONS, RATE CONSTANTS, AND SURFACE DIFFUSION 529 G.
WAHNSTROEM 16.1. INTRODUCTION 529 16.2. JUMP DIFFUSION MODELS 530 16.2.1.
NONINTERACTING ADATOMS 530 16.2.1.1. THE SELF-DIFFUSION CONSTANT 532
XVIII CONTENTS 16.2.1.2. MACROSCOPIC APPROXIMATION 533 16.2.1.3.
ONE-DIMENSIONAL EXAMPLE 534 16.2.2. INTERACTING ADATOMS 535 16.2.2.1.
MACROSCOPIC DESCRIPTION 536 16.2.2.2. HARD CORE INTERACTION 536
16.2.2.3. GENERAL INTERACTION 537 16.2.3. LIMITATIONS 538 16.3.
CONTINUOUS DIFFUSION MODELS 538 16.3.1. BROWNIAN MOTION THEORY 538
16.3.1.1. LANGEVIN S EQUATION 539 16.3.1.2. THE FLUCTUATION-DISSIPATION
THEOREM 539 16.3.1.3. THE SELF-DIFFUSION CONSTANT 540 16.3.2. ADATOM
DYNAMICS 542 16.3.2.1. ESCAPE FROM A POTENTIAL WELL 543 16.3.2.2.
DIFFUSION IN A PERIODIC POTENTIAL 544 16.3.3. LIMITATIONS WITH THE
BROWNIAN MOTION MODEL 545 16.3.3.1. THREE-DIMENSIONAL MOTION 545
16.3.3.2. POSITION-DEPENDENT FRICTION 545 16.3.3.3. MEMORY EFFECTS 545
16.3.3.4. QUANTUM EFFECTS 546 16.4. THERMAL RATE CONSTANTS 546 16.4.1.
THE BORN-OPPENHEIMER APPROXIMATION 546 16.4.2. TRANSITION STATE THEORY
547 16.4.2.1. ONE-DIMENSIONAL EXAMPLE 547 16.4.2.2. THE MULTIDIMENSIONAL
CASE 549 16.4.3. QUANTUM TRANSITION STATE THEORY 551 16.4.4. DYNAMIC
CORRECTION FACTOR 552 16.4.4.1. TWO-SITE SYSTEM-HEURISTIC DERIVATION 553
16.4.4.2. TWO-SITE SYSTEM-FORMAL DERIVATION 555 16.4.4.3. MULTISITE
SYSTEM 558 16.5. FRICTION COEFFICIENT AND MEMORY FUNCTION 559 16.5.1.
FORMAL EXACT EQUATION OF MOTION 559 16.5.2. FOKKER-PLANCK APPROXIMATION
561 16.5.2.1. ELECTRON-HOLE PAIR EXCITATIONS 562 16.5.2.2. PHONONS 563
16.5.3. MODE COUPLING APPROXIMATION 564 REFERENCES 564 17. THEORY OF
ADSORPTION-DESORPTION KINETICS AND DYNAMICS 567 S. HOLLOWAY 17.1.
INTRODUCTION 567 17.2. THE BORN-OPPENHEIMER APPROXIMATION AND
POTENTIAL-ENERGY SURFACES 568 CONTENTS XIX 17.2.1. ADIABATIC
REPRESENTATION 571 17.2.2. DIABATIC REPRESENTATION 571 17.3. DESORPTION
RATES AND THE TRANSITION STATE METHOD 573 17.4. THE INTERACTION OF H 2
WITH CU SURFACES; A BRIEF REVIEW . . . . 575 17.4.1. EXPERIMENTAL 575
17.4.2. THEORETICAL 579 17.5. THE ASSOCIATIVE DESORPTION OF H 2 /CU; A
CLASSICAL PICTURE . . . 582 17.6. THE DISSOCIATIVE ADSORPTION OF H 2
/CU; A QUANTUM WAVE-PACKET STUDY 587 17.7. DISSOCIATIVE ADSORPTION;
MULTIPLE ACTIVATION BARRIERS AND DIFFRACTION 591 17.8. SUMMARY 596
REFERENCES 597 18. ELEMENTARY CHEMICAL PROCESSES ON SURFACES AND
HETEROGENEOUS CATALYSIS 599 A. HAMNETT 18.1. INTRODUCTION 599 18.2.
FUNDAMENTAL PROCESSES THAT TAKE PLACE AT THE SURFACE 600 18.2.1.
