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Laser spectroscopy: 1 Basic principles

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Bibliographic Details
Main Author:	Demtröder, Wolfgang 1931- (Author)
Format:	Book
Language:	English
Published:	Berlin Springer 2008
Edition:	4. ed.
Subjects:	Laserspektroskopie
Online Access:	Inhaltsverzeichnis
Physical Description:	XVI, 457 S. Ill., graph. Darst.
ISBN:	9783540734154

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adam_text	Contents 1. Introduction ............................................................. 1 2. Absorption and Emission of Light .................................. 5 2.1 Cavity Modes ..................................................... 5 2.2 Thermal Radiation and Planck s Law .......................... 9 2.3 Absorption, Induced, and Spontaneous Emission ............. 11 2.4 Basic Photometric Quantities ................................... 15 2.4.1 Definitions ............................................... 16 2.4.2 Illumination of Extended Areas ...................... 18 2.5 Polarization of Light ............................................. 20 2.6 Absorption and Emission Spectra __,......................... 22 2.7 Transition Probabilities .......................................... 26 2.7.1 Lifetimes, Spontaneous and Radiationless Transitions ......................... 27 2.7.2 Semiclassical Description: Basic Equations ......... 29 2.7.3 Weak-Field Approximation ............................ 32 2.7.4 Transition Probabilities with Broad-Band Excitation 34 2.7.5 Phenomenological Inclusion of Decay Phenomena . 35 2.7.6 Interaction with Strong Fields ........................ 37 2.7.7 Relations Between Transition Probabilities, Absorption Coefficient, and Line Strength ........... 41 2.8 Coherence Properties of Radiation Fields ..................... 42 2.8.1 Temporal Coherence ................................... 43 2.8.2 Spatial Coherence ...................................... 44 2.8.3 Coherence Volume ..................................... 46 2.8.4 The Coherence Function and the Degree of Coherence ............................................ 49 2.9 Coherence of Atomic Systems .................................. 54 2.9.1 Density Matrix .......................................... 54 2.9.2 Coherent Excitation .................................... 56 2.9.3 Relaxation of Coherently Excited Systems .......... 58 Problems ................................................................. 58 3. Widths and Profiles of Spectral Lines .............................. 61 3.1 Natural Linewidth ................................................ 62 3.1.1 Lorentzian Line Profile of the Emitted Radiation .. 62 3.1.2 Relation Between Linewidth and Lifetime .......... 64 3.1.3 Natural Linewidth of Absorbing Transitions ........ 66 3.2 Doppler Width .................................................... 70 Contents 3 .3 Collisional Broadening of Spectral Lines ...................... 75 3.3.1 Phenomenological Description ........................ 75 3.3.2 Relations Between Interaction Potential, Line Broadening, and Shifts ........................... 80 3.3.3 Collisional Narrowing of Lines ....................... 84 3.4 Transit-Time Broadening ........................................ 84 3.5 Homogeneous and Inhomogeneous Line Broadening ........ 88 3.6 Saturation and Power Broadening .............................. 90 3.6.1 Saturation of Level Population by Optical Pumping 90 3.6.2 Saturation Broadening of Homogeneous Line Profiles ........................ 92 3.6.3 Power Broadening ...................................... 93 3.7 Spectral Line Profiles in Liquids and Solids .................. 95 Problems ................................................................. 97 Spectroscopie Instrumentation ....................................... 99 4.1 Spectrographs and Monochromators ........................... 99 4.1.1 Basic Properties ........................................ 101 4.1.2 Prism Spectrometer .................................... Ill 4.1.3 Grating Spectrometer .................................. 