Homogeneous catalysis with metal complexes: fundamentals and applications
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| Main Author: | |
|---|---|
| Format: | Book |
| Language: | English |
| Published: |
Berlin [u.a.]
Springer
2012
|
| Series: | Springer series in chemical physics
102 |
| Subjects: | |
| Online Access: | Inhaltstext Inhaltsverzeichnis |
| Physical Description: | XII, 478 S. graph. Darst. 235 mm x 155 mm |
| ISBN: | 3642246281 9783642246289 |
Staff View
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Record in the Search Index
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IMAGE 1
CONTENTS
1 INTRODUCTION 1
1.1 TYPES O F HOMOGENEOUS CATALYSIS WITH METAL COMPLEXES, THEIR
ADVANTAGES AND DRAWBACKS 1
1.2 PERSPECTIVES OF THE INDUSTRIAL USE OF HOMOGENEOUS CATALYSIS WITH
METAL COMPLEXES 5
REFERENCES 9
2 HOMOGENEOUS REDOX CATALYSIS WITH TRANSITION METAL COMPOUNDS IN OXIDE
AND PEROXIDE SYSTEMS 11
2.1 GENERAL PRINCIPLES O F CATALYTIC REDOX REACTIONS WITH METAL
COMPOUNDS 11
2.2 INTERMEDIATE COMPOUNDS, O2 MOLECULE ACTIVATION, AND FREE RADICALS IN
THE CATALYSIS OF OXIDATION PROCESSES 17
2.2 .1 NATURE O F FORMING INTERMEDIATE COMPOUNDS 17
2.2.2 OXYGEN MOLECULE ACTIVATION: INTERMEDIATE SPECIES, AND FREE
RADICALS 2 0
2.2.3 PEROXOCOMPLEXES O F SOME METALS 4 3
2.3 THEORETICAL ASPECTS OF CATALYSIS WITH METAL COMPLEXES 4 6
2.3.1 INFLUENCE O F COMPLEX FORMATION ON METAL ION REACTIVITY AND
CATALYTIC PROCESSES MECHANISMS (ROLE OF COORDINATION IN CATALYSIS) 4 6
2.3.2 QUALITATIVE MODEL O F THE THEORY O F PCT COMPLEXES 51
2.4 GENERAL PRINCIPLES O F REDOX CATALYSIS MECHANISMS DETERMINATION 54
2.4.1 POSSIBLE MECHANISMS O F CATALYTIC REDOX SYSTEMS F E Z + U Q - H 2
O 2 AND F E Z + L N - H 2 O 2 5 4
2.4.2 STAGES O F REVEALING CATALYTIC REDOX REACTIONS MECHANISM (METHODIC
ASPECT 2 ) 62
I X
HTTP://D-NB.INFO/1014977096
IMAGE 2
X
C O N T E N T S
2.5 MECHANISMS O F OXIDE AND PEROXIDE SYSTEMS REDOX
TRANSFORMATIONS CATALYSIS WITH TRANSITION METAL COMPOUNDS 75 2.5.1
MECHANISMS OF O2 TRANSFORMATION IN OXIDE CATALYTIC SYSTEMS 75
2.5.2 MECHANISMS O F H2O2 DECOMPOSITION IN THE PEROXIDE CATALYTIC
SYSTEMS 80
2.6 MECHANISMS OF ORGANIC SUBSTRATES (S) OXIDATION IN OXIDE AND PEROXIDE
SYSTEMS 91
2.6.1 MECHANISMS OF ORGANIC SUBSTRATES OXIDATION BY OXYGEN [SYSTEMS M Z
+ ( M Z + L N )-O2- S] 91
2.6.2 MECHANISMS O F ORGANIC SUBSTRATE'S OXIDATION BY HYDROGEN PEROXIDE
[SYSTEMS M Z + { M Z + L N ) ~ H 2 0 2 - S ) 9 6
2.7 FERRYL PARTICLES IN THE CATALYSIS O F OXIDATION PROCESSES 105
2.7.1 EXPERIMENTAL CONFIRMATION O F FERRYL PARTICLES FORMATION. 105
2.7.2 QUANTUM-CHEMICAL METHODS O F FERRYL (MANGANYL) PARTICLES FORMATION
STUDY 107
REFERENCES 113
3 BIOCHEMICAL PROCESSES AND METAL COMPLEXES'ROLE AS CATALYSTS 123 3.1
CATALYTIC INFLUENCE O F TRANSITION METAL COMPOUNDS ON BIOLOGICAL
PROCESSES 123
3.1.1 ROLE O F TRANSITION METAL IONS IN BIOLOGICAL SYSTEMS 124
3.1.2 CATALYTIC REACTIONS IN THE INITIATION OF LIPID PEROXIDATION .
128 3.1.3 LIGANDS INFLUENCE O F HABER-WEISS REACTION 133
3.1.4 TOXICITY O F O2 REDUCED FORMS WITH REGARD TO BIOLOGICAL SYSTEMS
AND METHODS O F PROTECTION 136
3.1.5 ROLE O F BLEOMYCIN AND ITS MODELS IN DNA DETERIORATION. 142
3.1.6 INTERMEDIATES OF FERRYL PARTICLES TYPE IN BIOCHEMICAL SYSTEMS 155
3.2 ENZYMES AND THEIR MODELING 161
