Aggregation induced emission: [1] Fundamentals
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| Sprache: | English |
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Wiley
2014
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| Ausgabe: | 1. publ. |
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| Beschreibung: | XVIII, 422 S. Ill., graph. Darst. |
| ISBN: | 9781118394304 |
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| 020 | |a 9781118394304 |9 978-1-118-39430-4 | ||
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| 245 | 1 | 0 | |a Aggregation induced emission |n [1] |p Fundamentals |c ed. by Anjun Qin ... |
| 250 | |a 1. publ. | ||
| 264 | 1 | |a Chichester |b Wiley |c 2014 | |
| 300 | |a XVIII, 422 S. |b Ill., graph. Darst. | ||
| 336 | |b txt |2 rdacontent | ||
| 337 | |b n |2 rdamedia | ||
| 338 | |b nc |2 rdacarrier | ||
| 700 | 1 | |a Qin, Anjun |4 edt | |
| 773 | 0 | 8 | |w (DE-604)BV041459875 |g 1 |
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Datensatz im Suchindex
| _version_ | 1804151589581094912 |
|---|---|
| adam_text | Contents
List of Contributors xijj
РФ
xvii
1
Synthesis of Siloles (and Germoles) that Exhibit the
AIE
Effect
1
Joyce Y. Corey
1.1 Introduction
1
1.2
Background
2
1.3
Synthesis of Siloles
4
1.3.
1 Reductive dimerization of tolan
4
1.3.2
Intramolecular cyclization of dialkynylsilanes
7
1
.3.3
Intramolecular cyclization of dialkynylsilanes utilizing
borane
reagents
10
1
.3.4
Synthesis of siloles using transition metal reagents
12
1.4
Modification of Preformed Siloles
14
1.4.1
Reactions at silicon centers
14
1
.4.2
Reactions of a ring carbon center
15
1.5
Related Germole Methodology
15
1.5.1
Germoles produced by metathesis and exchange reactions
15
1
.5.2
Germoles from other methods
16
1.5.3
Photoluminescence
and
AIE
of germoles
18
1
.6
Metallaindenes and Metallafluorenes of Si and Ge
19
1.6.1
Methods for the formation of silaindenes and germaindenes
19
1
.6.2
Methods for the formation of metallafluorenes
21
1.7
Oligomers
and Polymers of Metalloles and Benzene-Annulated
Metalloles
25
1
.7.1
Oligomers
that contain silole units connected at the
1,1-
and 2,5-positions
25
! .7.2
Polysiloles and silole polymers connected through 2,5-positions
26
1.7.3
Polymers with silole pendants and hyperbranched polymers
27
1.7.4
Polybenzosiloles and ladder polymers
28
1
.7.5
Polymers that contain silafluorenes
29
1.7.6
Germoles in
oligomers
and polymers
30
1.8
Summary and Future Directions
31
References
33
vi
Contents
2
Aggregation-Induced Emission in
(¡roup
14
IVletalloles (Siloles, (¡ermoles, and Stannoles):
Spectroscopic Considerations,
Substituent
Effects, and Applications
39
Jerome
L
Mitili))
and Henry J.
Trucy
2.1
Introduction
39
2.1.1
The group
14
melailoles
41
2.2
Characteristics of
AIE in
the Group
14
Metalloles
44
2.2.1
Aryl-substitLited siloles
44
2.2.2
Aryl-suhsiituted germoles ami stannoles
47
2.3
Origins of
AIE
in Group
14
Metalloles: Restricted Intramolecular Rotation
48
2.3.1
Effect of solvent viscosity
48
2.3.2
Effect of temperature
48
2.3.3
Room-temperature glasses
49
2.3.4
Effect of pressure
49
2.3.5
Excited-state lifetimes
49
2.3.6
Molecular geometry
50
2.3.7
Aggregate nanopartiele morphology
50
2.3.8
Internal structural control of intramolecular rotations
