Non-noble metal catalysis: molecular approaches and reactions
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| Other Authors: | , |
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| Format: | Book |
| Language: | English |
| Published: |
Weinheim
Wiley-VCH
[2019]
|
| Subjects: | |
| Online Access: | http://www.wiley-vch.de/publish/dt/books/ISBN978-3-527-34061-3/ Inhaltsverzeichnis Buchcover |
| Physical Description: | xix, 590 Seiten Illustrationen, Diagramme |
| ISBN: | 9783527340613 |
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MARC
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| 015 | |a 18,N32 |2 dnb | ||
| 016 | 7 | |a 1163620653 |2 DE-101 | |
| 020 | |a 9783527340613 |c hbk. |9 978-3-527-34061-3 | ||
| 035 | |a (OCoLC)1090779456 | ||
| 035 | |a (DE-599)DNB1163620653 | ||
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| 084 | |a VE 7040 |0 (DE-625)147136:253 |2 rvk | ||
| 084 | |a 540 |2 sdnb | ||
| 245 | 1 | 0 | |a Non-noble metal catalysis |b molecular approaches and reactions |c edited by Robertus J.M. Klein Gebbink, Marc-Etienne Moret |
| 264 | 1 | |a Weinheim |b Wiley-VCH |c [2019] | |
| 264 | 4 | |c © 2019 | |
| 300 | |a xix, 590 Seiten |b Illustrationen, Diagramme | ||
| 336 | |b txt |2 rdacontent | ||
| 337 | |b n |2 rdamedia | ||
| 338 | |b nc |2 rdacarrier | ||
| 650 | 0 | 7 | |a Homogene Katalyse |0 (DE-588)4160579-2 |2 gnd |9 rswk-swf |
| 650 | 0 | 7 | |a Übergangsmetallkomplexe |0 (DE-588)4131837-7 |2 gnd |9 rswk-swf |
| 653 | |a Catalysis | ||
| 653 | |a Chemie | ||
| 653 | |a Chemistry | ||
| 653 | |a Industrial Chemistry | ||
| 653 | |a Katalyse | ||
| 653 | |a Nachhaltige u. Grüne Chemie | ||
| 653 | |a Sustainable Chemistry & Green Chemistry | ||
| 653 | |a Technische u. Industrielle Chemie | ||
| 655 | 7 | |0 (DE-588)4143413-4 |a Aufsatzsammlung |2 gnd-content | |
| 689 | 0 | 0 | |a Übergangsmetallkomplexe |0 (DE-588)4131837-7 |D s |
| 689 | 0 | 1 | |a Homogene Katalyse |0 (DE-588)4160579-2 |D s |
| 689 | 0 | |5 DE-604 | |
| 700 | 1 | |a Klein Gebbink, Bert |0 (DE-588)1074662008 |4 edt | |
| 700 | 1 | |a Moret, Marc-Etienne |d 1982- |0 (DE-588)1116540541 |4 edt | |
| 710 | 2 | |a Wiley-VCH |0 (DE-588)16179388-5 |4 pbl | |
| 776 | 0 | 8 | |i Erscheint auch als |n Online-Ausgabe, ePDF |z 978-3-527-69911-7 |
| 776 | 0 | 8 | |i Erscheint auch als |n Online-Ausgabe, ePub |z 978-3-527-69910-0 |
| 776 | 0 | 8 | |i Erscheint auch als |n Online-Ausgabe, oBook |z 978-3-527-69908-7 |
| 856 | 4 | 2 | |m X:MVB |u http://www.wiley-vch.de/publish/dt/books/ISBN978-3-527-34061-3/ |
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| 856 | 4 | 2 | |m SWB Datenaustausch |q application/pdf |u http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=030852067&sequence=000003&line_number=0002&func_code=DB_RECORDS&service_type=MEDIA |3 Buchcover |
| 999 | |a oai:aleph.bib-bvb.de:BVB01-030852067 | ||
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| _version_ | 1804179381922299904 |
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| adam_text | PREFACE
XVII
1
APPLICATION
OF
STIMULI-RESPONSIVE
AND
NON-INNOCENT
LIGANDS
IN
BASE
METAL
CATALYSIS
1
ANDREI
CHIRILA,
BRAJA
GOPAL
DAS,
PETRUS
F.
