Thermoelectric Bi 2 Te 3 Nanomaterials:
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| Other Authors: | |
|---|---|
| Format: | Book |
| Language: | English |
| Published: |
Weinheim
Wiley-VCH
2015
|
| Subjects: | |
| Online Access: | Inhaltstext Inhaltsverzeichnis |
| Physical Description: | XXIII, 290 S. Ill., graph. Darst. |
| ISBN: | 3527334890 9783527334896 9783527672608 |
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| 245 | 1 | 0 | |a Thermoelectric Bi 2 Te 3 Nanomaterials |c ed. by Oliver Eibl ... |
| 264 | 1 | |a Weinheim |b Wiley-VCH |c 2015 | |
| 300 | |a XXIII, 290 S. |b Ill., graph. Darst. | ||
| 336 | |b txt |2 rdacontent | ||
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CONTENTS
PREFACE
XIII
LIST OF CONTRIBUTORS
XVII
ACKNOWLEDGMENTS
XXIII
1 OLD AND NEW THINGS IN THERMOELECTRICITY 1
RUDOLF P. HUEBENER
1.1 THREE THERMOELECTRIC EFFECTS 2
1.1.1 SEEBECK EFFECT 2
1.1.2 PELTIER EFFECT 3
1.1.3 THOMSON EFFECT 3
1.2 SEMICONDUCTORS 4
1.3 MY ENTRY INTO THERMOELECTRICITY
6
1.4 PELTIER CASCADES 9
1.5 CHALLENGE OF MATERIALS SCIENCE 9
REFERENCES 10
PART I: SYNTHESIS OF NANOWIRES, THIN FILMS, AND NANOSTRUCTURED
BULK
11
2 ELECTRODEPOSITION OF BI
2
TE
3
-BASED THIN FILMS AND NANOWIRES
13
WILLIAM TOLLNER,
SVENJA BAFFLER, NICOLA
PERANIO, ECKHARD PIPPEL,
OLIVER EIBL,
AND KORNELIUS NIELSCH
2.1 INTRODUCTION 13
2.2 FUNDAMENTALS OF BI
2
TE
3
-BASED ELECTRODEPOSITION 14
2.3 ELECTRODEPOSITION OF BI
2
TE
3
THIN FILMS 16
2.4 ELECTRODEPOSITION OF THERMOELECTRIC NANOWIRES 21
2.4.1 ELECTRODEPOSITION OF BI
2
TE
3
NANOWIRES 21
2.4.2 TERNARY BI
2
TE
3
-BASED NANOWIRES 28
2.5 CONCLUSION 31
REFERENCES 31
HTTP://D-NB.INFO/105870284X
VI | CONTENTS
3 BI
2
TE
3
NANOWIRES BY ELECTRODEPOSITION IN POLYMERIC ETCHED ION TRACK
MEMBRANES: SYNTHESIS AND CHARACTERIZATION
33
OLIVER PICHT,
JANINA KRIEG,
AND MARIA EUGENIA TOIMIL-MOLARES
3.1 INTRODUCTION 33
3.2 SYNTHESIS OF BI
2
TE
3
NWS WITH CONTROLLED SIZE AND
CRYSTALLOGRAPHY 36
3.2.1 FABRICATION OF ETCHED ION-TRACK MEMBRANES 36
3.2.1.1 SWIFT HEAVY-ION IRRADIATION 36
3.2.1.2 CHEMICAL ETCHING 37
3.2.2 ELECTRODEPOSITION OF BI
2
TE
3
NWS 38
3.2.2.1 EXPERIMENTAL SETUP 38
3.2.2.2 ELECTRODEPOSITION OF BI
2
TE
3
AND CHOICE OF THE
ELECTROLYTE 40
3.2.2.3 CHRONOAMPEROMETRIC CURRENT-TIME CURVES 41
3.2.3 MORPHOLOGICAL AND CRYSTALLOGRAPHIC CHARACTERIZATION OF
BI
2
TE
3
NWS 42
3.2.3.1 NW ARRAYS 42
3.2.3.2 MORPHOLOGY OF INDIVIDUAL NANOWIRES AS A FUNCTION OF THE
DEPOSITION PARAMETERS 43
3.2.3.3 ADJUSTING THE NANOWIRE DIMENSIONS 44
3.2.3.4 INVESTIGATION OF THE NANOWIRE CRYSTALLINITY AND COMPOSITION
BY TEM 45
3.2.3.5 INVESTIGATION OF THE PREFERRED CRYSTALLOGRAPHIC ORIENTATION OF
WIRE ARRAYS BY X-RAY DIFFRACTION 49
3.3 CONCLUSIONS SO
