Holdings: Single-molecule junctions with epitaxial graphene electrodes

Single-molecule junctions with epitaxial graphene electrodes: = Einzelmolekülkontakte mit Epitaktischen Graphen Elektroden

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Bibliographic Details
Main Author:	Ullmann, Konrad (Author)
Format:	Thesis Book
Language:	English
Published:	Erlangen ; Nürnberg 2018
Subjects:	Graphen Strom-Spannungs-Kennlinie Freies Molekül Fullerene Elektrode Elektrischer Kontakt Hochschulschrift
Online Access:	Inhaltsverzeichnis Inhaltsverzeichnis
Physical Description:	vi, 121 Seiten Illustrationen, Diagramme 21 cm

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MARC


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adam_text	C O N TE N TS ZUSAMMENFASSUNG I 1 INTRODUCTION 1 2 THEORY OF TRANSPORT IN NANOCONTACTS 3 2.1 LANDAUER-BUETTIKER M E TH O D .......................................................... 4 2.2 QUANTUM TUNNELING....................................................................... 8 2.3 COHERENT TRANSPORT IN SINGLE-MOLECULE J U N C TIO N S ........................ 11 2.3.1 SINGLE-LEVEL MODEL .......................................................... 12 3 NANOGAPS IN GRAPHENE 19 3.1 SAMPLE P REP ARATIO N ....................................................................... 19 3.1.1 SILICON CARBIDE S U B STRA TE ................................................. 19 3.1.2 GRAPHENE G RO W TH ............................................................. 21 3.1.3 PATTERNING OF METAL AND GRAPHENE S TRU CTU RES ............... 23 3.1.4 SAMPLE D ESIGN.................................................................... 27 3.2 FORMING NANOGAPS BY E LECTROBURNING ........................................ 28 3.2.1 FEEDBACK CONTROLLED ELECTROBURNING............................... 29 3.2.2 ANNEALING AND ^ -C LE A N IN G .............................................. 30 3.2.3 CURRENT ANNEALING ............................................................. 32 3.3 CHARACTERIZATION OF GRAPHENE NANOELECTRODES............................ 34 3.3.1 TOPOLOGY............................................................................. 34 3.3.2 TUNNELING C U RREN T ............................................................. 41 3.3.3 TEMPERATURE AND TIME S TA B ILITY ..................................... 42 3.3.4 INFLUENCE OF GASEOUS E NVIRONM ENT.................................. 43 3.4 FREESTANDING GRAPHENE E LECTRODES .............................................. 47 3.4.1 SUSPENDED G RA P H E N E ....................................................... 47 3.4.2 TEARING SUSPENDED G RAPHENE ........................................... 51 4 SINGLE-MOLECULE EXPERIMENTS 55 4.1 FULLERENE-CYCLOPHANE M OLECULE..................................................... 55 4.1.1 EMPLOYING EPITAXIAL GRAPHENE N ANOELECTRODES ............ 56 4.1.2 COMPARISON TO GOLD ELECTRODES ........................................ 62 4.1.3 THEORETICAL D ESCRIPTION..................................................... 67 4.2 FULLERENE-FE2+ M OLECULE................................................................. 80 4.2.1 HYSTERETIC S TRU C TU RE S ........................................................ 83 4.2.2 NEGATIVE DIFFERENTIAL RESISTANCE ..................................... 85 4.2.3 LONG-TERM FLUCTUATIONS .................................................... 89 4.3 POLYYNE MOLECULES.......................................................................... 91 4.3.1 PLATINUM-POLYYNE M OLECULES............................................ 93 4.4 CRITICAL DISCUSSION ON SINGLE-MOLECULE JUNCTIONS WITH GRAPHENE E LECTRO D ES......................................................................................... 101 5 SUMMARY 105 LIST OF PUBLICATIONS 107 ABBREVIATIONS AND SYMBOLS 109 BIBLIOGRAPHY 111
