Catalysis for sustainable energy production:
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| Format: | Book |
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| Language: | English |
| Published: |
Weinheim
Wiley-VCH-Verl.
2009
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| Subjects: | |
| Online Access: | Inhaltstext Inhaltsverzeichnis |
| Item Description: | Literaturangaben |
| Physical Description: | XXII, 452 S. Ill., graph. Darst. 25 cm |
| ISBN: | 9783527320950 |
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IMAGE 1
CONTENTS
FOREWORD XII I
EPILOGUE XVII
LIST OF CONTRIBUTORS XIX
PART ONE FUEL CELLS
THE DIRECT ETHANOL FUEL CELL: ACHALLENGE TO CONVERT BIOETHANOL CLEANLY
INTO ELECTRIC ENERGY 3 C1AUDE LAMY, CHRISTOPHE COUTANCEAU, AND
JEAN-MICHEL LEGER 1.1 INTRODUCTION 3
1.2 PRINCIPLES AND DIFFERENT KINDS OF FUEL CELLS 4 1.2.1 WORKING
PRINCIPLES OF A FUEL CELL 4 1.2.1.1 THE THERMODYNAMICS OF FUEL CELLS 5
1.2.1.2 THE KINETICS OF FUEL CELLS 6
1.2.1.3 CATALYSIS OF FUEL CELL REACTIONS 9 1.2.2 DIFFERENT TYPES OF FUEL
CELLS 14 1.2.2.1 FUELS FAR FUEL CELLS 14 1.2.2.2 HYDROGEN-FED FUEL CELLS
16 1.2.2.3 METHANOL- AND ETHANOL-FED FUEL CELLS 16 1.3 LOW-TEMPERATURE
FUEL CELLS (PEMFCS AND DAFCS) 17 1.3.1 PROTON EXCHANGE MEMBRANE FUEL
CELL (PEMFC) 17 1.3.1.1 PRINCIPLE OF A PEMFC 17
1.3.1.2 THE PROTON EXCHANGE MEMBRANE 18 1.3.1.3 THE ELECTRODE CATALYSTS
19 1.3.1.4 THE MEMBRANE-ELECTRODE ASSEMBLY 19 1.3.1.5 THE BIPOLAR PLATES
19
1.3.1.6 AUXILIARY AND CONTRAL EQUIPMENT 19 1.3.2 DIRECT ETHANOL FUEL
CELL (DEFC) 21 1.3.2.1 PRINCIPLE OF THE DIRECT ETHANOL FUEL CELL 21
1.3.2.2 REACTION MECHANISMS AF ETHANOLOXIDATION 22 1.3.2.3 DEFC TESTS 26
1.4 SOLID ALKALINE MEMBRANE FUEL CELL (SAMFC) 29
CO.TALYSIS FOR SUSTAINABLE ENERGY PRODUCTION. EDITED BY P. BARBARO AND
C. BIANCHINI COPYRIGHT 2009 WILEYVCH VERLAG GMBH & CO. KGAA, WEINHEIM
ISBN: 978352732095-0
IMAGE 2
VI I CONTENTS
1.4.1
1.4.2 1.4.3 1.5
2
2.1 2.2 2.3 2.3.1
2.3.2 2.3.3 2.3.4 2.4
3
3.1 3.2 3.2.1 3.2.2 3.2.3 3.2.4 3.3 3.3.1 3.3.2 3.3.3 3.3.4 3.3.5
3.4
4
4.1
DEVELOPMENT OF ASOLID ALKALINE MEMBRANE FOR FUEL CELL APPLICATION 29