KUIJPERS,
VIVEK
SINHA,
AND
BAS
DE
BRUIN
1.1
INTRODUCTION
1
1.2
STIMULI-RESPONSIVE
LIGANDS
2
1.2.1
REDOX-RESPONSIVE
LIGANDS
3
1.2.2
PH-RESPONSIVE
LIGANDS
5
1.2.3
LIGHT-RESPONSIVE
LIGANDS
7
1.3
REDOX-ACTIVE
LIGANDS
AS
ELECTRON
RESERVOIRS
8
1.3.1
BIS(IMINO)PYRIDINE
(BIP)
8
1.3.1.1
ETHYLENE
POLYMERIZATION
WITH
BIP
9
1.3.1.2
CYCLOADDITION REACTIONS
10
1.3.1.3
HYDROGENATION
AND
HYDRO-ADDITION
REACTIONS
12
1.3.2
OTHER
LIGANDS
AS
ELECTRON
RESERVOIRS
14
1.4
COOPERATIVE
LIGANDS
15
1.4.1
COOPERATIVE
REACTIVITY
WITH
LIGAND
RADICALS
16
1.4.1.1
GALACTOSE
OXIDASE
(GOASE)
AND
ITS
MODELS
16
1.4.1.2
ALCOHOL
OXIDATION
BY
SALEN
COMPLEXES
18
1.4.2
BASE
METAL
COOPERATIVE
CATALYSIS
WITH
LIGANDS
ACTING
AS
AN
INTERNAL
BASE
18
1.4.2.1
FE-PINCER
COMPLEXES
19
1.4.2.2
LIGANDS
CONTAINING
A
PENDANT
BASE
20
1.5
SUBSTRATE
RADICALS
IN
CATALYSIS
21
1.5.1
CARBENE
RADICALS
22
1.5.2
NITRENE
RADICALS
25
1.6
SUMMARY
AND
CONCLUSIONS
26
REFERENCES
27
2
COMPUTATIONAL
INSIGHTS
INTO
CHEMICAL
REACTIVITY
AND
ROAD
TO
CATALYST
DESIGN:
THE
PARADIGM
OF
CO
2
HYDROGENATION
33
BHASKAR
MONDAL,
FRANK
NEESE,
AND
SHENG
FA
YE
2.1
INTRODUCTION
33
2.1.1
CHEMICAL
REACTIONS:
CONCEPTUAL
THOUGHTS
33
2.1.2
MOTIVATION
BEHIND
STUDYING
CO
2
HYDROGENATION
35
2.1.3
CHALLENGES
OF
CO
2
REDUCTION
35
2.1.4
CO
2
HYDROGENATION
37
2.1.5
NOBLE
VS
NON-NOBLE
METAL
CATALYSIS
38
2.1.6
CO
2
HYDROGENATION:
BASIC
MECHANISTIC
CONSIDERATIONS
38
2.2
REACTION
ENERGETICS
AND
GOVERNING
FACTOR
39
2.3
NEWLY
DESIGNED
CATALYSTS
AND
THEIR
REACTIVITY
42
2.4
CORRELATION
BETWEEN
HYDRICITY
AND
REACTIVITY
43
2.5
CONCLUDING
REMARKS
45
ACKNOWLEDGMENTS
46
REFERENCES
47
3
CATALYSIS
WITH
MULTINUDEAR
COMPLEXES
49
NEAL
P.
MANKAD
3.1
INTRODUCTION
49
3.2
STOICHIOMETRIC
REACTION
PATHWAYS
50
3.2.1
BIMETALLIC
BINDING
AND
ACTIVATION
OF
SUBSTRATES
50
3.2.1.1
SMALL-MOLECULE
ACTIVATION
51
3.2.1.2
ALKYNE
ACTIVATION
52
3.2.2
BIMETALLIC
ANALOGS
OF
OXIDATIVE
ADDITION
AND
REDUCTIVE
ELIMINATION
53
3.2.2.1
E
*
H
ADDITION
AND
ELIMINATION
54
3.2.2.2
C
*
X
ACTIVATION
AND
C
*
C
COUPLING
56
3.2.2.3
C=O
CLEAVAGE
57
3.3
APPLICATION
IN
CATALYSIS
57
3.3.1
CATALYSIS
WITH
REACTIVE
METAL-METAL
BONDS
58
3.3.1.1
BIMETALLIC
ALKYNE
CYCLOADDITIONS
58
3.3.1.2
BIMETALLIC
OXIDATIVE
ADDITION/REDUCTIVE
ELIMINATION
CYCLING
59
3.3.2
BIFUNCTIONAL
AND
TANDEM
CATALYSIS
WITHOUT
METAL-METAL
BONDS
59
3.3.2.1
COOPERATIVE
ACTIVATION
OF
UNSATURATED
SUBSTRATES
59
3.3.2.2
COOPERATIVE
PROCESSES
WITH
BIMETALLIC
OXIDATIVE
ADDITION
AND/OR
REDUCTIVE
ELIMINATION
62
3.4
POLYNUCLEAR
COMPLEXES
64
3.5
OUTLOOK
65
ACKNOWLEDGMENTS
66
REFERENCES
66
4
COPPER-CATALYZED
HYDROGENATIONS
AND
AEROBIC
N
*
N
BOND
FORMATIONS:
ACADEMIC
DEVELOPMENTS
AND
INDUSTRIAL
RELEVANCE
69
PAUL
L
ALSTERS
AND
LAURENT
LEFORT
4.1
INTRODUCTION
69
4.2
CU-PROMOTED
N
*
N
BOND
FORMATION
70
4.2.1
NONCYCLIZATION
N
*
N
OR
N=N
BOND
FORMATIONS
71
4.2.1.1
N
*
N
SINGLE-BOND-FORMING
REACTIONS
71
4.2.1.2
N=N
DOUBLE
BOND-FORMING
REACTIONS
72
4.2.2
CYCLIZATION
N
*
N
BOND
FORMATIONS
74
4.2.2.1
DEHYDROGENATIVE
CYCLIZATIONS
77
4.2.2.2
ELIMINATIVE
CYCLIZATIONS
80
4.2.2.Z
ELIMINATIVE
DEHYDROGENATIVE
CYCLIZATIONS
81
4.3
CU-CATALYZED
HOMOGENEOUS
HYDROGENATION
82
4.3.1
HYDROGENATION
OF
CO
2
TO
FORMATE
AND
DERIVATIVES
84
4.3.2
HYDROGENATION
OF
CARBONYL
COMPOUNDS
86
4.3.3
HYDROGENATION
OF
OLEFINS
AND
ALKYNES
89
4.4
CONCLUSIONS
91
REFERENCES
92
5
C=C
HYDROGENATIONS
WITH
IRON
GROUP
METAL
CATALYSTS
97
TIM
N.
