Excitonic processes in solids:
Gespeichert in:
| Format: | Buch |
|---|---|
| Sprache: | English |
| Veröffentlicht: |
Berlin ; Heidelberg ; New York ; Tokyo
Springer
1986
|
| Schriftenreihe: | Springer series in solid-state sciences
60 |
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | Literaturverz. S. 499 - 519 |
| Beschreibung: | XII, 530 S. zahlr. graph. Darst. |
| ISBN: | 3540158898 0387158898 |
Internformat
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| 245 | 1 | 0 | |a Excitonic processes in solids |c by M. Ueta ... |
| 264 | 1 | |a Berlin ; Heidelberg ; New York ; Tokyo |b Springer |c 1986 | |
| 300 | |a XII, 530 S. |b zahlr. graph. Darst. | ||
| 336 | |b txt |2 rdacontent | ||
| 337 | |b n |2 rdamedia | ||
| 338 | |b nc |2 rdacarrier | ||
| 490 | 1 | |a Springer series in solid-state sciences |v 60 | |
| 500 | |a Literaturverz. S. 499 - 519 | ||
| 650 | 0 | 7 | |a Festkörper |0 (DE-588)4016918-2 |2 gnd |9 rswk-swf |
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| 689 | 1 | 0 | |a Exziton |0 (DE-588)4016091-9 |D s |
| 689 | 1 | |5 DE-604 | |
| 700 | 1 | |a Ueta, Masayasu |e Sonstige |4 oth | |
| 830 | 0 | |a Springer series in solid-state sciences |v 60 |w (DE-604)BV000016582 |9 60 | |
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Datensatz im Suchindex
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CONTENTS
1. INTRODUCTION . 1
1.1 THE GROUND STATE OF MANY-BODY SYSTEMS AND THE MODES OF
EXCITATION. 1
1.2 ELECTRONIC EXCITATION IN INSULATORS AND THE WANNIER-MOTT EXCITON 3
1.3 THE FRENKEL EXCITON. 5
1.4 THE GENERAL CASE. 6
1.4.1 EFFECTIVE MASS APPROXIMATION . 8
1.4.2 THE ROLE OF SPIN. 8
1.4.3 INTERPLAY OF SPIN-ORBIT AND EXCHANGE INTERACTIONS . 9
1.4.4 DAVYDOV SPLITTING. 10
1.4.5 CHARGE TRANSFER EXCITONS. 10
1.5 OPTICAL ABSORPTION SPECTRA. 11
1.5.1 ALLOWED EDGE CASE. 12
1.5.2 FORBIDDEN EDGE CASE. 13
1.5.3 TRANSITION FROM FRENKEL TO WANNIER-MOTT EXCITON . 13
1.6 THE POLARITON AND SPATIAL DISPERSION . 15
1.7 SCOPE OF THE PRESENT BOOK. 18
2. THEORETICAL ASPECTS OF EXCITONIC MOLECULES. 20
2.1 FISSION AND FUSION OF EXCITONS VS. CHEMICAL REACTION INTO
EXCITONIC MOLECULES. 20
2.2 THE EXCITONIC MOLECULE AND ELECTRON-HOLE LIQUID . 23
2.2.1 BINDING ENERGY AND ELECTRONIC STRUCTURE OF EXCITONIC
MOLECULE IN A SIMPLE SYSTEM - CUX. 23
2.2.2 THE METALLIC DROPLET AND EXCITONIC MOLECULE IN
MANY-VALLEY STRUCTURES - GE AND SI. 32
2.2.3 THE EXCITONIC MOLECULE IN MANY-VALLEY SYSTEMS - T1X AND
AGX. . 39
2.2.4 INFLUENCE OF THE POLARIZABLE LATTICE AND THE EFFECT OF
ANISOTROPIC EFFECTIVE MASS - CDS AND CDSE. 44
2.2.5 THE DIRECT FORBIDDEN EXCITON - CU20. 46
