Oxide ultrathin films: science and technology
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| Format: | Book |
| Language: | English |
| Published: |
Weinheim
Wiley-VCH
2012
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| Subjects: | |
| Online Access: | Inhaltstext Inhaltsverzeichnis |
| Physical Description: | XVI, 352 S. Ill., graph. Darst. |
| ISBN: | 352733016X 9783527330164 9783527640171 |
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IMAGE 1
CONTENTS
PREFACE XI LIST OF CONTRIBUTORS XIII
1 SYNTHESIS AND PREPARATION OF OXIDE ULTRATHIN FILMS 1 SERGIO VALERI AND
STEFANIA BENEDETTI 1.1 INTRODUCTION 1
1.2 BASIC ASPECTS OF FABRICATION 3
1.3 PHYSICAL METHODS 7
1.3.1 CONTROLLED OXIDATION OF BULK SINGLE-CRYSTAL SURFACES 7 1.3.2
SPUTTERING AND ABLATION OF OXIDE TARGETS 8 1.3.2.1 SPUTTER DEPOSITION 8
1.3.2.2 PULSED LASER DEPOSITION 8 1.3.3 REACTIVE PHYSICAL VAPOR
DEPOSITION 9 1.3.3.1 FILM GROWTH BY SPUTTERING OR ABLATION OF PURE
TARGETS IN OXIDIZING
ATMOSPHERE 10
1.3.3.2 FILM GROWTH BY REACTIVE MBE 10 1.3.4 POST-OXIDATION OF
PRE-DEPOSITED THIN METAL FILMS 13 1.4 CHEMICAL METHODS 14
1.4.1 CHEMICAL VAPOR DEPOSITION 15 1.4.2 LIQUID-PRECURSOR-BASED
THIN-FILM DEPOSITION TECHNIQUES 16 1.5 OXIDE NANOSHEETS AND BURIED
LAYERS 19 1.5.1 EXFOLIATED AND DETACHABLE LAYERS 19
1.5.1.1 EXFOLIATED OXIDE NANOSHEETS 19 1.5.1.2 DETACHABLE ULTRATHIN
OXIDE FILMS 19 1.5.2 BURIED OXIDE LAYERS 20 1.6 CONCLUSIONS AND
PERSPECTIVES 21
2 CHARACTERIZATION TOOLS OF ULTRATHIN OXIDE FILMS 27 DAVID C. GRINTER
AND GEOFF THORNTON 2.1 INTRODUCTION 27
2.2 STRUCTURE DETERMINATION TECHNIQUES 28
BIBLIOGRAFISCHE INFORMATIONEN HTTP://D-NB.INFO/1012093905
DIGITALISIERT DURCH
IMAGE 2
VI CONTENTS
2.2.1 SCANNED PROBE MICROSCOPY 28
2.2.2 SCANNING TUNNELING MICROSCOPY 28 2.2.2.1 CASE STUDY: CEO 2
(LLL)/PT(LLL) 30 2.2.3 NONCONTACT ATOMIC FORCE MICROSCOPY 30 2.2.4 X-RAY
PHOTOEMISSION ELECTRON MICROSCOPY 31 2.2.4.1 CASE STUDY: IRON OXIDE ON
A-AL 2 O 3 (0001) 33 2.2.5 SURFACE X-RAY DIFFRACTION 33
2.2.5.1 CASE STUDY: OXIDATION OF RH(L 11) 34 2.2.6 PHOTOELECTRON
DIFFRACTION 35 2.2.6.1 CASE STUDY: VO LAYERS ON TIO 2 (110) 36 2.3
SPECTROSCOPIC TECHNIQUES 36
2.3.1 X-RAY MAGNETIC CIRCULAR/LINEAR DICHROISM 36 2.3.1.1 CASE STUDY: FE
3 _ 8 O 4 (LLL) ULTRATHIN FILMS ON PT(LLL) 38 2.3.1.2 CASE STUDY:
NIO/FEO(001) 39 2.3.2 MAGNETO-OPTICAL KERR EFFECT 40 2.3.2.1 CASE STUDY:
FE/NIO/MGO(001) AND FE/NIO/AG(001) 40 2.3.3 CONVERSION ELECTRON
MOESSBAUER SPECTROSCOPY 41 2.3.3.1 CASE STUDY: FE 3 O 4 (LLL)/PT(LLL) 43