50
2.4
Polymer Films and Polymerized Siloles
51
2.5
Applications ol AIE-Active Metalloles ?>3
2.5.1
Electrooptical devices
53
2.5.2
Chemical sensors
53
References
54
3
Aggregation-Induced Emission ofUO-Distyrylanthracene Derivatives and
Their Applications
61
Bin
Хи,
Jiho
УЈшпц
and Wcnjiiif»
fian
3.1
Introduction
61
3.2
AIE
Molecules Based on
9,1
0-Dislyrylanthracene
63
3.2.1
Small molecules
63
3.2.2
Macromolecules
64
3.3
AIE
Mechanism of
9,
lO-Distyrylanthracene Molecule Systems
65
3.4
Application of
AIE
Luminogcns Based on
9,
lO-Distyrylanthracene
67
3.4.1
Solid-state emitters
67
3.4.2
Pie/ochromism
72
3.4.3
Fluorescent sensors and probes
74
3.4.4
Bioimaging
75
3.5
Conclusion
80
Acknowledgments
80
References
80
4
Diaminobenzene-Cored Fluorophores Exhibiting Highly Efficient Solid-State
Luminescence
83
Musaki Shimizu
4.1
Introduction
83
4.2
K4-Bis(alkenyl)-2,5-dipiperidinobenzenes
86
4.3 1
,4-Diamino-2,5-bis(arylethenyl)benzenes
89
4.4
2,5-Diaminoterephthalates
93
Contents
vii
4.5
2,5-Bis(diarylamino)-l,4-diaroylbenzenes
95
4.6
Applications
99
4.7
Conclusion
102
Acknowledgments
102
References
ЮЗ
5
Agrégation-
Induced Emission in Organic Ion Pairs
105
Suzanne Fery-Forgues
5.1
Introduction IO5
5.2
Historical Background
106
5.3
Preparation and Control of the Fluorophore Arrangement
107
5.3.1
Ту ре
of interactions
107
5.3.2
Preparation J07
5.3.3
Influence of the nature of the
counterion
on the fluorophore arrangement
108
5.3.4
Influence of stoichiometry on the
AIE
effect
11
1
5.4
AIE-Active Organic Ion Pairs in
Nano-
and Microparticles 111
5.4.1
Controlled preparation of nanoparticles
112
5.4.2
Nanoparticles for
biomedical
imaging
] 14
5.4.3
Preparation of nanocrystals, nanofibers, and reticulated materials
114
5.5
Applications as Fluorescent Probes and Sensors for Analytical Purposes
115
5.5.
1 Detection of small electrolytes
115
5.5.2
Detection of
рої у
electrolytes
116
5.6
Perspectives
122
Acknowledgments
122
References
123
6
Aggregation-Induced Emission Materials: the Art of Conjugation and Rotation
127
.////#
Huang, Qianqian Li and Zhen Li
6.1
Introduction
127
6.2
Rotation and Conjugation in
AIE
Molecules
128
6.3
Design of Functional Materials by Tuning the Conjugation Effect and
Restricting Rotations
134
6.3.1
Some
AIE
molecules with blue emission through modification of the
conjugation between the construction blocks
135
6.3.2
Some sensing systems by selectively controlling rotation
142
6.3.3
Some other systems utilizing the
AIE
concept
145
6.4
Outlook
151
References
152
Red-Emitting
AIE
Materials
155
Xiao Yuan Shen, Anjun Qin and Jing Zhi Sun
7.1
Introduction
155
7.2
Basic Principles of Molecular Design for Red-Emitting Materials
156
7.3
Acquirement of Red-Emitting
AIE
Materials by Reconstruction of Traditional
Red-Emitting Molecules
158
7.4
Preparation of Red-Emitting Materials by Introduction of Electron Donors/Acceptors
into AIE-Active Molecules
162
viii Contents
7.5
Outlook
164
Acknowledgments 165
References 1
65
8
Properties of Triarylamine Derivatives with
AIK
and Large Two-Photon
Absorbing Cross-Sections
169
Jianli
Hua,
He
Tian
and Hao Zhang
8.1
Introduction
169
8.2
Design and Synthesis of Triarylamine Derivatives with
AIE
and 2PA
170
8.3
AIE
Properties of Triarylamine Derivatives
170
8.3.
