Concepts of modern catalysis and kinetics:
Saved in:
| Main Authors: | , |
|---|---|
| Format: | Book |
| Language: | English |
| Published: |
Weinheim
Wiley-VCH
[2017]
|
| Edition: | Third, completely revised and enlarged edition |
| Subjects: | |
| Online Access: | http://www.wiley-vch.de/publish/dt/books/ISBN978-3-527-33268-7/ Inhaltsverzeichnis |
| Physical Description: | XVIII, 505 Seiten Illustrationen, Diagramme |
| ISBN: | 9783527332687 |
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MARC
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| 245 | 1 | 0 | |a Concepts of modern catalysis and kinetics |c I. Chorkendorff and J.W. Niemantsverdriet |
| 250 | |a Third, completely revised and enlarged edition | ||
| 264 | 1 | |a Weinheim |b Wiley-VCH |c [2017] | |
| 264 | 4 | |c © 2017 | |
| 300 | |a XVIII, 505 Seiten |b Illustrationen, Diagramme | ||
| 336 | |b txt |2 rdacontent | ||
| 337 | |b n |2 rdamedia | ||
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| 653 | |a Chemical Engineering | ||
| 653 | |a Chemie | ||
| 653 | |a Chemische Verfahrenstechnik | ||
| 653 | |a Chemistry | ||
| 653 | |a Industrial Chemistry | ||
| 653 | |a Katalyse | ||
| 653 | |a Kinetik | ||
| 653 | |a Methods - Synthesis & Techniques | ||
| 653 | |a Organische Chemie / Methoden, Synthesen, Verfahren | ||
| 653 | |a Physical Chemistry | ||
| 653 | |a Physikalische Chemie | ||
| 653 | |a Technische Chemie | ||
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Record in the Search Index
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| adam_text |
CONTENTS
PREFACE XIII
LIST OF ACRONYMS XVII
1 INTRODUCTION TO CATALYSIS 1
1.1 WHAT IS CATALYSIS? 2
1.2 CATALYSTS CAN BE ATOMS, MOLECULES, ENZYMES, AND SOLID SURFACES 4
1.2.1 HOMOGENEOUS CATALYSIS 5
1.2.2 BIOCATALYSIS 5
1.2.3 HETEROGENEOUS CATALYSIS 6
1.3 WHY IS CATALYSIS IMPORTANT? 9
1.3.1 CATALYSIS AND GREEN CHEMISTRY 9
1.3.2 ATOM EFFICIENCY, E FACTORS, AND ENVIRONMENTAL FRIENDLINESS 10
1.3.3 THE CHEMICAL INDUSTRY 11
1.4 CATALYSIS AS A MULTIDISCIPLINARY SCIENCE 16
1.4.1 THE MANY LENGTH SCALES OF A "CATALYST" 16
1.4.2 TIME SCALES IN CATALYSIS 17
1.5 THE SCOPE OF THIS BOOK 18
1.6 APPENDIX: CATALYSIS IN JOURNALS 18
REFERENCES 22
2 KINETICS 23
2.1 INTRODUCTION 23
2.2 THE RATE EQUATION AND POWER RATE LAWS 25
2.3 REACTIONS AND THERMODYNAMIC EQUILIBRIUM 28
2.3.1 EXAMPLE OF CHEMICAL EQUILIBRIUM: THE AMMONIA SYNTHESIS 31
2.3.2 CHEMICAL EQUILIBRIUM FOR A NONIDEAL GAS 33
2.4 THE TEMPERATURE DEPENDENCE OF THE RATE 35
2.5 INTEGRATED RATE EQUATIONS: TIME DEPENDENCE OF CONCENTRATIONS
IN REACTIONS OF DIFFERENT ORDERS 38
2.6 COUPLED REACTIONS IN FLOW REACTORS: THE STEADY STATE
APPROXIMATION 41
2.7 COUPLED REACTIONS IN BATCH REACTORS 45
