Asymmetric biocatalytic epoxidation in a scalable electrochemical reactor using FAD-dependent styrene monooxygenase:
Saved in:
| Main Author: | |
|---|---|
| Format: | Thesis Book |
| Language: | English |
| Published: |
Aachen
Shaker
2010
|
| Series: | Chemical biotechnology
2 |
| Subjects: | |
| Online Access: | Inhaltsverzeichnis |
| Physical Description: | XIV, 175 S. Ill., graph. Darst. |
| ISBN: | 9783832287924 |
Staff View
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| 245 | 1 | 0 | |a Asymmetric biocatalytic epoxidation in a scalable electrochemical reactor using FAD-dependent styrene monooxygenase |c Reto Ruinatscha |
| 264 | 1 | |a Aachen |b Shaker |c 2010 | |
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Record in the Search Index
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| adam_text | IMAGE 1
IV
TABLE OF CONTENTS
SUMMARY VI
ZUSAMMENFASSUNG VIL
LIST OF ABBREVIATIONS X
CHAPTER 1: INTRODUCTION 1
1.1 GENERAL INTRODUCTION 2
1.2 FLAVIN-DEPENDENT MONOOXYGENASES 3
1.2.} ONE-COMPONENT FLAVIN-DEPENDENT MONOOXYGENASES 5
1.2.2 TWO-COMPONENT FLAVIN-DEPENDENT MONOOXYGENASES 6
1.3 COFACTOR REGENERATION 9
1.4 OPERATIONAL WINDOWS OF ELECTROENZYMATIC PROCESSES 11
1.5 EVALUATION OF PROMISING ELECTROENZYMATIC PROCESSES WITH SYNTHETIC
POTENTIAL 15
1.6 PARAMETERS THAT LIMIT THE PERFORMANCE OF ELECTROENZYMATIC PROCESSES
AND PROMISING
DEVELOPMENTS IN REACTION ENGINEERING 21
1.7 CONCLUDING REMARKS AND FUTURE PROSPECTS 24
1.8 SCOPE OF THE THESIS 25
CHAPTER 2: DEVELOPMENT OF A HIGH PERFORMANCE ELECTROCHEMICAL COFACTOR
REGENERATION
MODULE AND ITS APPLICATION TO THE CONTINUOUS REDUCTION OF FAD 27
CHAPTER 3: PRODUCTIVE ASYMMETRIC STYRENE EPOXIDATTON BASED ON A NEXT
GENERATION
ELECTROENZYMATIC METHODOLOGY
CHAPTER 4: INTEGRATED ONE-POT ENRICHMENT AND IMMOBILIZATION OF STYRENE
MONOOXYGENASE
(STYA) USING SEPABEAD EC-EA AND EC-Q1A ANION-EXCHANGE CARRIERS
CHAPTER 5: CATALYST DESIGN AND CHARACTERIZATION FOR CELL-FREE
EPOXIDATIONS BASED ON
STYRENE MONOOXYGENASE (STYA) IMMOBILIZED ON SEPABEADS EC-EP
BIBLIOGRAFISCHE INFORMATIONEN HTTP://D-NB.INFO/1000544044
DIGITALISIERT DURCH
IMAGE 2
CHAPTER 6: SYNTHESIS AND EVALUATION OF 5-DEAZA FLAVIN ADENINE
DINUCLEOTIDE AS AN ARTIFICIAL
COFACTOR FOR THE TWO-COMPONENT STYRENE MONOOXYGENASE S T Y AB 105
CHAPTER 7: CONCLUDING REMARKS AND OUTLOOK 125
7.1 STATE OFTHE ART IN ELECTROENZYMATIC SYNTHESIS PERFORMANCE AND
REACTOR ENGINEERING 126
7.2 FACTORS INFLUENCING ELECTROCHEMICAL COFACTOR REGENERATION RATES 127
7.3 DEVELOPMENT OF A NOVEL, PRODUCTIVE AND SCALABLE ELECTROENZYMATIC
REACTOR CONCEPT 129
7.4 ELECTROENZYMATIC SYNTHESIS OF (S)-STYRENE OXIDE USING THE DEVELOPED
COFACTOR REGENERATION
CONCEPT 132
7.5 EXPLOITATION OF THE CATALYTIC PROPERTIES OF IMMOBILIZED STYA 139
7.5.1 ADSORPTIVE IMMOBILIZATION OF STYA ON SEPABEADS EC-EA AND EC-Q1A
139
7.5.2 COVALENT IMMOBILIZATION OF STYA ON SEPABEADS **-EP 141
7.6 CHALLENGING THE OXYGEN DILEMMA USING AN ARTIFICIAL COFACTOR 143
7.7 OUTLOOK 145
REFERENCES 147
CURRICULUM VITAE 173
|
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| id | DE-604.BV026780085 |
| illustrated | Illustrated |
| indexdate | 2024-07-09T23:18:52Z |
| institution | BVB |
| isbn | 9783832287924 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-022314845 |
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| owner_facet | DE-188 |
| physical | XIV, 175 S. Ill., graph. Darst. |
