On the aging of lithium ion batteries with focus on polyolefin separators and graphite negative electrodes:
Saved in:
| Main Author: | |
|---|---|
| Format: | Thesis Book |
| Language: | English |
| Published: |
2014
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| Series: | Physikalische Chemie
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| Subjects: | |
| Online Access: | Inhaltsverzeichnis |
| Physical Description: | VI, 481 S. Ill., graph. Darst. |
Staff View
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| 245 | 1 | 0 | |a On the aging of lithium ion batteries with focus on polyolefin separators and graphite negative electrodes |c vorgelegt von Claudia Colle |
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Record in the Search Index
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|---|---|
| adam_text | INTRODUCTION AND FUNDAMENTAL THEORY 7
1.1 GENERAL VIEW ON LITHIUM-ION BATTERIES 7
1.2 POSITIVE ELECTRODE MATERIALS 9
1.3 ELECTROLYTES 10
1.3.1 SOLVENTS 10
1.3.2 SALTS 11
1.3.3 ADDITIVES 11
1.4 NEGATIVE ELECTRODE MATERIALS 12
1.4.1 OVERVIEW 12
1.4.2 GRAPHITE 13
1.4.3 SOLID ELECTROLYTE INTERPHASE (SEI)..] 15
1.5 SEPARATORS 17
1.5.1 GENERAL 17
1.5.2 CHARACTERISTICS AND REQUIREMENTS 18
1.5.3 DIFFERENT TYPES OF SEPARATORS 33
1.5.4 PROPERTY IMPROVEMENT, NEW DEVELOPMENTS AND FUTURE TRENDS OF
SEPARATORS 41
1.5.5 CORRELATIONS BETWEEN SEPARATOR PROPERTIES, CELL PERFORMANCE AND
SAFETY 53
1.6 AGING OF LITHIUM-ION BATTERIES 62
1.6.1 GENERAL 62
1.6.2 POSITIVE ELECTRODE 63
1.6.3 NEGATIVE ELECTRODE 64
1.6.4 SEPARATOR 67
MOTIVATION
71
HTTP://D-NB.INFO/1052214088
METHODS 75
3.1 ELECTROCHEMICAL METHODS 75
3.1.1 CONSTANT CURRENT CYCLING 75
3.1.2 CYCLIC VOLTAMMETRY 78
3.1.3 ELECTROCHEMICAL IMPEDANCE SPECTROSCOPY 81
3.2 THERMAL ANALYSIS 82
3.2.1 DIFFERENTIAL SCANNING CALORIMETRY (DSC) 82
3.2.2 THERMOGRAVIMETRIC ANALYSIS (TGA) 85
3.2.3 THERMO-MECHANICAL ANALYSIS (TMA) 86
3.2.4 DYNAMIC MECHANICAL ANALYSIS (DMA) 88
3.3 SURFACE ANALYSIS TECHNIQUES 91
3.3.1 SCANNING ELECTRON MICROSCOPY (SEM) 91
3.3.2 ATOMIC FORCE MICROSCOPY (AFM) 92
3.3.3 X-RAY DIFFRACTION (XRD) 93
3.3.4 X-RAY PHOTOEIECTRON SPECTROSCOPY (XPS) 93
3.4 PHYSICAL ADSORPTION 94
3.4.1 GENERAL 94
3.4.2 SURFACE CHARACTERIZATION USING BET 95
3.4.3 SURFACE CHARACTERIZATION USING DFT 96
3.5 FURTHER METHODS 98
3.5.1 GURLEY 98
3.5.2 MACMULLIN 99
3.5.3 MIXED PENETRATION STRENGTH 101
3.5.4 MERCURY INTRUSION POROSIMETRY 103
3.5.5 BALL MILLING 103
EXPERIMENTAL 105
4.1 MATERIALS 105
4.2 ELECTRODE PREPARATION 106
4.2.1 GRAPHITE ELECTRODES FOR AGING EXPERIMENTS 106
4.2.2 GRAPHITE ELECTRODES FOR DFT-STUDIES 106
4.3 THERMAL TREATMENT OF SEPARATORS 107
4.3.1 TREATMENT WITHOUT ELECTROLYTE 107
4.3.2 TREATMENT IN THE PRESENCE OF ELECTROLYTE 107
4.4 CELL ASSEMBLY 107
4.4.1 POUCH BAG CELLS 107
4.4.2 SWAGELOK T-CELLS 108
RESULTS AND DISCUSSION 110
5.1 SEPARATORS 110
5.1.1 INTRODUCTION 110
5.1.2 CHARACTERIZATION OF THE PRISTINE MATERIAL 115
5.1.3 THERMAL TREATMENT 149
5.1.4 THERMAL TREATMENT IN THE PRESENCE OF ELECTROLYTE 212
5.1.5 CHARACTERIZATION OF SEPARATORS AGED IN COMMERCIAL CELLS 275
5.1.6 CONCLUSION 286
5.2 GRAPHITE NEGATIVE ELECTRODES 301
5.2.1 INTRODUCTION 301
5.2.2 CHARACTERIZATION OF THE ELECTRODE MATERIAL 304
5.2.3 AGING ATTEMPTS BY GALVANOSTATIC CYCLING IN HALF-CELLS VS. LITHIUM
327
5.2.4 EFFECT OF LONG TERM CYCLING AND CYCLING OF CYCLED ELECTRODES IN
NEW HALF-CELLS ON THE ELECTRODE MATERIAL 334
5.2.5 CONCLUSION 348
5.3 DFT-STUDIES ON DIFFERENT GRAPHITES 351
5.3.1 INTRODUCTION 351
5.3.2 CHARACTERIZATION AND COMPARISON OF THE GRAPHITES 353
5.3.3 GRAPHITE ELECTRODES: CAPACITY INVESTIGATIONS 378
5.3.4 CORRELATION BETWEEN DFT AND BET SURFACE AREA AND IRREVERSIBLE
CHARGE CAPACITY LOSS IN THE 1
ST
CYCLE 400
5.3.5 CORRELATION BETWEEN BASAL PLANE AND NON-BASAL PLANE SURFACE
AREA AND IRREVERSIBLE CHARGE CAPACITY LOSS IN THE 1
ST
CYCLE 404
5.3.6 CONCLUSION 410
CONCLUSION AND OUTLOOK 422
SEPARATORS 422
GRAPHITE 424
REFERENCES
428
LIST OF FIGURES 444
LIST OF TABLES 468
ACKNOWLEDGMENTS 476
