Low energy electrons and surface chemistry:
Gespeichert in:
| Hauptverfasser: | , |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Weinheim u.a.
Verl. Chemie
1985
|
| Ausgabe: | 2., completely rev. ed. |
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | XII, 374 S. Ill., graph. Darst. |
| ISBN: | 3527260560 0895730650 |
Internformat
MARC
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| 245 | 1 | 0 | |a Low energy electrons and surface chemistry |c G. Ertl ; J. Küppers |
| 250 | |a 2., completely rev. ed. | ||
| 264 | 1 | |a Weinheim u.a. |b Verl. Chemie |c 1985 | |
| 300 | |a XII, 374 S. |b Ill., graph. Darst. | ||
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Datensatz im Suchindex
| _version_ | 1804115610117865472 |
|---|---|
| adam_text | G Ertl, J Kuppers
Low Energy Electrons
and Surface Chemistry
VCH
Contents
1 Basic concepts 1
1 1 Introduction 1
1 2 Principles of ultrahigh vacuum techniques 2
121 Why is UHV necessary? 2
122 Production of ultrahigh vacuum 3
123 Pressure measurement 4
124 Gas handling 4
1 3 Preparation of clean surfaces 5
1 4 Interaction of low energy electrons with mailer 6
1 5 Electron energy analyzers 9
151 Retarding field grid analyzer (RFA) 9
152 Cylindrical mirror analyzer (CMA) 11
153 127 -analyzer 13
154 Concentric hemisphere analyzer (CHA) 14
1 6 References 15
2 Auger electron spectroscopy 17
2 1 Historical development 17
2 2 Instrumentation 18
221 Source of excitation 18
222 Sample 20
223 Analyzer and detector system 20
224 Further refinements 23
2 3 Mechanism of the Auger process 28
2 4 Energies and shapes of the Auger peaks 33
241 Free atoms 33
242 Condensed matter 34
243 Chemical effects 37
2 5 Intensity of the Auger electron emission 40
251 Auger yield 40
252 Ionization cross section 42
253 Auger electron emission from condensed matter 43
2 6 Detected volume 45
2 7 Qualitative analysis 47
2 8 Quantitative analysis 47
281 Determination of relative surface quantities 48
282 Absolute surface quantities 48
283 Alloys 49
284 Depth profiling - 55
285 Kinetic studies 56
VIII Contents
2 9 Deconvolution technique and band structure 57
2 10 References 61
3 X-ray photoelectron spectroscopy (X PS) 65
3 1 Introduction 65
3 2 Instrumentation 65
321 Light sources 65
322 Analyzer and detector 66
323 Data analysis 67
3 3 Physical principles 69
3 4 Qualitative surface analysis 70
341 Identification of elements 70
342 Core-level chemical shifts 71
3 5 Quantitative analysis 74
3 6 Final state effects 79
361 Relaxation effects 79
362 Multiplet splitting 79
363 Multi-electron excitations 80
364 Core-level satellites 81
3 7 Angular effects 82
3 8 References 83
4 Ultraviolet photoelectron spectroscopy (UPS) 87
4 1 Introduction 87
4 2 Instrumentation 89
421 Light sources 89
4211 Resonance sources 89
4212 Continuous sources 90
422 Sample 93
423 Analyzer and detector 93
4 3 Photoionization process 94
431 Photoionization of atoms 95
432 Photoionization of molecules 97
433 Photoemission from solids 101
4 4 UPS from clean surfaces 108
441 Angle integrated photoemmission 109
442 Angle resolved photoemission 110
4 5 UPS from adsorbate covered surfaces 114
451 Adsorbed atoms 117
452 Adsorbed noble gases 122
453 Adsorbed molecules 128
Contents IX
4531 Adsorbed CO 129
4532 Adsorbed polyatomics 138
4 6 References 143
5 Electron spectroscopy with noble gas ions and metastable atoms 147
5 1 Introduction 147
5 2 Instrumentation 147
5 3 Deexcitation mechanisms 148
5 4 Auger neutralization 150
5 5 Auger deexcitation (Penning ionization) 153
5 6 References 156
6 Appearance potential spectroscopy 157
6 1 Introduction 157
6 2 Instrumentation 158
6 3 Mechanism 160
6 4 Core-level binding energies 163
6 5 Surface analysis 165
6 6 Band structure and deconvolution 165
6 7 Adsorbate studies/Chemical effects 170
6 8 Extended fine structure 171
6 9 References 173
7 Inverse photoemission (IPE, BIS) 175