ANODIC CATALYSTS IN ALKALINE MEDIUM 32 CATHODIC CATALYSTS IN ALKALINE
MEDIUM 38 CONCLUSION 42
REFERENCES 42
PERFORMANCE OF DIRECT METHANOL FUEL CELLS FOR PORTABLE
POWER APPLICATIONS 47
XIAOMING REN INTRODUCTION 47 EXPERIMENTAL 49 RESULTS AND DISCUSSION 51
WATER BALANCE, MAXIMUM AIR FEED RATE AND IMPLICATIONS
FOR CATHODE PERFORMANCE 51 STACK PERFORMANCE 57 THERMAL BALANCE AND
WASTE HEAT REJECTION 64 STACK LIFE TEST RESULTS 65
CONCLUSIONS 67 REFERENCES 68
SELECTIVE SYNTHESIS OFCARBON NANOFIBERS AS BETTER CATALYST SUPPORTS
FOR LOW-TEMPERATURE FUEL CELLS 71
SEONG-HWA HONG, MUN-SUKJUN, FSAO MOCHIDA, AND SEONG-HO YOON INTRODUCTION
71 PREPARATION AND CHARACTERIZATION OF CNFS AND FUEL CELL CATALYSTS 73
PREPARATION OFTYPICAL CNFS 73 PREPARATION OF NANOTUNNELED MESOPOROUS H
-CNF 73 PREPARATION OF FUEL CELL CATALYSTS 74 PERFORMANCE
CHARACTERIZATION OF FUEL CELL CATALYSTS 74 RESULTS 74
STRUCTURAL EFFECTS OF CNFS 74 CATALYTIC PERFORMANCE OF CNFS IN HALF AND
SINGLE CELLS 76 STRUCTURE OF NANOTUNNELED MESOPOROUS THICK H-CNF 78
CATALYTIC PERFORMANCE OFNANOTUNNELED MESOPOROUS THICK H-CNF 78
EFFECT OF THE DISPERSION OF THIN AND VERY THIN H-CNFS ON THE CATALYST
ACTIVITY 81 DISCUSSION 84 REFERENCES 86
TOWARDS FULL ELECTRIC MOBILITY: ENERGY AND POWER SYSTEMS 89
PIETRO PERFO, MARCO OTTELLA, NICOFA CORINO, FRANCESCO PITZALIS, MAURO
BRIGNONE, DANIELE ZANELLO, GIANFRANCO INNOCENTI, LUCA BELFORTE, AND
ALESSANDRO ZIGGIOTTI INTRODUCTION 89
IMAGE 3
CONTENTS\ VII
4.2 THE CURRENT GRAND CHAILENGES 89
4.3 POWER-ENERGY NEEDED IN VEHIDES 90 4.3.1 BASIE FORMULATION 90 4.3.2
WEIL TO WHEEL EVALUATIONS 92 4.3.3 SPECIFIE CALCULATIONS FOR IDEAL
ELEETRIE POWERTRAINS 92 4.3.4 A ROADMAP OF FEASIBILITY WITH BATTERIES
AND SUPEREAPAEITORS 95 4.3.5 THE NEED FOR RANGE EXTENDERS 96 4.3.5.1
DIREET THERMOELEETRIE GENERATORS 98 4.4 A GREAT NEW OPPORTUNITY FOR TRUE
ZERO EMISSIONS 101
4.5 ADVANEED SYSTEMS INTEGRATION 102 4.6 CONDUSION AND PERSPEETIVES 103
REFERENEES 104
PART TWO HYDROGEN STORAGE 107
5 MATERIALS FOR HYDROGEN STORAGE 109
ANDREAS ZUETTEL
5.1 TBE PRIMITIVE PHASE DIAGRAM OFHYDROGEN 109 5.2 HYDROGEN STORAGE
METHODS 109 5.3 PRESSURIZED HYDROGEN 111
5.3.1 PROPERTIES OF COMPRESSED HYDROGEN 112 5.3.2 PRESSURE VESSEL 113