115 4.2 Interferometers .................................................... 124 4.2.1 Basic Concepts ......................................... 124 4.2.2 Michelson Interferometer .............................. 125 4.2.3 Fourier Spectroscopy ................................... 129 4.2.4 Mach-Zehnder Interferometer ........................ 131 4.2.5 Sagnac Interferometer .................................. 134 4.2.6 Multiple-Beam Interference ........................... 136 4.2.7 Plane Fabry-Perot Interferometer ..................... 144 4.2.8 Confocal Fabry-Perot Interferometer ................ 152 4.2.9 Multilayer Dielectric Coatings ........................ 157 4.2.10 Interference Filters ..................................... 162 4.2.11 Biréfringent Interferometer ............................ 165 4.2.12 Tunable Interferometers ................................ 169 4.3 Comparison Between Spectrometers and Interferometers .... 170 4.3.1 Spectral Resolving Power ............................. 170 4.3.2 Light-Gathering Power ................................. 173 4.4 Accurate Wavelength Measurements ........................... 174 4.4.1 Precision and Accuracy of Wavelength Measurements ......................... 175 4.4.2 Today s Wavemeters ................................... 178 4.5 Detection of Light ................................................ 188 4.5.1 Thermal Detectors ...................................... 191 4.5.2 Photodiodes ............................................. 198 4.5.3 Photodiode Arrays ...................................... 208 4.5.4 Charge-Coupled Devices (CCDs) ..................... 210 4.5.5 Photoemissive Detectors ............................... 212 4.5.6 Detection Techniques and Electronic Equipment ... 224 Contents XV 4.6 Conclusions ....................................................... 231 Problems ................................................................. 231 5. Lasers as Spectroscopie Light Sources ............................. 235 5.1 Fundamentals of Lasers .......................................... 235 5.1.1 Basic Elements of a Laser ............................ 235 5.1.2 Threshold Condition ................................... 236 5.1.3 Rate Equations .......................................... 238 5.2 Laser Resonators ................................................. 241 5.2.1 Open Optical Resonators .............................. 242 5.2.2 Spatial Field Distributions in Open Resonators ..... 245 5.2.3 Confocal Resonators ................................... 247 5.2.4 General Spherical Resonators ......................... 250 5.2.5 Diffraction Losses of Open Resonators .............. 251 5.2.6 Stable and Unstable Resonators ...................... 253 5.2.7 Ring Resonators ........................................ 258 5.2.8 Frequency Spectrum of Passive Resonators ......... 260 5.3 Spectral Characteristics of Laser Emission .................... 262 5.3.1 Active Resonators and Laser Modes ................. 263 5.3.2 Gain Saturation ......................................... 266 5.3.3 Spatial Hole Burning ................................... 268 5.3.4 Multimode Lasers and Gain Competition ........... 269 5.3.5 Mode Pulling ........................................... 273 5.4 Experimental Realization of Single-Mode Lasers ............ 274 5.4.1 Line Selection .......................................... 275 5.4.2 Suppression of Transverse Modes .................... 279 5.4.3 Selection of Single Longitudinal Modes ............. 281 5.4.4 Intensity Stabilization .................................. 288 5.4.5 Wavelength Stabilization .............................. 291 5.5 Controlled Wavelength Tuning of Single-Mode Lasers ...... 302 5.5.1 Continuous Tuning Techniques ....................... 303 5.5.2 Wavelength Calibration ................................ 308 5.5.3 Frequency Offset Locking ............................. 310 5.6 Linewidths of Single-Mode Lasers ............................. 310 5.7 Tunable Lasers .................................................... 314 5.7.1 Basic Concepts ......................................... 