7 1 Introduction 175
7 2 Instrumentation 175
7 3 Mechanism of IPE 176
7 4 Clean surfaces 178
7 5 Adsorbate studies 181
7 6 References 183
8 Electron energy loss spectroscopy (ELS, EELS) 185
8 1 Introduction 185
8 2 Instrumentation 186
8 3 Ionization losses 187
8 4 Plasmon losses and intraband transitions 190
8 5 Extended loss fine structure 195
8 6 Adsorbate induced losses 197
8 7 References 199
X Contents
9 Low energy electron diffraction (LEED) 201
9 1 Introduction and historical development 201
9 2 Classification of periodic surface structures 203
921 Substrate and surface structures 203
922 Surfaces with periodic steps and kinks 206
9 3 Formation of the diffraction pattern 207
9 4 Instrumentation 209
941 Introduction 209
942 Electron gun 209
943 Detector system 210
9 5 Geometrical theory of diffraction 214
951 Introduction 214
952 The reciprocal lattice 215
9 5 3V Interference conditions and the Evald construction 217
954 Analysis of a simple diffraction pattern 219
955 Domain structures 220
956 LEED patterns of incommensurai; structures 224
9 6 Kinematic theory 226
961 Introduction 226
962 Scattering at two-dimensional lattices 227
963 Kinematical structure factor 230
964 Intensity-voltage (I/V) curves 230
9 7 Disordered structures 232
971 Introduction 232
972 The transfer width 233
973 Size effects and one-dimensional c isorder 234
974 Lattice gas systems 238
975 Antiphase domains 242
976 Facets 244
977 Stepped surfaces 246
9 8 Simulation of diffraction patterns 248
9 9 Dynamical theories 250
991 Introduction 250
992 Physical parameters entering a dynamical theory 251
993 Multiple scattering 253
994 Data evaluation 255
9 10 Temperature effects 257
9 11 Spin-polarized LEED 261
9 12 References 262
10 X-ray absorption fine structure (EXAFS) 267
10 1 Introduction : 267
10 2 Instrumentation 268
Contents XI
10 3 Theory of EXAFS 270
10 4 EXAFS data analysis 272
10 5 Applications of EXAFS to surface problems 277
10 5 1 Supported catalysts 277
10 5 2 Adsorbed layers 277
10 6 Near-edge structure (XANES) 280
10 7 References 282
11 Vibrational spectroscopy (HREELS, EELS) 285
11 1 Introduction 285
11 2 Instrumentation 286
11 3 Symmetry aspects of vibrating adsorbed molecules 288
11 3 1 General remarks 288
11 3 2 Symmetry elements 289
11 3 3 Point groups and representations 291
11 3 4 Irreducible representations 293
11 3 5 Symmetry properties of displacements 294
11 3 6 Application to degenerate point groups 299
11 3 7 Symmetry of adsorbed atoms 302
11^3 8 Symmetry of adsorbed molecules 303
11 4 Normal vibrations 305
11 5 Group frequencies 308
11 6 Theory of the electron scattering mechanism 308
11 6 1 Surface dipole scattering 308
11 6 2 Electron impact mechanism 311
11 6 3 Negative ion resonances 313
11 7 Experimental results 313
11 7 1 Clean surfaces 313
11 7 2 Adsorbed atoms 315
11 7 3 Adsorbed diatomics 323
11 7 4 Adsorbed polyatomics 326
11 7 5 Reaction intermediates 329
11 8 References 332
12 Electron and photon stimulated desorption 335
12 1 Introduction 335
12 2 Experimental 335
12 2 1 Changes of surface properties 336
12 2 2 Detection of desorbing species 336
12 3 Cross sections for desorption : 339
12 4 Mechanisms for desorption 341
XII Contents
12 5 Angular distribution of desorbing ions (ESDIAD) 343
12 6 References 345
13 Appendix 347
13 1 Fundamental constants 347
13 2 Properties of selected elements 347
13 3 Line positions in XPS using Al-K(j radiation 350
13 4 XPS atomic sensitivity factors 354
13 5 Kinetic energies of Auger electron; 357
13 6 Relative Auger sensitivity factors 365
13 7 Character tables 365
13 8 Characteristic group frequencies 367
13 9 Abbreviations and acronyms 369
Index 371
|
| any_adam_object | 1 |
| author | Ertl, Gerhard 1936- Küppers, Jürgen 1943-2019 |
| author_GND | (DE-588)106105507 (DE-588)133762238 |
| author_facet | Ertl, Gerhard 1936- Küppers, Jürgen 1943-2019 |
| author_role | aut aut |
