Electrochemical Activation of Catalysis: Promotion, Electrochemical Promotion, and Metal-Support Interactions
I knew nothing of the work of C. G. Vayenas on NEMCA until the early nineties. Then I learned from a paper of his idea (gas interface reactions could be catalyzed electrochemically), which seemed quite marvelous; but I did not understand how it worked. Consequently, I decided to correspond with Prof...
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| Hauptverfasser: | , , , |
|---|---|
| Format: | Elektronisch E-Book |
| Sprache: | English |
| Veröffentlicht: |
Boston, MA
Springer US
2001
|
| Schlagworte: | |
| Online-Zugang: | UBT01 URL des Erstveröffentlichers |
| Zusammenfassung: | I knew nothing of the work of C. G. Vayenas on NEMCA until the early nineties. Then I learned from a paper of his idea (gas interface reactions could be catalyzed electrochemically), which seemed quite marvelous; but I did not understand how it worked. Consequently, I decided to correspond with Professor Vayenas in Patras, Greece, to reach a better understanding of this concept. I think that my early papers (1946, 1947, and 1957), on the relationship between the work function of metal surfaces and electron transfer reactions thereat to particles in solution, held me in good stead to be receptive to what Vayenas told me. As the electrode potential changes, so of course, does the work function at the interface, and gas metal reactions there involve adsorbed particles which have bonding to the surface. Whether electron transfer is complete in such a case, or whether the effect is on the desorption of radicals, the work function determines the strength of their bonding, and if one varies the work function by varying the electrode potential, one can vary the reaction rate at the interface. I got the idea. After that, it has been smooth sailing. Dr. Vayenas wrote a seminal article in Modern Aspects of Electrochemistry, Number 29, and brought the field into the public eye. It has since grown and its usefulness in chemical catalytic reactions has been demonstrated and verified worldwide |
| Beschreibung: | 1 Online-Ressource (XXXII, 574 p) |
| ISBN: | 9780306475511 |
| DOI: | 10.1007/b115566 |
Internformat
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| 520 | |a I knew nothing of the work of C. G. Vayenas on NEMCA until the early nineties. Then I learned from a paper of his idea (gas interface reactions could be catalyzed electrochemically), which seemed quite marvelous; but I did not understand how it worked. Consequently, I decided to correspond with Professor Vayenas in Patras, Greece, to reach a better understanding of this concept. I think that my early papers (1946, 1947, and 1957), on the relationship between the work function of metal surfaces and electron transfer reactions thereat to particles in solution, held me in good stead to be receptive to what Vayenas told me. As the electrode potential changes, so of course, does the work function at the interface, and gas metal reactions there involve adsorbed particles which have bonding to the surface. Whether electron transfer is complete in such a case, or whether the effect is on the desorption of radicals, the work function determines the strength of their bonding, and if one varies the work function by varying the electrode potential, one can vary the reaction rate at the interface. I got the idea. After that, it has been smooth sailing. Dr. Vayenas wrote a seminal article in Modern Aspects of Electrochemistry, Number 29, and brought the field into the public eye. It has since grown and its usefulness in chemical catalytic reactions has been demonstrated and verified worldwide | ||
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Datensatz im Suchindex
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| author | Vayenas, Costas G. Bebelis, Symeon Pliangos, Costas Brosda, Susanne |
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| dewey-full | 541.37 |
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| dewey-tens | 540 - Chemistry and allied sciences |
| discipline | Chemie / Pharmazie |
| doi_str_mv | 10.1007/b115566 |
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| id | DE-604.BV045151706 |
| illustrated | Not Illustrated |
| indexdate | 2024-07-10T08:10:06Z |
| institution | BVB |
| isbn | 9780306475511 |
