Electronic dissipation processes during chemical reactions on surfaces:
Saved in:
| Main Author: | |
|---|---|
| Format: | Thesis Book |
| Language: | English |
| Published: |
Hamburg
Disserta Verl.
2011
|
| Subjects: | |
| Online Access: | Inhaltstext Inhaltsverzeichnis |
| Physical Description: | III, 241 S. Ill., graph. Darst. |
| ISBN: | 9783942109888 |
Staff View
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Record in the Search Index
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| adam_text |
IMAGE 1
CONTENTS
1 INTRODUCTION 1
2 BASIC INFORMATION 3
2.1 ADIABATIC OR NON-ADIABATIC REACTION? 3
2.2 MOLECULAR BEAMS 9
2.3 CYCLIC VOLTAMMETIY 14
2.4 WATER FORMATION REACTION 18
3 EXPERIMENTAL DESIGN AND SAMPLE PREPARATION 25
3.1 THE ULTRA HIGH VACUUM RECIPIENT 25
3.2 THE MOLECULAR BEAM APPARATUS 27
3.3 THE ION BEAM SOURCE 27
3.4 TUNNEL DETECTORS 29
3.4.1 METAL-INSULATOR-METAL TUNNEL DETECTOR (MIM) 29 3.4.2 THE NEW
STEPPED METAL-INSULATOR-SEMICONDUCTOR TUNNEL DETECTOR (STEPPED-MIS) 30
4 MEASUREMENTS, RESULTS AND DISCUSSION 33
4.1 MOLECULAR BEAM 33
4.1.1 TRANSLATIONAL ENERGY OF THE PARTICLES 33
4.1.2 PARTICLE NUMBERS OF THE MOLECULAR BEAM 36
4.2 ION BEAM CHARACTERISTICS 42
4.3 ION MIGRATION IN ANODIC OXIDE FILMS AFTER POTENTIOSTATIC FORMATION .
43
4.3.1 INTRODUCTION 43
4.3.2 EXPERIMENTAL 46
4.3.3 RESULTS 49
4.3.4 DISCUSSION 56
4.3.5 CONCLUSION 64
4.3.6 APPENDIX 65
4.4 PREPARATION AND PROPERTIES OF THIN AMORPHOUS TANTALUM FILMS . . 66
4.4.1 INTRODUCTION 66
BIBLIOGRAFISCHE INFORMATIONEN HTTP://D-NB.INFO/1016934769
DIGITALISIERT DURCH
IMAGE 2
CONTENTS
4.4.2 EXPERIMENTAL 67
4.4.3 ELECTRICAL RESISTIVITY OF THIN TANTALUM FILMS 76
4.4.4 CONCLUSION 81
4.5 THIN TANTALUM FILMS ON CRYSTALLINE SILICON - A METALLIC GLASS 86
4.5.1 INTRODUCTION 86
4.5.2 EXPERIMENT AND DISCUSSION 86
4.5.3 CONCLUSION 91
4.6 CHARGE TRANSPORT THROUGH THIN AMORPHOUS TIOX AND TAOX LAYERS . 92
4.6.1 INTRODUCTION 92
4.6.2 SAMPLE PREPARATION 93
4.6.3 INTERNAL PHOTOEMISSION 97
4.6.4 BIAS-INDUCED CHARGE TRANSPORT 108
4.6.5 CHEMICURRENTS 113
4.6.6 CONCLUSION 114
4.6.7 APPENDIX 116
4.7 PHOTO-SENSITIVE MIS SENSORS WITH STEPPED INSULATING LAYER 118 4.8
TRANSPORT OF EXCITED HOLES THROUGH MIS SENSORS 125
4.8.1 INTRODUCTION 125
4.8.2 EXPERIMENTAL 127
4.8.3 ELECTRONIC SENSOR PROPERTIES 129
4.8.4 CAPACITANCE VOLTAGE PLOTS AT DIFFERENT THICKNESSES 135 4.8.5
THEORETICAL DESCRIPTION OF INTERNAL PHOTOEMISSION 137 4.8.6 EXPERIMENTAL
RESULTS 141
4.8.7 CONCLUSION 157
4.8.8 MATHEMATICAL APPENDIX 158
4.9 MOLECULAR REACTION CHEMICURRENT STUDIES WITH MIS SENSORS 160 4.9.1
STUDY OF EFFUSING MOLECULAR GASES WITH MIS SENSORS 160 4.9.2 DIRECT
DOSAGE OF EXCITED SPECIES ON A MIS SENSOR I 162 4.9.3 DIRECT DOSAGE OF
EXCITED SPECIES ON A MIS SENSOR II 165 4.9.4 THE ORIGIN OF THE
CHEMICURRENT SIGNALS 166
4.9.5 TIME DEPENDENT TRACE OF THE CHEMICURRENT SIGNALS 175 4.9.6
INDIRECT DOSAGE OF EXCITED SPECIES ON A MIS SENSOR 179 4.9.7 EFFUSION OF
DEUTERIUM AND OXYGEN MIXTURES 184
5 SUMMARY AND OUTLOOK 187
BIBLIOGRAPHY 193
IMAGE 3
CONTENTS
6 FURTHER EXPERIMENTAL RESULTS PLANNED FOR PUBLICATION 217 6.1
TEMPERATURE DEPENDENCE OF INTERNAL PHOTOEMISSION IN MIM SENSORS 217
6.2 TEMPERATURE DEPENDENCE OF INTERNAL PHOTOEMISSION IN MIS SENSORS 222
6.3 ABOUT THE STABILITY OF THIN AL-ALOX AND TA-TAOX INTERFACES 225 6.3.1
INTRODUCTION 225