2.3 OPTICAL RESPONSE OF AN EXCITONIC MOLECULE. 47
2.3.1 LUMINESCENCE SPECTRUM. 48
2.3.2 RELAXATION BY EMISSION OF ACOUSTIC PHONONS. 55
2.3.3 OPTICAL CONVERSION OF EXCITONS INTO EXCITONIC MOLECULES . 60
2.3.4 GIANT TWO-PHOTON ABSORPTION . 61
BIBLIOGRAFISCHE INFORMATIONEN
HTTP://D-NB.INFO/860086534
VIII CONTENTS
R
2.4 COHERENT OPTICAL PHENOMENA DUE TO THE EXCITONIC MOLECULE . 69
2.4.1 HYPER-RAMAN SCATTERING AND LUMINESCENCE . 69
2.4.2 TWO-POLARITON SCATTERING DUE TO THE EXCITONIC MOLECULE . 75
2.4.3 DISPERSION OF THE EXCITON POLARITON AND EXCITONIC
MOLECULE. 79
2.4.4 FOUR-WAVE MIXING DUE TO THE EXCITONIC MOLECULE . 83
2.4.5 PHASE-CONJUGATION BY FOUR-WAVE MIXING. 87
2.5 THE EXCITONIC MOLECULE AT HIGH DENSITIES. 91
2.5.1 RENORMALIZATION OF THE EXCITON POLARITON DUE TO THE
EXCITONIC MOLECULE GIANT TWO-PHOTON ABSORPTION . 91
2.5.2 POLARIZATION ROTATION EFFECTS DUE TO TWO-PHOTON
EXCITATION OF THE EXCITONIC MOLECULE . 95
2.5.3 MULTI-POLARITON SCATTERING VIA EXCITONIC MOLECULES . 102
2.5.4 OPTICAL BISTABILITY DUE TO THE EXCITONIC MOLECULE. 106
2.5.5 RELAXATION AND BOSE CONDENSATION OF EXCITONIC
MOLECULES. 110
3. THE EXCITON AND EXCITONIC MOLECULE IN CUPROUS HALIDES . 116
3.1 BAND STRUCTURE AND EXCITONIC STATES. 116
3.2 EXCITON ABSORPTION, REFLECTION, AND EMISSION SPECTRA. 117
3.2.1 ABSORPTION AND REFLECTION SPECTRA . 117
3.2.2 SPLITTING OF EXCITON BANDS BY PERTURBATIONS. 119
3.2.3 EMISSION SPECTRA . 121
3.2.4 PHONON STRUCTURE IN THE EXCITATION SPECTRA OF FREE-EXCITON
EMISSION. 125
3.2.5 BOUND EXCITONS. 127
3.2.6 CUCL-CUBR SOLID SOLUTIONS . 129
3.3 HIGH-DENSITY EXCITATION EFFECTS. 132
3.3.1 EXCITON-ELECTRON INTERACTION . 132
3.3.2 EFFECT ON EXCITON ABSORPTION BANDS. 136
3.3.3 CREATION OF THE EXCITONIC MOLECULE BY EXCITON-EXCITON
COLLISION. 140
3.4 GIANT TWO-PHOTON EXCITATION OF THE EXCITONIC MOLECULE . 144
3.4.1 EVIDENCE OF GIANT TWO-PHOTON CREATION . 144
3.4.2 GIANT TWO-PHOTON ABSORPTION . 146
3.5 TWO-PHOTON RESONANT RAMAN SCATTERING VIA THE EXCITONIC
MOLECULE. 148
3.5.1 BACKWARD SCATTERING. 148
3.5.2 FORWARD SCATTERING . 150
3.5.3 SCATTERING WITH RECOIL OF THE UPPER-BRANCH POLARITON . . . 152
3.5.4 POLARIZATION CHARACTER - GEOMETRICAL SELECTION RULES . . . 154
3.5.5 NONLINEAR CHANGE OF EXDTON-POLARITON DISPERSION
ASSOCIATED WITH THE GTA. 155
3.6 ACOUSTIC-PHONON INTERACTION OF THE EXCITONIC MOLECULE. 161
CONTENTS
IX
3.7 COEXISTENCE OF LUMINESCENCE AND RAMAN COMPONENTS IN THE
RESONANT EXCITATION. 166
3.8 REDISTRIBUTION OF EXCITONIC MOLECULES RESONANTLY GENERATED BY
TWO-PHOTON EXCITATION . 170
3.8.1 CALCULATION OF LINE-SHAPES OF THE EXCITONIC MOLCECULE
LUMINESCENCE. 172
