Scanning tunneling microscopy in surface science, nanoscience and catalysis:
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| Other Authors: | |
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| Format: | Book |
| Language: | English |
| Published: |
Weinheim
Wiley-VCH
2010
|
| Subjects: | |
| Online Access: | Inhaltstext Inhaltsverzeichnis |
| Physical Description: | XIV, 244 S. Ill., graph. Darst. |
| ISBN: | 9783527319824 |
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Record in the Search Index
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IMAGE 1
CONTENTS
PREFECE IX LIST OF CONTRIBUTORS XIII
1 CHIRALITY AT METAL SURFACES 1
CHRIS J. BADDELEY AND NEVILLE V. RICHARDSON 1.1 INTRODUCTION 1
1.1.1 DEFINITION OF CHIRALITY 1 1.1.2 NOMENCLATURE OF CHIRALITY: THE
(SS),(S) CONVENTION 2 1.2 SURFACE CHIRALITY FOLLOWING MOLECULAR
ADSORPTION 4 1.2.1 ACHIRAL MOLECULES ON ACHIRAL SURFACES 4
1.2.2 LATTICE MATCHING 8
1.2.3 CHIRAL MOLECULES ON ACHIRAL SURFACES 12 1.2.4 CHIRAL MOLECULES ON
CHIRAL SURFACES 15 1.2.5 CHIRAL ETCHING 16
1.3 CHIRAL AMPLIFICATION AND RECOGNITION 19 1.3.1 CHIRAL AMPLIFICATION
IN TWO DIMENSIONS 19 1.3.2 CHIRAL SWITCHING 20
1.3.3 CHIRAL RECOGNITION 21 1.3.4 PROCHIRAL MOLECULES INTERACTING WITH
CHIRAL SURFACES 24 1.4 CONCLUSIONS 25
REFERENCES 26
2 THE TEMPLATE ROUTE TO NANOSTRUCTURED MODEL CATALYSTS 29 CONRAD BECKER
AND KLAUS WANDELT 2.1 INTRODUCTION 29
2.2 SURFACES AS TWO-DIMENSIONAL TEMPLATES 3 I 2.3 STM IMAGING OF OXIDE
FILMS 34
2.4 STM IMAGING OF METAL PARTICLES ON OXIDE FILMS 39 2.5
TEMPLATE-CONTROLLED GROWTH OF MODEL CATALYSTS 44 2.5.1 OXIDES AS
TEMPLATES 44
BIBLIOGRAFISCHE INFORMATIONEN HTTP://D-NB.INFO/994711816
DIGITALISIERT DURCH
IMAGE 2
VI CONTENTS
2.5.2 MODIFIED TEMPLATES 50
2.6 CONCLUSIONS 51
REFERENCES 52
3 IN SITU STM STUDIES OF MODEL CATALYSTS 55
FAN YANG AND D. WAYNE GOODMAN 3.1 INTRODUCTION 55
3.2 INSTRUMENTATION 56
3.3 VISUALIZING THE PATHWAY OF CATALYTIC REACTIONS 59 3.3.1 IMAGING OF
ADSORBATES AND REACTION INTERMEDIATES 59 3.3.2 IMAGING CHEMISORPTION ON
METALS 61
3.3.3 DETERMINING THE SITES FOR CHEMISORPTION ON OXIDE SURFACES 64 3.3.4
VISUALIZING REACTION INTERMEDIATES AND THE MECHANISM OF HYDROGEN
OXIDATION 71 3.3.5 MEASURING THE REACTION KINETICS OF CO OXIDATION 73
3.4 METAL SURFACES AT HIGH PRESSURES 81
3.5 IN SITU STUDIES OF SUPPORTED MODEL CATALYSTS 85 3.5.1 MONITORING THE
GROWTH KINETICS OF SUPPORTED METAL CATALYSTS 85 3.5.2 STUDIES OF THE
SMSI EFFECT 88 3.5.3 SINTERING KINETICS OF SUPPORTED AU CLUSTERS 89 3.6
OUTLOOK 91
REFERENCES 92
4 THEORY OF SCANNING TUNNELING MICROSCOPY AND APPLICATIONS IN CATALYSIS
97 GILBERTO TEOBALDI, HAIPING LIN, AND WERNER HOFER 4.1 CATALYSIS AND
SCANNING TUNNELING MICROSCOPY 97 4.2 IMAGE FORMATION IN AN STM 98
4.3 SIMULATING TUNNELING CURRENTS 99 4.4 SIMULATING CHEMICAL REACTIVITY
100 4.5 CATALYTIC WATER PRODUCTION 101 4.5.1 TIO 2 : A CATALYTIC MODEL
SYSTEM 106 4.6 OUTLOOK 115
REFERENCES 136
5 CHARACTERIZATION AND MODIFICATION OF ELECTRODE SURFACES BY IN SITU STM
119 DIETER M. KOLB AND FELICE C. SIMEONE 5.1 INTRODUCTION 119
5.2 IN SITU STM: PRINCIPLE, TECHNICAL REALIZATION AND LIMITATIONS 120
5.2.1 PRINCIPLE CONSIDERATIONS FOR IN SITU OPERATION 120 5.2.2 TECHNICAL
REALIZATION 124 5.2.2.1 TIP PREPARATION AND ISOLATION 124 5.2.2.2
ELECTROCHEMICAL CELL 126 5.2.2.3 VIBRATION DAMPING 127
IMAGE 3
CONTENTS VII
5.2.3 LIMITATIONS 127
5.3 IMAGING SINGLE-CRYSTAL SURFACES OF CATALYTICALLY RELEVANT SYSTEMS
328 5.3.1 PREPARATION AND IMAGING OF METAL SINGLE-CRYSTAL SURFACES 128
5.3.2 BIMETALLIC SURFACES 230 5.4 STRATEGIES FOR NANOSTRUCTURING
SURFACES 132 5.4.1 OXIDATION-REDUCTION CYCLES FOR ROUGHENING AND
FACETING
SURFACES 232
5.4.2 SURFACE MODIFICATION BY AN STM: AN OVERVIEW 234 5.4.3 METAL
NANODUSTER DEPOSITION VIA JUMP-TO-CONTACT 239 REFERENCES 144