CURRICULUM VITAE 478
LIST OF PUBLICATIONS 480
|
| any_adam_object | 1 |
| author | Colle, Claudia 1981- |
| author_GND | (DE-588)1050799054 |
| author_facet | Colle, Claudia 1981- |
| author_role | aut |
| author_sort | Colle, Claudia 1981- |
| author_variant | c c cc |
| building | Verbundindex |
| bvnumber | BV042068407 |
| classification_rvk | ZN 8730 |
| ctrlnum | (OCoLC)891366992 (DE-599)DNB1052214088 |
| dewey-full | 621.312424 |
| dewey-hundreds | 600 - Technology (Applied sciences) |
| dewey-ones | 621 - Applied physics |
| dewey-raw | 621.312424 |
| dewey-search | 621.312424 |
| dewey-sort | 3621.312424 |
| dewey-tens | 620 - Engineering and allied operations |
| discipline | Elektrotechnik / Elektronik / Nachrichtentechnik |
| format | Thesis Book |
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| id | DE-604.BV042068407 |
| illustrated | Illustrated |
| indexdate | 2024-07-10T01:11:52Z |
| institution | BVB |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-027509134 |
| oclc_num | 891366992 |
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| owner_facet | DE-29T DE-355 DE-BY-UBR DE-83 |
| physical | VI, 481 S. Ill., graph. Darst. |
| publishDate | 2014 |
| publishDateSearch | 2014 |
| publishDateSort | 2014 |
| record_format | marc |
| series2 | Physikalische Chemie |
| spelling | Colle, Claudia 1981- Verfasser (DE-588)1050799054 aut On the aging of lithium ion batteries with focus on polyolefin separators and graphite negative electrodes vorgelegt von Claudia Colle 2014 VI, 481 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Physikalische Chemie Münster (Westfalen), Univ., Diss., 2014 Grafit (DE-588)4158067-9 gnd rswk-swf Lithium-Ionen-Akkumulator (DE-588)7681721-0 gnd rswk-swf Elektrode (DE-588)4014247-4 gnd rswk-swf Alterung (DE-588)4142063-9 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Lithium-Ionen-Akkumulator (DE-588)7681721-0 s Grafit (DE-588)4158067-9 s Elektrode (DE-588)4014247-4 s Alterung (DE-588)4142063-9 s DE-604 DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=027509134&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Colle, Claudia 1981- On the aging of lithium ion batteries with focus on polyolefin separators and graphite negative electrodes Grafit (DE-588)4158067-9 gnd Lithium-Ionen-Akkumulator (DE-588)7681721-0 gnd Elektrode (DE-588)4014247-4 gnd Alterung (DE-588)4142063-9 gnd |
| subject_GND | (DE-588)4158067-9 (DE-588)7681721-0 (DE-588)4014247-4 (DE-588)4142063-9 (DE-588)4113937-9 |
| title | On the aging of lithium ion batteries with focus on polyolefin separators and graphite negative electrodes |
| title_auth | On the aging of lithium ion batteries with focus on polyolefin separators and graphite negative electrodes |
| title_exact_search | On the aging of lithium ion batteries with focus on polyolefin separators and graphite negative electrodes |
| title_full | On the aging of lithium ion batteries with focus on polyolefin separators and graphite negative electrodes vorgelegt von Claudia Colle |
| title_fullStr | On the aging of lithium ion batteries with focus on polyolefin separators and graphite negative electrodes vorgelegt von Claudia Colle |
| title_full_unstemmed | On the aging of lithium ion batteries with focus on polyolefin separators and graphite negative electrodes vorgelegt von Claudia Colle |
| title_short | On the aging of lithium ion batteries with focus on polyolefin separators and graphite negative electrodes |
| title_sort | on the aging of lithium ion batteries with focus on polyolefin separators and graphite negative electrodes |
| topic | Grafit (DE-588)4158067-9 gnd Lithium-Ionen-Akkumulator (DE-588)7681721-0 gnd Elektrode (DE-588)4014247-4 gnd Alterung (DE-588)4142063-9 gnd |
| topic_facet | Grafit Lithium-Ionen-Akkumulator Elektrode Alterung Hochschulschrift |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=027509134&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
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