2.4 SUMMARY 43
3 ORDERED OXIDE NANOSTRUCTURES ON METAL SURFACES 47 FALKO P. HETZER AND
SVETLOZAR SURNEV 3.1 INTRODUCTION 47
3.2 FABRICATION OF OXIDE NANOSTRUCTURES 48 3.3 NOVEL STRUCTURE CONCEPTS
49
3.4 DIMENSIONALITY ASPECTS: FROM TWO- TO ONE- TO ZERO-DIMENSIONAL
STRUCTURES 58 3.5 TRANSITION FROM TWO- TO THREE-DIMENSIONAL STRUCTURES:
GROWTH OF BULK STRUCTURES OUT OF INTERFACIAL LAYERS 63 3.6 SYNOPSIS 69
ACKNOWLEDGMENT 69
4 UNUSUAL PROPERTIES OF OXIDES AND OTHER INSULATORS IN THE ULTRATHIN
LIMIT 75 LIVIA GIORDANO AND GIANFRANCO PACCHIONI 4.1 INTRODUCTION 75
4.2 EVOLUTION OF BAND GAP WITH FILM THICKNESS 77 4.3 ELECTRONIC
TRANSPORT THROUGH OXIDE ULTRATHIN FILMS 79 4.4 WORK FUNCTION CHANGES
INDUCED BY OXIDE FILMS 85 4.5 NANOPOROSITY: OXIDE FILMS AS MOLECULAR AND
ATOMIC SIEVES 89 4.6 FLEXIBILITY OF OXIDE THIN FILMS AND POLARONIC
DISTORTION 94 4.7 CONCLUSIONS 97
ACKNOWLEDGMENTS 97
IMAGE 3
CONTENTS I VII
5 SILICA AND HIGH-K DIELECTRIC THIN FILMS IN
MICROELECTRONICS 101 GENNADI BERSUKER, KEITH MCKENNA, AND ALEXANDER
SHLUGER 5.1 INTRODUCTION 101
5.2 ELECTRICAL CHARACTERIZATION OF HIGH-FC DIELECTRICS ON SILICON 103
5.3 THEORETICAL MODELING OF GATE DIELECTRIC FILMS 104 5.3.1 AIMS OF
THEORETICAL MODELING 104
5.3.2 COMPUTATIONAL METHODS 105 5.4 MODELS OF THE STRUCTURE AND
PROPERTIES OF HFO2 GATE DIELECTRIC FILMS 106 5.4.1 OXYGEN-DEFICIENT
DEFECT CENTERS IN BULK HFO 2 106 5.4.2 SELF-TRAPPED POLARONS IN HFO 2
107 5.4.3 USING DOPING TO INCREASE THE K VALUE IN HFO 2 108
5.4.4 MODELING OF SI/SIO 2 /HFO 2 FILMS AND INTERFACES 109 5.5
POLYCRYSTALLINE GATE OXIDE FILMS 110 5.5.1 IMPACT OF POLYCRYSTALLINITY
ON MICROELECTRONIC DEVICE CHARACTERISTICS 110
5.5.2 STRUCTURE AND ELECTRONIC PROPERTIES OF GRAIN BOUNDARIES 112 5.5.3
DEFECT SEGREGATION AT GRAIN BOUNDARIES 113 5.6 CONCLUSIONS AND OUTLOOK
114
ACKNOWLEDGMENTS 115
6 OXIDE PASSIVE FILMS AND CORROSION PROTECTION 119 PHILIPPE MARCUS AND
VINCENT MAURICE 6.1 INTRODUCTION 119
6.2 ELECTROCHEMICAL FUNDAMENTALS OF PASSIVATION OF METALS 119 6.3
CHEMICAL COMPOSITION, CHEMICAL STATES, AND THICKNESS OF PASSIVE FILMS ON
METALS AND ALLOYS 122 6.3.1 COPPER, SILVER, NICKEL, IRON, AND CHROMIUM
122 6.3.2 STAINLESS STEELS 124
6.4 TWO-DIMENSIONAL OXIDE PASSIVE FILMS ON METALS 126 6.4.1 COPPER 126
6.4.2 SILVER 128
6.5 GROWTH AND NANOSTRUCRURE OF THREE-DIMENSIONAL ULTRATHIN OXIDE FILMS
130 6.5.1 CU(I) AND CU(I)/CU(II) PASSIVE FILMS 131 6.5.2 NI(II) PASSIVE
FILMS 133
6.5.3 FE(II)/FE(III) PASSIVE FILMS 135 6.5.4 AGING EFFECTS ON