GIESHOFFANDAXELJ.
VON
WANGELIN
5.1
INTRODUCTION
97
5.2
IRON
99
5.2.1
INTRODUCTION
99
5.2.2
PINCER
COMPLEXES
100
5.2.3
OTHERS
106
5.3
COBALT
107
5.3.1
INTRODUCTION
107
5.3.2
PINCER
COMPLEXES
108
5.3.3
OTHERS
115
5.4
NICKEL
118
5.4.1
INTRODUCTION
118
5.4.2
PINCER
COMPLEXES
119
5.4.3
OTHERS
121
5.5
CONCLUSION
122
ACKNOWLEDGMENTS
REFERENCES
123
123
6
BASE
METAL-CATALYZED
ADDITION
REACTIONS
ACROSS
C
*
C
MULTIPLE
BONDS
127
RODRIGO
RAMIREZ-CONTRERAS
AND
BIIL
MORANDI
6.1
INTRODUCTION
127
6.2
CATALYTIC
ADDITION
TO
ALKENES
INITIATED
THROUGH
RADICAL
MECHANISMS
128
6.2.1
HYDROGEN
ATOM
TRANSFER
AS
A
GENERAL
APPROACH
TO
HYDROFUNCTIONALIZATION
OF
UNSATURATED
BONDS
128
6.2.2
HYDRAZINES
AND
AZIDES
VIA
HYDROHYDRAZINATION
AND
HYDROAZIDATION
OF
OLEFINS
128
6.2.2.1
CO-
AND
MN-CATALYZED
HYDROHYDRAZINATION
128
6.2.2.2
COBALT-
AND
MANGANESE-CATALYZED
HYDROAZIDATION
OF
OLEFINS
130
6.2.3
CO-CATALYZED
HYDROCYANATION
OF
OLEFINS
WITH
TOSYL
CYANIDE
133
6.2.4
CO-CATALYZED
HYDROCHLORINATION
OF
OLEFINS
WITH
TOSYL
CHLORIDE
133
6.2.5
FE
LN
/NABH
4
-MEDIATED
ADDITIONS
OF
UNACTIVATED
ALKENES
134
6.2.6
CO-CATALYZED MARKOVNIKOV
HYDROALKOXYLATION
OF
UNACTIVATED
OLEFINS
135
6.2.7
FE-CATALYZED
HYDROMETHYLATION
OF
UNACTIVATED
OLEFINS
137
6.2.8
HYDROAMINATION
OF
OLEFINS
USING
NITROARENES
TO
OBTAIN
ANILINES
137
6.2.9
DUAL-CATALYTIC
MARKOVNIKOV
HYDROARYLATION
OF
ALKENES
139
6.3
OTHER
CATALYTIC
ADDITIONS
TO
UNSATURATED
BONDS
PROCEEDING
THROUGH
INITIAL
R
(R
/
H)
ATTACK
139
6.3.1
CU-CATALYZED
TRIFLUOROMETHYLATION
OF
UNACTIVATED
ALKENES
139
6.3.2
MN-CATALYZED
AEROBIC
OXIDATIVE
HYDROXYAZIDATION
OF
ALKENES
139
6.3.3
FE-CATALYZED
AMINOHYDROXYLATION
OF
ALKENES
141
6.4
CATALYTIC
ADDITION
TO
ALKENES
INITIATED
THROUGH
POLAR
MECHANISMS
143
6.4.1
CU-CATALYZED
HYDROAMINATION
OF
ALKENES
AND
ALKYNES
143
6.4.2
NI-CATALYZED,
LEWIS-ACID-ASSISTED
CARBOCYANATION
OF
ALKYNES
147
6.4.3
NI-CATALYZED
TRANSFER HYDROCYANATION
148
6.5
HYDROSILYLATION
REACTIONS
150
6.5.1
FE-CATALYZED,
ANTI-MARKOVNIKOV
HYDROSILYLATION
OF
ALKENES
WITH
TERTIARY
SILANES
AND
HYDROSILOXANES
150
6.5.2
HIGHLY
CHEMOSELECTIVE
CO-CATALYZED
HYDROSILYLATION
OF
FUNCTIONALIZED
ALKENES
USING
TERTIARY
SILANES
AND
HYDROSILOXANES
151
6.5.3
ALKENE
HYDROSILYLATION
USING
TERTIARY
SILANES
WITH
A-DIIMINE
NI
CATALYSTS
151
6.5.4
CHEMOSELECTIVE
ALKENE
HYDROSILYLATION
CATALYZED
BY
NI
PINCER
COMPLEXES
154
6.5.5
FE-
AND
CO-CATALYZED
REGIODIVERGENT
HYDROSILYLATION
OF
ALKENES
155
6.5.6
CO-CATALYZED
MARKOVNIKOV
HYDROSILYLATION
OF
TERMINAL
ALKYNES
AND
HYDROBORYLATION
OF
A-VINYLSILANES
155
6.5.7
FE
AND
CO
PIVALATE
ISOCYANIDE-LIGATED
CATALYST
SYSTEMS
FOR
HYDROSILYLATION
OF
ALKENES
WITH
HYDROSILOXANES
157
6.6
CONCLUSION
159
REFERENCES
160
7
IRON-CATALYZED
CYCLOPROPANATION
OF
ALKENES
BY
CARBENE
TRANSFER
REACTIONS
163
DANIELA
INTRIERI,
DANIELA
M.