314 5.7.2 Semiconductor-Diode Lasers .......................... 315 5.7.3 Tunable Solid-State Lasers ............................ 321 5.7.4 Color-Center Lasers .................................... 325 5.7.5 Dye Lasers .............................................. 329 5.7.6 Excimer Lasers ......................................... 346 5.7.7 Free-Electron Lasers ................................... 349 5.8 Nonlinear Optical Mixing Techniques ......................... 352 5.8.1 Physical Background ................................... 353 5.8.2 Phase Matching ......................................... 358 5.8.3 Second-Harmonic Generation ......................... 360 5.8.4 Quasi Phase Matching ................................. 366 XVI Contents 5.8.5 Sum-Frequency and Higher-Harmonic Generation . 368 5.8.6 Х -Ray Lasers ........................................... 373 5.8.7 Difference-Frequency Spectrometer .................. 377 5.8.8 Optical Parametric Oscillator ......................... 380 5.8.9 Tunable Raman Lasers ................................. 384 5.9 Gaussian Beams .................................................. 388 Problems ................................................................. 394 Solutions ....................................................................... 397 References ..................................................................... 425 Subject Index ................................................................. 453
adam_txt	Contents 1. Introduction . 1 2. Absorption and Emission of Light . 5 2.1 Cavity Modes . 5 2.2 Thermal Radiation and Planck's Law . 9 2.3 Absorption, Induced, and Spontaneous Emission . 11 2.4 Basic Photometric Quantities . 15 2.4.1 Definitions . 16 2.4.2 Illumination of Extended Areas . 18 2.5 Polarization of Light . 20 2.6 Absorption and Emission Spectra _,. 22 2.7 Transition Probabilities . 26 2.7.1 Lifetimes, Spontaneous and Radiationless Transitions . 27 2.7.2 Semiclassical Description: Basic Equations . 29 2.7.3 Weak-Field Approximation . 32 2.7.4 Transition Probabilities with Broad-Band Excitation 34 2.7.5 Phenomenological Inclusion of Decay Phenomena . 35 2.7.6 Interaction with Strong Fields . 37 2.7.7 Relations Between Transition Probabilities, Absorption Coefficient, and Line Strength . 41 2.8 Coherence Properties of Radiation Fields . 42 2.8.1 Temporal Coherence . 43 2.8.2 Spatial Coherence . 44 2.8.3 Coherence Volume . 46 2.8.4 The Coherence Function and the Degree of Coherence . 49 2.9 Coherence of Atomic Systems . 54 2.9.1 Density Matrix . 54 2.9.2 Coherent Excitation . 56 2.9.3 Relaxation of Coherently Excited Systems . 58 Problems . 58 3. Widths and Profiles of Spectral Lines . 61 3.1 Natural Linewidth . 62 3.1.1 Lorentzian Line Profile of the Emitted Radiation . 62 3.1.2 Relation Between Linewidth and Lifetime . 64 3.1.3 Natural Linewidth of Absorbing Transitions . 66 3.2 Doppler Width . 70 Contents 3 .3 Collisional Broadening of Spectral Lines . 75 3.3.1 Phenomenological Description . 75 3.3.2 Relations Between Interaction Potential, Line Broadening, and Shifts . 80 3.3.3 Collisional Narrowing of Lines . 84 3.4 Transit-Time Broadening . 84 3.5 Homogeneous and Inhomogeneous Line Broadening . 88 3.6 Saturation and Power Broadening . 90 3.6.1 Saturation of Level Population by Optical Pumping 90 3.6.2 Saturation Broadening of Homogeneous Line Profiles . 92 3.6.3 Power Broadening . 93 3.7 Spectral Line Profiles in Liquids and Solids . 95 Problems . 97 Spectroscopie Instrumentation . 99 4.1 Spectrographs and Monochromators . 99 4.1.1 Basic Properties . 101 4.1.2 Prism Spectrometer . Ill 4.1.3 Grating Spectrometer . 115 4.2 Interferometers . 124 4.2.1 Basic Concepts . 124 4.2.2 Michelson Interferometer . 125 4.2.3 Fourier Spectroscopy . 129 4.2.4 Mach-Zehnder Interferometer . 131 4.2.5 Sagnac Interferometer . 134 4.2.6 Multiple-Beam Interference . 136 4.2.7 Plane Fabry-Perot Interferometer . 144 4.2.8 Confocal Fabry-Perot Interferometer . 152 4.2.9 Multilayer Dielectric Coatings . 157 4.2.10 Interference Filters . 162 4.2.11 Biréfringent Interferometer . 