| author_sort | Ertl, Gerhard 1936- |
| author_variant | g e ge j k jk |
| building | Verbundindex |
| bvnumber | BV001211084 |
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| classification_tum | CHE 250f CHE 180f PHY 608f |
| ctrlnum | (OCoLC)630753138 (DE-599)BVBBV001211084 |
| discipline | Chemie / Pharmazie Physik Chemie |
| edition | 2., completely rev. ed. |
| format | Book |
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| id | DE-604.BV001211084 |
| illustrated | Illustrated |
| indexdate | 2024-07-09T15:25:21Z |
| institution | BVB |
| isbn | 3527260560 0895730650 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-000731735 |
| oclc_num | 630753138 |
| open_access_boolean | |
| owner | DE-19 DE-BY-UBM DE-91 DE-BY-TUM DE-91G DE-BY-TUM DE-384 DE-703 DE-355 DE-BY-UBR DE-20 DE-29T DE-210 DE-11 DE-188 |
| owner_facet | DE-19 DE-BY-UBM DE-91 DE-BY-TUM DE-91G DE-BY-TUM DE-384 DE-703 DE-355 DE-BY-UBR DE-20 DE-29T DE-210 DE-11 DE-188 |
| physical | XII, 374 S. Ill., graph. Darst. |
| publishDate | 1985 |
| publishDateSearch | 1985 |
| publishDateSort | 1985 |
| publisher | Verl. Chemie |
| record_format | marc |
| spelling | Ertl, Gerhard 1936- Verfasser (DE-588)106105507 aut Low energy electrons and surface chemistry G. Ertl ; J. Küppers 2., completely rev. ed. Weinheim u.a. Verl. Chemie 1985 XII, 374 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier LEED (DE-588)4074082-1 gnd rswk-swf Oberflächenchemie (DE-588)4126166-5 gnd rswk-swf Langsames Elektron (DE-588)4166710-4 gnd rswk-swf Adsorption (DE-588)4000536-7 gnd rswk-swf Elektronenspektroskopie (DE-588)4014332-6 gnd rswk-swf Festkörperoberfläche (DE-588)4127823-9 gnd rswk-swf Auger-Spektroskopie (DE-588)4122843-1 gnd rswk-swf LEED (DE-588)4074082-1 s DE-604 Auger-Spektroskopie (DE-588)4122843-1 s Elektronenspektroskopie (DE-588)4014332-6 s Adsorption (DE-588)4000536-7 s Oberflächenchemie (DE-588)4126166-5 s Festkörperoberfläche (DE-588)4127823-9 s Langsames Elektron (DE-588)4166710-4 s Küppers, Jürgen 1943-2019 Verfasser (DE-588)133762238 aut HEBIS Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=000731735&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Ertl, Gerhard 1936- Küppers, Jürgen 1943-2019 Low energy electrons and surface chemistry LEED (DE-588)4074082-1 gnd Oberflächenchemie (DE-588)4126166-5 gnd Langsames Elektron (DE-588)4166710-4 gnd Adsorption (DE-588)4000536-7 gnd Elektronenspektroskopie (DE-588)4014332-6 gnd Festkörperoberfläche (DE-588)4127823-9 gnd Auger-Spektroskopie (DE-588)4122843-1 gnd |
| subject_GND | (DE-588)4074082-1 (DE-588)4126166-5 (DE-588)4166710-4 (DE-588)4000536-7 (DE-588)4014332-6 (DE-588)4127823-9 (DE-588)4122843-1 |
| title | Low energy electrons and surface chemistry |
| title_auth | Low energy electrons and surface chemistry |
| title_exact_search | Low energy electrons and surface chemistry |
| title_full | Low energy electrons and surface chemistry G. Ertl ; J. Küppers |
| title_fullStr | Low energy electrons and surface chemistry G. Ertl ; J. Küppers |
| title_full_unstemmed | Low energy electrons and surface chemistry G. Ertl ; J. Küppers |
| title_short | Low energy electrons and surface chemistry |
| title_sort | low energy electrons and surface chemistry |
| topic | LEED (DE-588)4074082-1 gnd Oberflächenchemie (DE-588)4126166-5 gnd Langsames Elektron (DE-588)4166710-4 gnd Adsorption (DE-588)4000536-7 gnd Elektronenspektroskopie (DE-588)4014332-6 gnd Festkörperoberfläche (DE-588)4127823-9 gnd Auger-Spektroskopie (DE-588)4122843-1 gnd |
| topic_facet | LEED Oberflächenchemie Langsames Elektron Adsorption Elektronenspektroskopie Festkörperoberfläche Auger-Spektroskopie |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=000731735&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT ertlgerhard lowenergyelectronsandsurfacechemistry AT kuppersjurgen lowenergyelectronsandsurfacechemistry |