REFERENCES SI
4 FABRICATION AND COMPREHENSIVE STRUCTURAL AND TRANSPORT PROPERTY
CHARACTERIZATION OF NANOALLOYED NANOSTRUCTURED V
2
VI
3
THIN FILM
MATERIALS
55
MARKUS WINKLER,
TORBEN DANKWORT, ULRICH SCHIIRMANN, XI LIU,
JAN D. KONIG, LORENZ KIENLE,
WOLFGANG BENSCH, HARALD BOTTNER, AND KILIAN
BARTHOLOME
4.1 SITUATION/STATE OF THE ART BEFORE THE START OF OUR COMBINED
RESEARCH PROJECT 55
4.2 MOTIVATION FOR RESEARCH ON V
2
VI
3
MULTILAYERED
STRUCTURES 56
4.2.1 BINARY THIN FILMS 58
4.2.2 RESULTS OBTAINED FOR SL STRUCTURES 62
4.2.3 RESULTS OBTAINED FROM A THEORETICAL ANALYSIS OF V
2
VI
3
BINARIES AND NANOSCALE SL STRUCTURES 66
CONTENTS | VII
4.3 CONCLUSION AND OUTLOOK 67
ACKNOWLEDGMENTS 69
REFERENCES 69
5 STRUCTURE AND TRANSPORT PROPERTIES OF BI
2
TE
3
FILMS
73
GUOYU WANG, LYNN ENDICOTT,
AND CTIRAD
UHER
5.1 INTRODUCTION 73
5.2 STRUCTURAL ASPECTS OF THE TETRADYMITE-TYPE LATTICE 75
5.3 MBE FILM DEPOSITION 76
5.4 STRUCTURAL CHARACTERIZATION OF BI
2
TE
3
FILMS 78
5.5 TRANSPORT PROPERTIES OF FILMS ON SAPPHIRE SUBSTRATES 85
5.6 CONCLUSION 95
ACKNOWLEDGMENT 95
REFERENCES 95
6 BULK-NANOSTRUCTURED BI
2
TE
3
-BASED MATERIALS: PROCESSING,
THERMOELECTRIC PROPERTIES, AND CHALLENGES 99
VICENTE PACHECO, HENRIK GORLITZ, NICOLA PERANIO,
ZAINUL AABDIN, AND OLIVER
EIBL
6.1 SUCCESS OF ZT ENHANCEMENT IN NANOSTRUCTURED BULK
MATERIALS 99
6.2 METHODOLOGY AT FRAUNHOFER IFAM-DD: PREVIOUS
RESEARCH 100
6.3 HIGH-ENERGY BALL MILLING TECHNOLOGY, SPS TECHNOLOGY, AND
THERMOELECTRIC CHARACTERIZATION 102
6.4 CONTROL OF CRYSTALLITE SIZE AND MASS DENSITY 103
6.4.1 OPTIMIZING BALL MILLING PARAMETERS 103
6.4.2 OPTIMIZING SPS PARAMETERS 105
6.5 NANOSTRUCTURE - TRANSPORT PROPERTIES - CORRELATIONS IN
SINTERED NANOMATERIALS 106
6.5.1 TRANSPORT PROPERTIES 106
6.5.2 NANOSTRUCTURE 108
6.5.3 CRYSTALLITE SIZE-LATTICE THERMAL CONDUCTIVITY
CORRELATION 110
6.5.4 COMPOSITION-ANTISITE DEFECT DENSITY-ELECTRIC TRANSPORT
CORRELATION 111
6.5.5 OXIDIZED SECONDARY PHASES - OXIDIZED MATRIX - ELECTRIC
TRANSPORT CORRELATION 112
6.6 SUMMARY AND STATE OF THE ART 113
VIII
| CONTENTS
6.7 OUTLOOK SECOND GENERATION SPS PREPARED
NANOMATERIALS 114
REFERENCES 115
PART II: STRUCTURE, EXCITATION, AND DYNAMICS
119
7 HIGH ENERGY X-RAY AND NEUTRON SCATTERING ON BI
2
TE
3
NANOWIRES,
NANOCOMPOSITES, AND BULK MATERIALS
121
BENEDIKT KLOBES, DIMITRIOS BESSAS,
AND RAPHAEL P. HERMANN
7.1 INTRODUCTION 121
7.2 REVIEW OF PUBLISHED HIGH-ENERGY X-RAY AND NEUTRON
SCATTERING STUDIES ON BI
2
TE
3
AND RELATED COMPOUNDS 122
7.3 ELEMENT SPECIFIC LATTICE DYNAMICS IN BULK BI
2
TE
3
AND
SB
2
TE
3
125
7.4 NANOSTRUCTURE AND PHONONS IN A BI
2
TE
3
NANOWIRE ARRAY 130
7.5 NANOCOMPOSITES AND SPEED OF SOUND 134
7.6 PERSPECTIVES OF HIGH-ENERGY X-RAY AND NEUTRON
SCATTERING 136