6 STM IMAGING OF OXIDE NANOLAYER MODEL SYSTEMS 147 FALKO P. HETZER AND
SVETLOZAR SURNEV 6.1 INTRODUCTION 147
6.2 EXPERIMENTAL ASPECTS AND TECHNICAL DEVELOPMENTS 249 6.3 CASE
STUDIES: SELECTED OXIDE-METAL SYSTEMS 152 6.3.1 ALUMINA NANOLAYERS ON
NIAL ALLOYS 252 6.3.2 TITANIUM OXIDE NANOLAYERS 155 6.3.3 VANADIUM OXIDE
NANOLAYERS 259 6.3.4 IRON OXIDES ON PT(L 1 1) 169
6.3.5 NICKEL OXIDE NANOLAYERS 173 6.3.6 CENA NANOLAYERS ON METAL
SURFACES 277 6.4 SYNOPSIS AND OUTLOOK 182
REFERENCES 283
7 SURFACE MOBILITY OF ATOMS AND MOLECULES STUDIED WITH HIGH-PRESSURE
SCANNING TUNNELING MICROSCOPY 189 GABOR A. SOMORJAI, FENG TAO, AND DEREK
BUTCHER 7.1 INTRODUCTION 189
7.2 CHARACTERIZATION OF SURFACE MOBILITY OF MOLECULES AND ATOMS 289 7.3
HIGH-PRESSURE STM TECHNIQUE AND INSTRUMENTATION 291 7.4 MOBILITY AND
FLEXIBILITY OF CATALYST SURFACES AT HIGH-PRESSURE HIGH-TEMPERATURE
REACTION CONDITIONS 197
7.5 ADSORBATE MOBILITY DURING CATALYTIC REACTIONS 206 7.5.1 ETHYLENE
HYDROGENATION ON PT(L 1 1) 207 7.5.2 HYDROGENATION OF C 6 CYCLIC
HYDROCARBONS ON PT(L 1 1) 209 7.5.3 CO/NO COADSORPTION ON RH(L 1 1) 213
7.6 SUMMARY 236
REFERENCES 226
IMAGE 4
VILI CONTENTS
8 POINT DEFECTS ON RUTILE TIO 2(1 1 0): REACTIVITY, DYNAMICS,
AND TUNABILITY 219 CHI L PANG AND GEOFF THORNTON 8.1 INTRODUCTION 219
8.2 METHODS 220
8.3 WATER DISSOCIATION AT OXYGEN VACANCIES AND THE IDENTIFICATION OF
POINT DEFECTS 221 8.4 O 2 DISSOCIATION AT OXYGEN VACANCIES 229 8.5
ALCOHOL DISSOCIATION AT OXYGEN VACANCIES 229 8.6 DIFFUSION OF OXYGEN
VACANCIES AND SURFACE HYDROXY 232 8.7 TUNING THE DENSITIES OF OXYGEN
VACANCIES AND SURFACE
HYDROXYL ON TIO 2 (L 1 0) 234 8.8 OUTLOOK 236
REFERENCES 236
INDEX 239 |
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| spelling | Scanning tunneling microscopy in surface science, nanoscience and catalysis ed. by Michael Bowker... Weinheim Wiley-VCH 2010 XIV, 244 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Scanning tunneling microscopy Surface chemistry Surfaces (Physics) Rastertunnelmikroskopie (DE-588)4252995-5 gnd rswk-swf (DE-588)4143413-4 Aufsatzsammlung gnd-content Rastertunnelmikroskopie (DE-588)4252995-5 s DE-604 Bowker, Michael edt text/html http://deposit.dnb.de/cgi-bin/dokserv?id=3320193&prov=M&dok_var=1&dok_ext=htm Inhaltstext DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=018651773&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Scanning tunneling microscopy in surface science, nanoscience and catalysis Scanning tunneling microscopy Surface chemistry Surfaces (Physics) Rastertunnelmikroskopie (DE-588)4252995-5 gnd |
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| title | Scanning tunneling microscopy in surface science, nanoscience and catalysis |
| title_auth | Scanning tunneling microscopy in surface science, nanoscience and catalysis |
| title_exact_search | Scanning tunneling microscopy in surface science, nanoscience and catalysis |
| title_full | Scanning tunneling microscopy in surface science, nanoscience and catalysis ed. by Michael Bowker... |
| title_fullStr | Scanning tunneling microscopy in surface science, nanoscience and catalysis ed. by Michael Bowker... |
| title_full_unstemmed | Scanning tunneling microscopy in surface science, nanoscience and catalysis ed. by Michael Bowker... |
| title_short | Scanning tunneling microscopy in surface science, nanoscience and catalysis |
| title_sort | scanning tunneling microscopy in surface science nanoscience and catalysis |
| topic | Scanning tunneling microscopy Surface chemistry Surfaces (Physics) Rastertunnelmikroskopie (DE-588)4252995-5 gnd |
| topic_facet | Scanning tunneling microscopy Surface chemistry Surfaces (Physics) Rastertunnelmikroskopie Aufsatzsammlung |
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