Chemistry of nanocarbons:
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| Other Authors: | |
|---|---|
| Format: | Book |
| Language: | English |
| Published: |
Chichester
Wiley
2010
|
| Edition: | 1. publ. |
| Subjects: | |
| Online Access: | Inhaltsverzeichnis |
| Physical Description: | XXVIII, 498 S. Ill., graph. Darst. |
| ISBN: | 9780470721957 |
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Record in the Search Index
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|---|---|
| adam_text | Titel: Chemistry of nanocarbons
Autor: Akasaka, Takeshi
Jahr: 2010
Contents
Preface xv
Acknowledgements
Contributors
Abbreviations
xvn
xix
xxiii
1 Noncovalent Functionalization of Carbon Nanotubes 1
Claudia Backes and Andreas Hirsch
1.1 Introduction 1
1.2 Overview of Functionalization Methods 2
1.3 The Noncovalent Approach 3
1.3.1 Dispersability of Carbon Nanotubes 3
1.3.2 The Role of Noncovalent Functionalization in
Nanotube Separation 26
1.4 Conclusion 35
References 35
2 Supramolecular Assembly of Fullerenes and Carbon Nanotubes Hybrids 49
M Angeles Herranz, Beatriz M. Illescas, Emilio M. Perez
and Nazario Martin
2.1 Introduction 49
2.2 Hydrogen Bonded C60* Donor Ensembles 50
2.3 Concave exTTF Derivatives as Recognizing Motifs for Fullerene 56
2.4 Noncovalent Functionalization of Carbon Nanotubes 61
2.5 Summary and Outlook 67
Acknowledgements 68
References 68
3 Properties of Fullerene-Containing Dendrimers 73
Juan-Jose Cid Martin and Jean-Francois Nierengarten
3.1 Introduction 73
3.2 Dendrimers with a Fullerene Core 74
3.2.1 A Fullerene Core to Probe Dendritic Shielding Effects 74
3.2.2 Light Harvesting Dendrimers with a Fullerene Core 77
3.3 Fullerene-Rich Dendrimers 79
3.4 Conclusions 89
Acknowledgements 89
References 89
4 Novel Electron Donor Acceptor Nanocomposites 93
Hiroshi Imahori, Dirk M. Guldi and Shunichi Fukuzumi
4.1 Introduction 93
4.2 Electron Donor-Fullerene Composites 94
4.2.1 General 94
4.2.2 Donor-Fullerene Dyads for Photoinduced Electron Transfer 94
4.2.3 Donor-Fullerene Linked Multicomponent Systems 96
4.2.4 Supramolecular Donor-Fullerene Systems 96
4.2.5 Photoelectrochemical Devices and Solar Cells 99
4.3 Carbon Nanotubes 106
4.3.1 General 106
4.3.2 Carbon Nanotube - Electron Donor Acceptor Conjugates 108
4.3.3 Carbon Nanotube - Electron Donor Acceptor Hybrids 113
4.4 Other Nanocarbon Composites 116
References 117
5 Higher Fullerenes: Chirality and Covalent Adducts 129
Agnieszka Kraszewska, Francois Diederich and Carlo Thilgen
5.1 Introduction 129
5.1.1 Fullerene Chirality - Classification and the Stereodescriptor
System 130
5.1.2 Reactivity and Regioselectivity 131
5.2 The Chemistry of C70 132
5.2.1 C70-Derivatives with an Inherently Chiral Functionalization
Pattern 132
5.2.2 Cyo-Derivatives with a Non-Inherently Chiral
Functionalization Pattern 148
5.2.3 Fullerene Derivatives with Stereogenic Centers in the
Addends 152
5.3 The Higher Fullerenes Beyond C70 152
5.3.1 Isolated and Structurally Assigned Higher Fullerenes 152
5.3.2 Inherently Chiral Fullerenes - Chiral Scaffolds 153
5.4 Concluding Remarks 162
Acknowledgement 163
References 163
6 Application of Fullerenes to Nanodevices 173
Yutaka Matsuo and Eiichi Nakamura
6.1 Introduction 173
6.2 Synthesis of Transition Metal Fullerene Complexes 174
6.3 Organometallic Chemistry of Metal Fullerene Complexes 176
6.4 Synthesis of Multimetal Fullerene Complexes 177