3.9 RELAXATION OF THE EXCITONIC MOLECULE DUE TO INTERMOLECULAR
COLLISIONS: INFLUENCE ON THE GTA AND SECONDARY EMISSIONS . 174
3.9.1 EFFECT ON THE GTA SPECTRA . 175
3.9.2 EFFECT ON SECONDARY EMISSIONS . 176
3.10 SPATIAL DISPERSION OF THE EXCITON AND EXCITONIC MOLECULE. 181
3.10.1 CUCL. 182
3.10.2 CUBR. 188
3.11 HIGHER EXCITED STATES OF THE EXCITONIC MOLECULE. 200
4. THEORY OF EXCITONS IN PHONON FIELDS . 203
4.1 ELECTRON-PHONON INTERACTIONS. 204
4.1.1 TYPES AND RANGES OF ELECTRON-PHONON INTERACTIONS . 204
4.1.2 THEPOLARON. 208
4.1.3 EXCITON-PHONON INTERACTIONS AND THE FORM FACTOR . 210
4.1.4 POLARON EFFECTS OF AN EXCITON. 211
4.2 THE EXCITON IN SPATIALLY FLUCTUATING FIELDS . 212
4.2.1 LOCALIZATION VERSUS DELOCALIZATION . 212
4.2.2 OVERALL LINE-SHAPE OF THE ABSORPTION SPECTRA. 215
4.2.3 COHERENT POTENTIAL APPROXIMATION FOR AN EXCITON IN A
MIXED CRYSTAL AND IN A PHONON FIELD. 220
4.2.4 THE URBACH RULE AND EXCITON LOCALIZATION. 228
4.3 PHONON STRUCTURES IN EXCITON SPECTRA. 234
4.3.1 MOTIONAL REDUCTION OF PHONON SIDEBANDS. 235
4.3.2 MULTICOMPONENT LINE-SHAPE FORMULA. 238
4.3.3 THE ELECTRON-HOLE RELATIVE MOTION AND THE PHONON
SIDEBAND OF AN EXCITON . 242
4.4 SELF-TRAPPING . 245
4.4.1 LOCAL STABILITIES OF FREE AND SELF-TRAPPED STATES . 245
4.4.2 CONTINUUM MODEL FOR SELF-TRAPPING. 247
4.4.3 ADIABATIC POTENTIALS FOR SELF-TRAPPING. 250
4.4.4 EFFECTIVE MASS CHANGE IN THE F-S TRANSITION . 254
4.4.5 EXTRINSIC SELF-TRAPPING AND SHALLOW-DEEP INSTABILITY . . . 258
4.4.6 INSTABILITIES IN THE RELATIVE MOTION OF A PAIR OF CHARGED
PARTICLES. 260
4.4.7 SURVEY OF EXPERIMENTAL STUDIES OF SELF-TRAPPING AND
RELATED INSTABILITIES. 264
4.5 ELECTRON-HOLE RECOMBINATION. 270
4.5.1 POLARITON BOTTLENECK. 270
X
CONTENTS
4.5.2 RESONANT SECONDARY RADIATION. 272
4.5.3 CAPTURE, RECOMBINATION, AND ENHANCED DEFECT REACTION
VIA A DEEP IMPURITY LEVEL IN A SEMICONDUCTOR. 273
4.5.4 SELF-TRAPPING AND RECOMBINATION OF AN EXCITON AS A
MULTIPHONON PROCESS . 275
4.6 EXCITONIC INSTABILITY AND PHASE CHANGES. 276
4.6.1 T-U-S PROBLEM. 278
4.6.2 TWO-SITE TWO-ELECTRON SYSTEM. 278
4.6.3 HIICKEL'S (4N + 2) RULE FOR RING SYSTEMS . 280
4.6.4 ONE-DIMENSIONAL HUBBARD-PEIERLS SYSTEM. 282
4.6.5 PROSPECTS . 283
5. EXCITONS IN CONDENSED RARE GASES. 285
5.1 ELECTRONIC STRUCTURE OF CONDENSED RARE GASES. 286
5.2 CHARGE CARRIERS IN CONDENSED RARE GASES. 288
5.3 EXCITONS AND EXCITON-PHONON INTERACTIONS IN CONDENSED RARE
GASES . 290
5.3.1 EXCITON ABSORPTION SPECTRA. 292
5.3.2 NATURE OF RELAXED EXCITONS IN CONDENSED RARE GASES . . 295
5.3.3 FORMATION OF SELF-TRAPPED EXCITON BUBBLES IN CONDENSED
NEON. 300
