Perovskite oxide for solid oxide fuel cells:
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| Format: | Book |
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| Language: | English |
| Published: |
New York, NY
Springer
2009
|
| Series: | Fuel cells and hydrogen energy
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| Subjects: | |
| Online Access: | Inhaltsverzeichnis |
| Physical Description: | XVI, 302 S. Ill., graph. Darst. |
| ISBN: | 9780387777078 |
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| 245 | 1 | 0 | |a Perovskite oxide for solid oxide fuel cells |c Tatsumi Ishihara ed. |
| 264 | 1 | |a New York, NY |b Springer |c 2009 | |
| 300 | |a XVI, 302 S. |b Ill., graph. Darst. | ||
| 336 | |b txt |2 rdacontent | ||
| 337 | |b n |2 rdamedia | ||
| 338 | |b nc |2 rdacarrier | ||
| 490 | 0 | |a Fuel cells and hydrogen energy | |
| 650 | 4 | |a Solid oxide fuel cells | |
| 650 | 4 | |a Perovskite | |
| 650 | 4 | |a Perovskite | |
| 650 | 4 | |a Solid oxide fuel cells | |
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| 689 | 0 | |5 DE-604 | |
| 700 | 1 | |a Ishihara, Tatsumi |e Sonstige |4 oth | |
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| 999 | |a oai:aleph.bib-bvb.de:BVB01-017098683 | ||
Record in the Search Index
| _version_ | 1804138591198117888 |
|---|---|
| adam_text | Contents
1 Structure and Properties of Perovskite Oxides
.................. 1
Tatsumi Ishihara
1.1
Introduction
....................................... 1
1.2
Structure of Perovskite Oxides
......................... 2
1.3
Typical Properties of Perovskite Oxides
.................. 7
1.4
Preparation of Perovskite Oxide
....................... 12
1.5
Perovskite Oxides for Solid Oxide Fuel Cells (SOFCs)
...... 15
References
.............................................. 16
2
Overview of Intermediate-Temperature Solid Oxide Fuel Cells
..... 17
Harumi Yokokawa
2.1
Introduction
....................................... 17
2.2
Characteristic Features of Solid Oxide Fuel Cells
.......... 18
2.2.1
Merits and Demerits of SOFCs
................... 18
2.2.2
Issues for Intermediate-Temperature SOFCs
........ 20
2.2.3
Stack Design
................................. 35
2.3
Development of Intermediate Temperature SOFC Stacks/
Systems
........................................... 36
2.3.1 Kyocera/Osaka Gas............................ 36
2.3.2
Mitsubishi Materials Corporation
................ 37
2.3.3
Micro SOFCs by
TOTO........................ 38
2.4
Perspective
........................................ 38
2.4.1
Applications
.................................. 38
2.4.2
Fuel Flexibility and Reliability in Relationship
to Intermediate-Temperature SOFCs
.............. 41
2.4.3
Hybrid Systems
............................... 41
2.5
Summary
......................................... 42
References
.............................................. 42
3
Ionic Conduction in Perovskite-Type Compounds
............... 45
Hiroyasu Iwahara
3.1
Introduction
....................................... 45
3.2
Conduction Behavior of Perovskite-Type Compounds
...... 46
viii Contents
3.3
Early Studies on Ionic Conduction in Perovskite-Type
Oxides
............................................ 49
3.4
Oxide Ion Conduction
............................... 52
3.5
Proton Conduction
.................................. 55
3.6
Lithium Ion Conduction
............................. 59
3.7
Halide Ion Conduction
............................... 60
3.8
Silver Ion Conduction
............................... 61
References
.............................................. 62
4
Oxide Ion Conductivity in Perovskite Oxide for SOFC
Electrolyte
............................................. 65
Tatsumi Ishihara
4.1
Introduction
....................................... 65
4.2
Oxide Ion Conductivity in Oxide
....................... 66
4.3
Oxide Ion Conductivity in Perovskite Oxides
............. 68
4.4
LaGaO^-Based Oxide Doped with Sr and
Mg (LSGM)
as a New Oxide Ion Conductor
........................ 71
4.4.1
Effects of Dopant for La and Ga Site
.............. 71
4.4.2
Transition Metal Doping Effects on Oxide Ion
Conductivity in LSGM
......................... 74
4.5
Basic Properties of the LSGM Electrolyte System
.......... 77
4.5.1
Phase Diagram of La-Sr-Ga-Mg-0
................ 77
4.5.2
Reactivity with SOFC Component
................ 77
4.5.3
Thermal Expansion Behavior and Other Properties
... 78
4.5.4
Behavior of Minor Carrier
...................... 79
4.5.5
Diffusivity of Oxide Ion
........................ 82
4.6