CARMINATI,
AND
EMMA
GALLO
7.1
INTRODUCTION
163
7.2
ACHIRAL
IRON
PORPHYRIN
CATALYSTS
165
7.3
CHIRAL
IRON
PORPHYRIN
CATALYSTS
172
7
A
IRON
PHTHALOCYANINES
AND CORROLES
176
7.5
IRON
CATALYSTS
WITH
N
OR
N,O
LIGANDS
180
7.6
THE
[CP(CO)
2
FE
N
(THF)]BF
4
CATALYST
184
7.7
CONCLUSIONS
186
REFERENCES
187
8
NOVEL
SUBSTRATES
AND
NUCLEOPHILES
IN
ASYMMETRIC
COPPER-CATALYZED
CONJUGATE
ADDITION
REACTIONS
191
RAVINDRA
P.
JUMDE,
SYUZANNA
R.
HARUTYUNYAN,
AND
ADRIAAN
J.
MINNAARD
8.1
INTRODUCTION
191
8.2
CATALYTIC
ASYMMETRIC
CONJUGATE
ADDITIONS
TO A-SUBSTITUTED
A,P-UNSATURATED
CARBONYL
COMPOUNDS
192
8.3
CATALYTIC
ASYMMETRIC
CONJUGATE
ADDITIONS
TO
ALKENYL-HETEROARENES
196
8.3.1
A
BRIEF
OVERVIEW
OF
ASYMMETRIC
NUCLEOPHILIC
CONJUGATE
ADDITIONS
TO
ALKENYL-HETEROARENES
197
8.3.2
COPPER-CATALYZED
ASYMMETRIC
NUCLEOPHILIC
CONJUGATE
ADDITIONS
TO ALKENYL-HETEROARENES
198
8.4
CONCLUSION
205
REFERENCES
207
9
ASYMMETRIC
REDUCTION
OF
POLAR
DOUBLE
BONDS
209
RAPHAEL
BIGLER,
LORENA
DE
LUCA,
RAFFAEL
HUBER,
AND
ANTONIO
MEZZETTI
9.1
INTRODUCTION
209
9.1.1
CATALYTIC
APPROACHES
FOR
POLAR
DOUBLE
BOND
REDUCTION
209
9.1.2
THE
ROLE
OF
HYDRIDE
COMPLEXES
210
9.1.3
LIGAND
CHOICE
AND
CATALYST
STABILITY
211
9.2
MANGANESE
211
9.3
IRON
212
9.3.1
IRON
CATALYSTS
IN
ASYMMETRIC
TRANSFER
HYDROGENATION
(ATH)
213
9.3.2
IRON
CATALYSTS
IN
ASYMMETRIC
DIRECT
(H
2
)
HYDROGENATION
(AH)
218
9.3.3
IRON
CATALYSTS
IN
ASYMMETRIC
HYDROSILYLATION
(AHS)
220
9.4
COBALT
223
9.4.1
COBALT
CATALYSTS
IN
THE
AH
OF
KETONES
223
9.4.2
COBALT
CATALYSTS
IN
THE
ATH
OF
KETONES
224
9.4.3
COBALT
CATALYSTS
IN
ASYMMETRIC
HYDROSILYLATION
225
9.4.4
ASYMMETRIC
BOROHYDRIDE
REDUCTION
AND HYDROBORATION
226
9.5
NICKEL
228
9.5.1
NICKEL
CATALYSTS
IN
ASYMMETRIC
H
2
HYDROGENATION
228
9.5.2
NICKEL
ATH
CATALYSTS
228
9.5.3
NICKEL
AHS
CATALYSTS 229
9.5.4
NICKEL-CATALYZED
ASYMMETRIC
BOROHYDRIDE
REDUCTION
230
9.5.5
NI-CATALYZED
ASYMMETRIC
HYDROBORATION
OF
A,P-UNSATURATED
KETONES
230
9.6
COPPER
231
9.6.1
COPPER-CATALYZED
AH
231
9.6.2
COPPER-CATALYZED
ATH
OF
A-KETOESTERS
232
9.6.3
COPPER-CATALYZED
AHS
OF
KETONES
AND
IMINES
232
9.7
CONCLUSION
235
REFERENCES
235
10
IRON-,
COBALT-,
AND
MANGANESE-CATALYZED
HYDROSILYLATION
OF
CARBONYL
COMPOUNDS
AND
CARBON
DIOXIDE
241
CHRISTOPHE
DARCEL,
JEAN-BAPTISTE
SORTAIS,
DUO
WEI,
AND
ANTOINE
BRUNEAU-VOISINE
10.1
INTRODUCTION
241
10.2
HYDROSILYLATION
OF
ALDEHYDES
AND
KETONES
241
10.2.1
IRON-CATALYZED
HYDROSILYLATION
242
10.2.2
COBALT-CATALYZED
HYDROSILYLATION
247
10.2.3
MANGANESE-CATALYZED
HYDROSILYLATION
248
10.3
REDUCTION
OF
IMINES
AND
REDUCTIVE
AMINATION
OF
CARBONYL
COMPOUNDS
251
10.4
REDUCTION
OF
CARBOXYLIC ACID
DERIVATIVES
252
10.4.1
CARBOXAMIDES
AND
UREAS
252
10.4.2
CARBOXYLIC
ESTERS
254
10.4.3
CARBOXYLIC
ACIDS
257
10.5
HYDROELEMENTATION
OF
CARBON
DIOXIDE
258
10.5.1
HYDROSILYLATION
OF
CARBON
DIOXIDE
258
10.5.2
HYDROBORATION
OF
CARBON
DIOXIDE 259
10.6
CONCLUSION
260
REFERENCES
261
11
REACTIVE
INTERMEDIATES
AND
MECHANISM
IN
IRON-CATALYZED
CROSS-COUPLING
265
JARED
L
KNEEBONE,
JEFFREY
D.