CLASSICAL MODELS FOR ATOMIC AND MOLECULAR SCATTERING AT SURFACES 600
18.2.2. QUANTUM EFFECTS IN ATOMIC AND MOLECULAR SCATTERING . . 609
18.2.2.1. BOUND STATE RESONANCES 609 18.2.2.2. MOLECULAR EFFECTS 612
18.2.3. TRAPPING 613 18.3. CHEMISORPTION 614 18.3.1. KINETICS OF
CHEMISORPTION 615 18.3.2. DESORPTION 621 18.3.3. MOBILITY ON SURFACES
623 18.4. THE CHEMISORBED LAYER 624 18.4.1. THERMODYNAMICS OF
CHEMISORBED LAYERS 624 18.4.2. ENTHALPIES OF CHEMISORPTION 627 18.4.3.
CHEMISORPTION ON NONELEMENTAL MATERIALS 628 18.4.3.1. SURFACE
COMPOSITION 629 18.4.3.2. DYNAMIC COMPOSITION EFFECTS 631 18.4.3.3.
INFLUENCE OF SURFACE GEOMETRY AND STRUCTURE . 632 18.4.4. MORE COMPLEX
ADSORPTION PROBLEMS 632 18.4.4.1. ADSORPTION OF CO ON METALS 632
18.4.4.2. ADSORPTION OF CO ON OXIDES 637 18.5. KINETICS AND MECHANISM IN
CATALYSIS . 639 18.5.1. FUNDAMENTALS 639 18.5.1.1. THE
LANGMUIR-HINSHELWOOD MECHANISM . . . 639 18.5.1.2. THE ELEY-RIDEAL
MECHANISM 642 XX CONTENTS 18.5.2. VARIATION OF CATALYTIC RATE WITH
SUBSTRATE 643 18.5.3. MASS TRANSPORT LIMITATIONS ON CATALYSIS 648
18.5.4. BRANCHING EFFECTS 649 18.5.5. THE FISCHER-TROPSCH PROCESS 649
REFERENCES 654 19. GROWTH PROCESSES AT SURFACES: MODELING AND
SIMULATIONS 657 M. DJAFARI ROUHANI AND D. ESTEVE 19.1. INTRODUCTION 657
19.2. THERMODYNAMIC AND KINETIC MODELS 658 19.3. ATOMIC-SCALE PROCESSES
661 19.4. APPLICATION OF MONTE CARLO SIMULATIONS 662 19.5. GAS-SURFACE
INTERACTIONS 663 19.6. SURFACE REACTION SIMULATIONS 665 19.7.
INTERACTION POTENTIAL MODELS 666 19.8. HETEROEPITAXIAL GROWTH 668 19.9.
CONCLUSION 669 REFERENCES 670 INDEX 673
|
| any_adam_object | 1 |
| building | Verbundindex |
| bvnumber | BV004318746 |
| callnumber-first | Q - Science |
| callnumber-label | QC173 |
| callnumber-raw | QC173.4.S94 |
| callnumber-search | QC173.4.S94 |
| callnumber-sort | QC 3173.4 S94 |
| callnumber-subject | QC - Physics |
| classification_rvk | UP 7500 UP 7700 |
| ctrlnum | (OCoLC)21483790 (DE-599)BVBBV004318746 |
| dewey-full | 530.4/27 |
| dewey-hundreds | 500 - Natural sciences and mathematics |
| dewey-ones | 530 - Physics |
| dewey-raw | 530.4/27 |
| dewey-search | 530.4/27 |
| dewey-sort | 3530.4 227 |
| dewey-tens | 530 - Physics |
| discipline | Physik |
| format | Book |
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| id | DE-604.BV004318746 |
| illustrated | Illustrated |
| indexdate | 2024-07-09T16:11:24Z |
| institution | BVB |
| isbn | 0306434245 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-002685559 |
| oclc_num | 21483790 |
| open_access_boolean | |
| owner | DE-12 DE-384 DE-703 DE-355 DE-BY-UBR DE-29T DE-188 |
| owner_facet | DE-12 DE-384 DE-703 DE-355 DE-BY-UBR DE-29T DE-188 |
| physical | XX, 679 S. graph. Darst. |
| publishDate | 1990 |
| publishDateSearch | 1990 |
| publishDateSort | 1990 |
| publisher | Plenum Press |
| record_format | marc |
| series2 | Physics of solids and liquids |
