Photocatalysis: fundamentals and perspectives
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| Other Authors: | , , , , |
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| Format: | Book |
| Language: | English |
| Published: |
Cambridge
Royal Society of Chemistry
[2016]
|
| Series: | RSC energy and environment series
no. 14 |
| Subjects: | |
| Online Access: | Inhaltsverzeichnis Klappentext |
| Physical Description: | xvi, 436 Seiten Illustrationen, Diagramme (teilweise farbig) |
| ISBN: | 9781782620419 9781782627142 |
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| adam_text | Contents
Part 1: Fundamental Aspects of Photocatalysis
Chapter 1 Photoelectrochemistry: From Basic Principles to
Photocatalysis 3
Laurence M. Peter
1.1 Introduction 3
1.2 A Brief Summary of Semiconductor Physics 4
1.3 Conventional Semiconductor Photoelectrodes 6
1.3.1 Potential and Charge Distribution Across the
Semiconductor-Inert Electrolyte Junction 6
1.3.2 The Semiconductor-Redox Electrolyte
Junction 9
1.3.3 The Semiconductor-Electrolyte Junction
Under Illumination 13
1.3.4 Quasi-Fermi Levels (QFLs) 15
1.4 Nanostructured Semiconductor Electrodes and
Colloidal Particles in the Dark 17
1.4.1 Band Bending in Nanostructures 17
1.4.2 Determination of Quasi-Fermi Level
Positions in Nanoparticie Suspensions 19
1.5 Surface States and Fermi Level Pinning 20
1.6 Surface Recombination 22
1.7 Charge Compensation and Charge Trapping in
Mesoporous Electrodes 25
1.8 Conclusions 25
References 26
RSC Energy and Environment Series No. 14
Photocatalysis: Fundamentals and Perspectives
Edited by Jenny Schneider, Detlef Bahnemann, Jinhua Ye, Gianluca Li Puma,
and Dionysios D. Dionysiou
© The Royal Society of Chemistry 2016
Published by the Royal Society of Chemistry, www.rsc.org
ix
X
Contents
Chapter 2 Understanding the Chemistry of Photocatalytic
Processes 29
Amer Hakki, Jenny Schneider, and Detlef Bahnemann
2.1 Thermodynamic Constraints for Photocatalytic
Processes 29
2.2 Single and Multiple Electron Transfer Reactions 35
2.3 Role of the Substrate Structure in the
Photocatalytic Process 37
2.4 Importance of the Reduction Pathway in
Photocatalytic Oxidation Reactions 40
2.5 Importance of the Oxidation Pathway in
Photocatalytic Reduction Reactions 45
2.6 Conclusions 48
References 48
Chapter 3 Current Issues Concerning the Mechanism of Pristine
Ti02 Photocatalysis and the Effects on Photonic Crystal
Nanostructures 51
Cecilia B. Mendive, Mariano Curti, and Detlef Bahnemann
3.1 Photocatalysis and Sustainability 51
3.2 The Basic Principle of Ti02 Photocatalysis 53
3.3 Current Mechanisms 57
3.3.1 Antenna Mechanism 57
3.3.2 Deaggregation of Particle Agglomerates 59
3.3.3 Band-Gap Coupling: Z-Scheme and
Heterojunctions 61
3.3.4 Wettability 64
3.3.5 Photo-Thermal Desorption of Water 69
3.4 Ti02 Photonic Crystal Nanostructures 70
3.5 Concluding Remarks 74
References 76
Chapter 4 Specificity in Photocatalysis 80
Yaron Paz
4.1 Introduction 80
4.2 Mass Transport to the Photocatalyst and Adsorption 82
4.2.1 Complexation in the Fluid Phase 83
4.2.2 Surface Charge Effects 84
4.2.3 Overcoating the Photocatalyst 85
4.2.4 Adsorb Shuttle 86
4.2.5 Doping 93
4.2.6 Selection by Size 94
4.2.7 Molecular Imprinting 95
Contents
xi
4.3 The Redox Reaction 99
4.3.1 Recombination Versus Interfacial Electron
Transfer 99
4.3.2 Doping as a Means to Control Oxidation
Versus Reduction 99
4.3.3 Shifting the Location of Energy Bands 100
4.3.4 Co-Existing Compounds as a Means to Alter
Specificity 100
4.3.5 Utilizing Specific Adsorbate-Adsorbent
Interactions 101
4.3.6 Surface Derivatization 101
4.3.7 Sensitization as a Means to Induce Specificity 102
4.4 Desorption of Products 103
4.4.1 Preferential Desorption from Imprinted
Photocatalysts 103
4.4.2 Effect of Solvents on the Desorption of
Intermediate Products 104
4.4.3 Surface Derivatization for Controlling the
Distribution of Products 105
4.5 Summary and Perspectives 106
References 106
Chapter 5 Photoexcitation in Pure and Modified Semiconductor
Photocatalysts 110
Gonu Kim, Yiseul Park, Gun-hee Moon, and Choi
5.1 Band-Gap Excitation of Semiconductor
