Chemical ozone loss in the arctic polar stratosphere: an analysis of twelve years of satellite observations
Saved in:
| Main Author: | |
|---|---|
| Format: | Thesis Book |
| Language: | English |
| Published: |
Jülich
Forschungszentrum, Zentralbibliothek
2004
|
| Series: | Schriften des Forschungszentrums Jülich
Reihe Umwelt ; 43 |
| Subjects: | |
| Online Access: | Inhaltsverzeichnis |
| Physical Description: | V, 162 S. Ill., graph. Darst. 24 cm |
| ISBN: | 3893363475 |
Staff View
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Record in the Search Index
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| adam_text | Titel: Chemical ozone loss in the arctic polar stratosphere
Autor: Tilmes, Simone
Jahr: 2004
Contents
Abstract i
1 Introduction 1
1.1 Stratospheric Ozone - Overview .................. 1
1.2 Polar Ozone Depletion........................ 5
2 Stratospheric Chemistry 9
2.1 The Chemistry of Stratospheric Ozone............... 9
2.1.1 Loss Cycles of Ozone .................... 9
2.1.2 Chlorine-Containing Trace Species ............. 11
2.2 The Chemistry of Stratospheric Polar Ozone ........... 12
2.2.1 Polar Stratospheric Clouds (PSCs) and Sulphate Aerosols 12
2.2.2 Heterogeneous Chemistry .................. 13
2.2.3 Deactivation of Chlorine................... 14
2.2.4 Denitrification ........................ 15
3 The Arctic Polar Vortex 17
3.1 Dynamics of the Stratospheric Polar Vortex ............ 17
3.1.1 The Polar Vortex Edge Region ............... 22
3.2 Dynamical Tracers.......................... 23
3.3 Total Ozone in High Northern Latitudes Based on TOMS Obser-
vations ................................ 24
4 The Quantification of Chemical Ozone Loss in the Polar Region 29
4.1 The Principles of the Tracer-Tracer Correlation (TRAC) Tech-
nique ................................. 30
4.2 Presentation of Several Methods of Calculating Ozone Loss ... 35
4.3 Criticism of the TRAC Technique ................. 37
4.4 Specific Improvements and Extentions in the TRAC Methodology 39
4.4.1 New Methodology for the Meteorological Analysis .... 39
4.4.2 Improved Determination of the Early Winter Reference
Function ........................... 41
4.4.3 Specific Improvements to the HALOE Analysis ...... 45
iii
iv Contents
5 Verification of the (TRAC) Technique Using ILAS Data in 1996-
97 47
5.1 Meteorology of the Polar Vortex 1996-97 ............. 47
5.2 Evolution of Ozone-Tracer Relations in the Early Vortex..... 49
5.3 Evolution of Ozone Loss over the Entire Lifetime of the Vortex . 51
5.4 Influence of Mixing on the Ozone-Tracer Relationship ...... 54
6 Re-analysis of HALOE and ILAS Observations in Winter 1996-
97 57
6.1 Comparison of ILAS and HALOE Ozone Observations ...... 57
6.2 Ozone Loss in the Winter 1996^97, ILAS and HALOE in Comparison 60
6.2.1 Ozone Loss Derived From HALOE Measurements..... 60
6.2.2 Ozone Loss Derived From ILAS Measurements ...... 70
6.2.3 Comparison of HALOE and ILAS Results......... 70
7 Development of the Tracer-Tracer Relation from 1991 to 2003 75
7.1 The CH4/HF Relation for all Winters ............... 75
7.2 The Early Winter Ozone-Tracer Reference Relation........ 79
7.3 Meteorological Conditions and the HCl-Tracer and O3-Tracer Re-
lation in Arctic Winters 1991-2003................. 87
8 Column Ozone Loss and Ozone Loss Profiles 95
8.1 Vertical Ozone Loss Profiles in Arctic Winters 1991-2003 .... 95
8.2 Column Ozone Loss in Arctic Winters 1991-2003......... 99
8.3 Discussion of the TRAC Technique................. 106
9 Comparison of Results With Earlier Studies 111
9.1 HALOE Results in Comparison With Earlier Studies Based on
HALOE................................ Ill
9.2 Comparison of Ozone Loss Derived Using Different Methods ... 114
9.3 Impact of Meteorological Conditions on Ozone Loss........ 119
10 Summary and Outlook 125
A Satellite Measurements 127
A.I ILAS .................................127
A.2 HALOE................................128
B Tracer-Tracer Reference Relations 131