ACKNOWLEDGMENTS 136
REFERENCES 137
8 ADVANCED STRUCTURAL CHARACTERIZATION OF BI
2
TE
3
NANOMATERIALS
141
NICOLA PERANIO,
ZAINUL AABDIN, MICHAEL DURRSCHNABEL, AND OLIVER EIBL
8.1 FROM BULK TO NANOMATERIALS 141
8.2 SYNTHESIS OF NANOMATERIALS AND TRANSPORT
MEASUREMENTS 142
8.3 RELEVANCE OF ADVANCED MICROSCOPY AND SPECTROSCOPY FOR
BI
2
TE
3
NANOMATERIALS 143
8.4 NANOSTRUCTURE - PROPERTY RELATIONS IN BULK AND
NANOMATERIALS 147
8.4.1 CHEMICAL MODULATIONS AND STRUCTURAL DISORDER IN
COMMERCIAL BULK MATERIALS 147
8.4.2 NEAR STOICHIOMETRIC, SINGLE CRYSTALLINE NANOWIRES FOR
TRANSPORT IN THE BASAL PLANE 150
8.4.3 EPITAXIAL AND NANO-ALLOYED THIN FILMS WITH LOW CHARGE
CARRIER DENSITIES AND HIGH POWER FACTORS 152
8.4.4 HIGHLY DENSE, ULTRA-FINE NANOSTRUCTURED BULK WITH LOW
THERMAL CONDUCTIVITIES 153
8.5 SIMULATION OF ELECTRON TRANSPORT AND ELECTRON SCATTERING IN
BI
2
TE
3
-BASED MATERIALS 155
8.5.1 CALCULATION OF ELECTRONIC TRANSPORT COEFFICIENTS 156
CONTENTS
IIX
8.5.2 CALCULATION OF HIGH-ENERGY ELECTRON SCATTERING IN
BI
2
TE
3
-BASED MATERIALS 158
8.6 EXPERIMENTAL TECHNIQUES AND SIMULATION 161
REFERENCES 161
PART III:
THEORY AND MODELING
165
9 DENSITY-FUNCTIONAL THEORY STUDY OF POINT DEFECTS IN BI
2
TE
3
167
ADHAM HASHIBON AND CHRISTIAN ELSASSER
9.1 INTRODUCTION 167
9.2 THERMOELECTRIC PROPERTIES 168
9.3 THE LATTICE STRUCTURE OF BI
2
TE
3
173
9.4 POINT DEFECTS IN BI
2
TE
3
-RELATED MATERIALS 174
9.5 CONCENTRATION OF POINT DEFECTS 177
9.6 CALCULATION OF FORMATION ENERGIES FROM FIRST PRINCIPLES 178
9.7 RECENT DFT RESULTS FOR THE POINT DEFECT ENERGIES IN
BI
2
TE
3
180
9.8 SUMMARY AND OUTLOOK 183
ACKNOWLEDGMENTS 184
REFERENCES 184
10 AB INITIO DESCRIPTION OF THERMOELECTRIC PROPERTIES BASED ON THE
BOLTZMANN THEORY
187
NICKI F. HINSCHE, MARTIN HOLZER,
ARTHUR ERNST, INGRID MERTIG,
AND PETER ZAHN
10.1 INTRODUCTION 187
10.1.1 LOW-DIMENSIONAL THERMOELECTRICS 188
10.1.2 PHONON-GLASS ELECTRON-CRYSTAL 189
10.1.3 PHONON-BLOCKING AND ELECTRON-TRANSMITTING
SUPERLATTICES 191
10.2 TRANSPORT THEORY 193
10.2.1 LINEARIZED BOLTZMANN EQUATION AND RELAXATION TIME
APPROXIMATION 193
10.2.2 TRANSPORT COEFFICIENTS 194
10.3 RESULTS 197
10.3.1 INFLUENCE OF STRAIN 197
10.3.2 SUPERLATTICES 203
10.3.3 THERMAL CONDUCTIVITY - TOWARD THE FIGURE OF MERIT 206
10.3.4 LORENZ FUNCTION OF SUPERLATTICES 208
10.3.5 PHONONS 211
10.4 SUMMARY 213
REFERENCES 214
X CONTENTS
PART IV: TRANSPORT PROPERTIES MEASUREMENT TECHNIQUES
223
11 MEASURING TECHNIQUES FOR THERMAL CONDUCTIVITY AND THERMOELECTRIC
FIGURE OF MERIT OF V-VI COMPOUND THIN FILMS AND NANOWIRES
225
F. VOLKLEIN,
H. REITH,
A. MEIER,
AND M. SCHMITT
11.1 INTRODUCTION 225
11.2 METHODS FOR THE INVESTIGATION OF THE IN-PLANE THERMAL
CONDUCTIVITY OF THIN FILMS 227
