Model studies of ceria-based catalysts for fuel cell applications: = Modelluntersuchungen von Ceroxid-haltigen Katalysatoren für Anwendungen in Brennstoffzellen
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| Format: | Thesis Book |
| Language: | German English |
| Published: |
Erlangen ; Nürnberg
2016
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| Subjects: | |
| Online Access: | Inhaltsverzeichnis |
| Item Description: | Enthalten mehrere Sonderdrucke |
| Physical Description: | 163 Seiten in getrennter Zählung Illustrationen, Diagramme |
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| 245 | 1 | 0 | |a Model studies of ceria-based catalysts for fuel cell applications |b = Modelluntersuchungen von Ceroxid-haltigen Katalysatoren für Anwendungen in Brennstoffzellen |c vorgelegt von Armin Neitzel aus Nürnberg |
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Record in the Search Index
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|---|---|
| adam_text | FRIEDRICH-ALEXANDER
UNIVERSITAET
ERLANGEN-NUERNBERG
DEPARTMENT
CHEMIE UND PHARMAZIE
NATURWISSENSCHAFTLICHE
FAKULTAET
MODEL STUDIES OF CERIA-BASED CATALYSTS
FOR FUEL CELL APPLICATIONS
MODELLUNTERSUCHUNGEN VON CEROXID-HALTIGEN
KATALYSATOREN FUR ANWENDUNGEN IN BRENNSTOFFZELLEN
DER NATURWISSENSCHAFTLICHEN FAKULTAET DER
FRIEDRICH-ALEXANDER-UNIVERSITAET ERLANGEN-NUERNBERG
ZUR ERLANGUNG DES DOKTORGRADES DR. RER. NAT.
VORGELEGT VON
ARMIN NEITZEL
AUS NUERNBERG
CONTENTS
1.
INTRODUCTION..............................................................................................................................1
1.1 FUEL
CELLS.............................................................................................................................1
1.2 FUNDAMENTALS OF CATALYSIS AND THE MODEL
APPROACH..........................................................2
1.3 CERIA AS A CATALYST AND ITS DOPING WITH OTHER
METALS.........................................................4
2. EXPERIMENTAL
TECHNIQUES.........................................................................................................
6
2.1 SYNCHROTRON RADIATION PHOTOELECTRON SPECTROSCOPY
(SRPES)............................................6
2.2 RESONANT PHOTOEMISSION SPECTROSCOPY
(RPES).................................................................9
3. EXPERIMENTAL
SETUP.................................................................................................................12
SRPES MACHINE SETUP AT THE MATERIALS SCIENCE BEAMLINE AT ELETTRA IN
TRIESTE....................12
4. ATOMICALLY DISPERSED (NOBLE) METALS IN M-CEC
2
MIXED OXIDES
............................................
13
4.1 MAXIMUM NOBLE METAL EFFICIENCY IN CATALYTIC MATERIALS: ATOMICALLY
DISPERSED SURFACE
PLATINUM[PL].............................................................................................................................14
4.2 SURFACE SITES ON PT-CEC
2
MIXED OXIDE CATALYSTS PROBED BY CO ADSORPTION: A
SYNCHROTRON RADIATION PHOTOELECTRON SPECTROSCOPY STUDY[P2]
..............................................
17
4.3 REACTIVITY OF ATOMICALLY DISPERSED PT2+ SPECIES TOWARDS H
2
: MODEL PT-CE02 FUEL CELL
CATALYST[P3]..............................................................................................................................20
4.4 REACTIVITY OF PT2+ SPECIES IN MODEL PT-CE02 FUEL CELL CATALYSTS UPON
REACTION WITH
METHANOL[P4].............................................................................................................................22
4.5 ATOMICALLY DISPERSED PD, NI AND PT IN CERIA-BASED CATALYSTS: THE
PRINCIPAL DIFFERENCES
IN STABILITY AND
REACTIVITY[P5]..................................................................................
25
5. CHARACTERIZATION OF CERIA SUPPORTED PT-SN BIMETALLIC
NANOALLOYS.........................................27
5.1 HYDROGEN ACTIVATION ON PT-SN NANOALLOYS SUPPORTED ON MIXED SN-CE
OXIDE FILMS[P6-*... 28
5.2 ATOMIC ORDERING AND SN SEGREGATION IN PT-SN NANOALLOYS SUPPORTED ON
CEC
2
THIN
FILMS[P7]...................................................................................................................................31
6.