Performance of a Single Cell Using LSGM Electrolyte
...... 84
4.7
Preparation of LaGaO3 Thin-Film Electrolytes
for Application at Temperatures Lower Than
773
К
....... 87
4.8
Oxide Ion Conductivity in the Perovskite-Related
Oxides
............................................ 89
4.9
Summary
......................................... 92
References
.............................................. 92
5
Diffusivity of the Oxide Ion in Perovskite Oxides
............... 95
J. A. Kilner, A. Berenov, and J. Rossiny
5.1
Introduction
....................................... 95
. 1
Definitions of Diffusion Coefficients
.............. 96
.2
The Oxygen Tracer Diffusion Coefficient
........... 96
.3
The Surface Exchange Coefficient
................. 98
.4
Defect Chemistry and Oxygen Transport
........... 99
1.5
Defect Equilibria
.............................. 99
5.2
Diffusion in Mixed Electronic-Ionic Conducting Oxides
(MEICs)
.......................................... 102
5.2.1
Effect of
А
-Site
Cation on Oxygen Diffusivity
....... 103
Contents
5.2.2
The Effect
of
B-Site
Cation on Oxygen Diffusivity
___ 104
5.2.3
The Effect of
А
-Site
Cation Vacancies on Oxygen
Diffusivity
................................... 105
5.2.4
Temperature Dependence of the Oxygen Diffusion
Coefficient
................................... 105
5.2.5
The Effect of Oxygen Pressure
................... 108
5.3
Oxygen Diffusion in Ionic Conducting Perovskites
......... 108
5.4
Oxygen Diffusion in Perovskite-Related Materials
......... 110
5.5
Correlations Between Oxygen Diffusion Parameters
........ 110
5.6
Conclusions
....................................... 112
References
.............................................. 113
Structural Disorder, Diffusion Pathway of Mobile Oxide Ions,
and Crystal Structure in Perovskite-Type Oxides and Related
Materials
.............................................. 117
Masatomo Yashima
6.1
Introduction
....................................... 117
6.2
High-Temperature Neutron Powder Diffractometry
........ 118
6.3
Data Processing for Elucidation of the Diffusion Paths
of Mobile Oxide Ions in Ionic Conductors:
Rietveld
Analysis, Maximum Entropy Method (MEM),
and MEM-Based Pattern Fitting (MPF)
................. 120
6.4
Diffusion Path of Oxide Ions in the Fast Oxide Ion
Conductor (Lao.8Sro.2XGao.8Mgo.
15^0.05)02.8 [10]......... 121
6.4.1
Introduction
.................................. 121
6.4.2
Experiments and Data Processing
................. 121
6.4.3
Results and Discussion
......................... 122
6.5
Diffusion Path of Oxide Ions in an Oxide Ion Conductor,
La0.64(Tio.92Nb0.o8)02.99,
with a Double Perovskite-Type
Structure
[11]...................................... 126
6.5.1
Introduction
.................................. 126
6.5.2
Experiments and Data Processing
................. 126
6.5.3
Results and Discussion
......................... 127
6.6
Crystal Structure and Structural Disorder of Oxide Ions
in Cathode Materials, Lao^Sro^CoO,^ and
Lao.6Sro
^Оо.ѕРео.гОз-л,
with a Cubic Perovskite-Type
Structure
[12, 13]................................... 131
6.6.1
Introduction
.................................. 131
6.6.2
Experiments and Data Processing
................. 131
6.6.3
Results and Discussion
......................... 132
6.7
Structural Disorder and Diffusion Path of Oxide Ions in a
Doped P^NiO^Based Mixed Ionic-Electronic Conductor
(Pro.9Lao.i)2(Nio.74Cuo.2iGao.o5)04+¿
with a KzNiF^Type
Structure
[15]...................................... 137
6.7.1
Introduction
.................................. 137
к
Contents
6.7.2 Experiments and Data Processing................. 138
6.7.3
Results and Discussion
......................... 138
6.8
Conclusions
....................................... 141
References
.............................................. 143
7
Perovskite Oxide for Cathode of SOFCs
...................... 147
Tatsuya Kawada
7.1
Introduction
....................................... 147
7.2
Properties Required for a Cathode Material
.............. 148
7.2.1
Catalytic Activity
.............................. 148
7.2.2
Electronic Conductivity
......................... 149
7.2.3
Oxygen Transport (Bulk or Surface)
............... 151
7.2.4
Chemical Stability and Compatibility
.............. 152
7.2.5
Morphological Stability
......................... 152
7.3
General Description of Cathode Reaction and Polarization
. . 153
7.3.1
Oxygen Electrode Process
....................... 153
7.3.2
Equivalent Circuit for a Cathode-Electrolyte
Interface
..................................... 154
7.4