SEARS,
AND
MICHAEL
L
NEIDIG
11.1
INTRODUCTION
265
11.2
CROSS-COUPLING
CATALYZED
BY
SIMPLE
IRON
SALTS
266
11.2.1
METHODS
OVERVIEW
266
11.2.2
MECHANISTIC
INVESTIGATIONS
267
11.3
TMEDA IN
IRON-CATALYZED
CROSS-COUPLING
273
11.3.1
METHODS
OVERVIEW
273
11.3.2
MECHANISTIC
INVESTIGATIONS
275
11.4
NHCS
IN
IRON-CATALYZED
CROSS-COUPLING
276
11.4.1
METHODS
OVERVIEW
276
11.4.2
MECHANISTIC
INVESTIGATIONS
279
11.5
PHOSPHINES
IN
IRON-CATALYZED
CROSS-COUPLING
283
11.5.1
METHODS
OVERVIEW
283
11.5.2
MECHANISTIC
INVESTIGATIONS
285
11.6
FUTURE
OUTLOOK
291
ACKNOWLEDGMENTS
291
REFERENCES
291
12
RECENT
ADVANCES
IN
COBALT-CATALYZED
CROSS-COUPLING
REACTIONS
297
ORIOLPLANAS,
CHRISTOPHER
J.
WHITEOAK,
AND
XAVI
RIBAS
12.1
INTRODUCTION
297
12.2
COBALT-CATALYZED
C
*
C
COUPLINGS
THROUGH
A
C
*
H
ACTIVATION
APPROACH
299
12.2.1
LOW-VALENT
COBALT
CATALYSIS
299
12.2.2
HIGH-VALENT
COBALT
CATALYSIS
302
12.3
COBALT-CATALYZED
C
*
C
COUPLINGS
USING
A
PREACTIVATED
SUBSTRATE
APPROACH
(ARYL
HALIDES
AND
PSEUDOHALIDES)
308
12.3.1
ARYL
OR
ALKENYL
HALIDES,
C(SP
2
)-X
308
12.3.2
ALKYL
HALIDES,
C(SP
3
)-X
309
12.3.3
ALKYNYL
HALIDES,
C(SP)-X
311
12.3.4
ARYL
HALIDES
WITHOUT
ORGANOMAGNESIUM
311
12.4
COBALT-CATALYZED
C
*
X
COUPLINGS
USING
C
*
H
ACTIVATION
APPROACHES
312
12.4.1
C
*
N
BOND
FORMATION
313
12.4.2
C
*
O
AND
C
*
S
BOND
FORMATION
317
12.4.3
C
*
X
BOND
FORMATION
(X
*
CL,
BR,
I,
AND
CN)
318
12.5
COBALT-CATALYZED
C
*
X
COUPLINGS
USING
A
PREACTIVATED
SUBSTRATE
APPROACH
(ARYL
HALIDES
AND
PSEUDOHALIDES)
320
12.5.1
C(SP
2
)-S
COUPLING
320
12.5.2
C(SP
2
)-N
COUPLING
321
12.5.3
C(SP
2
)-O
COUPLING
322
12.6
MISCELLANEOUS
322
12.7
CONCLUSIONS
AND
FUTURE
PROSPECTS
323
ACKNOWLEDGMENTS
323
REFERENCES
324
13
TRIFLUOROMETHYLATION
AND
RELATED
REACTIONS
329
JEREMY
JACQUET,
LOUIS
FENSTERBANK
;
AND
MARINE
DESAGE-EL
MURR
13.1
TRIFLUOROMETHYLATION
REACTIONS
329
13.1.1
COPPER(I)
SALTS
WITH
NUCLEOPHILIC
TRIFLUOROMETHYL
SOURCES
329
13.1.1.1
REACTIONS
WITH
ELECTROPHILES
330
13.1.1.2
REACTIONS
WITH
NUCLEOPHILES:
OXIDATIVE
COUPLING
331
13.1.2
GENERATION OF
CF
3
*
RADICALS
USING
LANGLOIS
*
REAGENT
332
13.1.3
COPPER
AND
ELECTROPHILIC
CF
3
+
SOURCES
333
13.2
TRIFLUOROMETHYLTHIOLATION
REACTIONS
341
13.2.1
NUCLEOPHILIC
TRIFLUOROMETHYLTHIOLATION
342
13.2.1.1
COPPER-CATALYZED
NUCLEOPHILIC
TRIFLUOROMETHYLTHIOLATION
342
13.2.1.2
NICKEL-CATALYZED NUCLEOPHILIC
TRIFLUOROMETHYLTHIOLATION
344
13.2.2
ELECTROPHILIC
TRIFLUOROMETHYLTHIOLATION
345
13.3
PERFLUOROALKYLATION
REACTIONS
348
13.4
CONCLUSION
350
REFERENCES
350
14
CATALYTIC
OXYGENATION
OF
C=C
AND
C
*
H
BONDS
355
PRADIP
GHOSH,
MARC-ETIENNE
MORET,
AND
ROBERT
J.