5.3.3 VOLUMETRIE AND GRAVIMETRIE HYDROGEN DENSITY 114 5.3.4 MIEROSPHERES
115
5.4 LIQUID HYDROGEN 117
5.4.1 LIQUEFAETION PROEESS 118 5.4.2 STORAGEVESSEL 119
5.4.3 GRAVIMETRIE AND VOLUMETRIE HYDROGEN DENSITY 120 5.5 PHYSISORPTION
121
5.5.1 VAN DER WAALS INTERAETION 121 5.5.2 ADSORPTION ISOTHERM 122 5.5.3
HYDROGEN AND CARBON NANOTUBES 123 5.6 METAL HYDRIDES 128
5.6.1 INTERSTITIAL HYDRIDES 128 5.6.2 HYDROGEN ABSORPTION 130 5.6.3
EMPIRIEAL MODELS 133 5.6.4 LATTIEE GAS MODEL 137
5.7 COMPLEX HYDRIDES 141
5.7.1 TETRAHYDROALANATES 143 5.7.2 TETRAHYDROBORATES 148 5.8 CHEMIEAL
HYDRIDES (HYDROLYSIS) 154 5.8.1 ZINE CYDE 154
5.8.2 BOROHYDRIDE 156
5.9 NEW HYDROGEN STORAGE MATERIALS 157 5.9.1 AMIDES AND IMIDES (-NH B
=NH) 158
IMAGE 4
VIII I CONTENTS
5.9.2 BCC ALLOYS 160
5.9.3 ALH 3 160
5.9.4 META! HYDRIDES WITH SHORT H-H-DISTANCE 161 5.9.5 MGH 2 WITH A NEW
STRUCTURE 162 5.9.6 DESTABILIZATION OF MGH 2 BY ALLOY FORMATION 162
5.9.7 AMMONIA STORAGE 163 5.9.8 BORAZANE 163
REFERENCES 165
PART THREE H 2 AND HYDROGEN VECTORS PRODUCTION 171
6 CATALYST DESIGN FOR REFORMING OFOXYGENATES 173
LOREDANA OE ROGATIS AND PAOLO FORNASIERO 6.1 INTRODUCTION 173
6.2 CATALYST DESIGN 179
6.2.1 IMPREGNATED CATALYSTS: THE ROLE OFMETAL, SUPPORT AND PROMOTERS 181
6.2.2 EMERGING STRATEGIES: EMBEDDED CATALYSTS 183 6.3 REFORMING
REACTIONS: PROCESS PRINCIPLES 185 6.3.1 CATALYTIC STEAM REFORMING 185
6.3.2 CATALYTIC PARTIAL OXIDATION 188 6.3.3 AUTOTHERMAL REFORMING 189
6.3.4 AQUEOUS PHASE REFORMING 190 6.4 KEY EXAMPLES OF OXYGENATE
REFORMING REACTIONS 193 6.4.1 METHANOL 193
6.4.2 ETHANOL 197
6.4.3 DIMETHYL ETHER 203
6.4.4 ACETIC ACID 207
6.4.5 SUGARS 210
6.4.6 ETHYLENE GLYCOL 214 6.4.7 GLYCEROL 219
6.5 CONC1USIONS 222
6.6 LIST OF ABBREVIATIONS 223
REFERENCES 224
7 ELECTROCATALYSIS IN WATER ELECTROLYSIS 235 EDOARDO GUERRINI AND SERGIO
TRASATTI 7.1 INTRODUCTION 235
7.2 THERMODYNAMIC CONSIDERATIONS 237 7.3 KINETIC CONSIDERATIONS 239
7.3.1 EQUILIBRIUM TERM (L1E) 240 7.3.2 OHMIC DISSIPATION TERM (IR) 240
7.3.2.1 CELL DESIGN 241 7.3.3 STABILITY TERM (L1 V T ) 242
7.3.4 OVERPOTENTIAL DISSIPATION TERM (LLL) 243 7.3.5 ELECTROCATALYSIS
244
.