Cathode for High-Temperature SOFC: (La, Sr)MnO3
...... 156
7.4.1
Transport Properties and Electrochemical
Reaction
..................................... 156
7.4.2
Chemical and Morphological Stability of LSM
...... 158
7.5
Cathode for Intermediate-Temperature SOFC:
(La, Sr)CoO3, (La, Sr)(Co, Fe)O3
...................... 160
7.5.1
General Features of Co-Based Perovskite Cathode
... 160
7.5.2
Electrochemical Reaction of a Model Electrode:
A (La,Sr)CoO3 Dense Film
...................... 161
7.5.3
Electrochemical Response of (La, Sr)CoO3
on Zirconia with and Without
Cena Interlayer
...... 163
7.6
Summary
......................................... 164
References
.............................................. 165
8
Perovskite Oxide Anodes for SOFCs
......................... 167
J. T. S. Irvine
8.1
Introduction
....................................... 167
8.2
Anode Materials for SOFCs
.......................... 168
8.3
Perovskite Chemistry
................................ 169
8.4
Doping, Nonstoichiometry, and Conductivity
............. 170
8.5
Perovskite Anode Materials
........................... 173
8.6
A(B,B )O3 Perovskites
............................... 177
8.7
Tungsten Bronze Anode Materials
...................... 178
8.8
Anode Materials for All-Perovskite Fuel Cells
............ 179
8.9
Conclusions
....................................... 180
References
.............................................. 180
Contents xj
9
Intermediate-Temperature
Solid Oxide
Fuel Cells Using
LaGaO3............................................... 183
Tañer
Akbay
9.1
Introduction
....................................... 183
9.2
Cell Development
................................... 184
9.2.1
Electrolyte
................................... 184
9.2.2
Anode
...................................... 185
9.2.3
Cathode
..................................... 188
9.3
Stack Development
.................................. 190
9.4
Module Development
................................ 192
9.4.1
A 1-kW Class Single-Stack Module
............... 192
9.4.2
A 10-kW Class Multi-Stack Module
............... 195
9.5
System Development
................................ 196
9.6
Stack Modeling
..................................... 198
References
.............................................. 202
10
Quick-Start-Up Type SOFC Using LaGaCb-Based New
Electrolyte
............................................. 205
Akira Kawakami
10.1
Introduction
...................................... 205
10.2
Micro-Tubular Cell Development
..................... 206
10.3
Rapid Thermal Cycling
............................. 211
10.4
Fuel Flexibility
.................................... 211
10.5
Stack Development
................................. 214
10.6
Summary
......................................... 216
References
.............................................. 216
11
Proton Conductivity in Perovskite Oxides
..................... 217
Truls Norby
11.1
Introduction
...................................... 217
11.2
Proton Conductivity in Acceptor-Doped Perovskites
...... 219
1.2.1
Protons in Oxides
............................ 219
1.2.2 Hydration
of Acceptor-Doped Perovskites
......... 219
1.2.3
Proton Diffusion
............................. 222
1.2.4
Charge Mobility and Conductivity of Protons
...... 224
1.2.5
Proton Conductivity in Acceptor-Doped Simple
Perovskites, ABO3
............................ 225
11.2.6
Effects of Defect-Acceptor Interactions
........... 228
11.2.7
Grain Boundaries
............................ 229
11.3
Proton Conduction in Inherently Oxygen-Deficient
Perovskites
....................................... 230
11.3.1 Hydration
of Ordered Oxygen Deficiency
.......... 230
11.3.2
Nomenclature and
Hydration
of Disordered
Intrinsic Oxygen Deficiency
..................... 231
x¡¡
Contents
11.3.3
Order-Disorder Reactions Involving
Hydrated
Inherently Oxygen-Deficient Perovskites
(Oxyhydroxides)
............................. 232
11.4 Hydration
of Undoped Perovskites
.................... 233
11.5
Proton Conductivity in Selected Classes Of Non-Perovskite
Oxides and Phosphates
.............................. 233
11.6
Developments of Proton-Conducting SOFCs
............ 236
11.7
Conclusions
...................................... 237
References
.............................................. 238
12
Proton Conduction in Cerium- and Zirconium-Based Perovskite
Oxides
................................................ 243
Hiroshige Matsumoto
12.1
Introduction
...................................... 243
12.2
Conductivity
...................................... 245
12.3