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author	Ullmann, Konrad
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spelling	Ullmann, Konrad Verfasser (DE-588)1174851074 aut Single-molecule junctions with epitaxial graphene electrodes = Einzelmolekülkontakte mit Epitaktischen Graphen Elektroden vorgelegt von Konrad Ullmann Einzelmolekülkontakte mit Epitaktischen Graphen Elektroden Erlangen ; Nürnberg 2018 vi, 121 Seiten Illustrationen, Diagramme 21 cm txt rdacontent n rdamedia nc rdacarrier Dissertation Friedrich-Alexander-Universität Erlangen-Nürnberg 2018 Graphen (DE-588)7591667-8 gnd rswk-swf Strom-Spannungs-Kennlinie (DE-588)4314420-2 gnd rswk-swf Freies Molekül (DE-588)4489205-6 gnd rswk-swf Fullerene (DE-588)4305238-1 gnd rswk-swf Elektrode (DE-588)4014247-4 gnd rswk-swf Elektrischer Kontakt (DE-588)4151733-7 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Graphen (DE-588)7591667-8 s Elektrode (DE-588)4014247-4 s Freies Molekül (DE-588)4489205-6 s Fullerene (DE-588)4305238-1 s Elektrischer Kontakt (DE-588)4151733-7 s Strom-Spannungs-Kennlinie (DE-588)4314420-2 s DE-604 B:DE-101 application/pdf http://d-nb.info/1171494610/04 Inhaltsverzeichnis DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=030762100&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis
spellingShingle	Ullmann, Konrad Single-molecule junctions with epitaxial graphene electrodes = Einzelmolekülkontakte mit Epitaktischen Graphen Elektroden Graphen (DE-588)7591667-8 gnd Strom-Spannungs-Kennlinie (DE-588)4314420-2 gnd Freies Molekül (DE-588)4489205-6 gnd Fullerene (DE-588)4305238-1 gnd Elektrode (DE-588)4014247-4 gnd Elektrischer Kontakt (DE-588)4151733-7 gnd
subject_GND	(DE-588)7591667-8 (DE-588)4314420-2 (DE-588)4489205-6 (DE-588)4305238-1 (DE-588)4014247-4 (DE-588)4151733-7 (DE-588)4113937-9
title	Single-molecule junctions with epitaxial graphene electrodes = Einzelmolekülkontakte mit Epitaktischen Graphen Elektroden
title_alt	Einzelmolekülkontakte mit Epitaktischen Graphen Elektroden
title_auth	Single-molecule junctions with epitaxial graphene electrodes = Einzelmolekülkontakte mit Epitaktischen Graphen Elektroden
title_exact_search	Single-molecule junctions with epitaxial graphene electrodes = Einzelmolekülkontakte mit Epitaktischen Graphen Elektroden
title_full	Single-molecule junctions with epitaxial graphene electrodes = Einzelmolekülkontakte mit Epitaktischen Graphen Elektroden vorgelegt von Konrad Ullmann
title_fullStr	Single-molecule junctions with epitaxial graphene electrodes = Einzelmolekülkontakte mit Epitaktischen Graphen Elektroden vorgelegt von Konrad Ullmann
title_full_unstemmed	Single-molecule junctions with epitaxial graphene electrodes = Einzelmolekülkontakte mit Epitaktischen Graphen Elektroden vorgelegt von Konrad Ullmann
title_short	Single-molecule junctions with epitaxial graphene electrodes
title_sort	single molecule junctions with epitaxial graphene electrodes einzelmolekulkontakte mit epitaktischen graphen elektroden
title_sub	= Einzelmolekülkontakte mit Epitaktischen Graphen Elektroden
topic	Graphen (DE-588)7591667-8 gnd Strom-Spannungs-Kennlinie (DE-588)4314420-2 gnd Freies Molekül (DE-588)4489205-6 gnd Fullerene (DE-588)4305238-1 gnd Elektrode (DE-588)4014247-4 gnd Elektrischer Kontakt (DE-588)4151733-7 gnd
topic_facet	Graphen Strom-Spannungs-Kennlinie Freies Molekül Fullerene Elektrode Elektrischer Kontakt Hochschulschrift
url	http://d-nb.info/1171494610/04 http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=030762100&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA
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