M.
KLEIN
GEBBINK
14.1
INTRODUCTION
355
14.2
OXYGENATION
OF
C=C
BONDS
356
14.2.1
MANGANESE
CATALYSTS
356
14.2.2
IRON
CATALYSTS
363
14.2.3
COBALT,
NICKEL,
AND
COPPER
CATALYSTS
372
14.3
OXYGENATION
OF
C
*
H
BONDS
376
14.3.1
MANGANESE
CATALYSTS
376
14.3.2
IRON
CATALYSTS
377
14.3.3
COBALT
CATALYSTS
380
14.3.4
NICKEL
CATALYSTS
381
14.3.5
COPPER
CATALYSTS
383
14.4
CONCLUSIONS
AND
OUTLOOK
384
ACKNOWLEDGMENT
385
REFERENCES
385
15
ORGANOMETALLIC
CHELATION-ASSISTED
C-H
FUNCTIONALIZATION
391
PARTHASARATHY
GANDEEPAN
AND
LUTZ
ACKERMANN
15.1
INTRODUCTION
391
15.2
C
*
C
BOND
FORMATION
VIA
C
*
H
ACTIVATION
392
15.2.1
REACTION
WITH
UNSATURATED
SUBSTRATES
392
15.2.1.1
ADDITION
TO
C
*
C
MULTIPLE
BONDS
392
15.2.1.2
ADDITION
TO
C
*
HETEROATOM
MULTIPLE
BONDS
393
15.2.1.3
OXIDATIVE
C
*
H
OLEFINATION
396
15.2.1.4
C
*
H
ALLYLATION
397
15.2.1.5
OXIDATIVE
C
*
H
FUNCTIONALIZATION
AND
ANNULATIONS
397
15.2.1.6
C
*
H
ALKYNYLATIONS
403
15.2.2
C
*
H
CYANATION
404
15.2.3
C
*
H
ARYLATION
404
15.2.4
C
*
H
ALKYLATION
407
15.3
C
*
HETEROATOM
FORMATION
VIA
C
*
H
ACTIVATION
409
15.3.1
C
*
N
FORMATION
VIA
C
*
H
ACTIVATION
409
15.3.1.1
C
*
H
AMINATION
WITH UNACTIVATED
AMINES
409
15.3.1.2
C
*
H
AMINATION
WITH
ACTIVATED
AMINE
SOURCES
409
15.3.2
C
*
O
FORMATION
VIA
C
*
H
ACTIVATION
412
15.3.3
C
*
HALOGEN
FORMATION
VIA
C
*
H
ACTIVATION
412
15.3.4
C
*
CHALCOGEN
FORMATION
VIA
C
*
H
ACTIVATION
414
15.4
CONCLUSIONS
415
ACKNOWLEDGMENTS
415
REFERENCES
415
16
CATALYTIC
WATER
OXIDATION:
WATER
OXIDATION
TO
O
2
MEDIATED
BY
3D
TRANSITION
METAL
COMPLEXES
425
ZOEI
CODOLA,
JULIO
LLORET-FILLOL,
AND
MIQUEL
COSTAS
16.1
WATER
OXIDATION
-
FROM
INSIGHTS
INTO
FUNDAMENTAL
CHEMICAL
CONCEPTS
TO
FUTURE
SOLAR
FUELS
425
16.1.1
THE
OXYGEN-EVOLVING
COMPLEX.
A
WELL-DEFINED
TETRAMANGANESE
CALCIUM
CLUSTER
425
16.1.2
SYNTHETIC
MODELS
FOR
THE
NATURAL
WATER
OXIDATION
REACTION
428
16.1.3
OXIDANTS
IN
WATER
OXIDATION
REACTIONS
428
16.2
MODEL
WELL-DEFINED
WATER
OXIDATION
CATALYSTS
430
16.2.1
MANGANESE
WATER
OXIDATION
CATALYSTS
430
16.2.1.1
BIOINSPIRED
MN
4
O
4
MODELS
430
16.2.1.2
BIOMIMETIC
MODELS
INCLUDING
A
LEWIS
ACID
432
16.2.1.3
CATALYTIC
WATER
OXIDATION
WITH
MANGANESE COORDINATION
COMPLEXES
433
16.2.2
WATER
OXIDATION
WITH
MOLECULAR
IRON
CATALYSTS
435
16.2.2.1
IRON
CATALYSTS
WITH
TETRA-ANIONIC
TETRA-AMIDO
MACROCYCLIC
LIGANDS
436
16.2.2.2
MONONUCLEAR
COMPLEXES
WITH
MONOANIONIC
POLYAMINE
LIGANDS
437
16.2.2.3
IRON
CATALYSTS
WITH
NEUTRAL
LIGANDS
437
16.2.2.4
WATER
OXIDATION
BY
A
MULTI-IRON
CATALYST
440
16.2.3
COBALT
WATER
OXIDATION
CATALYSTS
440
16.2.4
NICKEL-BASED
WATER
OXIDATION
CATALYSTS
443
16.2.5
COPPER-BASED
WATER
OXIDATION
CATALYSTS
445
16.3
CONCLUSION
AND
OUTLOOK
446
REFERENCES
448
17
BASE-METAL-CATALYZED
HYDROGEN
GENERATION
FROM
CARBON-
AND
BORON
NITROGEN-BASED
SUBSTRATES
453
ELISABETTA
ALBERICO,
LYDIA
K.