List of Figures 137
List of Tables 141
Abbreviations and Symbols 143
Bibliography 147
Contents____________________________________________________ v
Acknowledgements 161
|
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| id | DE-604.BV023831555 |
| illustrated | Illustrated |
| indexdate | 2024-07-09T21:37:37Z |
| institution | BVB |
| isbn | 3893363475 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-017473716 |
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| physical | V, 162 S. Ill., graph. Darst. 24 cm |
| publishDate | 2004 |
| publishDateSearch | 2004 |
| publishDateSort | 2004 |
| publisher | Forschungszentrum, Zentralbibliothek |
| record_format | marc |
| series | Schriften des Forschungszentrums Jülich |
| series2 | Schriften des Forschungszentrums Jülich : Reihe Umwelt |
| spelling | Tilmes, Simone 1973- Verfasser (DE-588)128707577 aut Chemical ozone loss in the arctic polar stratosphere an analysis of twelve years of satellite observations Simone Tilmes Jülich Forschungszentrum, Zentralbibliothek 2004 V, 162 S. Ill., graph. Darst. 24 cm txt rdacontent n rdamedia nc rdacarrier Schriften des Forschungszentrums Jülich : Reihe Umwelt 43 Zugl.: Frankfurt (Main), Univ., Diss., 2003 Geschichte 1991-2002 gnd rswk-swf Satellitenfernerkundung (DE-588)4224344-0 gnd rswk-swf Abbaureaktion (DE-588)4136352-8 gnd rswk-swf Ozon (DE-588)4173038-0 gnd rswk-swf Stratosphäre (DE-588)4132622-2 gnd rswk-swf Arktis (DE-588)4002924-4 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Arktis (DE-588)4002924-4 g Stratosphäre (DE-588)4132622-2 s Ozon (DE-588)4173038-0 s Abbaureaktion (DE-588)4136352-8 s Satellitenfernerkundung (DE-588)4224344-0 s Geschichte 1991-2002 z DE-604 Schriften des Forschungszentrums Jülich Reihe Umwelt ; 43 (DE-604)BV011951674 43 HBZ Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=017473716&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Tilmes, Simone 1973- Chemical ozone loss in the arctic polar stratosphere an analysis of twelve years of satellite observations Schriften des Forschungszentrums Jülich Satellitenfernerkundung (DE-588)4224344-0 gnd Abbaureaktion (DE-588)4136352-8 gnd Ozon (DE-588)4173038-0 gnd Stratosphäre (DE-588)4132622-2 gnd |
| subject_GND | (DE-588)4224344-0 (DE-588)4136352-8 (DE-588)4173038-0 (DE-588)4132622-2 (DE-588)4002924-4 (DE-588)4113937-9 |
| title | Chemical ozone loss in the arctic polar stratosphere an analysis of twelve years of satellite observations |
| title_auth | Chemical ozone loss in the arctic polar stratosphere an analysis of twelve years of satellite observations |
| title_exact_search | Chemical ozone loss in the arctic polar stratosphere an analysis of twelve years of satellite observations |
| title_full | Chemical ozone loss in the arctic polar stratosphere an analysis of twelve years of satellite observations Simone Tilmes |
| title_fullStr | Chemical ozone loss in the arctic polar stratosphere an analysis of twelve years of satellite observations Simone Tilmes |
| title_full_unstemmed | Chemical ozone loss in the arctic polar stratosphere an analysis of twelve years of satellite observations Simone Tilmes |
| title_short | Chemical ozone loss in the arctic polar stratosphere |
| title_sort | chemical ozone loss in the arctic polar stratosphere an analysis of twelve years of satellite observations |
| title_sub | an analysis of twelve years of satellite observations |
| topic | Satellitenfernerkundung (DE-588)4224344-0 gnd Abbaureaktion (DE-588)4136352-8 gnd Ozon (DE-588)4173038-0 gnd Stratosphäre (DE-588)4132622-2 gnd |
| topic_facet | Satellitenfernerkundung Abbaureaktion Ozon Stratosphäre Arktis Hochschulschrift |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=017473716&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| volume_link | (DE-604)BV011951674 |
| work_keys_str_mv | AT tilmessimone chemicalozonelossinthearcticpolarstratosphereananalysisoftwelveyearsofsatelliteobservations |