6.5 Supramolecular Structures of Penta(organo)[60]fullerene Derivatives 179
6.6 Reduction of Penta(organo)[60]fullerenes to Generate Polyanions 179
6.7 Photoinduced Charge Separation 180
6.8 Photocurrent-Generating Organic and Organometallic Fullerene
Derivatives 181
6.8.1 Attaching Legs to Fullerene Metal Complexes 181
6.8.2 Formation of Self-Assembled Monomolecular Films 182
6.8.3 Photoelectric Current Generation Function of Lunar
Lander-Type Molecules 183
6.9 Conclusion 185
References 185
7 Supramolecular Chemistry of Fullerenes: Host Molecules for
Fullerenes on the Basis of tt-it Interaction 189
Takeshi Kawase
7.1 Introduction 189
7.2 Fullerenes as an Electron Acceptor 190
7.3 Host Molecules Composed of Aromatic 7r-systems 192
7.3.1 Hydrocarbon Hosts 192
7.3.2 Hosts Composed of Electron Rieh Aromatic 7t-Systems 194
7.3.3 Host Molecules Bearing Appendants 195
7.3.4 Host Molecules with Dimeric or Polymerie Structures 197
7.4 Complexes with Host Molecules Based on Porphyrin n Systems 199
7.4.1 Hosts with a Porphyrin n System 199
7.4.2 Hosts with Two Porphyrin n Systems 200
7.5 Complexes with Host Molecules Bearing a Cavity Consisting
of Curved % System 203
7.5.1 Host with a Concave Structure 203
7.5.2 Complexes with Host Molecules Bearing a Cylindrical Cavity 204
7.6 The Nature of the Supramolecular Property of Fullerenes 208
References 208
8 Molecular Surgery toward Organic Synthesis
of Endohedral Fullerenes 215
Michihisa Murata, Yasujiro Murata and Koichi Komatsu
8.1 Introduction 215
8.2 Molecular-Surgery Synthesis of Endohedral C60 Encapsulating
Molecular Hydrogen 216
8.2.1 CageOpening 216
8.2.2 Encapsulation of a H2 Molecule 219
8.2.3 Encapsulation of a He Atom 219
8.2.4 Closure of the Opening 220
8.3 Chemical Functionalization of H2@C6o 222
8.4 Utilization of the Encapsulated H2 as an NMR Probe 224
8.5 Physical Properties of an Encapsulated H2 in C60 226
8.6 Molecular-Surgery Synthesis of Endohedral C70 Encapsulating
Molecular Hydrogen 227
8.6.1 Synthesis of (H2)2@C70 and H2@C70 227
8.6.2 Diels-Alder Reaction of (H2)2@C70 and H2@C70 231
8.7 Outlook 233
References 233
9 New Endohedral Metallofullerenes: Trimetallic Nitride
Endohedral Fullerenes 239
Marilyn M. Olmstead, Alan L. Balch, Julio R. Pinzön, Luis Echegoyen,
Harry W. Gibson and Harry C. Dorn
9.1 Discovery, Preparation, and Purification 239
9.2 Structural Studies 240
9.2.1 Cycloaddition Reactions 246
9.2.2 Free Radical and Nucleophilic Addition Reactions 250
9.2.3 Electrochemistry Studies of TNT-EMFs 252
9.3 Summary and Conclusions 254
References 254
10 Recent Progress in Chemistry of Endohedral Metallofullerenes 261
Takahiro Tsuchiya, Takeshi Akasaka and Shigeru Nagase
10.1 Introduction 261
10.2 Chemical Derivatization of Mono-Metallofullerenes 262
10.2.1 Carbene Reaction 263
10.2.2 Nucleophilic Reaction 263
10.3 Chemical Derivatization of Di-Metallofullerenes 265
10.3.1 Bis-silylation 266
10.3.2 Cycloaddition with Oxazolidinone 267
10.3.3 Carbene Reaction 267
10.4 Chemical Derivatization of Trimetallic Nitride Template Fullerene 269
10.5 Chemical Derivatization of Metallic Carbaide Fullerene 271
10.6 Missing Metallofullerene 271
10.7 Supramolecular Chemistry 274
10.7.1 Supramolecular System with Macrocycles 274
10.7.2 Supramolecular System with Organic Donor 276
10.8 Conclusion 277
References 278
11 Gadonanostructures as Magnetic Resonance Imaging Contrast Agents 287
Jeyarama S. Ananta and Lon J. Wilson
11.1 Magnetic Resonance Imaging (MRI) and the Role of