3.2.1 MECHANISMS O F SOME ENZYMES' FUNCTIONING AND THEIR MODELING:
MODELING O F MONOOXIDASES IN ALKANES, ALKENES, AND OTHER SUBSTRATES
HYDROXYLATION AND EPOXIDATION 161
3.2.2 DOPAMINE/J-HYDROXYLASE AND ITS MODELS 203
3.2.3 MODEL SYSTEMS O F DIOXYGENASES 206
3.2.4 MODEL SYSTEMS OF CATALASE 212
3.2.5 PEROXIDASES AND THEIR MODEL SYSTEMS 219
3.2.6 SUPEROXIDE DISMUTASE AND ITS MODELS 231
3.2.7 MODELS OF OXIDASES (LACCASE, CYTOCHROME C, AND GALACTOSE OXIDASE)
236
REFERENCES 244
IMAGE 3
CONTENTS XI
4 CATALYTIC PROCESSES AND HUMAN DISEASES 261
4.1 CATALYTIC FREE RADICAL PROCESSES IN VIVO AND TOXICITY O F OXYGEN
REDUCTION PRODUCTS 261
4.2 STRESS AND CATALYTIC PROCESSES 267
4.3 INFLAMMATORY PROCESSES AND ROLE O F METAL COMPOUNDS 279
4.4 ROLE OF ENZYMES AND METAL COMPOUNDS IN PHAGOCYTOSIS 284
4.5 METAL-CATALYZED OXIDATION AND AGEING 289
4.5.1 OXIDATIVE DAMAGE O F PROTEINS AND ENZYMES, AND AGEING 289 4.5.2
MITOCHONDRIA DAMAGE WITH FREE RADICALS AND AGEING 292 4.5.3 MECHANISM O
F LIPOFUSCIN FORMATION AND AGEING 294
4.5.4 THE ROLE O F ANTIOXIDANT ENZYMES AND SUBSTANCES IN CELLULAR AGEING
295
4.6 DISEASES O F JOINTS AND TISSUES AND CATALYTIC FREE RADICAL PROCESSES
299
4.7 CATALYTIC AND RADICAL PROCESSES ON ATHEROSCLEROSIS AND MYOCARDIAL
ISCHEMIA 301
4.7.1 CATALYTIC AND RADICAL PROCESSES ON ATHEROSCLEROSIS 301
4.7.2 MYOCARDIAL DETERIORATIONS AND CATALYTIC PROCESSES WITH FREE
RADICALS FORMATION 307
REFERENCES 310
5 CATALYTIC OXIDATION O F OXYACIDS AND NATURAL POLYPHENOLS 319
5.1 METABOLIC CYCLES O F TRI-AND DICARBONIC ACIDS 319
5.2 CATALYTIC PROCESSES O F DICARBONIC ACIDS O F BAROUD CYCLE
TRANSFORMATIONS 322
5.2.1 CATALYTIC PROCESSES O F BAROUD CYCLE OXYACIDS TRANSFORMATIONS 322
5.2.2 GENERAL REGULARITIES O F THE REDUCTION-OXIDATION CONVERSIONS OF
THE BAROUD CYCLE OXYACIDS 338
5.3 CATALYTIC TRANSFORMATIONS O F NATURAL POLYPHENOLS 341
5.3.1 ROLE O F NATURAL POLYPHENOLS AND THEIR CATALYTIC OXIDATIVE
TRANSFORMATIONS 341
5.3.2 CATALYSIS OF CATECHINS OXIDATION WITH OXYGEN AND HYDROGEN PEROXIDE
IN THE PRESENCE OF F E 3 + AND F E 2 + IONS 342
REFERENCES 347
6 CATALYTIC PROCESSES IN ECOLOGICAL CHEMISTRY 351
6.1 ECOLOGICAL CHEMISTRY AND CATALYSIS WITH METAL COMPLEXES 351 6.2
CATALYTIC PROCESSES IN THE ATMOSPHERE AND ACID RAIN FORMATION 355 6.3
CATALYTIC REDOX PROCESSES IN NATURAL WATER AND ITS SELF-PURIFICATION 369
6.3.1 MAIN SOURCES O F H 2 0 2 , OH*" AND 0 * ~ ( H 0 * ) RADICALS
FORMATION IN NATURAL WATER 369
6.3.2 H2O2 AND O2 ACTIVATION IN NATURAL WATER AND THE ROLE O F METAL
COMPOUNDS 374
IMAGE 4
XII C O N T E N T S
6.3.3 PHOTOCATALYTIC TRANSFORMATION OF NITROGEN
MINERAL FORMS IN WATER 381
6.3.4 PHOTOCATALYTIC TRANSFORMATIONS O F ANTHROPOGENIC ORGANIC
POLLUTANTS IN WATER COMPARTMENTS 387
6.3.5 MODELING O F POLLUTANT TRANSFORMATION AND SELF-PURIFICATION
CAPACITY O F NATURAL WATER 390
6.4 WASTEWATER TREATMENT AND CATALYTIC PROCESSES 396
6.4.1 PRINCIPLES OF CATALYTIC WASTEWATER TREATMENT 396
6.4.2 COMBINED REDOX-PHOTOCATALYTIC PROCESSES 401
6.5 CATALYMETRY OF ENVIRONMENTAL OBJECTS 408
REFERENCES 415
7 HOMOGENEOUS CATALYSIS WITH METAL COMPLEXES IN THE CHEMICAL INDUSTRY
AND FOODSTUFFS CHEMISTRY 423
7.1 CATALYTIC PROCESSES IN THE CHEMICAL INDUSTRY 423
7.1.1 CATALYTIC OXIDATION OF ORGANIC COMPOUNDS IN MODEL SYSTEMS AND
THEIR POSSIBLE INDUSTRIAL APPLICATIONS 423
7.1.2 CATALYTIC HYDROXYLATION AND EPOXIDATION IN INDUSTRIAL PROCESSES
