Metal-organic frameworks: applications from catalysis to gas storage
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| Format: | Book |
| Language: | English |
| Published: |
Weinheim
Wiley-VCH
2011
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| Subjects: | |
| Online Access: | Inhaltstext Inhaltsverzeichnis |
| Physical Description: | XXII, 392 S. Ill., graph. Darst. |
| ISBN: | 9783527328703 352732870X |
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IMAGE 1
CONTENTS
PREFACE XV LIST OF CONTRIBUTORS XIX
PART ONE DESIGN OF MULTIFUNCTIONAL POROUS MOFS 1
1 DESIGN OF POROUS COORDINATION POLYMERS/METAL-ORGANIC FRAMEWORKS: PAST,
PRESENT AND FUTURE 3 SATOSHI HORIKE AND SUSUMU KITAGAWA 1.1 INTRODUCTION
3
1.2 BACKGROUND AND ONGOING CHEMISTRY OF POROUS COORDINATION POLYMERS 3
1.2.1 FRAMEWORKS WITH HIGH SURFACE AREA 5 1.2.2 LEWIS ACIDIC FRAMEWORKS
6 1.2.3 SOFT POROUS CRYSTALS 8
1.3 MULTIFUNCTIONAL FRAMEWORKS 10 1.3.1 POROSITY AND MAGNETISM 10 1.3.2
POROSITY AND CONDUCTIVITY/DIELECTRICITY 12 1.3.3 POROUS FLEXIBILITY AND
CATALYSIS 12
1.4 PREPARATION OF MULTIFUNCTIONAL FRAMEWORKS 13 1.4.1 MIXED LIGANDS AND
MIXED METALS 13 1.4.2 CORE-SHELL 16
1.4.3 PCPS AND NANOPARTIDES 17 1.5 PERSPECTIVES 18
REFERENCES 19
2 DESIGN OF FUNCTIONAL METAL-ORGANIC FRAMEWORKS BY POST-SYNTHETIC
MODIFICATION 23 DAVID FARRUSSENG, JEROME CANIVET, AND ALESSANDRA
QUADRELLI
2.1 BUILDING A MOFS TOOLBOX BY POST-SYNTHETIC MODIFICATION 23 2.1.1
TAKING ADVANTAGE OF IMMOBILIZATION IN A POROUS SOLID 23 2.1.2 UNIQUE
REACTIVITY OF MOFS 24 2.2 POST-FUNCTIONALIZATION OF MOFS BY HOST-GUEST
INTERACTIONS 26
BIBLIOGRAFISCHE INFORMATIONEN HTTP://D-NB.INFO/1010591738
DIGITALISIERT DURCH
IMAGE 2
VIII CONTENTS
5.6.4 MOFS FOR POST-COMBUSTION CO 2 CAPTURE 113
5.7 CONCLUSIONS 116
REFERENCES 116
6 MANUFACTURE OF MOF THIN FILMS ON STRUCTURED SUPPORTS FOR SEPARATION
AND CATALYSIS 121 SONIA AGUADO AND DAVID FARRUSSENG
6.1 ADVANTAGES AND LIMITATIONS OF MEMBRANE TECHNOLOGIES FOR GAS AND
LIQUID SEPARATION 121 6.2 MECHANISM OF MASS TRANSPORT AND SEPARATION 123
6.3 SYNTHESIS OF MOLECULAR SIEVE MEMBRANES 127 6.3.1 SYNTHESIS OF
ZEOLITE MEMBRANES 127 6.3.1.1 DIRECT NUDEATION-GROWTH ON THE SUPPORT 128
6.3.1.2 SECONDARY GROWTH 129 6.3.2 PREPARATION OF MOF MEMBRANESAND FILMS
129 6.3.2.1 SELF-ASSEMBLED LAYERS 130 6.3.2.2 SOLVOTHERMAL SYNTHESIS:
DIRECT AND SECONDARY GROWTH 131
6.4 APPLICATION OF MOF MEMBRANES 137 6.4.1 GAS SEPARATION 137
6.4.1.1 METAL CARBOXYLATE-BASED MEMBRANES 137 6.4.1.2 ZINC
IMIDAZOLATE-BASED MEMBRANES 138 6.4.2 SHAPED STRUCTURED REACTORS 141
6.4.3 PERSPECTIVES FOR FUTURE APPLICATIONS 143 6.5 LIMITATIONS 143
6.6 CONDUSIONS AND OUTLOOK 246
REFERENCES 147
7 RESEARCH STATUS OF METAL-ORGANIC FRAMEWORKS FOR ON-BOARD
CRYO-ADSORPTIVE HYDROGEN STORAGE APPLICATIONS 151 ANNE DAILLY 7.1
INTRODUCTION - RESEARCH PROBLEM AND SIGNIFICANCE 151
7.1.1 CHALLENGES IN HYDROGEN STORAGE TECHNOLOGIES FOR HYDROGEN FUEL CELL
VEHIDES 151 7.1.2 CURRENT STATUS OF HYDROGEN STORAGE OPTIONS AND R&D FOR