Photocatalysts 110
5.2 Photoexcitation of Impurity-Doped
Semiconductors 112
5.3 Photoexcitation of Coupled Semiconductors 115
5.4 Dye-Sensitized Semiconductors and Dye
Discoloration 117
5.5 LMCT-Sensitized Semiconductors 119
5.6 Photoexcitation at Metal/Semiconductor Interfaces 121
5.7 Conclusions 124
Acknowledgements 124
References 124
Chapter 6 New Concepts in Photocatalysis 129
Ying Wu and Michael Wark
6.1 Introduction 129
6.2 Graphene 130
6.3 Carbon Nitride 134
6.4 Z-Scheme Photocatalytic Systems 139
xii
Contents
6.4.1 Z-Scheme Systems with Redox Mediator 140
6.4.2 Z-Scheme Systems Without Redox Mediator 142
6.5 Plasmonic Photocatalysis 147
6.6 New Applications of Photocatalysis 153
6.7 Perspectives 156
References 157
Part 2: Primary Processes in Photocatalysis
Chapter 7 Kinetic Processes in the Presence of Photogenerated
Charge Carriers 165
Yoshio Nosaka and Atsuko Y. Nosaka
7.1 Outline of the Processes in Photocatalysis 165
7.1.1 Environmental Clean-up or Solar
Hydrogen Production 165
7.1.2 Energy Levels of Ti02 and Water 166
7.1.3 Adsorption of Water Molecules 167
7.2 Primary Processes of Photogenerated Charge Carriers 169
7.2.1 Trapping of Free Charge Carriers 169
7.2.2 Trapped Electrons and Reduction of 02 171
7.2.3 Trapped Holes and Oxidation of Alcohols 172
7.3 Kinetic Processes at Pure TiOz Photocatalysts 172
7.3.1 02 Production at Rutile Surfaces 172
7.3.2 OH Radical Formation over Rutile and
Anatase Photocatalysts 173
7.3.3 Kinetics of Methanol Oxidation 176
7.4 Modified Ti02 Photocatalysts for Visible
Light Response 178
7.4.1 Copper(n) deposited TiOz and W03 178
7.4.2 Iron(m)-deposited Ru-doped TiOz 179
7.4.3 Platinum Complex Sensitized Ti02 180
7.4.4 Gold-Nanoparticle Deposited Ti02 181
References 182
Chapter 8 Traps and Interfaces in Photocatalysis: Model Studies
on Ti02 Particle Systems 185
Thomas Berger and Oliver Diwald
8.1 Introduction 185
8.2 The Solid-Gas Interface: Trapping Sites and
Spectroscopic Manifestations 188
8.2.1 Trapped Electrons 188
8.2.2 Trapped Holes 192
8.2.3 Trapped Hydrogen 193
8.2.4 Trapped Charges and Optical Fingerprints 194
xiii
195
199
201
204
209
211
211
218
218
223
226
230
230
235
243
243
243
247
249
252
253
253
254
255
256
8.3 Slow Charge Trapping and Charge Carrier
Quantification at the Solid-Gas Interface
8.4 From Solid (Particle)-Gas to Solid (Particle)-Liquid
Interfaces: Changes on Different Size Scales
8.5 Microstructural Changes of Particle Ensembles
and Solid-Solid Interface Formation
8.6 Charge Separation and Trapping at the Solid-Liquid
Interface - Slow Processes
8.7 Summary and Outlook
Acknowledgements
References
Interplay Between Physical and Chemical Events in
Photoprocesses in Heterogeneous Systems
Alexei V Emeline, Vladimir K. Ryabchuk,
Vyacheslav N. Kuznetsov, and Nick Serpone
9.1 Introduction
9.2 Physical and Chemical Relaxation through
Surface-Active Centers
9.3 Photoinduced Defect Formation
9.4 Interconnection Between the Activity and
Selectivity of Photocatalysts
9.4.1 Activity of Photocatalysts
9.4.2 Selectivity of Photocatalysts
9.5 Concluding Remarks
Acknowledgements
References
Part 3: New Materials
New Materials: Outline
Jinhua Ye
References
New Materials for Degradation of Organics
Shuxin Ouyang and Hua Xu
11.1 Basic Characterizations by which to Judge
a New Material as Photocatalyst
11.1.1 Dark and Light Experiments
11.1.2 Wavelength-Dependence Test
11.1.3 Evidence for Catalytic Process
11.2 Typical New Materials for Photodegradation of
Organics
xiv
Contents
11.2.1 New-Generation Ti02-Based Materials 256
11.2.2 Photocatalysts Comprising d-Block Elements 261
11.2.3 Photocatalysts Containing p-Block Elements 265
11.2.4 Organic Photocatalysts 273
11.2.5 Composite and Heterojunction
Photocatalysts 275
11.3 Photodegradation Mechanism 281
11.3.1 Intrinsic Semiconductor-Based
Photocatalysis or Dye-Sensitized
Photocatalysis 286
11.3.2 Reactive Species Analysis 287
11.4 Summary and Prospects 289
References 289
Chapter 12 New Materials for Water Splitting 295
Kazuhiko Maeda
12.1 Introduction 295
12.1.1 Research Background 295
12.1.2 Basic Principles of Water Splitting on