CR(III)-RICH PASSIVE FILMS I36 6.6 CORROSION MODELING BY DFT 137 6.7
CONCLUSION 140
IMAGE 4
VIII I CONTENTS
7 OXIDE FILMS AS CATALYTIC MATERIALS AND MODELS OF REAL
CATALYSTS 145 HANS-JOACHIM FREUND
7.1 INTRODUCTION 145
7.2 OXIDE THIN FILMS GROWN AS SUPPORTS 146
7.3 SYSTEMS TO MODEL REAL CATALYSTS 154 7.3.1 SUPPORTED GOLD 154
7.3.2 OXIDES ON OXIDES: VANADIA NANOPARTICLES ON CERIA 163 7.4
ULTRATHIN-FILM CATALYSTS 166
7.5 SYNOPSIS 173
ACKNOWLEDGMENTS 174
8 OXIDE FILMS IN SPINTRONICS 181 RICCARDO BERTACCO AND FRANCO CICCACCI
8.1 INTRODUCTION 181
8.2 HISTORICAL NOTES 182
8.3 HALF-METALLIC MANGANITES: THE CASE OF LSMO 183 8.4 ELECTRIC CONTROL
OF MAGNETIZATION IN OXIDE HETEROSTRUCTURES 189 8.4.1 PROXIMITY AND
ELECTRIC FIELD EFFECTS ON MAGNETIC PROPERTIES
OF LSMO FILMS 189
8.4.2 MAGNETOELECTRIC COUPLING AT FE-BTO INTERFACES I96 8.5 CONCLUSIONS
AND PERSPECTIVES 197 ACKNOWLEDGMENTS 197
9 OXIDE ULTRATHIN FILMS FOR SOLID OXIDE FUEL CELLS 201 TATSUMI ISHIHARA
9.1 OVERVIEW OF SOLID OXIDE FUEL CELL TECHNOLOGY 201 9.2 PREPARATION OF
OXIDE ION CONDUCTOR THIN FILMS 203 9.3 NANO SIZE EFFECTS ON OXIDE ION
CONDUCTOR FILMS 206 9.4 POWER GENERATING PROPERTY OF SOFCS USING LAGAO 3
THIN
FILMS 208
9.5 DEVELOPMENT OF /I-SOFCS 216
9.6 CONCLUDING REMARKS 217
10 TRANSPARENT CONDUCTING AND CHROMOGENIC OXIDE FILMS AS SOLAR ENERGY
MATERIALS 221 CLAES-GOERAN GRANQVIST 10.1 INTRODUCTION 221
10.2 TRANSPARENT INFRARED REFLECTORS AND TRANSPARENT ELECTRICAL
CONDUCTORS 223 10.2.1 OVERVIEW 223 10.2.2 COMPUTED OPTICAL DATA FOR ITO
FILMS 225 10.2.3 ALTERNATIVE TRANSPARENT CONDUCTORS 226
IMAGE 5
CONTENTS IX
10.3 THERMOCHROMICS 228
10.3.1 OVERVIEW 228 10.3.2 VO 2 FILMS AND NANOPARTIDES: HOW TO IMPROVE
THE MODULATION OFT SOL 229
10.3.3 MAGNESIUM DOPING OF VO 2 : HOW TO ENHANCE TI UM 231 10.4
ELECTROCHROMICS 232 10.4.1 OVERVIEW 232 10.4.2 NANOSTRUCTURAL FEATURES:
A CLOSER LOOK AT EC FILMS 233 10.4.3 EC FOILS BY ROLL-TO-ROLL
MANUFACTURING: SOME INITIAL RESULTS 234 10.5 SUMMARY AND CONCLUDING
REMARKS 235
11 OXIDE ULTRATHIN FILMS IN SENSOR APPLICATIONS 239 ELISE BRUNEI,
GIORGIO C. MUTINATI, STEPHAN STEINHAUER, AND ANTON KB'CK 11.1
INTRODUCTION 239
11.2 SENSOR APPLICATIONS 241 11.2.1 MAGNETIC SENSORS 243 11.2.2
PHOTODETECTORS AND DETECTORS FOR THE (F)IR REGION 246 11.2.3
ELECTROCHEMICAL SENSORS 246 11.2.4 GAS SENSORS 247 11.2.4.1 OPTICAL GAS
SENSORS 248 11.2.4.2 MASS-SENSITIVE GAS SENSORS 249 11.2.4.3 ELECTRICAL
GAS SENSORS 250 11.3 SNO 2 -BASED GAS SENSORS 254 11.3.1 SENSOR