Contrast Agents (CAs) 287
11.2 The Advantages of Gadonanostructures as MRI Contrast
Agent Synthons 289
11.3 Gadofullerenes as MRI Contrast Agents 290
11.4 Understanding the Relaxation Mechanism of Gadofullerenes 291
11.5 Gadonanotubes as MRI Contrast Agents 294
Acknowledgement 297
References 297
12 Chemistry of Soluble Carbon Nanotubes: Fundamentals
and Applications 301
Tsuyohiko Fujigaya and Naotoshi Nakashima
12.1 Introduction 301
12.2 Characterizations of Dispersion States 303
12.3 CNT Solubilization by Small Molecules 303
12.3.1 Surfactants 303
12.3.2 Aromatic Compounds 305
12.4 Solubilization by Polymers 309
12.4.1 Vinyl Polymers 309
12.4.2 Conducting Polymers 313
12.4.3 Condensation Polymers 314
12.4.4 Block Copolymers 314
12.5 Nanotube/Polymer Hybrids and Composites 315
12.5.1 DNA/Nanotube Hybrids 315
12.5.2 Curable Monomers and Nanoimprinting 317
12.5.3 Nanotube/Polymer Gel-Near IR Responsive Materials 318
12.5.4 Conductive Nanotube Honeycomb Film 320
12.6 Summary 323
References 323
13 Functionalization of Carbon Nanotubes for Nanoelectronic
and Photovoltaic Applications 333
Stephane Campidelli and Maurizio Prato
13.1 Introduction 333
13.2 Functionalization of Carbon Nanotubes 333
13.3 Properties and Applications 336
13.3.1 Electron Transfer Properties and Photovoltaic Applications 336
13.3.2 Functionalized Carbon Nanotubes for Electrical
Measurements and Field Effect Transistors 346
13.3.3 Biosensors 351
13.4 Conclusion 356
References 356
14 Dispersion and Separation of Single-walled Carbon Nanotubes 365
Yutaka Maeda, Takeshi Akasaka, Jing Lu and Shigeru Nagase
14.1 Introduction 365
14.2 Dispersion of SWNTs 366
x/7 Contents
14.2.1 Dispersion of SWNTs Using Amine 366
14.2.2 Dispersion of SWNTs Using C60 Derivatives 368
14.2.3 Dispersion of SWNTs in Organic Solvents 371
14.3 Purification and Separation of SWNTs Using Amine 373
14.3.1 Purification and Separation of SWNTs Prepared
by CVD Methods 373
14.3.2 Purification and Separation of Metallic SWNTs Prepared
by Arc-Discharged Method 375
14.3.3 Preparation of SWNTs and Metallic SWNTs Films 377
14.4 Conclusion 380
References 380
15 Molecular Encapsulations into Inferior Spaces of Carbon
Nanotubes and Nanohorns 385
T. Okazaki, S. Iijima and M. Yudasaka
15.1 Introduction 385
15.2 SWCNT Nanopeapods 386
15.2.1 Synthesis Methods 386
15.2.2 Electronic Structures of C60 Nanopeapods 387
15.3 Material Incorporation and Release in/from SWNH 394
15.3.1 Structure of SWNH and SWNHox 394
15.3.2 Liquid Phase Incorporation at Room Temperature 395
15.3.3 Adsorption Sites of SWNHox 397
15.3.4 Release of Materials from inside SWNHox 398
15.3.5 Plug 401
15.4 Summary 401
References 401
16 Carbon Nanotube for Imaging of Single Molecules in Motion 405
Eiichi Nakamura
16.1 Introduction 405
16.2 Electron Microscopic Observation of Small Molecules 406
16.3 TEM Imaging of Alkyl Carborane Molecules 407
16.4 Alkyl Chain Passing through a Hole 408
16.5 3D Structural Information on Pyrene Amide Molecule 409
16.6 Complex Molecule 4 Fixed outside of Nanotube 410
16.7 Conclusion 411
Acknowledgements 411
References 412
17 Chemistry of Single-Nano Diamond Particles 413
Eiji Ösawa
17.1 Introduction 413
17.2 Geometrical Structure 417
17.3 Electronic Structure 419
17.4 Properties 422
17.4.1 Tight Hydration 422
17.4.2 Gels 424
17.4.3 Number Effect 425
17.5 Applications 425
17.5.1 Lubrication Water 426
17.6 Recollection and Perspectives 428