IMAGE 5
7.3.5.1 7.4 7.4.1 7.4.2 7.4.3 7.4.4 7.5 7.5.1 7.5.2 7.5.3
7.5.4 7.5.5 7.5.6 7.6
7.7 7.8
8
8.1 8.2 8.2.1 8.2.2
8.2.2.1 8.2.2.2 8.2.2.3 8.2.2.4 8.2.2.5 8.3 8.3.1 8.3.2
9
9.1 9.2 9.2.1 9.2.2
9.3 9.3.1
CONTENTS IIX
THEORY OF ELECTROCATALYSIS 245 THE HYDROGEN EVOLUTION REACTION 248
REACTION MECHANISMS 248
THE OXYGEN EVOLUTION REACTION
ELECTROCATALYSTS: STATE-OF-THEART
ELECTROCATALYSIS 249 MATERIALS FOR CATHODES 251 FACTORS OF
ELECTROCATALYSIS 252
REACTION MECHANISMS 255 ANODIC OXIDES 256 THERMAL OXIDES (DSA) 257
ELECTROCATALYSIS 259
FACTORS OF ELECTROCATALYSIS 260 INTERMITTENT ELECTROLYSIS 263
255
264
WATER ELECTROLYSIS: STATE-OF-THE-ART 265 BEYOND OXYGEN EVOLUTION 265
REFERENCES 267
ENERGY FROM ORGANIC WASTE: INFLUENCE OFTHE PROCESS PARAMETERS ON
THE PRODUCTION OF METHANE AND HYDROGEN 271 MICHE/E ARESTA AND ANGE/A
DIBENEDETTO INTRODUCTION 271 EXPERIMENTAL 273
METHANATION OF RESIDUAL BIOMASS 273 BIOCONVERSION OF GLYCEROL 274
CHARACTERIZATION OF STRAINS KI-K4 274 USE OF STRAINS KL, K2 AND K3 274
USE OF STRAIN K4 274 TESTS UNDER AEROBIC CONDITIONS 275
TESTS UNDER MICROAEROBIC OR ANAEROBIC CONDITIONS 275 RESULTS AND
DISCUSSION 275 BIOGAS FROM WASTE 275 DIHYDROGEN FROM BIOGLYCEROL 279
REFERENCES 284
NATURAL GAS AUTOTHERMAL REFORMING: AN EFFECTIVE OPTION FOR A SUSTAINABLE
DISTRIBUTED PRODUCTION OF HYDROGEN 287 PAOLO GAMBEL/I, VINCENZO PA/MA,
EMMA PA/O, AND GAETANO LAQUANIEL/O
INTRODUCTION 287 AUTOTHERMAL REFORMING: FROM CHEMISTRY TO ENGINEERING
294 THE CATALYST 294 KILOWATT-SCALE ATR FUEL PROCESSORS 298
THERMODYNAMIC ANALYSIS 299
EFFECT OF PREHEATING THE REACTANTS 300
IMAGE 6
X I CONTENTS
9.3.2 9.4 9.4.1 9.4.2 9.4.3
9.4.4 9.4.5 9.5 9.6
PART FOUR
10
10.1 10.2 10.2.1
10.2.2 10.3 10.4
11
11.1 11.2 11.3 11.3.1 11.3.2
11.3.3 11.4 11.4.1
11.5 11.6 11.7 11.8
12
12.1 12.2 12.2.1 12.2.2
EFFECT OF 02:CH4 AND H 2 0:CH 4 MOLAR FEED RATIOS 300 A CASE STUDY 303
LABORATORY APPARATUS AND ATR REACTOR 303 ATR REACTOR SETUP: OPERATING
CONDITIONS 306 ATR REACTOR SETUP: START-UP PHASE 306
ATR REACTOR SETUP: LNFLUENCE OF PREHEATING THE REACTANTS 307 CATALYTIC
ACTIVITY TEST RESULTS 309 ECONOMIC ASPECTS 313 CONCLUSIONS AND
PERSPECTIVES 316
REFERENCES 317
INDUSTRIAL CATALYSIS FOR SUSTAINABLE ENERGY 321
THE USE OF CATALYSIS IN THE PRODUCTION OF HIGH-QUALITY BIODIESEL 323
NICO/ETTA RAVASIO, FEDERICA ZACCHERIA, AND RINA/DO PSARO INTRODUCTION
323 HETEROGENEOUS TRANSESTERIFICATION AND ESTERIFICATION CATALYSTS 328
HETEROGENEOUS BASIC CATALYSTS 328 HETEROGENEOUS ACID CATALYSTS 330
SELECTIVE HYDROGENATION IN BIODIESEL PRODUCTION 336
CONCLUSIONS AND PERSPECTIVES 341 REFERENCES 342
PHOTOVOLTAICS - CURRENT TRENDS AND VISION FOR THE FUTURE 345 FRANCESCA
FERRAZZA INTRODUCTION 345 MARKET: PRESENT SITUATION AND CHALLENGES AHEAD
346 CRYSTALLINE SILICON TECHNOLOGY 348
FROM FEEDSTOCK TO WAFERS 348 FROM WAFERS TO CELLS AND MODULES 349 WHERE