THE FUTURE 152 7.2 MOFS AS ADSORPTIVE HYDROGEN STORAGE OPTIONS 154 7.3
EXPERIMENTAL TEDINIQUES AND METHODS FOR PERFORMANCE
AND THERMODYNAMIC ASSESSMENT OF POROUS MOFS FOR HYDROGEN STORAGE 256 7.4
MATERIAL RESEARCH RESULTS 259
7.4.1 STRUCTURE-HYDROGEN STORAGE PROPERTIES CORRELATIONS 159 7.4.2
NATURE OF THE ADSORBED HYDROGEN PHASE 162 7.5 FROM LABORATORY-SCALE
MATERIALS TO ENGINEERING 165 7.6 CONDUSION 267
REFERENCES 268
IMAGE 3
CONTENTS IX
PART THREE BULK CHEMISTRY APPLICATIONS 272
8 SEPARATION OF XYLENE ISOMERS 273 JOERI FM DENAYER, DIRK DE VOS, AND
PHILIBERT LEFLAIVE 8.1 XYLENE SEPARATION: INDUSTRIAL PROCESSES,
ADSORBENTS, AND SEPARATION PRINCIPLES 173 8.2 PROPERTIES OF MOFS VERSUS
ZEOLITES IN XYLENE SEPARATIONS 276 8.3 SEPARATION OF XYLENES USING
MIL-47 AND MIL-53 278
8.3.1 LOW-COVERAGE GAS-PHASE ADSORPTION PROPERTIES 179 8.3.2 MOLECULAR
PACKING 280 8.3.3 SEPARATION OF XYLENE-MIXTURES 284 8.4 CONDUSIONS 285
REFERENCES 287
9 METAL-ORGANIC FRAMEWORKS AS CATALYSTS FOR ORGANIC REACTIONS 292 LIK
HONG WEE, LUC ALAERTS, JOHAN A. MARTENS, AND DIRK DE VOS 9.1
INTRODUCTION 292
9.2 MOFS WITH CATALYTICALLY ACTIVE METAL NODES IN THE FRAMEWORK 2 92
9.2.1 TRANSITION METAL NODES 292 9.2.2 COORDINATIVELY UNSATURATED METAL
NODES 294 9.3 CATALYTIC FUNCTIONAH'ZATION OF ORGANIC FRAMEWORK LINKERS
295 9.3.1 PORPHYRIN FUNCTIONAL GROUPS 195 9.3.2 AMINE AND AMIDE
FUNCTIONS INCORPORATED VIA GRAFTING 296
9.4 HOMOCHIRAL MOFS 298
9.4.1 MOFS WITH INTRINSIC CHIRALITY 198 9.4.2 CHIRAL ORGANIC CATALYTIC
FUNCTIONS 299 9.4.3 METALLOLIGANDS 200 9.5 MOF-ENCAPSULATED
CATALYTICALLY ACTIVE GUESTS 201 9.5.1 POLYOXOMETALATES (POMS) 201 9.5.2
METALLOPORPHYRINS 203 9.5.3 METAL NANOPARTIDES 204 9.6 MESOPOROUS MOFS
206
9.7 CONDUSIONS 209
REFERENCES 220
PART FOUR MEDICAL APPLICATIONS 223
10 BIOMEDICAL APPLICATIONS OF METAL-ORGANIC FRAMEWORKS 225 PATRICIA
HORCAJADA, CHRISTIAN SERRE, ALISTAIR C. MCKINLAY, AND RUSSELL E. MORRIS
10.1 INTRODUCTION 215
10.2 MOFS FOR BIOAPPLICATIONS 216 10.2.1 CHOOSING THE RIGHT COMPOSITION
216 10.2.2 THE ROLE OF FLEXIBILITY 227 10.2.3 THE ROLE OF
FUNCTIONALIZATION 219
IMAGE 4
XIII CONTENTS
13.5.4
13.5.5 13.5.6 13.5.7
13.6
LIQUID-PHASE EPITAXY 325 TOWARD HETEROEPITAXIAL GROWTH OF MULTIPLE MOF
LAYERS 328 GROWTH OF MOF FILMS IN CONFINED SPACES 329
COMPARISON OF THE DIFFERENT METHODS FOR MOF THIN FILM GROWTH 331
CONDUSIONS AND PERSPECTIVES 332
REFERENCES 332
PART SIX LARGE-SCALE SYNTHESIS AND SHAPING OF MOFS 337
14 INDUSTRIAL MOF SYNTHESIS 339 ALEXANDER CZAJA, EMI LEUNG, NATALIA
TRUKHAN, AND ULRICH MUELLER 14.1 INTRODUCTION 339
14.2 RAW MATERIALS 340
14.2.1 METAL SOURCES 340 14.2.2 LINKERS 340
14.3 SYNTHESIS 343
14.3.1 HYDROTHERMAL SYNTHESIS 344 14.3.2 ELECTROCHEMICAL SYNTHESIS 345
14.4 SHAPING 347
14.5 APPLICATIONS 349
14.5.1 NATURAL GAS STORAGE FOR AUTOMOBILE APPLICATIONS 349 14.5.2
ETHYLENE ADSORPTION FOR FOOD STORAGE 350 14.6 CONDUSION AND OUTLOOK 351
REFERENCES 352
15 MOF SHAPING AND IMMOBILIZATION 353 BERTRAM BOEHRINGER, ROLAND FISCHER,