FABRICATION 254 11.3.2 SENSOR PERFORMANCE 255 11.4 CONCLUSION 258
12 FERROELECTRICITY IN ULTRATHIN-FILM CAPACITORS 265 CELINE
LICHTENSTEIGER, PAVLO ZUBKO, MASSIMILIANO STENGEL, PABLO AGUADO- PUENTE,
JEAN-MARC TRISCONE, PHILIPPE GHOSEZ, AND JAVIERJUNQUERA 12.1
INTRODUCTION 265
12.2 FERROELECTRICITY: BASIC DEFINITIONS 266 12.3 THEORETICAL METHODS
FOR THE STUDY OF BULK FERROELECTRIC MATERIALS 269 12.3.1
DEVONSHIRE-GINZBURG-LANDAU PHENOMENOLOGICAL THEORY 269 12.3.2
FIRST-PRINCIPLES SIMULATIONS 270
12.3.3 SECOND-PRINCIPLES METHODS: MODEL HAMILTONIANS AND SHELL MODELS
272 12.4 MODELING FERROELECTRICITY IN OXIDES 274 12.5 THEORY OF
FERROELECTRIC THIN FILMS 277 12.5.1 MECHANICAL BOUNDARY CONDITIONS:
STRAIN 277
12.5.2 ELECTRICAL BOUNDARY CONDITIONS: IMPERFECT SCREENING 280 12.5.3
ELECTRICAL FUNCTIONALS WITH A DEPOLARIZATION FIELD 284 12.5.4 CHEMICAL
BONDING CONTRIBUTIONS TO ELECTRICAL BOUNDARY CONDITIONS 285
IMAGE 6
CONTENTS
12.6 POLARIZATION DOMAINS AND DOMAIN WALLS 287
12.6.1 KITTEL LAW 287
12.6.2 DOMAIN MORPHOLOGY 289 12.6.3 DOMAIN WALLS 290 12.7 ARTIFICIALLY
LAYERED FERROELECTRICS 291
12.7.1 ELECTROSTATIC COUPLING 291 12.7.2 ENGINEERING FERROELECTRICITY AT
INTERFACES 294 12.8 CONCLUSION AND PERSPECTIVES 296
13 TITANIA THIN FILMS IN BIOCOMPATIBLE MATAIS AND MEDICAL IMPLANTS 309
FABIO VARIOLA AND ANTONIO NANCI 13.1 THE ADVENT OF TITANIUM-BASED
MATERIALS 309 13.2 BIOLOGICALLY RELEVANT PHYSICOCHEMICAL PROPERTIES OF
NATIVE
TITANIA THIN FILMS 310 13.3 STRATEGIES FOR MODIFICATION OF THE SURFACE
OXIDE LAYER 311 13.3.1 CHEMICAL METHODS 312 13.3.1.1 OXIDE GROWTH MODELS
FOR OXIDATIVE TREATMENTS 313 13.3.1.2 DOPING OF OXIDE LAYERS WITH
BIOACTIVE ELEMENTS 314 13.3.2 PHYSICAL METHODS 315 13.3.3 BIOCHEMICAL
FUNCTIONALIZATION 315 13.4 BIOLOGICAL SURFACE SCIENCE 316 13.5
BIOLOGICAL RESPONSE TO SURFACE OXIDE LAYERS 317 13.5.1 PROTEIN
ADSORPTION 317 13.5.2 IN VITRO STUDIES 317
13.5.3 IN VIVO AND CLINICAL STUDIES 319 13.5.4 ANTIBACTERIAL CAPACITY
320 13.6 SLOW RELEASE CAPACITY OF NANOPOROUS TITANIUM OXIDE LAYERS 321
13.7 CONCLUSION AND PERSPECTIVES 322
ACKNOWLEDGMENTS 324
14 OXIDE NANOWIRES FOR NEW CHEMICAL SENSOR DEVICES 329 ALBERTO VOMIERO,
ELISABETTA COMINI, AND GIORGIO SBERVEGLIERI 14.1 OUTLINE 329
14.2 INTRODUCTION 329
14.3 SYNTHESIS 331
14.4 INTEGRATION 334
14.5 METAL OXIDE CHEMICAL SENSORS 335 14.6 CONDUCTOMETRIC SENSORS 336
14.7 OPTICAL SENSORS 340
INDEX 345 |
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| id | DE-604.BV039885879 |
| illustrated | Illustrated |
| indexdate | 2024-07-21T00:24:24Z |