2.8 CATALYTIC REACTIONS 48
2.8.1 THE MEAN-FIELD APPROXIMATION 52
2.9 LANGMUIR ADSORPTION ISOTHERMS 53
2.9.1 ASSOCIATIVE ADSORPTION 53
2.9.2 DISSOCIATIVE ADSORPTION 54
2.9.3 COMPETITIVE ADSORPTION 55
2.10 REACTION MECHANISMS 55
2.10.1 LANGMUIR-HINSHELWOOD OR ELEY-RIDEAL MECHANISMS 56
2.10.2 LANGMUIR-HINSHELWOOD KINETICS 56
2.10.3 THE COMPLETE SOLUTION 57
2.10.4 THE STEADY STATE APPROXIMATION 58
2.10.5 THE QUASI-EQUILIBRIUM APPROXIMATION 59
2.10.6 STEPS WITH SIMILAR RATES 60
2.10.7 IRREVERSIBLE STEP APPROXIMATION 61
2.10.8 THE MARI APPROXIMATION 61
2.10.9 THE NEARLY EMPTY SURFACE 62
2.10.10 THE REACTION ORDER 63
2.10.11 THE APPARENT ACTIVATION ENERGY 63
2.11 ENTROPY, ENTROPY PRODUCTION, AUTO CATALYSIS, AND OSCILLATING
REACTIONS 67
2.12 KINETICS OF ENZYME-CATALYZED REACTIONS 73
REFERENCES 77
3 REACTION RATE THEORY 79
3.1 INTRODUCTION 79
3.2 THE BOLTZMANN DISTRIBUTION AND THE PARTITION FUNCTION
80
3.3 PARTITION FUNCTIONS OF ATOMS AND MOLECULES 83
3.3.1 THE BOLTZMANN DISTRIBUTION 83
3.3.2 MAXWELL-BOLTZMANN DISTRIBUTION OF VELOCITIES 86
3.3.3 TOTAL PARTITION FUNCTION OF A SYSTEM 87
3.4 MOLECULES IN EQUILIBRIUM 93
3.5 COLLISION THEORY 7M
3.5.1 REACTION PROBABILITY 104
3.5.2 FUNDAMENTAL OBJECTION AGAINST COLLISION THEORY 105
3.6 ACTIVATION OF REACTING MOLECULES BY COLLISIONS:
THE LINDEMANN THEORY 106
3.7 TRANSITION STATE THEORY 107
3.8 TRANSITION STATE THEORY OF SURFACE REACTIONS 113
3.8.1 ADSORPTION OF ATOMS 113
3.8.2 ADSORPTION OF MOLECULES 118
3.8.3 REACTION BETWEEN ADSORBATES 121
3.8.4 DESORPTION OF MOLECULES 123
3.9 SUMMARY 124
REFERENCES 127
4 CATALYST CHARACTERIZATION 729
4.1 INTRODUCTION 129
4.2 X-RAY DIFFRACTION (XRD) 731
4.3 X-RAY PHOTOELECTRON SPECTROSCOPY (XPS) 134
4.4 X-RAY ABSORPTION SPECTROSCOPY (EXAFS AND XANES) 139
4.4.1 EXTENDED X-RAY ABSORPTION FINE STRUCTURE (EXAFS) 139
4.4.2 X-RAY ABSORPTION NEAR-EDGE SPECTROSCOPY (XANES) 143
4.5 ELECTRON MICROSCOPY 744
4.6 MOESSBAUER SPECTROSCOPY 148
4.7 ION SPECTROSCOPY: SIMS, LEIS, RBS 757
4.8 TEMPERATURE-PROGRAMMED REDUCTION, OXIDATION,
AND SULFIDATION 155
4.9 INFRARED SPECTROSCOPY 158
4.10 SURFACE SCIENCE TECHNIQUES 160
4.10.1 LOW ELECTRON ENERGY DIFFRACTION (FEED) 767
4.10.2 SCANNING PROBE MICROSCOPY 164
4.11 CONCLUDING REMARKS 769
REFERENCES 7 70
5 SOLID CATALYSTS 173
5.1 REQUIREMENTS OF A SUCCESSFUL CATALYST 773
5.2 THE STRUCTURE OF METALS, OXIDES, AND SULFIDES AND THEIR SURFACES 175
5.2.1 METAL STRUCTURES 175
5.2.2 SURFACE CRYSTALLOGRAPHY OF METALS 7 76
5.2.3 OXIDES AND SULFIDES 782
5.2.4 SURFACE FREE ENERGY 185
5.3 CHARACTERISTICS OF SMALL PARTICLES AND POROUS MATERIAL 187
5.3.1 THE WULFF CONSTRUCTION 187
5.3.2 THE PORE SYSTEM 790
5.3.3 THE SURFACE AREA 797
5.4 CATALYST SUPPORTS 797