1
AIE
properties of diketopyrrolopyrrole (DPP)-based triarylamine derivatives
170
8.3.2
AIE
properties of sturbursl triarylamine derivatives based on
cyano-substituted diphenylamineslyrylbenzene
173
8.3.3
AIL properties of multibranehed triarylamine end-capped tria/.mes
174
8.4
One-Photon and Two-Photon Absorption Properties ol Triarylamine
Derivatives with AIL
176
8.5
Application
oí
Triarylamine Materials with
AIE
and 2PA
180
8.5.1
Fluorescence switching
180
8.5.2
Organic light-emitting diodes
180
8.5.3
Fluorescence probes for
Ніг
180
8.6
Conclusion
181
References 1
82
9
Photoisomerization and Light-Driven Fluorescence Enhancement
of Azobenzene Derivatives
185
Mina Hati
and Yusiw Norikaiw
9.1
Introduction
185
9.2
Photoisomerization and Fluorescence of Azobenzene Derivatives
186
9.2.1
Ground-state structure of azobenzene
186
9.2.2
Reversible
isomerizution
of azobenzene
187
9.2.3
Sterically hindered azobenzene derivatives
188
9.2.4
Fluorescence from azobenzene derivatives
190
9.3
Aggregation-Induced Emission
(AIE)
191
9.4
Fluorescence from Azobenzene-Based Aggregates
193
9.4.1
Light-driven self-assembly and fluorescence enhancement
194
9.4.2
Factors affecting fluorescence enhancement of azobenzenes
195
9.4.3
Modulation of fluorescence color
196
9.4.4
Fluorescent organic films
198
9.5
Conclusion
199
References
199
10
Supramolecular Structure and Aggregation-Induced Emission
205
Hongyu Zhang and Yue Wang
10.1
Introduction
205
10.2
Hydrogen Bonding-Based Molecular Dimer and
AIE
206
10.2.1
The role of hydrogen bonds in
AIE
206
10.2.2
AIE
and single crystal structures
208
Contents ix
1
0.2.3
Relationship between supramolecualr structures and
AIE
209
10.2.4
Amplified spontaneous emission
(ASE)
property
210
10.3
Quinacridine Derivatives with ID Aggregation-Induced Red Emission
210
10.3.1
Contradiction between ID self-assembly and
AIE
210
10.3.2
Design of novel QA with
AIE
and ID self-assembly
211
10.3.3
AIE
behavior
212
10.3.4
Morphology transition from 0D nanostructures to IDmicrowires
214
10.3.5
ID self-assembly
214
10.3.6
Crystal structure
215
10.4
Multi-Stimuli-Responsive Fluorescence Switching of AIE/AIEE Luminogens
217
10.4.1
Mechanism of stimuli-responsive fluorescence switching
217
1
0.4.2
Design strategy towards stimuli-responsive AIE/AIEE molecules
218
10.4.3
AIE
phenomenon in neutral and acid states
218
10.4.4
Molecular and supramolecular structures in crystal
220
10.4.5
Multi-stimuli-responsive
AIE
switching
220
1
0.4.6
Multi-stimuli-responsive fluorescence of other AIE/AIEE molecules
221
10.5
Pt·
■
Pt
Interaction-Induced Emissive and Conductive ID Crystals
222
10.5.1
AIE
of organometallic complexes
222
10.5.2
Pt·
·
Pt interaction-induced luminescent crystals
223
10.5.3 1
D
nano-Zmicro aggregation and photophysical properties
223
10.5.4
Vapor-responsive emission behavior of nanowires
225
10.5.5
Pt-
■
Pt interaction-induced ID semiconductor
225
10.6
Conclusion
226
References
227
11
Aggregation-Induced Emission in Supramolecular jr-Organogels
233
ľcngchong Xue
and Ran
Lu
M.I Introduction
233
1
1
.2
Organogels Based on Discotic Molecules with
AIE
234
1
1
.2.1
Triphenylbenzene-cored discotic molecules
234
11.2.2
Other discotic gelators
237
11.3
Organogels Based on Rod-Like Molecules with
AIE
238
1
1.3.1
Styrene
derivatives
238
11.3.2
Other linear molecules
241
1 1.4
Organogels Based on Banana-Shaped Molecules with
AIE
242
11.4.1
Salicylideneaniline derivatives
242
11.4.2
Other banana-shaped gelators
245
1
1
.5
Organogels Based on Dendritic Molecules with
AIE
246
1
1.6
Conclusion
249
References
250
12
AIE-Acti
ve
Polymers
253
Rongrong
Ни,
Jacky W.Y. Lam and Ben Zhong Tang
12.1
Introduction
253
12.2
Polyolefins
254
12.3
Polyacetylenes
258
12.4
Polydiynes
259
χ
Contents
Ι Ί
ϊ Δ
.5
Polyarylenes
12
.6
Polytria/oles
12
.7
Poly
si lyleneviny
lenes
12
.8
P()ly(
Vinylene
Sul
lide
)s
12.
,9
Other
Systems
12.