| institution | BVB |
| isbn | 352733016X 9783527330164 9783527640171 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-024745003 |
| oclc_num | 768068334 |
| open_access_boolean | |
| owner | DE-703 DE-20 DE-11 |
| owner_facet | DE-703 DE-20 DE-11 |
| physical | XVI, 352 S. Ill., graph. Darst. |
| publishDate | 2012 |
| publishDateSearch | 2012 |
| publishDateSort | 2012 |
| publisher | Wiley-VCH |
| record_format | marc |
| spelling | Oxide ultrathin films science and technology ed. by Gianfranco Pacchioni ... Weinheim Wiley-VCH 2012 XVI, 352 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Dünne Schicht (DE-588)4136925-7 gnd rswk-swf Metalloxide (DE-588)4169619-0 gnd rswk-swf (DE-588)4143413-4 Aufsatzsammlung gnd-content Metalloxide (DE-588)4169619-0 s Dünne Schicht (DE-588)4136925-7 s DE-604 Pacchioni, Gianfranco 1954- (DE-588)172299640 edt Erscheint auch als Online-Ausgabe, EPUB 978-3-527-64018-8 Erscheint auch als Online-Ausgabe, MOBI 978-3-527-64020-1 Erscheint auch als Online-Ausgabe, PDF 978-3-527-64019-5 X:MVB text/html http://deposit.dnb.de/cgi-bin/dokserv?id=3830301&prov=M&dok_var=1&dok_ext=htm Inhaltstext DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=024745003&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Oxide ultrathin films science and technology Dünne Schicht (DE-588)4136925-7 gnd Metalloxide (DE-588)4169619-0 gnd |
| subject_GND | (DE-588)4136925-7 (DE-588)4169619-0 (DE-588)4143413-4 |
| title | Oxide ultrathin films science and technology |
| title_auth | Oxide ultrathin films science and technology |
| title_exact_search | Oxide ultrathin films science and technology |
| title_full | Oxide ultrathin films science and technology ed. by Gianfranco Pacchioni ... |
| title_fullStr | Oxide ultrathin films science and technology ed. by Gianfranco Pacchioni ... |
| title_full_unstemmed | Oxide ultrathin films science and technology ed. by Gianfranco Pacchioni ... |
| title_short | Oxide ultrathin films |
| title_sort | oxide ultrathin films science and technology |
| title_sub | science and technology |
| topic | Dünne Schicht (DE-588)4136925-7 gnd Metalloxide (DE-588)4169619-0 gnd |
| topic_facet | Dünne Schicht Metalloxide Aufsatzsammlung |
| url | http://deposit.dnb.de/cgi-bin/dokserv?id=3830301&prov=M&dok_var=1&dok_ext=htm http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=024745003&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT pacchionigianfranco oxideultrathinfilmsscienceandtechnology |