11.2.1 STEADY-STATE JOULE HEATING METHOD FOR DETERMINING THE
THERMAL CONDUCTIVITY AND EMISSIVITY OF ELECTRICALLY
CONDUCTING FILMS
227
11.2.2 MICROFABRICATED X-CHIPS FOR MEASUREMENTS OF IN-PLANE
THERMAL CONDUCTIVITY 230
11.2.3 THE A-CHIPS FOR TRANSIENT MEASUREMENTS OF THE IN-PLANE
THERMAL CONDUCTIVITY AND THE SPECIFIC HEAT CAPACITY OF THIN
FILMS 235
11.3 STEADY-STATE MEASUREMENTS OF THE CROSS-PLANE THERMAL
CONDUCTIVITY OF THIN FILMS 236
11.4 INVESTIGATION OF CROSS-PLANE THERMAL CONDUCTIVITY OF
NANOWIRE ARRAYS 243
11.5 CHARACTERIZATION OF THERMAL CONDUCTIVITY AND THERMOELECTRIC
FIGURE OF MERIT OF SINGLE NANOWIRES 245
11.5.1 DESIGN OF THE Z-CHIP 245
11.5.2 ELECTRICAL CONDUCTIVITY MEASUREMENT 248
11.5.3 THERMOPOWER MEASUREMENTS 248
11.5.4 THERMAL CONDUCTIVITY MEASUREMENT 250
ACKNOWLEDGMENTS 251
REFERENCES 251
12 DEVELOPMENT OF A THERMOELECTRIC NANOWIRE CHARACTERIZATION PLATFORM
(TNCP) FOR
STRUCTURAL AND THERMOELECTRIC INVESTIGATION OF SINGLE
NANOWIRES
253
ZHI
WANG, S. HODA
MOOSAVI, MICHAEL KROENER,
AND PETER WOIAS
12.1 INTRODUCTION 253
12.2 TNCP INITIAL DESIGN 256
12.3 FIRST AND SECOND GENERATIONS OF TNCP 257
12.3.1 DESIGN, MODELING, AND SIMULATION 257
12.3.2 DESIGN IMPROVEMENTS AND NEW CHARACTERISTICS FOR THE SECOND
GENERATION CHIP DESIGN 259
12.3.3 FABRICATION 262
12.4 NANOWIRE ASSEMBLY UTILIZING DIELECTROPHORESIS 264
CONTENTS | XI
12.4.1 THEORY 264
12.4.2 EXPERIMENTAL DETAILS 267
12.4.2.1 LIQUID MEDIUM SELECTION 267
12.4.2.2 NANOWIRE ASSEMBLY PROCESS 267
12.4.2.3 ACCELERATION OF WATER DROPLET EVAPORATION 269
12.4.2.4 RECOGNITION OF PROPERLY ASSEMBLED NANOWIRES 269
12.4.2.5 RESULTS AND DISCUSSION 270
12.5 OHMIC CONTACT GENERATION 271
12.5.1 SEM ELECTRON BEAM INDUCED DEPOSITION (EBID) 271
12.5.2 SHADOW MASK TECHNIQUES 275
12.5.2.1 DESIGN AND FABRICATION 275
12.5.2.2 EXPERIMENTAL PROCESS 277
12.6 SUMMARY AND OUTLOOK 277
REFERENCES 279
APPENDIX
283
INDEX
287 |
| any_adam_object | 1 |
| author2 | Eibl, Oliver |
| author2_role | edt |
| author2_variant | o e oe |
| author_GND | (DE-588)135937523 |
| author_facet | Eibl, Oliver |
| building | Verbundindex |
| bvnumber | BV042546762 |
| classification_rvk | UP 5100 ZM 7028 ZN 3700 ZN 8900 |
| ctrlnum | (OCoLC)892071315 (DE-599)DNB105870284X |
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| dewey-hundreds | 600 - Technology (Applied sciences) |
| dewey-ones | 620 - Engineering and allied operations |
| dewey-raw | 620.115 |
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| dewey-sort | 3620.115 |
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| genre | (DE-588)4143413-4 Aufsatzsammlung gnd-content |
| genre_facet | Aufsatzsammlung |
| id | DE-604.BV042546762 |
| illustrated | Illustrated |