a Semiconductor Particle 296
12.1.3 Development of Visible-Light-Responsive
Photocatalysts for Overall Water Splitting 299
12.1.4 Scope of This Chapter 301
12.2 Modified Oxynitrides for Efficient Water Splitting 301
12.2.1 Surface Modified Tantalum Oxynitrides with
Zr(iv) Species for Enhanced Hydrogen
Evolution 302
12.2.2 Oxynitrides Modified with Cobalt Oxide for
Highly Efficient Water Oxidation 306
12.3 Metal Oxide Based Photocatalysts for Overall
Water Splitting 307
12.3.1 Doped SrTi03 308
12.3.2 Dye-Sensitized Lamellar Niobate for
Z-Scheme Water Splitting 312
12.4 Summary and Outlook 314
References 315
Chapter 13 New Materials for C02 Photoreduction 318
YongZhou, WenguangTu, and Zhigang Zou
13.1 Introduction 318
13.2 Basic Principles of Photocatalytic Reduction of C02 319
13.3 Materials for C02 Photoreduction 322
13.3.1 Metal Oxides with d° and d10 Electronic
Configurations 322
13.3.2 Metal Sulfides and Phosphides 324
13.3.3 Other Materials 325
Contents
XV
13.4 Strategies for Designing Effective Photocatalytic
Materials 325
13.4.1 Surface Sites for Reactant Adsorption and
Chemical Reaction 326
13.4.2 Light Harvesting for Effectively Utilizing
Solar Energy 331
13.4.3 Charge Separation for Effectively Utilizing
Solar Energy 333
13.5 Conclusions and Perspectives 337
References 337
Part 4: Reactor and Reaction Engineering
Chapter 14 Fundamentals of Radiation Transport in Absorbing
Scattering Media 351
Orlando M. Alfano, Alberto E.
and Rafael van Grieken
14.1 Introduction 351
14.2 Definitions 352
14.2.1 Radiation Intensity 353
14.2.2 Incident Radiation 353
14.2.3 Local Volumetric Rate of Photon
Absorption (LVRPA) 354
14.2.4 Net Radiation Flux 354
14.2.5 Local Surface Rate of Photon Absorption
(LSRPA) 354
14.3 The Radiative Transport Equation (RTE) 355
14.4 Boundary Conditions for the RTE 357
14.4.1 Extended Source with Superficial
Emission (ESSE) 358
14.4.2 Extended Source with Voluminal
Emission (ESVE) 358
14.4.3 Solar Radiation 360
14.4.4 Chemical Actinometry 361
14.5 Solution Methods of the RTE 363
Acknowledgements 364
References 365
Chapter 15 Photocatalytic Reactor Design 367
Javier Marugan, Rafael van Grieken, Alberto E. Cassano,
and Orlando M. Alfano
15.1 Predictive Design of Photocatalytic Reactors 367
15.2 Optical Properties of Photocatalytic Suspensions
and Films 369
15.3 Radiation Field Inside the Reactor 373
xvi Contents
15.4 Photocatalytic Efficiencies 373
15.4.1 Quantum Yield and Quantum Efficiency 373
15.4.2 Photonic Yield and Photonic Efficiency 374
15.5 Kinetic Modeling 375
15.6 Mass Balance Equations 377
15.7 Case Study: Photocatalytic Oxidation of Cyanide
with Ti02/Si02 Materials 378
15.7.1 Experimental Determination of the
Optical Properties of the Materials 378
15.7.2 Estimation of the Quantum Efficiency 379
15.7.3 Development of a Suitable Intrinsic
Kinetic Model 382
15.7.4 Scaling-Up of the Process to a Larger
Photocatalytic Reactor 383
Acknowledgements 386
References 387
Chapter 16 Photocatalytic Reactor Modeling 388
Fiderman Machuca-Martinez,
José Colina-Mârquez, and Gianluca Li Puma
16.1 Introduction 388
16.2 Radiation Field Evaluation 390
16.3 Emission Model (Lamps) 390
16.4 Solar Emission Model 391
16.5 Photon Absorption-Scattering Model: Evaluation
of the Local Volumetric Rate of Photon
Absorption, LVRPA 393
16.5.1 Two-Flux and Six-Flux Absorption-
Scattering Models 394
16.6 Application of SFM in Flat-Plate Photoreactors 397
16.7 Application of SFM in Solar CPC and FPR Reactors 399
16.8 Photocatalytic Reaction Kinetics Model 401
16.9 Generalized Model 405
16.10 Thin-Film Slurry Photocatalytic Reactors 408
16.11 Kinetic Parameters Optimization 412
16.12 Application of Models to the Photocatalytic
Degradation of Organic Compounds in Water 414
16.12.1 DCA Solar Photodegradation 415
16.12.2 Phenol and 4-Chlorophenol Solar
Photodegradation 416
16.13 Photodegradation of Organic Mixtures 418
References 420
Subject Index
425
Combining the basic concepts of photocatalysis with the synthesis of
new catalysts, reactor and reaction engineering reaction engineering,
this book provides a comprehensive resource on the topic.