5.4.1 SILICA 797
5.4.2 ALUMINA 799
5.4.3 CARBON 207
5.4.4 SHAPING OF CATALYST SUPPORTS 207
5.5 PREPARATION OF SUPPORTED CATALYSTS 203
5.5.1 COPRECIPITATION 203
5.5.2 IMPREGNATION, ADSORPTION, AND ION EXCHANGE 203
5.5.3 DEPOSITION PRECIPITATION 205
5.6 UNSUPPORTED CATALYSTS 206
5.7 ZEOLITES 206
5.7.1 STRUCTURE OF A ZEOLITE 207
5.7.2 COMPENSATING CATIONS AND ACIDITY 208
5.7.3 APPLICATIONS OF ZEOLITES 209
5.8 CATALYST TESTING 270
5.8.1 TEN COMMANDMENTS FOR TESTING CATALYSTS 211
5.8.2 ACTIVITY MEASUREMENTS 213
REFERENCES 223
6 SURFACE REACTIVITY 225
6.1 INTRODUCTION 225
6.2 PHYSISORPTION 226
6.2.1 THE VAN DER WAALS INTERACTION 226
6.2.2 INCLUDING THE REPULSIVE PART 227
6.3 CHEMICAL BONDING 228
6.3.1 BONDING IN MOLECULES 229
6.3.2 THE SOLID SURFACE 233
6.4 CHEMISORPTION 246
6.4.1 THE NEWNS-ANDERSON MODEL 246
6.4.2 SUMMARY OF THE NEWNS-ANDERSON APPROXIMATION IN QUALITATIVE
TERMS 252
6.4.3 ELECTROSTATIC EFFECTS IN ATOMIC ADSORBATES ON JELLIUM 254
6.5 IMPORTANT TRENDS IN SURFACE REACTIVITY 256
6.5.1 TREND IN ATOMIC CHEMISORPTION ENERGIES 257
6.5.2 TRENDS IN MOLECULAR CHEMISORPTION 267
6.5.3 TRENDS IN SURFACE REACTIVITY 265
6.5.4 UNIVERSALITY IN HETEROGENEOUS CATALYSIS 274
6.5.5 SCALING RELATIONS 276
6.5.6 APPENDIX: DENSITY FUNCTIONAL THEORY (DFT) 278
REFERENCES 280
7 KINETICS OF REACTIONS ON SURFACES 283
7.1 ELEMENTARY SURFACE REACTIONS 283
7.1.1 ADSORPTION AND STICKING 283
7.1.2 DESORPTION 289
7.1.3 LATERAL INTERACTIONS IN SURFACE REACTIONS 295
7.1.4 DISSOCIATION REACTIONS ON SURFACES 297
7.1.5 INTERMEDIATES IN SURFACE REACTIONS 301
7.1.6 ASSOCIATION REACTIONS 301
7.2 KINETIC PARAMETERS FROM FITTING LANGMUIR-HINSHELWOOD MODELS 304
7.3 MICROKINETIC MODELING 306
7.3.1 REACTION SCHEME AND RATE EXPRESSIONS
307
7.3.2 ACTIVATION ENERGY AND REACTION ORDERS 310
7.3.3 AMMONIA SYNTHESIS CATALYST UNDER WORKING CONDITIONS 373
REFERENCES 315
8 CATALYSIS IN PRACTICE: SYNTHESIS GAS AND HYDROGEN 379
8.1 INTRODUCTION 379
8.2 SYNTHESIS GAS AND HYDROGEN 379
8.2.1 STEAM REFORMING: BASIC CONCEPTS OF THE PROCESS 327
8.2.2 MECHANISTIC DETAIL OF STEAM REFORMING 323
8.2.3 CHALLENGES IN THE STEAM REFORMING PROCESS 326
8.2.4 THE SPARG PROCESS: SELECTIVE POISONING BY SULFUR 328
8.2.5 GOLD-NICKEL ALLOY CATALYST FOR STEAM REFORMING 329
8.2.6 DIRECT USES OF METHANE 330
8.3 REACTION OF SYNTHESIS GAS 332
8.3.1 METHANOL SYNTHESIS 332
8.3.2 FISCHER-TROPSCH PROCESS 343
8.4 WATER-GAS SHIFT REACTION 351
8.5 SYNTHESIS OF AMMONIA 353
8.5.1 HISTORY OF AMMONIA SYNTHESIS 353
8.5.2 AMMONIA SYNTHESIS PLANT 355
8.5.3 OPERATING THE REACTOR 356
8.5.4 SCIENTIFIC RATIONALE FOR IMPROVING CATALYSTS 359
8.6 PROMOTERS AND INHIBITORS 361
8.7 THE "HYDROGEN SOCIETY* 364
8.7.1 THE NEED FOR SUSTAINABLE ENERGY 364