TO CUT COSTS 351 THIN FILMS 353 TECHNOLOGY AND IMPROVEMENT REQUIREMENTS
354
OTHER TECHNOLOGY-RELATED ASPECTS 355 ADVANCED AND EMERGING TECHNOLOGIES
357 SYSTEM ASPECTS 359 CONCLUSIONS 361
REFERENCES 362
CATALYTIC COMBUSTION FOR THE PRODUCTION OF ENERGY 363 GIANPIERO GROPPI,
CINZIA CRISTIANI, A/ESSANDRA BERETTA, AND PIO FORZATTI INTRODUCTION 363
LEAN CATALYTIC COMBUSTION FOR GAS TURBINES 364
PRINCIPLES AND SYSTEM REQUIREMENTS 364 DESIGN CONCEPTS AND PERFORMANCE
366
IMAGE 7
12.2.2.1 12.2.2.2 12.2.2.3 12.3 12.4 12.5
12.6 12.6.1 12.6.2 12.6.2.1
12.6.2.2 12.6.2.3 12.7
13
13.1 13.2 13.2.1 13.2.2
13.2.3 13.2.3.1 13.2.3.2 13.2.3.3
13.2.4 13.2.4.1 13.2.4.2
13.3 13.3.1 13.3.2 13.3.2.1
13.3.2.2 13.3.2.3 13.3.3 13.3.3.1
13.3.3.2
13.4
CONTENTS I XI
FUHY CATALYTIC COMBUSTOR 366 FUEL STAGING 367 PARTIAL CATALYTIC HYBRID
COMBUSTOR 367 FUEL-RICH CATALYTIC COMBUSTION 370 OXY-FUEL COMBUSTION 372
MICROCOMBUSTORS 373 CATALYTIC MATERIALS 375 STRUCTURED SUBSTRATE 376
ACTIVE CATALYST LAYER 376
PDO-BASED CATALYSTS 377 METALSUBSTITUTED HEXAALUMINATE CATALYSTS 381
RICH COMBUSTION CATALYSTS 382 CONCLUSIONS 387
REFERENCES 388
CATALYTIC REMOVAL OF NO X UNDER LEAN CONDITIONS FROM STATIONARY AND
MOBILE SOURCES 393
PIO FORZATTI, LUCA LIETTI, AND ENRICO TRONCONI
INTRODUCTION 393
UNSTEADY-STATE MODELS OFTHE MONOLITH NO/NOZ/NH 3 SCR
IDENTIFICATION OF THE REACTION NETWORK DURING REDUCTION
SELECTIVE CATALYTIC REDUCTION 395 STANDARD SCR PROCESS 395 SCR
APPLICATIONS: PAST AND FUTURE 399 MODELING OF THE SCR REACTOR 400
STEADY-STATE MODELING OF THE SCR REACTOR 400 UNSTEADY-STATE KINETICS OF
THE STANDARD SCR REACTION 401 UNSTEADY-STATE MODELS OF THE MONOLITH SCR
REACTOR 406 FAST SCR 409 MECHANISM OF FAST SCR 409
REACTOR 412 NO" STORAGE REDUCTION 414 NSR TECHNOLOGY 414 STORAGE OFNO"
415 MECHANISTIC FEATURES 415 KINETICS 421 EFFECT OF CO Z 422 REDUCTION
OF STORED NO" 424
MECHANISM OF THE REDUCTION BY HZ OF STORED NO" 425
OF STORED NO" BY HZ 428 OPEN ISSUES AND FUTURE OPPORTUNITIES 432
REFERENCES 433
INDEX 439 |
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| genre | (DE-588)1071861417 Konferenzschrift gnd-content |
| genre_facet | Konferenzschrift |
| id | DE-604.BV035430052 |
| illustrated | Illustrated |
| indexdate | 2024-07-20T10:07:37Z |
| institution | BVB |
| isbn | 9783527320950 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-017350458 |
| oclc_num | 234432082 |
| open_access_boolean | |
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| owner_facet | DE-91G DE-BY-TUM DE-634 DE-1102 DE-29T DE-703 DE-83 DE-M347 |
| physical | XXII, 452 S. Ill., graph. Darst. 25 cm |
| publishDate | 2009 |
| publishDateSearch | 2009 |
| publishDateSort | 2009 |
| publisher | Wiley-VCH-Verl. |
| record_format | marc |