| spelling | Interaction of atoms and molecules with solid surfaces ed. by V. Bortolani ... New York u.a. Plenum Press 1990 XX, 679 S. graph. Darst. txt rdacontent n rdamedia nc rdacarrier Physics of solids and liquids Atomes Chimie des surfaces Molécules Surfaces (Physique) Atoms Molecules Surface chemistry Surfaces (Physics) Atom (DE-588)4003412-4 gnd rswk-swf Schwingungsverhalten (DE-588)4180569-0 gnd rswk-swf Oberflächenphysik (DE-588)4134881-3 gnd rswk-swf Festkörperoberfläche (DE-588)4127823-9 gnd rswk-swf Metall (DE-588)4038860-8 gnd rswk-swf Wechselwirkung (DE-588)4064937-4 gnd rswk-swf Molekül (DE-588)4039972-2 gnd rswk-swf Elektronenstruktur (DE-588)4129531-6 gnd rswk-swf Oberflächenchemie (DE-588)4126166-5 gnd rswk-swf Festkörperoberfläche (DE-588)4127823-9 s Atom (DE-588)4003412-4 s Wechselwirkung (DE-588)4064937-4 s DE-604 Molekül (DE-588)4039972-2 s Oberflächenchemie (DE-588)4126166-5 s Oberflächenphysik (DE-588)4134881-3 s Schwingungsverhalten (DE-588)4180569-0 s 1\p DE-604 Metall (DE-588)4038860-8 s 2\p DE-604 Elektronenstruktur (DE-588)4129531-6 s 3\p DE-604 Bortolani, V. Sonstige oth GBV Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=002685559&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis 1\p cgwrk 20201028 DE-101 https://d-nb.info/provenance/plan#cgwrk 2\p cgwrk 20201028 DE-101 https://d-nb.info/provenance/plan#cgwrk 3\p cgwrk 20201028 DE-101 https://d-nb.info/provenance/plan#cgwrk |
| spellingShingle | Interaction of atoms and molecules with solid surfaces Atomes Chimie des surfaces Molécules Surfaces (Physique) Atoms Molecules Surface chemistry Surfaces (Physics) Atom (DE-588)4003412-4 gnd Schwingungsverhalten (DE-588)4180569-0 gnd Oberflächenphysik (DE-588)4134881-3 gnd Festkörperoberfläche (DE-588)4127823-9 gnd Metall (DE-588)4038860-8 gnd Wechselwirkung (DE-588)4064937-4 gnd Molekül (DE-588)4039972-2 gnd Elektronenstruktur (DE-588)4129531-6 gnd Oberflächenchemie (DE-588)4126166-5 gnd |
| subject_GND | (DE-588)4003412-4 (DE-588)4180569-0 (DE-588)4134881-3 (DE-588)4127823-9 (DE-588)4038860-8 (DE-588)4064937-4 (DE-588)4039972-2 (DE-588)4129531-6 (DE-588)4126166-5 |
| title | Interaction of atoms and molecules with solid surfaces |
| title_auth | Interaction of atoms and molecules with solid surfaces |
| title_exact_search | Interaction of atoms and molecules with solid surfaces |
| title_full | Interaction of atoms and molecules with solid surfaces ed. by V. Bortolani ... |
| title_fullStr | Interaction of atoms and molecules with solid surfaces ed. by V. Bortolani ... |
| title_full_unstemmed | Interaction of atoms and molecules with solid surfaces ed. by V. Bortolani ... |
| title_short | Interaction of atoms and molecules with solid surfaces |
| title_sort | interaction of atoms and molecules with solid surfaces |
| topic | Atomes Chimie des surfaces Molécules Surfaces (Physique) Atoms Molecules Surface chemistry Surfaces (Physics) Atom (DE-588)4003412-4 gnd Schwingungsverhalten (DE-588)4180569-0 gnd Oberflächenphysik (DE-588)4134881-3 gnd Festkörperoberfläche (DE-588)4127823-9 gnd Metall (DE-588)4038860-8 gnd Wechselwirkung (DE-588)4064937-4 gnd Molekül (DE-588)4039972-2 gnd Elektronenstruktur (DE-588)4129531-6 gnd Oberflächenchemie (DE-588)4126166-5 gnd |
| topic_facet | Atomes Chimie des surfaces Molécules Surfaces (Physique) Atoms Molecules Surface chemistry Surfaces (Physics) Atom Schwingungsverhalten Oberflächenphysik Festkörperoberfläche Metall Wechselwirkung Molekül Elektronenstruktur Oberflächenchemie |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=002685559&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT bortolaniv interactionofatomsandmoleculeswithsolidsurfaces |