| indexdate | 2024-08-03T02:21:59Z |
| institution | BVB |
| isbn | 3527334890 9783527334896 9783527672608 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-027980728 |
| oclc_num | 892071315 |
| open_access_boolean | |
| owner | DE-11 DE-29T DE-83 |
| owner_facet | DE-11 DE-29T DE-83 |
| physical | XXIII, 290 S. Ill., graph. Darst. |
| publishDate | 2015 |
| publishDateSearch | 2015 |
| publishDateSort | 2015 |
| publisher | Wiley-VCH |
| record_format | marc |
| spelling | Thermoelectric Bi 2 Te 3 Nanomaterials ed. by Oliver Eibl ... Weinheim Wiley-VCH 2015 XXIII, 290 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Nanostrukturiertes Material (DE-588)4342626-8 gnd rswk-swf Thermoelektrischer Effekt (DE-588)4223155-3 gnd rswk-swf Bismuttellurid (DE-588)1071749803 gnd rswk-swf (DE-588)4143413-4 Aufsatzsammlung gnd-content Bismuttellurid (DE-588)1071749803 s Nanostrukturiertes Material (DE-588)4342626-8 s Thermoelektrischer Effekt (DE-588)4223155-3 s DE-604 Eibl, Oliver (DE-588)135937523 edt Erscheint auch als Online-Ausgabe, EPUB 978-3-527-67262-2 Erscheint auch als Online-Ausgabe, MOBI 978-3-527-67261-5 Erscheint auch als Online-Ausgabe, PDF 978-3-527-67263-9 X:MVB text/html http://deposit.dnb.de/cgi-bin/dokserv?id=4783429&prov=M&dok_var=1&dok_ext=htm Inhaltstext DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=027980728&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Thermoelectric Bi 2 Te 3 Nanomaterials Nanostrukturiertes Material (DE-588)4342626-8 gnd Thermoelektrischer Effekt (DE-588)4223155-3 gnd Bismuttellurid (DE-588)1071749803 gnd |
| subject_GND | (DE-588)4342626-8 (DE-588)4223155-3 (DE-588)1071749803 (DE-588)4143413-4 |
| title | Thermoelectric Bi 2 Te 3 Nanomaterials |
| title_auth | Thermoelectric Bi 2 Te 3 Nanomaterials |
| title_exact_search | Thermoelectric Bi 2 Te 3 Nanomaterials |
| title_full | Thermoelectric Bi 2 Te 3 Nanomaterials ed. by Oliver Eibl ... |
| title_fullStr | Thermoelectric Bi 2 Te 3 Nanomaterials ed. by Oliver Eibl ... |
| title_full_unstemmed | Thermoelectric Bi 2 Te 3 Nanomaterials ed. by Oliver Eibl ... |
| title_short | Thermoelectric Bi 2 Te 3 Nanomaterials |
| title_sort | thermoelectric bi 2 te 3 nanomaterials |
| topic | Nanostrukturiertes Material (DE-588)4342626-8 gnd Thermoelektrischer Effekt (DE-588)4223155-3 gnd Bismuttellurid (DE-588)1071749803 gnd |
| topic_facet | Nanostrukturiertes Material Thermoelektrischer Effekt Bismuttellurid Aufsatzsammlung |
| url | http://deposit.dnb.de/cgi-bin/dokserv?id=4783429&prov=M&dok_var=1&dok_ext=htm http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=027980728&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT eibloliver thermoelectricbi2te3nanomaterials |