IO
Conclusion
References
263
269
271
272
277
280
280
13
Enhanced Emission by Restriction of Molecular Rotation
285
J
in-
Lon
я
H on
χ
13.1
Background
285
13.2
Strategy to Restrict Molecular Rotation
286
13.2.1
Introduction of bulky Mibslituents by chemical links
287
13.2.2
Introduction ol bulky groups by complexalion
290
13.2.3
Hindered molecular rolalion by hydrogen bonding
292
13.2.4
Hindered molecular rotation by metal or metal ion chcLition
296
13.3
Characterizations of Hindered Molecular Rotations
297
13.3.1
Solution fluorescence spectroseopy
297
13.3.2
Ή
NMR spectroseopy
298
13.4
Conclusion
302
References
303
14
Restricted Intramolecular Rotations: a Mechanism for Aggregation-Induced
Emission
307
Jumvti Chen and Hen /.hong Tung
14.1
Introduction: 2,3,4,5-Telraphenylsilolc, the Prototype Molecule
of Aggregation-Induced Hmission (Alb)
307
14.2
Crystal Structures ol
2,3.4,5-
Tetraphenylsiloles
310
14.2.1
Twisted arrangements of phenyl groups on the silole core
310
14.2.2
Enlarged distance between silole cores: far beyond
π-π
interactions
3 1 1
14.3
Restricted Intramolecular Rotation
(RIR)
312
14.3.1
Thickening-enhanced emission of silole solutions (viscochcomism)
З ІЗ
14.3.2
Piezochromism
313
14.3.3
Cooling-enhanced emission (thermochromism)
314
14.3.4
On-off fluorescence switching of silole thin films: activation
of rotations in solvent vapors (vapochromism)
316
14.3.5
Fluorescence decay dynamics
317
14.3.6
Highly emissive silole solutions: restriction of rotation by internal
structural tuning
318
14.4
Conclusion
320
Acknowledgments
320
References
320
15
Crystallization-Induced Emission Enhancement
323
Yongqiang Dong
15.1
Introduction
323
15.2
Traditional Luminogens
324
Contents xi
15.3 Crystallization-Induced Emission Enhancement (CIEE) 324
15.3.1 CIEE luminogens 325
15.3.2 Potential
applications
330
15.4
Conclusion
333
References
334
16
Time-Resolved
Spectroscopie
Study of the Aggregation-Induced Emission
Mechanism
337
Bmg
-гощ
Gao, Hai-yu
Wang, Qi-dai Chen and Hong-bo Sun
16.1
Introduction
337
16.2
Time-Resolved Spectroscopy
338
16.2.
1 Femtosecond time-resolved fluorescence system
338
16.2.2
Femtosecond transient absorption system
339
16.2.3
Time-correlated single-photon counting (TCSPC) system
341
16.3
AIE
Molecules Without Electron Donor-Acceptor Units
341
í
6.3.1
Time-resolved fluorescence study of HPS
341
16.3.2
Time-resolved fluorescence study of CNDPDSB
342
16.3.3
Transient absorption study of CNDPDSB
343
16.4
AIE
Molecules with Electron Donor-Acceptor Units
344
16.4.1
Steady-state properties of CNDPASDB
344
16.4.2
Time-resolved fluorescence study of CNDPASDB
346
16.4.3
Transient absorption study of CNDPASDB
351
16.4.4
Discussion
353
16.5
Conclusion
353
Acknowledgments
354
References
354
17
Theoretical Understanding of
AIE
Phenomena Through Computational
Chemistry
357
Qian Peng, Yingli Niu, Qunyan Wu, Xing
Gao
and Zhigang Shuai
17.1
Introduction
357
17.2
Fundamental Photophysics Relating to
AIE
Phenomena
358
1
7.2.1
Absorption and emission
358
1
7.2.2
Luminescence quantum efficiency
359
17.3
Computational Approaches to Investigate
AIE
Molecules
360
17.3.1
Molecular optical spectra formalisms
360
} 7.3.2
Molecular radiative and nonradiative rate formalisms
365
1
7.3.3
Computational details
367
17.4
Computational Results
370
17.4.1
Optical spectra
370
17.4.2
Excited-state decay processes
376
17.4.3
A nonadiabatic dynamic simulation
385
17.5
Summary and Outlook
389
References
390
xii
Contents
18
Recent Theoretical Advances in Understanding the Mechanism of Aggregation-Induced
Emission for Small Organic Molecules
399
Jim-Ling
Jiti,
Yun
Gelig
and
Zliouiţ-Miu
Su
18.1
Introduction
399
18.2
Theoretical Methods
400
18.2.1
Main phoiophysicul processes of organic molecules
400
18.2.2
Theoretical estimation of pholophysical parameters
402
1
8.3
Recent Theoretical Advances in Understanding the Mechanism of
Aggregation-Induced Km
issi
on
406
18.3.1
Restriction of intramolecular rotation (R1R)
406
18.3.2
Influence of molecular packing and intermolecular interactions on the
photophysical properties and fluorescence efficiencies in the solid phase
41 1
18.4
Prospects
413
18.4.1
Other
AIE
mechanisms except for the conventional
RIR
mechanism
413
18.4.2
Design ol multifunctional materials with
AIK
413
Acknowledgments
414
References
414
index
4
Ì
9
AGGREGATION-INDUCED
EMISSION
FUNDAMENTALS
EDITORS
ANJUN QIN
Department
of Polymer
Science
and Engineering, Zhejiang University,
China
BEN ZHONG
TANG
Department
of Chemistry, The
Hong Kong
University of
Science
and Technology China
Aggregation-Induced Emission
(AIE)
is a novel photophysical phenomenon which offers a new platform
for researchers to look into the light-emitting processes from luminogen aggregates, from which useful
information on structure-property relationships may be collected and mechanistic insights may be
gained. The discovery of the
AIE
effect opens a new avenue for the development of new luminogen
materials in the aggregate or solid state. By enabling light emission in the practically useful solid state,
AIE
has the potential to expand significantly the technological applications of luminescent materials.