The book introduces the fundamental aspects of photocatalysis
including the role of surface chemistry and understanding the
chemistry of photocatalytic processes before exploring the theory
and experimental studies of charge carrier dynamics. Specific
chapters then cover new materials for the degradation of organics;
water splitting and C02 reduction; as well as reactor and reaction
engineering. Researchers new to this discipline can learn the first
principles, whilst experienced researchers can gain further information
about aspects in photocatalysis beyond their area of expertise.
Together with Photocatalysis: Applications, these volumes provide a
complete overview of photocatalysis.
|
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| id | DE-604.BV043499776 |
| illustrated | Illustrated |
| indexdate | 2024-07-10T07:27:21Z |
| institution | BVB |
| isbn | 9781782620419 9781782627142 |
| language | English |
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| series | RSC energy and environment series |
| series2 | RSC energy and environment series |
| spelling | Photocatalysis fundamentals and perspectives edited by Jenny Schneider, Detlef Bahnemann, Jinhua Ye, Gianluca Li Puma, Dionysios D Dionysiou Cambridge Royal Society of Chemistry [2016] © 2016 xvi, 436 Seiten Illustrationen, Diagramme (teilweise farbig) txt rdacontent n rdamedia nc rdacarrier RSC energy and environment series no. 14 Fotokatalyse (DE-588)4193873-2 gnd rswk-swf Fotokatalyse (DE-588)4193873-2 s DE-604 Schneider, Jenny (DE-588)1100701605 edt Bahnemann, Detlef 1953- (DE-588)171963172 edt Ye, Jinhua edt Li Puma, Gianluca edt Dionysiou, Dionysios D. (DE-588)1100723498 edt Erscheint auch als Online-Ausgabe, EPUB 978-1-78262-826-2 Erscheint auch als Online-Ausgabe, PDF 978-1-78262-233-8 RSC energy and environment series no. 14 (DE-604)BV036744686 14 Digitalisierung UB Bayreuth - ADAM Catalogue Enrichment application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=028916201&sequence=000003&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis Digitalisierung UB Bayreuth - ADAM Catalogue Enrichment application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=028916201&sequence=000004&line_number=0002&func_code=DB_RECORDS&service_type=MEDIA Klappentext |
| spellingShingle | Photocatalysis fundamentals and perspectives RSC energy and environment series Fotokatalyse (DE-588)4193873-2 gnd |
| subject_GND | (DE-588)4193873-2 |
| title | Photocatalysis fundamentals and perspectives |
| title_auth | Photocatalysis fundamentals and perspectives |
| title_exact_search | Photocatalysis fundamentals and perspectives |
| title_full | Photocatalysis fundamentals and perspectives edited by Jenny Schneider, Detlef Bahnemann, Jinhua Ye, Gianluca Li Puma, Dionysios D Dionysiou |
| title_fullStr | Photocatalysis fundamentals and perspectives edited by Jenny Schneider, Detlef Bahnemann, Jinhua Ye, Gianluca Li Puma, Dionysios D Dionysiou |
| title_full_unstemmed | Photocatalysis fundamentals and perspectives edited by Jenny Schneider, Detlef Bahnemann, Jinhua Ye, Gianluca Li Puma, Dionysios D Dionysiou |
| title_short | Photocatalysis |
| title_sort | photocatalysis fundamentals and perspectives |
| title_sub | fundamentals and perspectives |
| topic | Fotokatalyse (DE-588)4193873-2 gnd |
| topic_facet | Fotokatalyse |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=028916201&sequence=000003&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=028916201&sequence=000004&line_number=0002&func_code=DB_RECORDS&service_type=MEDIA |
| volume_link | (DE-604)BV036744686 |
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