| publishDate | 2010 |
| publishDateSearch | 2010 |
| publishDateSort | 2010 |
| publisher | Shaker |
| record_format | marc |
| series | Chemical biotechnology |
| series2 | Chemical biotechnology |
| spelling | Ruinatscha, Reto 1978- Verfasser (DE-588)140716297 aut Asymmetric biocatalytic epoxidation in a scalable electrochemical reactor using FAD-dependent styrene monooxygenase Reto Ruinatscha Aachen Shaker 2010 XIV, 175 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Chemical biotechnology 2 Zugl: Dortmund, Techn. Univ., Diss., 2009 Enzymkatalyse (DE-588)4152480-9 gnd rswk-swf Elektrokatalyse (DE-588)4151819-6 gnd rswk-swf Asymmetrische Synthese (DE-588)4135603-2 gnd rswk-swf Styroloxid (DE-588)7704126-4 gnd rswk-swf Epoxidation (DE-588)4152560-7 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Styroloxid (DE-588)7704126-4 s Asymmetrische Synthese (DE-588)4135603-2 s Epoxidation (DE-588)4152560-7 s Enzymkatalyse (DE-588)4152480-9 s Elektrokatalyse (DE-588)4151819-6 s DE-604 Chemical biotechnology 2 (DE-604)BV026780082 2 DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=022314845&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Ruinatscha, Reto 1978- Asymmetric biocatalytic epoxidation in a scalable electrochemical reactor using FAD-dependent styrene monooxygenase Chemical biotechnology Enzymkatalyse (DE-588)4152480-9 gnd Elektrokatalyse (DE-588)4151819-6 gnd Asymmetrische Synthese (DE-588)4135603-2 gnd Styroloxid (DE-588)7704126-4 gnd Epoxidation (DE-588)4152560-7 gnd |
| subject_GND | (DE-588)4152480-9 (DE-588)4151819-6 (DE-588)4135603-2 (DE-588)7704126-4 (DE-588)4152560-7 (DE-588)4113937-9 |
| title | Asymmetric biocatalytic epoxidation in a scalable electrochemical reactor using FAD-dependent styrene monooxygenase |
| title_auth | Asymmetric biocatalytic epoxidation in a scalable electrochemical reactor using FAD-dependent styrene monooxygenase |
| title_exact_search | Asymmetric biocatalytic epoxidation in a scalable electrochemical reactor using FAD-dependent styrene monooxygenase |
| title_full | Asymmetric biocatalytic epoxidation in a scalable electrochemical reactor using FAD-dependent styrene monooxygenase Reto Ruinatscha |
| title_fullStr | Asymmetric biocatalytic epoxidation in a scalable electrochemical reactor using FAD-dependent styrene monooxygenase Reto Ruinatscha |
| title_full_unstemmed | Asymmetric biocatalytic epoxidation in a scalable electrochemical reactor using FAD-dependent styrene monooxygenase Reto Ruinatscha |
| title_short | Asymmetric biocatalytic epoxidation in a scalable electrochemical reactor using FAD-dependent styrene monooxygenase |
| title_sort | asymmetric biocatalytic epoxidation in a scalable electrochemical reactor using fad dependent styrene monooxygenase |
| topic | Enzymkatalyse (DE-588)4152480-9 gnd Elektrokatalyse (DE-588)4151819-6 gnd Asymmetrische Synthese (DE-588)4135603-2 gnd Styroloxid (DE-588)7704126-4 gnd Epoxidation (DE-588)4152560-7 gnd |
| topic_facet | Enzymkatalyse Elektrokatalyse Asymmetrische Synthese Styroloxid Epoxidation Hochschulschrift |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=022314845&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| volume_link | (DE-604)BV026780082 |
| work_keys_str_mv | AT ruinatschareto asymmetricbiocatalyticepoxidationinascalableelectrochemicalreactorusingfaddependentstyrenemonooxygenase |