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| spelling | Vayenas, Costas G. Verfasser aut Electrochemical Activation of Catalysis Promotion, Electrochemical Promotion, and Metal-Support Interactions by Costas G. Vayenas, Symeon Bebelis, Costas Pliangos, Susanne Brosda, Demetrios Tsiplakides Boston, MA Springer US 2001 1 Online-Ressource (XXXII, 574 p) txt rdacontent c rdamedia cr rdacarrier I knew nothing of the work of C. G. Vayenas on NEMCA until the early nineties. Then I learned from a paper of his idea (gas interface reactions could be catalyzed electrochemically), which seemed quite marvelous; but I did not understand how it worked. Consequently, I decided to correspond with Professor Vayenas in Patras, Greece, to reach a better understanding of this concept. I think that my early papers (1946, 1947, and 1957), on the relationship between the work function of metal surfaces and electron transfer reactions thereat to particles in solution, held me in good stead to be receptive to what Vayenas told me. As the electrode potential changes, so of course, does the work function at the interface, and gas metal reactions there involve adsorbed particles which have bonding to the surface. Whether electron transfer is complete in such a case, or whether the effect is on the desorption of radicals, the work function determines the strength of their bonding, and if one varies the work function by varying the electrode potential, one can vary the reaction rate at the interface. I got the idea. After that, it has been smooth sailing. Dr. Vayenas wrote a seminal article in Modern Aspects of Electrochemistry, Number 29, and brought the field into the public eye. It has since grown and its usefulness in chemical catalytic reactions has been demonstrated and verified worldwide Chemistry Electrochemistry Physical Chemistry Analytical Chemistry Industrial Chemistry/Chemical Engineering Ceramics, Glass, Composites, Natural Methods Analytical chemistry Physical chemistry Chemical engineering Elektrokatalyse (DE-588)4151819-6 gnd rswk-swf Elektrokatalyse (DE-588)4151819-6 s 1\p DE-604 Bebelis, Symeon aut Pliangos, Costas aut Brosda, Susanne aut Erscheint auch als Druck-Ausgabe 9780306467196 https://doi.org/10.1007/b115566 Verlag URL des Erstveröffentlichers Volltext 1\p cgwrk 20201028 DE-101 https://d-nb.info/provenance/plan#cgwrk |
| spellingShingle | Vayenas, Costas G. Bebelis, Symeon Pliangos, Costas Brosda, Susanne Electrochemical Activation of Catalysis Promotion, Electrochemical Promotion, and Metal-Support Interactions Chemistry Electrochemistry Physical Chemistry Analytical Chemistry Industrial Chemistry/Chemical Engineering Ceramics, Glass, Composites, Natural Methods Analytical chemistry Physical chemistry Chemical engineering Elektrokatalyse (DE-588)4151819-6 gnd |
| subject_GND | (DE-588)4151819-6 |
| title | Electrochemical Activation of Catalysis Promotion, Electrochemical Promotion, and Metal-Support Interactions |
| title_auth | Electrochemical Activation of Catalysis Promotion, Electrochemical Promotion, and Metal-Support Interactions |
| title_exact_search | Electrochemical Activation of Catalysis Promotion, Electrochemical Promotion, and Metal-Support Interactions |
| title_full | Electrochemical Activation of Catalysis Promotion, Electrochemical Promotion, and Metal-Support Interactions by Costas G. Vayenas, Symeon Bebelis, Costas Pliangos, Susanne Brosda, Demetrios Tsiplakides |
| title_fullStr | Electrochemical Activation of Catalysis Promotion, Electrochemical Promotion, and Metal-Support Interactions by Costas G. Vayenas, Symeon Bebelis, Costas Pliangos, Susanne Brosda, Demetrios Tsiplakides |
| title_full_unstemmed | Electrochemical Activation of Catalysis Promotion, Electrochemical Promotion, and Metal-Support Interactions by Costas G. Vayenas, Symeon Bebelis, Costas Pliangos, Susanne Brosda, Demetrios Tsiplakides |
| title_short | Electrochemical Activation of Catalysis |
| title_sort | electrochemical activation of catalysis promotion electrochemical promotion and metal support interactions |
| title_sub | Promotion, Electrochemical Promotion, and Metal-Support Interactions |
| topic | Chemistry Electrochemistry Physical Chemistry Analytical Chemistry Industrial Chemistry/Chemical Engineering Ceramics, Glass, Composites, Natural Methods Analytical chemistry Physical chemistry Chemical engineering Elektrokatalyse (DE-588)4151819-6 gnd |
| topic_facet | Chemistry Electrochemistry Physical Chemistry Analytical Chemistry Industrial Chemistry/Chemical Engineering Ceramics, Glass, Composites, Natural Methods Analytical chemistry Physical chemistry Chemical engineering Elektrokatalyse |
| url | https://doi.org/10.1007/b115566 |
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