VOGT,
NILS
ROCKSTROH,
AND
HENRIK
JUNGE
17.1
INTRODUCTION
453
17.1.1
STATE
OF
THE
ART
OF
HYDROGEN
GENERATION
FROM
CARBON-
AND
BORON
NITROGEN-BASED
SUBSTRATES
453
17.1.2
DEVELOPMENT
OF
BASE
METAL
CATALYSTS
FOR
CATALYTIC
HYDROGEN
GENERATION
458
17.2
HYDROGEN
GENERATION
FROM
FORMIC
ACID
460
17.2.1
IRON
461
17.2.2
NICKEL
466
17.2.3
ALUMINUM
467
17.2.4
MISCELLANEOUS
467
17.3
HYDROGEN
GENERATION
FROM
ALCOHOLS
469
17.3.1
HYDROGEN
GENERATION
WITH
RESPECT
TO
ENERGETIC
APPLICATION
469
17.3.2
HYDROGEN
GENERATION
COUPLED
WITH
THE
SYNTHESIS
OF
ORGANIC
COMPOUNDS
470
17.4
HYDROGEN
STORAGE
IN
LIQUID
ORGANIC
HYDROGEN
CARRIERS
473
17.5
DEHYDROGENATION
OF
AMMONIA
BORANE
AND
AMINE
BORANES
474
17.5.1
OVERVIEW
ON
CONDITIONS
FOR
H
2
LIBERATION
FROM
AMMONIA
BORANE
AND
AMINE
BORANES
474
17.5.2
NON-NOBLE
METAL-CATALYZED
DEHYDROGENATION
OF
AMMONIA
BORANE
AND
AMINE
BORANES
476
17.6
CONCLUSION
480
REFERENCES
481
18
MOLECULAR
CATALYSTS
FOR
PROTON
REDUCTION
BASED
ON
NON-NOBLE
METALS
489
CATHERINE
ELLEOUET,
FRANCOIS
Y.
PETITION,
AND
PHILIPPE
SCHOLLHAMMER
18.1
INTRODUCTION
489
18.2
IRON AND
NICKEL
CATALYSTS
489
18.2.1
BIOINSPIRED
DI-IRON
MOLECULES
490
18.2.2
MONO-
AND
POLY-IRON
COMPLEXES
496
18.2.3
BIOINSPIRED
[NIFE]
COMPLEXES
AND
[NIMN]
ANALOGS
501
18.2.4
OTHER
NICKEL-BASED
CATALYSTS
506
18.3
OTHER
NON-NOBLE
METAL-BASED
CATALYSTS:
CO,
MN,
CU,
MO,
AND
W
508
18.3.1
COBALT
508
18.3.2
MANGANESE
512
18.3.3
COPPER
514
18.3.4
GROUP
6
METALS
(MO,
W)
514
18.4
CONCLUSION
518
REFERENCES
518
19
NONREDUCTIVE
REACTIONS
OF
CO
2
MEDIATED
BY
COBALT
CATALYSTS:
CYCLIC
AND
POLYCARBONATES
529
THOMAS
A.
ZEVACO
AND
ARJAN
W.
KLEI
/
19.1
INTRODUCTION
529
19.2
COCATALYSTS
FOR
CO
2
/EPOXIDE
COUPLINGS:
SALEN-BASED
SYSTEMS
530
19.3
CO-PORPHYRINS
AS
CATALYSTS FOR
EPOXIDE/CO
2
COUPLING
537
19.4
COCATALYSTS
BASED
ON
OTHER
N
4
-LIGATED
AND
RELATED
SYSTEMS
540
19.5
AMINOPHENOXIDE-BASED
CO
COMPLEXES
542
19.6
CONCLUSION
AND
OUTLOOK
544
ACKNOWLEDGMENTS
545
REFERENCES
545
20
DINITROGEN
REDUCTION
549
FENNA
F.
VAN
DE
WATERING
AND
WOJCIECH
/.