SUMMARY................................................................................................................................33
7.
ZUSAMMENFASSUNG.................................................................................................................
36
8.
ACKNOWLEDGEMENTS...............................................................................................................
39
9.
REFERENCES..............................................................................................................................41
10. LIST OF
ABBREVIATIONS............................................................................................................
45
11. APPENDIX: PAPER 1 - PAPER 7 AND ADDITIONAL
PUBLICATIONS..................................................48
III
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| indexdate | 2024-07-10T07:33:07Z |
| institution | BVB |
| language | German English |
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| physical | 163 Seiten in getrennter Zählung Illustrationen, Diagramme |
| publishDate | 2016 |
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| spelling | Neitzel, Armin Verfasser aut Model studies of ceria-based catalysts for fuel cell applications = Modelluntersuchungen von Ceroxid-haltigen Katalysatoren für Anwendungen in Brennstoffzellen vorgelegt von Armin Neitzel aus Nürnberg Modelluntersuchungen von Ceroxid-haltigen Katalysatoren für Anwendungen in Brennstoffzellen Erlangen ; Nürnberg 2016 163 Seiten in getrennter Zählung Illustrationen, Diagramme txt rdacontent n rdamedia nc rdacarrier Enthalten mehrere Sonderdrucke Dissertation Friedrich-Alexander-Universität Erlangen-Nürnberg 2016 Katalysator (DE-588)4029919-3 gnd rswk-swf Cerdioxid (DE-588)4336485-8 gnd rswk-swf Brennstoffzelle (DE-588)4008195-3 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Cerdioxid (DE-588)4336485-8 s Katalysator (DE-588)4029919-3 s Brennstoffzelle (DE-588)4008195-3 s DE-604 DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=029121763&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Neitzel, Armin Model studies of ceria-based catalysts for fuel cell applications = Modelluntersuchungen von Ceroxid-haltigen Katalysatoren für Anwendungen in Brennstoffzellen Katalysator (DE-588)4029919-3 gnd Cerdioxid (DE-588)4336485-8 gnd Brennstoffzelle (DE-588)4008195-3 gnd |
| subject_GND | (DE-588)4029919-3 (DE-588)4336485-8 (DE-588)4008195-3 (DE-588)4113937-9 |
| title | Model studies of ceria-based catalysts for fuel cell applications = Modelluntersuchungen von Ceroxid-haltigen Katalysatoren für Anwendungen in Brennstoffzellen |
| title_alt | Modelluntersuchungen von Ceroxid-haltigen Katalysatoren für Anwendungen in Brennstoffzellen |
| title_auth | Model studies of ceria-based catalysts for fuel cell applications = Modelluntersuchungen von Ceroxid-haltigen Katalysatoren für Anwendungen in Brennstoffzellen |
| title_exact_search | Model studies of ceria-based catalysts for fuel cell applications = Modelluntersuchungen von Ceroxid-haltigen Katalysatoren für Anwendungen in Brennstoffzellen |
| title_full | Model studies of ceria-based catalysts for fuel cell applications = Modelluntersuchungen von Ceroxid-haltigen Katalysatoren für Anwendungen in Brennstoffzellen vorgelegt von Armin Neitzel aus Nürnberg |
| title_fullStr | Model studies of ceria-based catalysts for fuel cell applications = Modelluntersuchungen von Ceroxid-haltigen Katalysatoren für Anwendungen in Brennstoffzellen vorgelegt von Armin Neitzel aus Nürnberg |
| title_full_unstemmed | Model studies of ceria-based catalysts for fuel cell applications = Modelluntersuchungen von Ceroxid-haltigen Katalysatoren für Anwendungen in Brennstoffzellen vorgelegt von Armin Neitzel aus Nürnberg |
| title_short | Model studies of ceria-based catalysts for fuel cell applications |
| title_sort | model studies of ceria based catalysts for fuel cell applications modelluntersuchungen von ceroxid haltigen katalysatoren fur anwendungen in brennstoffzellen |
| title_sub | = Modelluntersuchungen von Ceroxid-haltigen Katalysatoren für Anwendungen in Brennstoffzellen |
| topic | Katalysator (DE-588)4029919-3 gnd Cerdioxid (DE-588)4336485-8 gnd Brennstoffzelle (DE-588)4008195-3 gnd |
| topic_facet | Katalysator Cerdioxid Brennstoffzelle Hochschulschrift |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=029121763&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
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