MARTIN R. LOHE, MARCUS ROSE, STEFAN KASKEL, AND PIA KUESGENS 15.1
INTRODUCTION 353
15.2 MOF@FIBER COMPOSITE MATERIALS 354 15.2.1 MOF-CONTAINING PAPER
SHEETS 354 15.2.2 MOF@PULP FIBERS 355 15.2.3 ELECTROSPINNING OF
MOF@POLYMER
COMPOSITE FIBERS 356 15.2.4 MOF FIXATION IN TEXTILE STRUCTURES 359
15.2.4.1 PRETREATMENT 360 15.2.4.2 WET PARTIDE INSERTION 362 15.2.4.3
DRY PARTIDE INSERTION 363 15.3 REQUIREMENTS OF ADSORBENTS FOR INDIVIDUAL
PROTECTION 367 15.3.1 RELEVANT PROTECTIVE CLOTHING APPLICATIONS 367
15.3.2 FILTER PERFORMANCE 368 15.3.3 TESTING THE CHEMICAL PROTECTION
PERFORMANCE OF FILTERS 371 15.3.4 CONCEPTS FOR APPLICATION 373 15.4 MOFS
IN MONOLITHIC STRUCTURES 373
IMAGE 5
CONTENTS XIII
15.4.1 15.4.2 15.4.3
MOF@POLYMERIC BEADS EXTRUDED MOF BODIES MONOLITHIC MOF GELS REFERENCES
379
INDEX 383
374
374 375 |
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| spelling | Metal-organic frameworks applications from catalysis to gas storage ed. by David Farrusseng Weinheim Wiley-VCH 2011 XXII, 392 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Metallorganisches Netzwerk (DE-588)7755315-9 gnd rswk-swf Polymerkomplexe (DE-588)4137334-0 gnd rswk-swf Nanoporöser Stoff (DE-588)4800345-1 gnd rswk-swf (DE-588)4143413-4 Aufsatzsammlung gnd-content Metallorganisches Netzwerk (DE-588)7755315-9 s DE-604 Polymerkomplexe (DE-588)4137334-0 s Nanoporöser Stoff (DE-588)4800345-1 s Farrusseng, David (DE-588)1014076870 edt X:MVB text/html http://deposit.dnb.de/cgi-bin/dokserv?id=3702197&prov=M&dok%5Fvar=1&dok%5Fext=htm Inhaltstext DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=024375712&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Metal-organic frameworks applications from catalysis to gas storage Metallorganisches Netzwerk (DE-588)7755315-9 gnd Polymerkomplexe (DE-588)4137334-0 gnd Nanoporöser Stoff (DE-588)4800345-1 gnd |
| subject_GND | (DE-588)7755315-9 (DE-588)4137334-0 (DE-588)4800345-1 (DE-588)4143413-4 |
| title | Metal-organic frameworks applications from catalysis to gas storage |
| title_auth | Metal-organic frameworks applications from catalysis to gas storage |
| title_exact_search | Metal-organic frameworks applications from catalysis to gas storage |
| title_full | Metal-organic frameworks applications from catalysis to gas storage ed. by David Farrusseng |
| title_fullStr | Metal-organic frameworks applications from catalysis to gas storage ed. by David Farrusseng |
| title_full_unstemmed | Metal-organic frameworks applications from catalysis to gas storage ed. by David Farrusseng |
| title_short | Metal-organic frameworks |
| title_sort | metal organic frameworks applications from catalysis to gas storage |
| title_sub | applications from catalysis to gas storage |
| topic | Metallorganisches Netzwerk (DE-588)7755315-9 gnd Polymerkomplexe (DE-588)4137334-0 gnd Nanoporöser Stoff (DE-588)4800345-1 gnd |
| topic_facet | Metallorganisches Netzwerk Polymerkomplexe Nanoporöser Stoff Aufsatzsammlung |
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