8.7.2 SUSTAINABLE ENERGY SOURCES 366
8.7.3 ENERGY STORAGE 368
8.7.4 HYDROGEN FUEL CELLS 377
REFERENCES 385
9 OIL REFINING AND PETROCHEMISTRY 391
9.1 CRUDE OIL 391
9.2 HYDROTREATING 394
9.2.1 HETEROATOMS AND UNDESIRED COMPOUNDS 395
9.2.2 HYDROTREATING CATALYSTS 397
9.2.3 HYDRODESULFURIZATION REACTION MECHANISMS 399
9.3 GASOLINE PRODUCTION 402
9.3.1 FLUIDIZED CATALYTIC CRACKING 404
9.3.2 REFORMING AND BIFUNCTIONAL CATALYSIS 406
9.3.3 ALKYLATION 410
9.4 PETROCHEMISTRY: REACTIONS OF SMALL OLEFINS 412
9.4.1 ETHYLENE EPOXIDATION 412
9.4.2 PARTIAL OXIDATION AND AMMOXIDATION OF PROPYLENE 413
9.4.3 POLYMERIZATION CATALYSIS 415
REFERENCES 418
10 ENVIRONMENTAL CATALYSIS 421
10.1 INTRODUCTION 421
10.2 AIR POLLUTION BY AUTOMOTIVE EXHAUST 422
10.2.1 THE THREE-WAY CATALYST 423
10.2.2 CATALYTIC REACTIONS IN THE THREE-WAY CATALYST:
MECHANISM AND KINETICS 429
10.2.3 CONCLUDING REMARKS ON AUTOMOTIVE CATALYSTS 436
10.3 AIR POLLUTION BY LARGE STATIONARY SOURCES 437
10.3.1 SELECTIVE CATALYTIC REDUCTION: THE SCR PROCESS 437
10.3.2 THE SCR PROCESS FOR MOBILE UNITS 443
REFERENCES 444
APPENDIX 447
QUESTIONS AND EXERCISES 449
INDEX 497 |
| any_adam_object | 1 |
| author | Chorkendorff, Ib 1955- Niemantsverdriet, Johannes W. 1951- |
| author_GND | (DE-588)173347088 (DE-588)122259742 |
| author_facet | Chorkendorff, Ib 1955- Niemantsverdriet, Johannes W. 1951- |
| author_role | aut aut |
| author_sort | Chorkendorff, Ib 1955- |
| author_variant | i c ic j w n jw jwn |
| building | Verbundindex |
| bvnumber | BV043630438 |
| classification_rvk | VE 7040 |
| ctrlnum | (OCoLC)1004312407 (DE-599)DNB1099098424 |
| dewey-full | 540 |
| dewey-hundreds | 500 - Natural sciences and mathematics |
| dewey-ones | 540 - Chemistry and allied sciences |
| dewey-raw | 540 |
| dewey-search | 540 |
| dewey-sort | 3540 |
| dewey-tens | 540 - Chemistry and allied sciences |
| discipline | Chemie / Pharmazie |
| edition | Third, completely revised and enlarged edition |
| format | Book |
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| id | DE-604.BV043630438 |
| illustrated | Illustrated |
| indexdate | 2025-02-06T13:01:34Z |
| institution | BVB |
| institution_GND | (DE-588)16179388-5 |
| isbn | 9783527332687 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-029044485 |
| oclc_num | 1004312407 |
| open_access_boolean | |
| owner | DE-703 DE-29T DE-11 DE-20 DE-83 DE-634 DE-19 DE-BY-UBM |
| owner_facet | DE-703 DE-29T DE-11 DE-20 DE-83 DE-634 DE-19 DE-BY-UBM |
| physical | XVIII, 505 Seiten Illustrationen, Diagramme |
| publishDate | 2017 |
| publishDateSearch | 2017 |
| publishDateSort | 2017 |
| publisher | Wiley-VCH |
| record_format | marc |