426
7.1.3 MECHANISMS OF SOME INDUSTRIAL CATALYTIC PROCESSES 434
7.2 FOODSTUFFS CHEMISTRY AND CATALYSIS 438
7.2.1 CATALYTIC LIPIDS PEROXIDATION IN FOODSTUFFS 438
7.2.2 DISTRIBUTION OF IRON COMPOUNDS IN FOODSTUFFS AND THEIR INFLUENCE
ON LIPIDS PEROXIDATION 446
7.2.3 ROLE OF ANTIOXIDANTS IN FOODSTUFFS PRESERVATION 449
7.3 REDOX CATALYTIC PROCESSES IN WINE-MAKING 454
7.3.1 REDOX CATALYTIC NON-ENZYMATIC PROCESSES DURING WINE MATURING AND
AGEING 454
7.3.2 METHODS OF WINE STABILIZATION AND IMPROVING O F ITS ORGANOLEPTIC
PROPERTIES 457
REFERENCES 461
INDEX 467 |
| any_adam_object | 1 |
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| discipline | Chemie / Pharmazie Physik Chemie Chemie-Ingenieurwesen |
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| indexdate | 2024-07-21T00:15:53Z |
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| isbn | 3642246281 9783642246289 |
| language | English |
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| publishDate | 2012 |
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| series2 | Springer series in chemical physics |
| spelling | Duca, Gheorghe 1952- Verfasser (DE-588)138810117 aut Homogeneous catalysis with metal complexes fundamentals and applications Gheorghe Duca Berlin [u.a.] Springer 2012 XII, 478 S. graph. Darst. 235 mm x 155 mm txt rdacontent n rdamedia nc rdacarrier Springer series in chemical physics 102 Homogene Katalyse (DE-588)4160579-2 gnd rswk-swf Übergangsmetallkomplexe (DE-588)4131837-7 gnd rswk-swf (DE-588)4143413-4 Aufsatzsammlung gnd-content Übergangsmetallkomplexe (DE-588)4131837-7 s Homogene Katalyse (DE-588)4160579-2 s DE-604 Erscheint auch als Online-Ausgabe 978-3-642-24629-6 Springer series in chemical physics 102 (DE-604)BV000000670 102 X:MVB text/html http://deposit.dnb.de/cgi-bin/dokserv?id=3876231&prov=M&dok_var=1&dok_ext=htm Inhaltstext DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=024550834&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Duca, Gheorghe 1952- Homogeneous catalysis with metal complexes fundamentals and applications Springer series in chemical physics Homogene Katalyse (DE-588)4160579-2 gnd Übergangsmetallkomplexe (DE-588)4131837-7 gnd |
| subject_GND | (DE-588)4160579-2 (DE-588)4131837-7 (DE-588)4143413-4 |
| title | Homogeneous catalysis with metal complexes fundamentals and applications |
| title_auth | Homogeneous catalysis with metal complexes fundamentals and applications |
| title_exact_search | Homogeneous catalysis with metal complexes fundamentals and applications |
| title_full | Homogeneous catalysis with metal complexes fundamentals and applications Gheorghe Duca |
| title_fullStr | Homogeneous catalysis with metal complexes fundamentals and applications Gheorghe Duca |
| title_full_unstemmed | Homogeneous catalysis with metal complexes fundamentals and applications Gheorghe Duca |
| title_short | Homogeneous catalysis with metal complexes |
| title_sort | homogeneous catalysis with metal complexes fundamentals and applications |
| title_sub | fundamentals and applications |
| topic | Homogene Katalyse (DE-588)4160579-2 gnd Übergangsmetallkomplexe (DE-588)4131837-7 gnd |
| topic_facet | Homogene Katalyse Übergangsmetallkomplexe Aufsatzsammlung |
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