X-ray photoemission studies of bimetallic Pt-Ga, Pd-Ga and Rh-Ga catalysts: = Untersuchungen an bimetallischen Pt-Ga, Pd-Ga und Rh-Ga Katalysatoren mittels Röntgenphotoelektronenspektroskopie
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| Main Author: | |
|---|---|
| Format: | Thesis Book |
| Language: | English |
| Published: |
Erlangen ; Nürnberg
[2018]
|
| Subjects: | |
| Online Access: | Inhaltsverzeichnis Inhaltsverzeichnis |
| Physical Description: | II, 83, LXVI Seiten Illustrationen, Diagramme 21 cm |
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MARC
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| 245 | 1 | 0 | |a X-ray photoemission studies of bimetallic Pt-Ga, Pd-Ga and Rh-Ga catalysts |b = Untersuchungen an bimetallischen Pt-Ga, Pd-Ga und Rh-Ga Katalysatoren mittels Röntgenphotoelektronenspektroskopie |c vorgelegt von Mathias F. Grabau |
| 246 | 1 | 3 | |a Untersuchungen an bimetallischen Pt-Ga, Pd-Ga und Rh-Ga Katalysatoren mittels Röntgenphotoelektronenspektroskopie |
| 246 | 1 | 1 | |a Untersuchungen an bimetallischen Pt-Ga, Pd-Ga und Rh-Ga Katalysatoren mittels Röntgenphotoelektronenspektroskopie |
| 264 | 1 | |a Erlangen ; Nürnberg |c [2018] | |
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| 336 | |b txt |2 rdacontent | ||
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| 338 | |b nc |2 rdacarrier | ||
| 502 | |b Dissertation |c Friedrich-Alexander-Universität Erlangen-Nürnberg |d 2018 | ||
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Record in the Search Index
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|---|---|
| adam_text | 1.
INTRODUCTION
1
1.1.
GENERAL
ASPECTS
OF
CATALYSIS
............................................................
1
1.2.
PRESSURE
AND
MATERIAL
GAPS
............................................................
3
1.3.
THE
PD/PT/RH-GA
BIMETALLIC
CATALYSTS
IN
THE
DEHYDROGENATION
OF
LIGHT
ALKANES
.....................................................................................
5
2.
FUNDAMENTALS
9
2.1.
X-RAY
PHOTOELECTRON
SPECTROSCOPY
..................................................
9
2.1.1.
THE
BINDING
ENERGY
IN
XPS
..................................................
9
2.1.2.
SURFACE
SENSITIVITY
IN
XPS
......................................................
12
2.1.3.
NEAR-AMBIENT
PRESSURE
XPS
...................................................
14
2.1.4.
QUANTITATIVE
XPS
......................................................................
15
2.2.
PLASMON
LOSS
SATELLITES
IN
GA
................................................................
19
3.
INSTRUMENTATION
AND
EXPERIMENTAL
DETAILS
23
3.1.
THE
GAP
INSTRUMENT
............................................................................
23
3.2.
THE
DASSA
INSTRUMENT
.........................................................................24
3.3.
SAMPLE
PREPARATION
............................................................................
24
4.
RESULTS
AND
DISCUSSION
27
4.1.
SUPPORTED
PD/RH-GA
BIMETALLIC
CATALYST
............................................ 27
4.1.1.
PD-GA
ON
POROUS
SIO2
-
P1
...................................................
28
4.1.2.
RH-GA
ON
AI
2
O
3
..................................................................... 30
4.2.
ANGLE-RESOLVED
PHOTOEMISSION
SPECTROSCOPY
OF
PT/PD/RH-GA
ALLOYS
33
4.2.1.
ARXPS
OF
PD-GA
ALLOYS
-P2
...................................................
34
4.2.2.
ARXPS
OF
RH/PT-GA
ALLOYS
......................................................40
4.3.
OXIDATION
OF
PT/PD-GA
ALLOYS
............................................................... 44
4.3.1.
OXIDATION
OF
PT-GA
-
P3
.........................................................44
4.3.2.
OXIDATION
OF
PD-GA
..................................................................
50
4.4.
DEPOSITION
OF
GA
ON
GOLD
SURFACES
......................................................
54
4.4.1.
GA
ON
POLYCRYSTALLINE
AU
SURFACES
-
P4
.....................................
54
5.
SUMMARY
61
6.
ZUSAMMENFASSUNG
65
7.
REFERENCES
71
8.
ACKNOWLEDGMENTS
81
9.
THE
AUTHOR
*
S
CONTRIBUTIONS
TO
P1
-
P4
83
A.
APPENDIX
A
I
A.1.
P1
.....................................................................................................
I
A.2.
P2
....................................................................................................
XXV
A.3.
P3
......................................................................................................
XXXIX
A.
4.
P4
.....................................................................................................
LI
B.
APPENDIX
B
LXV
B.
1.
GA
EVAPORATOR
.................................................................................LXV
8.2.
DRAWINGS
APERATURE
AI
....................................................................
