Principles and applications of resonance ionisation spectroscopy:
Gespeichert in:
| Hauptverfasser: | , |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Bristol [u.a.]
Hilger
1988
|
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | XII, 417 S. |
| ISBN: | 0852744609 |
Internformat
MARC
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Datensatz im Suchindex
| _version_ | 1804115325337206784 |
|---|---|
| adam_text | Principles and Applications of
Resonance Ionisation
Spectroscopy
G S Hurst
Institute of Resonance Ionisation Spectroscopy, Department
of Physics, University of Tennessee, and Consultant to the
Oak Ridge National Laboratory
and
M G Payne
Oak Ridge National Laboratory
Adam Hilger, Bristol and Philadelphia
Contents
Preface xi
1 The origin of resonance ionisation spectroscopy 1
1 1 Introduction 1
1 2 Excitation and ionisation of gases with charged particles,
W values 2
1 3 The Hornbeck-Molnar reactions 5
1 4 Jesse effects 6
1 5 Energy pathways research - 8
1 6 Energy pathways in helium 14
1 7 Resonance ionisation spectroscopy 20
References 22
2 RIS studies on He(2 S) 24
2 1 Introduction 24
2 2 Gaseous electronics 24
2 3 Pulsed ionisation measurements 32
2 4 Concept of the RIS experiment on He(2 S) 36
2 5 Results of the RIS experiment on He(2 S) involving
photo-ionisation 40
2 6 The RIS experiments on He(2 S) using associative
ionisation 44
References 48
3 One-atom detection 50
3 1 RIS of atoms in their ground states 50
3 2 Sensitive ionisation measurements 58
33A demonstration of one-atom detection 60
3 4 One-atom detection in time coincidence with nuclear
decay 67
References 72
viii Contents
4 The interaction of laser light with atoms 74
4 1 Introduction 74
4 2 Review of electromagnetic fields 75
4 3 Interaction of a laser field with isolated atoms 83
4 4 The two-state model 91
4 5 Excitation involving three bound states 102
46A more general adiabatic method 104
4 7 Multiphoton excitation 108
References 113
5 Theory of resonance ionisation spectroscopy 114
5 1 Introduction 114
5 2 Thermodynamic arguments concerning the absorption and
emission of radiation by an atomic vapour 115
5 3 Density matrix formulation of atomic response 118
5 4 Finite band width effects in a two-state model 119
5 5 The incorporation of laser ionisation into the equations of
motion 129
5 6 Near-resonant two-photon ionisation 133
5 7 Methods of RIS using commercial lasers 140
5 8 Effective volumes of ionisation 146
References 149
6 Chemical physics 151
6 1 Introduction 151
6 2 Photodissociation of Csl - 151
6 3 Diffusion of caesium atoms in argon gas 156
6 4 Chemical reaction of caesium atoms with O2 in the
presence of an argon buffer gas 158
6 5 Precision measurements of the diffusion of reactive atoms 160
6 6 Photodissociation of Lil , 165
6 7 Chemical reactions of lithium atoms with O2 170
6 8 Diffusion of lithium atoms in argon gas 172
6 9 Concluding remarks 174
References 176
7 Statistical mechanics 178
7 1 Introduction 178
7 2 Density fluctuations in atomic populations 178
7 3 Fluctuations in ionisation by swift particles: the
Fano factor 180
7 4 Fluctuations in atomic and molecular processes 188
7 5 The ergodic hypothesis: an Einstein Gedanken experiment 196
Contents ix
7 6 An experimental test of the ergodic hypothesis 199
7 7 Further comments on the ergodic hypothesis 202
References 203
8 Elemental analyses of solids and related applications of RIS 205
8 1 Introduction 205
8 2 Laser ablation methods LARIS 206
8 3 RIMS using pulsed lasers 209
8 4 RIMS using continuous wave lasers 219
8 5 Atomisation by ion sputtering 223
8 6 Elemental analyses of solids using SIRIS 230
8 7 Comparison of RIS with accelerator mass spectroscopy
(AMS) 237
8 8 On-line RIMS in nuclear physics 239
8 9 Some additional applications of RIS 241
References 242
9 Non-linear optics: applications to resonance ionisation