| spelling | Catalysis for sustainable energy production ed. by Pierluigi Barbaro ... Weinheim Wiley-VCH-Verl. 2009 XXII, 452 S. Ill., graph. Darst. 25 cm txt rdacontent n rdamedia nc rdacarrier Literaturangaben Biomass chemicals Congresses Catalysis Congresses Energy development Congresses Renewable energy sources Congresses Katalyse (DE-588)4029921-1 gnd rswk-swf Brennstoffzelle (DE-588)4008195-3 gnd rswk-swf Elektrochemische Energietechnik (DE-588)4151756-8 gnd rswk-swf Wasserstoffenergietechnik (DE-588)4121905-3 gnd rswk-swf (DE-588)1071861417 Konferenzschrift gnd-content Elektrochemische Energietechnik (DE-588)4151756-8 s Katalyse (DE-588)4029921-1 s DE-604 Brennstoffzelle (DE-588)4008195-3 s Wasserstoffenergietechnik (DE-588)4121905-3 s Barbaro, Pierluigi Sonstige oth text/html http://deposit.dnb.de/cgi-bin/dokserv?id=3112784&prov=M&dok_var=1&dok_ext=htm Inhaltstext OEBV Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=017350458&sequence=000003&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Catalysis for sustainable energy production Biomass chemicals Congresses Catalysis Congresses Energy development Congresses Renewable energy sources Congresses Katalyse (DE-588)4029921-1 gnd Brennstoffzelle (DE-588)4008195-3 gnd Elektrochemische Energietechnik (DE-588)4151756-8 gnd Wasserstoffenergietechnik (DE-588)4121905-3 gnd |
| subject_GND | (DE-588)4029921-1 (DE-588)4008195-3 (DE-588)4151756-8 (DE-588)4121905-3 (DE-588)1071861417 |
| title | Catalysis for sustainable energy production |
| title_auth | Catalysis for sustainable energy production |
| title_exact_search | Catalysis for sustainable energy production |
| title_full | Catalysis for sustainable energy production ed. by Pierluigi Barbaro ... |
| title_fullStr | Catalysis for sustainable energy production ed. by Pierluigi Barbaro ... |
| title_full_unstemmed | Catalysis for sustainable energy production ed. by Pierluigi Barbaro ... |
| title_short | Catalysis for sustainable energy production |
| title_sort | catalysis for sustainable energy production |
| topic | Biomass chemicals Congresses Catalysis Congresses Energy development Congresses Renewable energy sources Congresses Katalyse (DE-588)4029921-1 gnd Brennstoffzelle (DE-588)4008195-3 gnd Elektrochemische Energietechnik (DE-588)4151756-8 gnd Wasserstoffenergietechnik (DE-588)4121905-3 gnd |
| topic_facet | Biomass chemicals Congresses Catalysis Congresses Energy development Congresses Renewable energy sources Congresses Katalyse Brennstoffzelle Elektrochemische Energietechnik Wasserstoffenergietechnik Konferenzschrift |
| url | http://deposit.dnb.de/cgi-bin/dokserv?id=3112784&prov=M&dok_var=1&dok_ext=htm http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=017350458&sequence=000003&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT barbaropierluigi catalysisforsustainableenergyproduction |