5.3.4 RELAXATION OF FREE EXCITONS IN PHOTO-EXCITED RARE GAS
SOLIDS . 305
6. EXCITON-PHONON PROCESSES IN SILVER HALIDES. 309
6.1 ELECTRONIC AND LATTICE PROPERTIES OF SILVER HALIDES . 309
6.2 EXCITONS AND EXCITON-PHONON INTERACTIONS IN SILVER HALIDES . 316
6.2.1 EXCITON TRANSITIONS IN PURE CRYSTALS. 317
6.2.2 EXCITON TRANSITIONS IN MIXED CRYSTALS. 331
6.2.3 BOUND-EXCITON TRANSITIONS AT AN ISOELECTRONIC IODINE
IMPURITY. 339
6.3 RELAXATION PROCESSES OF PHOTO-EXCITED STATES IN SILVER AND ALKALI
HALIDES. 347
6.4 LOCALIZED ELECTRONS AND HOLES IN SILVER HALIDES. 351
6.4.1 NATURE OF LOCALIZED CENTERS IN SILVER HALIDES COMPARED TO
COLOR CENTERS IN ALKALI HALIDES. 352
6.4.2 BOUND POLARONS IN SILVER AND ALKALI HALIDES. 358
6.4.3 PHOTOCHEMICAL REACTIONS IN SILVER HALIDES AT HIGHER
TEMPERATURES. 364
7. EXCITONS AND THEIR INTERACTIONS WITH PHONONS AND EXTERNAL FIELDS IN
THALLOUS HALIDES . 370
7.1 BAND STRUCTURES AND EXCITON STATES OF THALLOUS HALIDES. 371
7.1.1 THALLOUS HALIDES. 371
CONTENTS
XI
7.1.2 BAND STRUCTURES. 372
7.1.3 EXCITON STATES. 374
7.2 OPTICAL SPECTRA OF THALLOUS HALIDES. 378
7.2.1 ABSORPTION AND REFLECTION SPECTRA IN A WIDE ENERGY
RANGE. 378
7.2.2 SPECTRA OF XG X X^ DIRECT EXCITONS. 380
7.2.3 SPECTRA OF X X R^ INDIRECT EXCITONS. 388
7.2.4 FREE-EXCITON EMISSION. 392
7.2.5 EXCITONIC MOLECULES OF X X R^ EXCITONS. 398
7.3 RESONANT RAMAN SCATTERING BY EXCITONS IN THALLOUS HALIDES . . . 403
7.3.1 LO PHONON SCATTERING RESONANT TO A DIRECT EXCITON . . . 403
7.3.2 INTERVALLEY SCATTERING OF A DIRECT EXCITON. 411
7.4 EXCITONS AND INDUCED SELF-TRAPPING IN MIXED CRYSTALS OF THALLOUS
HALIDES. 412
7.4.1 EXCITON STATES IN A MIXED CRYSTAL. 412
7.4.2 SELF-TRAPPING INDUCED BY ALLOYING . 418
7.5 EXCITONS IN THALLOUS HALIDES IN EXTERNAL FIELDS. 422
7.5.1 MAGNETIC FIELD. 422
7.5.2 ELECTRIC FIELD . 432
7.5.3 UNIAXIAL STRESS FIELD. 435
8. PHOTOCARRIER MOTION IN IONIC CRYSTALS. 437
8.1 PHOTOCURRENT AND MEASUREMENT. 438
8.1.1 PHOTOCURRENT. 438
8.1.2 BLOCKING ELECTRODE METHOD AND RESPONSE . 439
8.1.3 SPECTRAL DEPENDENCE OF PHOTOCONDUCTIVITY. 442
8.2 MEASUREMENTS OF CARRIER MOBILITY AND CYCLOTRON RESONANCE IN
INSULATING PHOTOCONDUCTORS. 444
8.2.1 CARRIER MOBILITY. 444
8.2.2 DRIFT MOBILITY MEASUREMENT. 447
8.2.3 HALL AND MAGNETORESISTANCE MOBILITY MEASUREMENTS . . . 447
8.2.4 DETECTION OF CYCLOTRON RESONANCE . 450
8.3 POLARON AND MOBILITY . 451
8.3.1 POLARON MASSES AND COUPLING CONSTANTS. 451
8.3.2 POLARON MOBILITIES. 452
8.4 MAGNETOCONDUCTIVITY . 461
8.4.1 SPIN-DEPENDENT MAGNETOCONDUCTIVITY. 461
8.4.2 PHOTOMAGNETOCURRENT. 464
8.5 POLARONS WITH HIGH ENERGY . 468
8.5.1 NONPARABOLICITY OF THE POLARON ENERGY SPECTRUM. 468