165 4.2.12 Tunable Interferometers . 169 4.3 Comparison Between Spectrometers and Interferometers . 170 4.3.1 Spectral Resolving Power . 170 4.3.2 Light-Gathering Power . 173 4.4 Accurate Wavelength Measurements . 174 4.4.1 Precision and Accuracy of Wavelength Measurements . 175 4.4.2 Today's Wavemeters . 178 4.5 Detection of Light . 188 4.5.1 Thermal Detectors . 191 4.5.2 Photodiodes . 198 4.5.3 Photodiode Arrays . 208 4.5.4 Charge-Coupled Devices (CCDs) . 210 4.5.5 Photoemissive Detectors . 212 4.5.6 Detection Techniques and Electronic Equipment . 224 Contents XV 4.6 Conclusions . 231 Problems . 231 5. Lasers as Spectroscopie Light Sources . 235 5.1 Fundamentals of Lasers . 235 5.1.1 Basic Elements of a Laser . 235 5.1.2 Threshold Condition . 236 5.1.3 Rate Equations . 238 5.2 Laser Resonators . 241 5.2.1 Open Optical Resonators . 242 5.2.2 Spatial Field Distributions in Open Resonators . 245 5.2.3 Confocal Resonators . 247 5.2.4 General Spherical Resonators . 250 5.2.5 Diffraction Losses of Open Resonators . 251 5.2.6 Stable and Unstable Resonators . 253 5.2.7 Ring Resonators . 258 5.2.8 Frequency Spectrum of Passive Resonators . 260 5.3 Spectral Characteristics of Laser Emission . 262 5.3.1 Active Resonators and Laser Modes . 263 5.3.2 Gain Saturation . 266 5.3.3 Spatial Hole Burning . 268 5.3.4 Multimode Lasers and Gain Competition . 269 5.3.5 Mode Pulling . 273 5.4 Experimental Realization of Single-Mode Lasers . 274 5.4.1 Line Selection . 275 5.4.2 Suppression of Transverse Modes . 279 5.4.3 Selection of Single Longitudinal Modes . 281 5.4.4 Intensity Stabilization . 288 5.4.5 Wavelength Stabilization . 291 5.5 Controlled Wavelength Tuning of Single-Mode Lasers . 302 5.5.1 Continuous Tuning Techniques . 303 5.5.2 Wavelength Calibration . 308 5.5.3 Frequency Offset Locking . 310 5.6 Linewidths of Single-Mode Lasers . 310 5.7 Tunable Lasers . 314 5.7.1 Basic Concepts . 314 5.7.2 Semiconductor-Diode Lasers . 315 5.7.3 Tunable Solid-State Lasers . 321 5.7.4 Color-Center Lasers . 325 5.7.5 Dye Lasers . 329 5.7.6 Excimer Lasers . 346 5.7.7 Free-Electron Lasers . 349 5.8 Nonlinear Optical Mixing Techniques . 352 5.8.1 Physical Background . 353 5.8.2 Phase Matching . 358 5.8.3 Second-Harmonic Generation . 360 5.8.4 Quasi Phase Matching . 366 XVI Contents 5.8.5 Sum-Frequency and Higher-Harmonic Generation . 368 5.8.6 Х -Ray Lasers . 373 5.8.7 Difference-Frequency Spectrometer . 377 5.8.8 Optical Parametric Oscillator . 380 5.8.9 Tunable Raman Lasers . 384 5.9 Gaussian Beams . 388 Problems . 394 Solutions . 397 References . 425 Subject Index . 453
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spelling	Demtröder, Wolfgang 1931- Verfasser (DE-588)120579774 aut Laser spectroscopy 1 Basic principles Wolfgang Demtröder 4. ed. Berlin Springer 2008 XVI, 457 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Laserspektroskopie (DE-588)4034620-1 gnd rswk-swf Laserspektroskopie (DE-588)4034620-1 s DE-604 (DE-604)BV023307227 1 Erscheint auch als Online-Ausgabe 978-3-540-73418-5 Digitalisierung UB Regensburg application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=016491586&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis
spellingShingle	Demtröder, Wolfgang 1931- Laser spectroscopy Laserspektroskopie (DE-588)4034620-1 gnd
subject_GND	(DE-588)4034620-1
title	Laser spectroscopy
title_auth	Laser spectroscopy
title_exact_search	Laser spectroscopy
title_exact_search_txtP	Laser spectroscopy
title_full	Laser spectroscopy 1 Basic principles Wolfgang Demtröder
title_fullStr	Laser spectroscopy 1 Basic principles Wolfgang Demtröder
title_full_unstemmed	Laser spectroscopy 1 Basic principles Wolfgang Demtröder
title_short	Laser spectroscopy
title_sort	laser spectroscopy basic principles
topic	Laserspektroskopie (DE-588)4034620-1 gnd
topic_facet	Laserspektroskopie
url	http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=016491586&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA
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work_keys_str_mv	AT demtroderwolfgang laserspectroscopy1

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