Acknowledgements 430
References 430
18 Properties of iT-electrons in Graphene Nanoribbons
and Nanographenes 433
De-en Jiang, Xingfa Gao, Shigeru Nagase and Zhongfang Chen
18.1 Introduction 433
18.2 Edge Effects in Graphene Nanoribbons and Nanographenes 435
18.3 Electronic and Magnetic Properties of Graphene Nanoribbons
and Nanographenes 438
18.3.1 Graphene Nanoribbons 438
18.3.2 Nanographenes 444
18.4 Outlook 456
Acknowledgement 456
References 456
19 Carbon Nano Onions 463
Luis Echegoyen, Angy Ortiz, Manuel N. Chaur and Amit J. Palkar
19.1 Introduction 464
19.2 Physical Properties of Carbon Nano Onions Obtained
from Annealing 465
19.2.1 Annealing Process 465
19.3 Raman Spectroscopy of Carbon Nano Onions Prepared
by Annealing Nanodiamonds 466
19.3.1 X-Ray Diffraction Studies 467
19.3.2 Electrical Resistivity Studies 468
19.4 Electron Paramagnetic Resonance Spectroscopy 469
19.5 Carbon Nano Onions Prepared from Arcing Graphite
Underwater 470
19.5.1 Mechanism of Formation 471
19.5.2 Properties of Carbon Nano Onions Obtained from
Are Discharge 471
19.6 Reactivity of Carbon Nano Onions (CNOs) 473
19.6.1 1,3-Dipolar Cycloaddition Reaction 473
19.6.2 Amidation Reactions 474
19.6.3 [2+1] Cycloaddition Reactions 475
19.6.4 Free-Radical Addition Reactions 476
19.7 Potential Applications of CNOs 478
Acknowledgements 481
References 481
Index 485
|
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| indexdate | 2024-07-09T22:12:29Z |
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| isbn | 9780470721957 |
| language | English |
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| spelling | Chemistry of nanocarbons ed. by Takeshi Akasaka ... 1. publ. Chichester Wiley 2010 XXVIII, 498 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Nanotubes Fullerenes Nanodiamonds Nanostrukturiertes Material (DE-588)4342626-8 gnd rswk-swf Kohlenstoff-Nanoröhre (DE-588)4581365-6 gnd rswk-swf Fullerene (DE-588)4305238-1 gnd rswk-swf Kohlenstoff (DE-588)4164538-8 gnd rswk-swf Fullerene (DE-588)4305238-1 s DE-604 Kohlenstoff-Nanoröhre (DE-588)4581365-6 s Kohlenstoff (DE-588)4164538-8 s Nanostrukturiertes Material (DE-588)4342626-8 s Akasaka, Takeshi edt HBZ Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=019009241&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Chemistry of nanocarbons Nanotubes Fullerenes Nanodiamonds Nanostrukturiertes Material (DE-588)4342626-8 gnd Kohlenstoff-Nanoröhre (DE-588)4581365-6 gnd Fullerene (DE-588)4305238-1 gnd Kohlenstoff (DE-588)4164538-8 gnd |
| subject_GND | (DE-588)4342626-8 (DE-588)4581365-6 (DE-588)4305238-1 (DE-588)4164538-8 |
| title | Chemistry of nanocarbons |
| title_auth | Chemistry of nanocarbons |
| title_exact_search | Chemistry of nanocarbons |
| title_full | Chemistry of nanocarbons ed. by Takeshi Akasaka ... |
| title_fullStr | Chemistry of nanocarbons ed. by Takeshi Akasaka ... |
| title_full_unstemmed | Chemistry of nanocarbons ed. by Takeshi Akasaka ... |
| title_short | Chemistry of nanocarbons |
| title_sort | chemistry of nanocarbons |
| topic | Nanotubes Fullerenes Nanodiamonds Nanostrukturiertes Material (DE-588)4342626-8 gnd Kohlenstoff-Nanoröhre (DE-588)4581365-6 gnd Fullerene (DE-588)4305238-1 gnd Kohlenstoff (DE-588)4164538-8 gnd |
| topic_facet | Nanotubes Fullerenes Nanodiamonds Nanostrukturiertes Material Kohlenstoff-Nanoröhre Fullerene Kohlenstoff |
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