DZIK
20.1
INTRODUCTION
549
20.2
ACTIVATION
OF
N
2
550
20.3
REDUCTION
OF
N
2
TO
AMMONIA
551
20.3.1
HABER-BOSCH-INSPIRED
SYSTEMS
551
20.3.2
NITROGENASE-INSPIRED
SYSTEMS
555
20.3.2.1
EARLY
MECHANISTIC
STUDIES
ON
N
2
REDUCTION
BY
METAL
COMPLEXES
556
20.3.2.2
IRON-SULFUR
SYSTEMS
557
20.3.3
CATALYTIC
AMMONIA FORMATION
559
20.3.3.1
TRIPODAL
SYSTEMS
560
20.3.3.2
IRON
AND
COBALT
PNP
SYSTEMS
566
20.3.3.3
THE
CYCLIC
AMINOCARBENE
IRON
SYSTEM
567
20.3.3.4
THE
DIPHOSPHINE IRON
SYSTEM
568
20.4
REDUCTION
OF
N
2
TO
SILYLAMINES
569
20.4.1
IRON
570
20.4.2
COBALT
572
20.5
CONCLUSIONS
AND
OUTLOOK
575
ACKNOWLEDGMENTS
576
REFERENCES
576
INDEX
583
|
| any_adam_object | 1 |
| author2 | Klein Gebbink, Bert Moret, Marc-Etienne 1982- |
| author2_role | edt edt |
| author2_variant | g b k gb gbk m e m mem |
| author_GND | (DE-588)1074662008 (DE-588)1116540541 |
| author_facet | Klein Gebbink, Bert Moret, Marc-Etienne 1982- |
| building | Verbundindex |
| bvnumber | BV045466880 |
| classification_rvk | VK 5560 VE 7040 |
| ctrlnum | (OCoLC)1090779456 (DE-599)DNB1163620653 |
| discipline | Chemie / Pharmazie |
| format | Book |
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| genre | (DE-588)4143413-4 Aufsatzsammlung gnd-content |
| genre_facet | Aufsatzsammlung |
| id | DE-604.BV045466880 |
| illustrated | Illustrated |
| indexdate | 2024-07-10T08:18:49Z |
| institution | BVB |
| institution_GND | (DE-588)16179388-5 |
| isbn | 9783527340613 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-030852067 |
| oclc_num | 1090779456 |
| open_access_boolean | |
| owner | DE-29T DE-703 DE-11 |
| owner_facet | DE-29T DE-703 DE-11 |
| physical | xix, 590 Seiten Illustrationen, Diagramme |
| publishDate | 2019 |
| publishDateSearch | 2019 |
| publishDateSort | 2019 |
| publisher | Wiley-VCH |
| record_format | marc |
| spelling | Non-noble metal catalysis molecular approaches and reactions edited by Robertus J.M. Klein Gebbink, Marc-Etienne Moret Weinheim Wiley-VCH [2019] © 2019 xix, 590 Seiten Illustrationen, Diagramme txt rdacontent n rdamedia nc rdacarrier Homogene Katalyse (DE-588)4160579-2 gnd rswk-swf Übergangsmetallkomplexe (DE-588)4131837-7 gnd rswk-swf Catalysis Chemie Chemistry Industrial Chemistry Katalyse Nachhaltige u. Grüne Chemie Sustainable Chemistry & Green Chemistry Technische u. Industrielle Chemie (DE-588)4143413-4 Aufsatzsammlung gnd-content Übergangsmetallkomplexe (DE-588)4131837-7 s Homogene Katalyse (DE-588)4160579-2 s DE-604 Klein Gebbink, Bert (DE-588)1074662008 edt Moret, Marc-Etienne 1982- (DE-588)1116540541 edt Wiley-VCH (DE-588)16179388-5 pbl Erscheint auch als Online-Ausgabe, ePDF 978-3-527-69911-7 Erscheint auch als Online-Ausgabe, ePub 978-3-527-69910-0 Erscheint auch als Online-Ausgabe, oBook 978-3-527-69908-7 X:MVB http://www.wiley-vch.de/publish/dt/books/ISBN978-3-527-34061-3/ DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=030852067&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis SWB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=030852067&sequence=000003&line_number=0002&func_code=DB_RECORDS&service_type=MEDIA Buchcover |
| spellingShingle | Non-noble metal catalysis molecular approaches and reactions Homogene Katalyse (DE-588)4160579-2 gnd Übergangsmetallkomplexe (DE-588)4131837-7 gnd |
| subject_GND | (DE-588)4160579-2 (DE-588)4131837-7 (DE-588)4143413-4 |
| title | Non-noble metal catalysis molecular approaches and reactions |
| title_auth | Non-noble metal catalysis molecular approaches and reactions |
| title_exact_search | Non-noble metal catalysis molecular approaches and reactions |
| title_full | Non-noble metal catalysis molecular approaches and reactions edited by Robertus J.M. Klein Gebbink, Marc-Etienne Moret |
| title_fullStr | Non-noble metal catalysis molecular approaches and reactions edited by Robertus J.M. Klein Gebbink, Marc-Etienne Moret |
| title_full_unstemmed | Non-noble metal catalysis molecular approaches and reactions edited by Robertus J.M. Klein Gebbink, Marc-Etienne Moret |
| title_short | Non-noble metal catalysis |
| title_sort | non noble metal catalysis molecular approaches and reactions |
| title_sub | molecular approaches and reactions |
| topic | Homogene Katalyse (DE-588)4160579-2 gnd Übergangsmetallkomplexe (DE-588)4131837-7 gnd |
| topic_facet | Homogene Katalyse Übergangsmetallkomplexe Aufsatzsammlung |
| url | http://www.wiley-vch.de/publish/dt/books/ISBN978-3-527-34061-3/ http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=030852067&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=030852067&sequence=000003&line_number=0002&func_code=DB_RECORDS&service_type=MEDIA |
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