LXVI
|
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| genre | (DE-588)4113937-9 Hochschulschrift gnd-content |
| genre_facet | Hochschulschrift |
| id | DE-604.BV045548620 |
| illustrated | Illustrated |
| indexdate | 2024-07-10T08:21:11Z |
| institution | BVB |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-030932636 |
| oclc_num | 1099923792 |
| open_access_boolean | |
| owner | DE-29T DE-29 |
| owner_facet | DE-29T DE-29 |
| physical | II, 83, LXVI Seiten Illustrationen, Diagramme 21 cm |
| publishDate | 2018 |
| publishDateSearch | 2018 |
| publishDateSort | 2018 |
| record_format | marc |
| spelling | Grabau, Mathias F. Verfasser aut X-ray photoemission studies of bimetallic Pt-Ga, Pd-Ga and Rh-Ga catalysts = Untersuchungen an bimetallischen Pt-Ga, Pd-Ga und Rh-Ga Katalysatoren mittels Röntgenphotoelektronenspektroskopie vorgelegt von Mathias F. Grabau Untersuchungen an bimetallischen Pt-Ga, Pd-Ga und Rh-Ga Katalysatoren mittels Röntgenphotoelektronenspektroskopie Erlangen ; Nürnberg [2018] II, 83, LXVI Seiten Illustrationen, Diagramme 21 cm txt rdacontent n rdamedia nc rdacarrier Dissertation Friedrich-Alexander-Universität Erlangen-Nürnberg 2018 Röntgen-Photoelektronenspektroskopie (DE-588)4076787-5 gnd rswk-swf Katalysator (DE-588)4029919-3 gnd rswk-swf Gadolinium (DE-588)4155786-4 gnd rswk-swf Platinmetalllegierung (DE-588)4377223-7 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Platinmetalllegierung (DE-588)4377223-7 s Gadolinium (DE-588)4155786-4 s Katalysator (DE-588)4029919-3 s Röntgen-Photoelektronenspektroskopie (DE-588)4076787-5 s DE-604 B:DE-101 application/pdf http://d-nb.info/1180525957/04 Inhaltsverzeichnis DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=030932636&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Grabau, Mathias F. X-ray photoemission studies of bimetallic Pt-Ga, Pd-Ga and Rh-Ga catalysts = Untersuchungen an bimetallischen Pt-Ga, Pd-Ga und Rh-Ga Katalysatoren mittels Röntgenphotoelektronenspektroskopie Röntgen-Photoelektronenspektroskopie (DE-588)4076787-5 gnd Katalysator (DE-588)4029919-3 gnd Gadolinium (DE-588)4155786-4 gnd Platinmetalllegierung (DE-588)4377223-7 gnd |
| subject_GND | (DE-588)4076787-5 (DE-588)4029919-3 (DE-588)4155786-4 (DE-588)4377223-7 (DE-588)4113937-9 |
| title | X-ray photoemission studies of bimetallic Pt-Ga, Pd-Ga and Rh-Ga catalysts = Untersuchungen an bimetallischen Pt-Ga, Pd-Ga und Rh-Ga Katalysatoren mittels Röntgenphotoelektronenspektroskopie |
| title_alt | Untersuchungen an bimetallischen Pt-Ga, Pd-Ga und Rh-Ga Katalysatoren mittels Röntgenphotoelektronenspektroskopie |
| title_auth | X-ray photoemission studies of bimetallic Pt-Ga, Pd-Ga and Rh-Ga catalysts = Untersuchungen an bimetallischen Pt-Ga, Pd-Ga und Rh-Ga Katalysatoren mittels Röntgenphotoelektronenspektroskopie |
| title_exact_search | X-ray photoemission studies of bimetallic Pt-Ga, Pd-Ga and Rh-Ga catalysts = Untersuchungen an bimetallischen Pt-Ga, Pd-Ga und Rh-Ga Katalysatoren mittels Röntgenphotoelektronenspektroskopie |
| title_full | X-ray photoemission studies of bimetallic Pt-Ga, Pd-Ga and Rh-Ga catalysts = Untersuchungen an bimetallischen Pt-Ga, Pd-Ga und Rh-Ga Katalysatoren mittels Röntgenphotoelektronenspektroskopie vorgelegt von Mathias F. Grabau |
| title_fullStr | X-ray photoemission studies of bimetallic Pt-Ga, Pd-Ga and Rh-Ga catalysts = Untersuchungen an bimetallischen Pt-Ga, Pd-Ga und Rh-Ga Katalysatoren mittels Röntgenphotoelektronenspektroskopie vorgelegt von Mathias F. Grabau |
| title_full_unstemmed | X-ray photoemission studies of bimetallic Pt-Ga, Pd-Ga and Rh-Ga catalysts = Untersuchungen an bimetallischen Pt-Ga, Pd-Ga und Rh-Ga Katalysatoren mittels Röntgenphotoelektronenspektroskopie vorgelegt von Mathias F. Grabau |
| title_short | X-ray photoemission studies of bimetallic Pt-Ga, Pd-Ga and Rh-Ga catalysts |
| title_sort | x ray photoemission studies of bimetallic pt ga pd ga and rh ga catalysts untersuchungen an bimetallischen pt ga pd ga und rh ga katalysatoren mittels rontgenphotoelektronenspektroskopie |
| title_sub | = Untersuchungen an bimetallischen Pt-Ga, Pd-Ga und Rh-Ga Katalysatoren mittels Röntgenphotoelektronenspektroskopie |
| topic | Röntgen-Photoelektronenspektroskopie (DE-588)4076787-5 gnd Katalysator (DE-588)4029919-3 gnd Gadolinium (DE-588)4155786-4 gnd Platinmetalllegierung (DE-588)4377223-7 gnd |
| topic_facet | Röntgen-Photoelektronenspektroskopie Katalysator Gadolinium Platinmetalllegierung Hochschulschrift |
| url | http://d-nb.info/1180525957/04 http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=030932636&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
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