Activation/Deactivation of Electrodes
.................. 247
12.4
Stability
.......................................... 248
12.5
Dopant
.......................................... 251
12.6
Proton Hole Mixed Conduction
....................... 255
References
.............................................. 258
13
Mechanisms of Proton Conduction in Perovskite-Type
Oxides
................................................ 261
K. D. Kreuer
13.1
Introduction
...................................... 261
13.2
Proton Sites
...................................... 262
13.3
Mechanisms of Proton Conduction (Undoped, Cubic
Perovskites)
....................................... 264
13.4
Complications (Symmetry Reduction, Doping, Mixed
Site Occupancy)
................................... 268
13.5
Implications for the Development of Proton-Conducting
Electrolytes for Fuel Cell Applications
................. 270
References
.............................................. 271
14
Intermediate-Temperature SOFCs Using Proton-Conducting
Perovskite
............................................. 273
Naoki
Ito
14.1
Introduction
...................................... 273
14.2
Preparation of Fuel Cells
............................ 277
14.3
Characterization of Fuel Cells
........................ 277
14.4
Operation and Evaluation of Fuel Cells
................. 279
14.5
Conclusion
....................................... 282
References
.............................................. 283
Contents xiii
15 LaCrCb-Based Perovskite
for SOFC Interconnects
.............. 285
Teruhisa
Horită
15.1
Introduction......................................
285
15.2
Sintering Properties and Chemical Compatibility
with the Other Components
.......................... 286
15.3
Electronic Conductivity
............................. 287
15.4
Defect Chemistry and Oxygen Electrochemical Leak
...... 289
15.5
Lattice Expansion During Reduction and Temperature
Change
.......................................... 293
15.6
Mechanical Strength
................................ 293
15.7
Summary
......................................... 294
References
.............................................. 295
Index
..................................................... 297
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| id | DE-604.BV035293677 |
| illustrated | Illustrated |
| indexdate | 2024-07-09T21:30:37Z |
| institution | BVB |
| isbn | 9780387777078 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-017098683 |
| oclc_num | 262509430 |
| open_access_boolean | |
| owner | DE-703 |
| owner_facet | DE-703 |
| physical | XVI, 302 S. Ill., graph. Darst. |
| publishDate | 2009 |
| publishDateSearch | 2009 |
| publishDateSort | 2009 |
| publisher | Springer |
| record_format | marc |
| series2 | Fuel cells and hydrogen energy |
| spelling | Perovskite oxide for solid oxide fuel cells Tatsumi Ishihara ed. New York, NY Springer 2009 XVI, 302 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Fuel cells and hydrogen energy Solid oxide fuel cells Perovskite Festoxidbrennstoffzelle (DE-588)4811042-5 gnd rswk-swf Perowskit (DE-588)4173836-6 gnd rswk-swf Perowskit (DE-588)4173836-6 s Festoxidbrennstoffzelle (DE-588)4811042-5 s DE-604 Ishihara, Tatsumi Sonstige oth Digitalisierung UB Bayreuth application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=017098683&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Perovskite oxide for solid oxide fuel cells Solid oxide fuel cells Perovskite Festoxidbrennstoffzelle (DE-588)4811042-5 gnd Perowskit (DE-588)4173836-6 gnd |
| subject_GND | (DE-588)4811042-5 (DE-588)4173836-6 |
| title | Perovskite oxide for solid oxide fuel cells |
| title_auth | Perovskite oxide for solid oxide fuel cells |
| title_exact_search | Perovskite oxide for solid oxide fuel cells |
| title_full | Perovskite oxide for solid oxide fuel cells Tatsumi Ishihara ed. |
| title_fullStr | Perovskite oxide for solid oxide fuel cells Tatsumi Ishihara ed. |
| title_full_unstemmed | Perovskite oxide for solid oxide fuel cells Tatsumi Ishihara ed. |
| title_short | Perovskite oxide for solid oxide fuel cells |
| title_sort | perovskite oxide for solid oxide fuel cells |
| topic | Solid oxide fuel cells Perovskite Festoxidbrennstoffzelle (DE-588)4811042-5 gnd Perowskit (DE-588)4173836-6 gnd |
| topic_facet | Solid oxide fuel cells Perovskite Festoxidbrennstoffzelle Perowskit |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=017098683&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT ishiharatatsumi perovskiteoxideforsolidoxidefuelcells |