6.3.2 EXPERIMENTAL 225
6.3.3 DISCUSSION 226
6.3.4 CONCLUSION 231
7 APPENDIX 233
7.1 REFEREED PAPERS PUBLISHED 233
7.2 REFEREED PAPERS IN PREPARATION 234
7.3 INVITED TALK 235
7.4 POSTER AND TALKS 235
CURRICULUM VITAE 238
ERKLAERUNG 239
DANKSAGUNG 240
III |
| any_adam_object | 1 |
| author | Stella, Kevin 1984- |
| author_GND | (DE-588)1018031499 |
| author_facet | Stella, Kevin 1984- |
| author_role | aut |
| author_sort | Stella, Kevin 1984- |
| author_variant | k s ks |
| building | Verbundindex |
| bvnumber | BV040270340 |
| classification_rvk | VE 7007 |
| ctrlnum | (OCoLC)778114345 (DE-599)DNB1016934769 |
| dewey-full | 541.3724 |
| dewey-hundreds | 500 - Natural sciences and mathematics |
| dewey-ones | 541 - Physical chemistry |
| dewey-raw | 541.3724 |
| dewey-search | 541.3724 |
| dewey-sort | 3541.3724 |
| dewey-tens | 540 - Chemistry and allied sciences |
| discipline | Chemie / Pharmazie |
| format | Thesis Book |
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| isbn | 9783942109888 |
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| physical | III, 241 S. Ill., graph. Darst. |
| publishDate | 2011 |
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| spelling | Stella, Kevin 1984- Verfasser (DE-588)1018031499 aut Electronic dissipation processes during chemical reactions on surfaces Kevin Stella Hamburg Disserta Verl. 2011 III, 241 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Zugl.: Duisburg, Essen, Univ., Diss., 2011 Energieverlust (DE-588)4014735-6 gnd rswk-swf Elektrode (DE-588)4014247-4 gnd rswk-swf Oberflächenreaktion (DE-588)4140095-1 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Oberflächenreaktion (DE-588)4140095-1 s Elektrode (DE-588)4014247-4 s Energieverlust (DE-588)4014735-6 s DE-604 X:MVB text/html http://deposit.dnb.de/cgi-bin/dokserv?id=3885766&prov=M&dok_var=1&dok_ext=htm Inhaltstext DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=025125923&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Stella, Kevin 1984- Electronic dissipation processes during chemical reactions on surfaces Energieverlust (DE-588)4014735-6 gnd Elektrode (DE-588)4014247-4 gnd Oberflächenreaktion (DE-588)4140095-1 gnd |
| subject_GND | (DE-588)4014735-6 (DE-588)4014247-4 (DE-588)4140095-1 (DE-588)4113937-9 |
| title | Electronic dissipation processes during chemical reactions on surfaces |
| title_auth | Electronic dissipation processes during chemical reactions on surfaces |
| title_exact_search | Electronic dissipation processes during chemical reactions on surfaces |
| title_full | Electronic dissipation processes during chemical reactions on surfaces Kevin Stella |
| title_fullStr | Electronic dissipation processes during chemical reactions on surfaces Kevin Stella |
| title_full_unstemmed | Electronic dissipation processes during chemical reactions on surfaces Kevin Stella |
| title_short | Electronic dissipation processes during chemical reactions on surfaces |
| title_sort | electronic dissipation processes during chemical reactions on surfaces |
| topic | Energieverlust (DE-588)4014735-6 gnd Elektrode (DE-588)4014247-4 gnd Oberflächenreaktion (DE-588)4140095-1 gnd |
| topic_facet | Energieverlust Elektrode Oberflächenreaktion Hochschulschrift |
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