8.5.2 HOT-POLARON TRANSPORT PHENOMENA. 470
9. EXCITONS AND PHONON COUPLINGS IN QUASI-ONE-DIMENSIONA! CRYSTALS . .
475
9.1 HALOGEN-BRIDGED MIXED-VALENCE CHAIN COMPOUNDS . . 476
9.2 POLY ACETYLENE. 482
XII
CONTENTS
9.3 MIXED STACKED DONOR-ACCEPTOR CHARGE TRANSFER COMPLEXES . 489
9.4 SEGREGATED STACKED DONOR-ACCEPTOR CHARGE TRANSFER COMPLEXES 495
REFERENCES. 499
SUBJECT INDEX. 521 |
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| id | DE-604.BV025873402 |
| illustrated | Illustrated |
| indexdate | 2024-08-27T00:25:21Z |
| institution | BVB |
| isbn | 3540158898 0387158898 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-019120610 |
| oclc_num | 260113274 |
| open_access_boolean | |
| owner | DE-11 |
| owner_facet | DE-11 |
| physical | XII, 530 S. zahlr. graph. Darst. |
| publishDate | 1986 |
| publishDateSearch | 1986 |
| publishDateSort | 1986 |
| publisher | Springer |
| record_format | marc |
| series | Springer series in solid-state sciences |
| series2 | Springer series in solid-state sciences |
| spelling | Excitonic processes in solids by M. Ueta ... Berlin ; Heidelberg ; New York ; Tokyo Springer 1986 XII, 530 S. zahlr. graph. Darst. txt rdacontent n rdamedia nc rdacarrier Springer series in solid-state sciences 60 Literaturverz. S. 499 - 519 Festkörper (DE-588)4016918-2 gnd rswk-swf Exziton (DE-588)4016091-9 gnd rswk-swf Exziton (DE-588)4016091-9 s Festkörper (DE-588)4016918-2 s DE-604 Ueta, Masayasu Sonstige oth Springer series in solid-state sciences 60 (DE-604)BV000016582 60 DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=019120610&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Excitonic processes in solids Springer series in solid-state sciences Festkörper (DE-588)4016918-2 gnd Exziton (DE-588)4016091-9 gnd |
| subject_GND | (DE-588)4016918-2 (DE-588)4016091-9 |
| title | Excitonic processes in solids |
| title_auth | Excitonic processes in solids |
| title_exact_search | Excitonic processes in solids |
| title_full | Excitonic processes in solids by M. Ueta ... |
| title_fullStr | Excitonic processes in solids by M. Ueta ... |
| title_full_unstemmed | Excitonic processes in solids by M. Ueta ... |
| title_short | Excitonic processes in solids |
| title_sort | excitonic processes in solids |
| topic | Festkörper (DE-588)4016918-2 gnd Exziton (DE-588)4016091-9 gnd |
| topic_facet | Festkörper Exziton |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=019120610&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| volume_link | (DE-604)BV000016582 |
| work_keys_str_mv | AT uetamasayasu excitonicprocessesinsolids |