| spelling | Chorkendorff, Ib 1955- Verfasser (DE-588)173347088 aut Concepts of modern catalysis and kinetics I. Chorkendorff and J.W. Niemantsverdriet Third, completely revised and enlarged edition Weinheim Wiley-VCH [2017] © 2017 XVIII, 505 Seiten Illustrationen, Diagramme txt rdacontent n rdamedia nc rdacarrier Enzymes Catalysis Environmental chemistry Industrial applications Reaktionskinetik (DE-588)4048655-2 gnd rswk-swf Heterogene Katalyse (DE-588)4123377-3 gnd rswk-swf Chemical Engineering Chemie Chemische Verfahrenstechnik Chemistry Industrial Chemistry Katalyse Kinetik Methods - Synthesis & Techniques Organische Chemie / Methoden, Synthesen, Verfahren Physical Chemistry Physikalische Chemie Technische Chemie Technische u. Industrielle Chemie Heterogene Katalyse (DE-588)4123377-3 s Reaktionskinetik (DE-588)4048655-2 s DE-604 Niemantsverdriet, Johannes W. 1951- Verfasser (DE-588)122259742 aut Wiley-VCH (DE-588)16179388-5 pbl Erscheint auch als Online-Ausgabe, ePDF 978-3-527-69128-9 Erscheint auch als Online-Ausgabe, ePub 978-3-527-69130-2 Erscheint auch als Online-Ausgabe, Mobi 978-3-527-69129-6 http://www.wiley-vch.de/publish/dt/books/ISBN978-3-527-33268-7/ Verlag DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=029044485&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Chorkendorff, Ib 1955- Niemantsverdriet, Johannes W. 1951- Concepts of modern catalysis and kinetics Enzymes Catalysis Environmental chemistry Industrial applications Reaktionskinetik (DE-588)4048655-2 gnd Heterogene Katalyse (DE-588)4123377-3 gnd |
| subject_GND | (DE-588)4048655-2 (DE-588)4123377-3 |
| title | Concepts of modern catalysis and kinetics |
| title_auth | Concepts of modern catalysis and kinetics |
| title_exact_search | Concepts of modern catalysis and kinetics |
| title_full | Concepts of modern catalysis and kinetics I. Chorkendorff and J.W. Niemantsverdriet |
| title_fullStr | Concepts of modern catalysis and kinetics I. Chorkendorff and J.W. Niemantsverdriet |
| title_full_unstemmed | Concepts of modern catalysis and kinetics I. Chorkendorff and J.W. Niemantsverdriet |
| title_short | Concepts of modern catalysis and kinetics |
| title_sort | concepts of modern catalysis and kinetics |
| topic | Enzymes Catalysis Environmental chemistry Industrial applications Reaktionskinetik (DE-588)4048655-2 gnd Heterogene Katalyse (DE-588)4123377-3 gnd |
| topic_facet | Enzymes Catalysis Environmental chemistry Industrial applications Reaktionskinetik Heterogene Katalyse |
| url | http://www.wiley-vch.de/publish/dt/books/ISBN978-3-527-33268-7/ http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=029044485&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
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