Holdings: Towards molecular photocatalysts for overall water splitting

Towards molecular photocatalysts for overall water splitting:

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Bibliographic Details
Main Author:	Staehle, Robert Oliver 1984- (Author)
Format:	Thesis Book
Language:	English
Published:	Ulm 2014
Subjects:	Wasserstofferzeugung Fotokatalyse Hochschulschrift
Online Access:	Inhaltsverzeichnis Inhaltsverzeichnis
Item Description:	Enthällt Sonderabdrucke
Physical Description:	233 Blätter Diagramme 30 cm

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MARC


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adam_text	QLI 30^ ULM UNIVERSITY UNIVERSITAT TOWARDS MOLECULAR PHOTOCATALYSTS FOR OVERALL WATER SPLITTING DISSERTATION ZUR ERLANGUNG DES DOKTORGRADES DR.RER.NAT. DER FAKULTAT FUR NATURWISSENSCHAFTEN DER UNIVERSITAT ULM VORGELEGT VON DIPLOMCHEMIKER ROBERT OLIVER STAEHLE GEBOREN AM 25.07.1984 IN STUTTGART 2014 HTTP://D-NB.INFO/1059371332 TABLE OF CONTENT 1. MOTIVATION 1 2. STATE OF THE ART 4 3. SCOPE OF THE THESIS 31 4. INVESTIGATED SYSTEMS 33 4.1. INFLUENCE OF PLANAR AROMATIC ORGANIC MOLECULES ON THE CATALYTIC PERFORMANCE 33 4.2. WATER REDUCTION IN THE PRESENCE OF OXYGEN 36 4.2.1. MECHANISTIC STUDIES 36 4.2.2. MODIFICATION OF THE CHROMOPHORE 41 4.3. CARBENES IN THE CATALYTIC WATER SPLITTING 43 4.3.1. INTRAMOLECULAR SYSTEMS CONTAINING N-HETEROCYCLIC CARBENES 43 4.3.2. INTERMOLECULAR SYSTEMS - MODIFICATIONS OF THE CHROMOPHORE 46 4.3.2.1. MODIFICATION OF THE PHENANTHROLINE BACKBONE 46 4.3.2.2. MODIFICATION OF THE N-HETEROCYCLIC CARBENE UNIT 47 4.3.2.3. MODIFICATION OF THE TERMINAL LIGANDS 49 4.3.2.4. CATALYTIC ACTIVITY OF MODIFIED COMPLEXES 54 4.3.2.5. MODIFICATION OF THE METAL CENTRE 58 5. SUMMARY AND OUTLOOK 60 6. REFERENCES 63 T 7. PUBLICATIONS 67 7.1. [RSI]: SUPRAMOLECULAR ACTIVATION OF A MOLECULAR PHOTOCATALYST 68 7.2. [RS2]: PHOTOCATALYTIC GENERATION OF HYDROGEN FROM WATER UNDER AEROBIC CONDITIONS 95 7.3. [RS3]: AN IMPROVED SYNTHESIS OF 4-CYANO-L,10-PHENANTHROLINE, 4,7-DICYANO-L 5 10- PHENANTHROLINE AND THEIR BIS (4,4'-DI-TERT-BUTYL-2 S 2'-BIPYRIDINE)RUTHENIUM(IL) COMPLEXES 109 7.4. [RS4]: CARBENE BASED PHOTOCHEMICAL MOLECULAR ASSEMBLIES FOR SOLAR DRIVEN HYDROGEN GENERATION 130 7.5. [RS5]: IMPROVED OXYGEN RESISTANCE IN RUTHENIUM PHOTOCENTRES BY LIGAND DESIGN. 178 7.6. [RS6]: WATER OXIDATION CATALYZED BY MONONUCLEAR RUTHENIUM COMPLEXES WITH A 2,2'- BIPYRIDINE-6,6'-DICARBOXYLATE (BDA) LIGAND: HOW LIGAND ENVIRONMENT INFLUENCES THE CATALYTIC BEHAVIOR 194 8. CURRICULUM VITAE 231 9. PUBLICATIONS AND CONFERENCE CONTRIBUTIONS 232 9.1. PUBLICATIONS IN PEER REVIEWED JOURNALS 232 9.2. SPECIALIST BOOKS 232 9.3. CONFERENCE PROCEEDINGS 232 9.3.1. ORAL PRESENTATIONS 232 9.3.2. POSTER CONTRIBUTIONS 233 10. ABBREVIATIONS 234 11. ACKNOWLEDGMENTS 237 12. DECLARATION OF HONESTY IN ACADEMIC WORK 238
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spelling	Staehle, Robert Oliver 1984- Verfasser (DE-588)1059652714 aut Towards molecular photocatalysts for overall water splitting vorgelegt von Robert Oliver Staehle Ulm 2014 233 Blätter Diagramme 30 cm txt rdacontent n rdamedia nc rdacarrier Enthällt Sonderabdrucke Dissertation Universität Ulm 2014 Wasserstofferzeugung (DE-588)4189271-9 gnd rswk-swf Fotokatalyse (DE-588)4193873-2 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Wasserstofferzeugung (DE-588)4189271-9 s Fotokatalyse (DE-588)4193873-2 s DE-604 B:DE-101 application/pdf http://d-nb.info/1059371332/04 Inhaltsverzeichnis DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=031256151&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis
spellingShingle	Staehle, Robert Oliver 1984- Towards molecular photocatalysts for overall water splitting Wasserstofferzeugung (DE-588)4189271-9 gnd Fotokatalyse (DE-588)4193873-2 gnd
subject_GND	(DE-588)4189271-9 (DE-588)4193873-2 (DE-588)4113937-9
title	Towards molecular photocatalysts for overall water splitting
title_auth	Towards molecular photocatalysts for overall water splitting
title_exact_search	Towards molecular photocatalysts for overall water splitting
title_full	Towards molecular photocatalysts for overall water splitting vorgelegt von Robert Oliver Staehle
title_fullStr	Towards molecular photocatalysts for overall water splitting vorgelegt von Robert Oliver Staehle
title_full_unstemmed	Towards molecular photocatalysts for overall water splitting vorgelegt von Robert Oliver Staehle
title_short	Towards molecular photocatalysts for overall water splitting
title_sort	towards molecular photocatalysts for overall water splitting
topic	Wasserstofferzeugung (DE-588)4189271-9 gnd Fotokatalyse (DE-588)4193873-2 gnd
topic_facet	Wasserstofferzeugung Fotokatalyse Hochschulschrift
url	http://d-nb.info/1059371332/04 http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=031256151&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA
work_keys_str_mv	AT staehlerobertoliver towardsmolecularphotocatalystsforoverallwatersplitting

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