spectroscopy 248
9 1 Introduction 248
9 2 Introduction to non-linear processes 249
9 3 An example of a non-linear process with an unfocused
laser beam: third harmonic generation near three-photon
resonances in xenon 253
9 4 Third harmonic generation with focused laser beams 264
9 5 Sum mixing with unfocused laser beams 270
9 6 Four-wave sum and difference mixing in Xe and Kr 277
9 7 Two-photon excitation and the stimulated Raman process 279
References 284
10 Maxwell s demon and other noble concepts 286
10 1 Concept of the Maxwell demon 286
10 2 The atom buncher 289
10 3 Mass spectrometer 295
10 4 Atom bank 297
10 5 Atom counter 304
10 6 A demonstration using 81Kr atoms 306
10 7 A Maxwell demon using time-of-flight principles 310
10 8 RISTRON 311
10 9 Other methods of atom counting 314
10 10 Isotopic enrichment 315
10 11 Concluding remarks 318
References 319
Contents
Cosmology and particle physics
11 1 Introduction
11 2 Connection of cosmology with particle physics
11 3 Time evolution of the universe
11 4 Standard cosmology and its problems
11 5 Inflationary cosmology and magnetic monopoles
11 6 Searches for magnetic monopoles
11 7 Concept of a monopole detector using RIS
References
Search for other primordial particles
12 1 Introduction
12 2 Quark composition of matter and quark confinement
12 3 Other predictions of particle physics theories
12 4 Searches for fractional charge
12 5 RIS searches for fractional charge
12 6 Previous searches for stable, heavy, elementary particles
12 7 RIS search for heavy elementary particles
References
Stellar evolution and the solar neutrino mystery
13 1 Introduction
13 2 Stellar evolution and stellar structure
13 3 Energy production in the sun
13 4 Solar models and neutrino production
13 5 The 37Cl(v, e~)37Ar solar neutrino experiment
13 6 The 81Br(v, e~)81Kr solar neutrino experiment
References
Earth and planetary sciences
14 1 Introduction
14 2 Origin of meteorites and atmospheric xenon
14 3 Age of the solar system
14 4 Principles of environmental dating
14 5 Age of ground-water and polar ice
14 6 Ocean water circulation
14 7 Concluding remarks
References
Index
|
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| spelling | Hurst, G. S. 1927- Verfasser (DE-588)120462133 aut Principles and applications of resonance ionisation spectroscopy G. S. Hurst and M. G. Payne Bristol [u.a.] Hilger 1988 XII, 417 S. txt rdacontent n rdamedia nc rdacarrier Resonance ionization spectroscopy REMPI (DE-588)4174508-5 gnd rswk-swf REMPI (DE-588)4174508-5 s DE-604 Payne, Marvin G. Verfasser aut HEBIS Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=000547393&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Hurst, G. S. 1927- Payne, Marvin G. Principles and applications of resonance ionisation spectroscopy Resonance ionization spectroscopy REMPI (DE-588)4174508-5 gnd |
| subject_GND | (DE-588)4174508-5 |
| title | Principles and applications of resonance ionisation spectroscopy |
| title_auth | Principles and applications of resonance ionisation spectroscopy |
| title_exact_search | Principles and applications of resonance ionisation spectroscopy |
| title_full | Principles and applications of resonance ionisation spectroscopy G. S. Hurst and M. G. Payne |
| title_fullStr | Principles and applications of resonance ionisation spectroscopy G. S. Hurst and M. G. Payne |
| title_full_unstemmed | Principles and applications of resonance ionisation spectroscopy G. S. Hurst and M. G. Payne |
| title_short | Principles and applications of resonance ionisation spectroscopy |
| title_sort | principles and applications of resonance ionisation spectroscopy |
| topic | Resonance ionization spectroscopy REMPI (DE-588)4174508-5 gnd |
| topic_facet | Resonance ionization spectroscopy REMPI |
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