Aggregation-Induced Emission: Fundamentals is the first book to explore the fundamental issues of
AIE,
including the design, synthesis, and photophysical behavior of AlE-active molecules and polymers. The
control of the morphological structures of the aggregates of AlE-active materials, and the experimental
investigation and theoretical understanding of the
AIE
mechanism, are also covered in this volume.
Topics covered include:
•
AIE
in group
14
metalloles
•
AIE in
organic ion pairs
•
Red light-emitting
AIE
materials
•
Supramolecular structure and
AIE
•
AlE-active polymers
•
Enhanced emission by restriction of molecular rotation
•
Crystallization-induced emission enhancement
•
Theoretical understanding of
AIE
phenomena
This book is essential reading for scientists and engineers who are designing optoelectronic materials
and
biomedical
sensors, and will also be of interest to academic researchers in materials science and
physical and synthetic organic chemistry, as well as physicists and biological chemists.
Also available
as an e-book
ISBN
978-1-118-39430-«
9 781 1 1
S
391304
|
| any_adam_object | 1 |
| author2 | Qin, Anjun |
| author2_role | edt |
| author2_variant | a q aq |
| author_facet | Qin, Anjun |
| building | Verbundindex |
| bvnumber | BV041460130 |
| classification_rvk | UH 5830 |
| ctrlnum | (OCoLC)884740569 (DE-599)BVBBV041460130 |
| discipline | Physik |
| edition | 1. publ. |
| format | Book |
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| id | DE-604.BV041460130 |
| illustrated | Illustrated |
| indexdate | 2024-07-10T00:57:13Z |
| institution | BVB |
| isbn | 9781118394304 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-026906513 |
| oclc_num | 884740569 |
| open_access_boolean | |
| owner | DE-11 DE-703 |
| owner_facet | DE-11 DE-703 |
| physical | XVIII, 422 S. Ill., graph. Darst. |
| publishDate | 2014 |
| publishDateSearch | 2014 |
| publishDateSort | 2014 |
| publisher | Wiley |
| record_format | marc |
| spelling | Aggregation induced emission [1] Fundamentals ed. by Anjun Qin ... 1. publ. Chichester Wiley 2014 XVIII, 422 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Qin, Anjun edt (DE-604)BV041459875 1 Digitalisierung UB Bayreuth - ADAM Catalogue Enrichment application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=026906513&sequence=000003&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis Digitalisierung UB Bayreuth - ADAM Catalogue Enrichment application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=026906513&sequence=000004&line_number=0002&func_code=DB_RECORDS&service_type=MEDIA Klappentext |
| spellingShingle | Aggregation induced emission |
| title | Aggregation induced emission |
| title_auth | Aggregation induced emission |
| title_exact_search | Aggregation induced emission |
| title_full | Aggregation induced emission [1] Fundamentals ed. by Anjun Qin ... |
| title_fullStr | Aggregation induced emission [1] Fundamentals ed. by Anjun Qin ... |
| title_full_unstemmed | Aggregation induced emission [1] Fundamentals ed. by Anjun Qin ... |
| title_short | Aggregation induced emission |
| title_sort | aggregation induced emission fundamentals |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=026906513&sequence=000003&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=026906513&sequence=000004&line_number=0002&func_code=DB_RECORDS&service_type=MEDIA |
| volume_link | (DE-604)BV041459875 |
| work_keys_str_mv | AT qinanjun aggregationinducedemission1 |