Laser chemistry: spectroscopy, dynamics and applications
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| Main Authors: | , , |
|---|---|
| Format: | Book |
| Language: | English |
| Published: |
Chichester [u.a.]
Wiley
2007
|
| Subjects: | |
| Online Access: | Inhaltsverzeichnis |
| Physical Description: | XIV, 502 S. Ill., graph. Darst. |
| ISBN: | 9780471485704 9780471485711 |
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| 100 | 1 | |a Telle, Helmut H. |e Verfasser |4 aut | |
| 245 | 1 | 0 | |a Laser chemistry |b spectroscopy, dynamics and applications |c Helmut H. Telle ; Angel González Ureña ; Robert J. Donovan |
| 264 | 1 | |a Chichester [u.a.] |b Wiley |c 2007 | |
| 300 | |a XIV, 502 S. |b Ill., graph. Darst. | ||
| 336 | |b txt |2 rdacontent | ||
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| 700 | 1 | |a Donovan, Robert J. |d 1912-2003 |e Verfasser |0 (DE-588)123674239 |4 aut | |
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Contents
Preface
xi
About the authors
xiii
1
Introduction
1
1.1
Basic concepts in laser chemistry
1
1.2
Organization of the book
10
PART
1
PRINCIPLES OF LASERS AND LASER SYSTEMS
15
2
Atoms and molecules, and their interaction with light waves
17
2.1
Quantum states, energy levels and wave functions
17
2.2 Dipole
transitions and transition probabilities
20
2.3
Einstein coefficients and excited-state lifetimes
23
2.4
Spectroscopie
line shapes
24
2.5
The polarization of light waves
26
2.6
Basic concepts of coherence
26
2.7
Coherent superposition of quantum states and the concept of wave packets
29
3
The basics of lasers
35
3.1
Fundamentals of laser action
35
3.2
Laser resonators
39
3.3
Frequency and spatial properties of laser radiation
41
3.4
Gain in continuous-wave and pulsed lasers
43
3.5
g-switching and the generation of nanosecond pulses
45
3.6
Mode locking and the generation of picosecond and femtosecond pulses
48
4
Laser systems
51
4.1
Fixed-wavelength gas lasers: helium-neon, rare-gas ion and excimer lasers
51
4.2
Fixed-wavelength solid-state lasers: the Nd:YAG laser
55
4.3
Tuneable dye laser systems
57
4.4
Tuneable Ti:sapphire laser systems
60
4.5
Semiconductor diode lasers
63
4.6
Quantum cascade lasers
67
4.7
Non-linear crystals and frequency-mixing processes
68
4.8
Three-wave mixing processes: doubling, sum and
difference frequency
72
4.9
Optical parametric oscillation
74
vi
CONTENTS
PART
2
SPECTROSCOPIC TECHNIQUES IN LASER CHEMISTRY
77
5
General concepts of laser spectroscopy
79
5.1
Spectroscopy based on photon detection
80
5.2
Spectroscopy based on charged particle detection
81
5.3
Spectroscopy based on measuring changes of macroscopic physical properties
of the medium
82
6
Absorption spectroscopy
87
6.1
Principles of absorption spectroscopy
87
6.2
Observable transitions in atoms and molecules
89
6.3
Practical implementation of absorption spectroscopy
91
6.4
Multipass absorption techniques
95
7
Laser-induced fluorescence spectroscopy
101
7.1
Principles of laser-induced fluorescence spectroscopy
102
7.2
Important parameters in laser-induced fluorescence
105
7.3
Practical implementation of laser-induced fluorescence spectroscopy
113
8
Light scattering methods: Raman spectroscopy and other processes
119
8.1
Light scattering
119
8.2
Principles of Raman spectroscopy
121
8.3
Practical implementation of Raman spectroscopy
125
9
Ionization spectroscopy
129
9.1
Principles of ionization spectroscopy
129
9.2 Photoion
detection
131
9.3
Photoelectron detection
135
9.4 Photoion
imaging
138
PART
3
OPTICS AND MEASUREMENT CONCEPTS
143
10
Reflection, refraction and diffraction
145
10.1
Selected properties of optical materials and light waves
145
10.2
Reflection and refraction at a plane surface
149
10.3
Light transmission through prisms
153
10.4
Light transmission through lenses and imaging
155
10.5
Imaging using curved mirrors
158
10.6
Superposition, interference and diffraction of light waves
158
10.7
Diffraction by single and multiple apertures
161
10.8
Diffraction gratings J64
11
Filters and thin-film coatings
169
11.1
Attenuation of light beams
159
11.2
Beamsplitters j7q
11.3
Wavelength-selective filters j72
11.4
Polarization filters
,j->
11.5
Reflection and filtering at optical component interfaces
176
11.6
Thin-film coatings ,77
CONTENTS
Vii
12
Optical fibres
183
12.1
Principles of optical fibre transmission
183
12.2
Attenuation in fibre transmission
185
12.3
Mode propagation in fibres
186
13
Analysis instrumentation and detectors
189
13.1
Spectrometers
189
13.2
Interferometers
190
13.3
Photon detectors exploiting the photoelectric effect
193
13.4
Photodetectors based on band-gap materials
194
13.5
Measuring laser power and pulse energy
197
13.6
Analysis of charged particles for charge, mass and energy
198
13.7
Charged-particle detectors
202
14
Signal processing and data acquisition
205
14.1
Signals, noise and noise reduction
205
14.2
DC, AC and balanced detection methods
208
14.3
Lock-in detection techniques
209
14.4
Gated integration/boxcar averaging techniques
212
14.5
Event counting
213
14.6
Digital conversion and data acquisition
216
PART
4
LASER STUDIES OF PHOTODISSOCIATION,
PHOTOIONIZATION AND UNIMOLECULAR PROCESSES
219
15
Photodissociation
of diatomic molecules
223
15.1
Photofragment
kinetic energy
223
15.2
Angular distributions and anisotropic scattering
225
15.3
Predissociation and curve crossing
226
15.4
Femtosecond studies: chemistry in the fast lane
228
15.5
Dissociation and oscillatory continuum emission
230
16
Photodissociation
of triatomic molecules
233
16.1
Photodissociation
of water
233
16.2
Photodissociation
of ozone
235
16.3
Laser-induced fluorescence and cavity ring-down studies
238
16.4
Femtosecond studies: transition-state spectroscopy
238
17
Photodissociation
of larger polyatomic molecules:
energy landscapes
241
17.1
Rydberg
tagging
241
17.2
Photodissociation
of ammonia
242
17.3
Selective bond breaking
243
17.4
Molecular elimination and three-body dissociation
244
18
Multiple and multiphoton excitation,
and photoionization
245
18.1
Infrared multiple-photon activation and unimolecular dissociation
246
18.2
Continuum intermediate states and bond stretching
247
viii CONTENTS
18.3
High-resolution zero kinetic energy photoelectron spectroscopy
251
18.4
Autoionization
254
18.5
Photoion-pair formation
256
19
Coherent control and the future of ultra-short probing
259
19.1
Coherent control of chemical processes
259
19.2
Time-resolved diffraction and attosecond probing
263
PART
5
LASER STUDIES OF BIMOLECULAR REACTIONS
265
20
Basic concepts of kinetics and reaction dynamics
267
20.1
Resumé
of kinetics
267
20.2
Introduction to reaction dynamics: total and differential reaction cross-sections
269
20.3
The Connection between dynamics and kinetics
272
20.4
Basic concepts of potential energy surfaces
273
20.5
Calculating potential energy surfaces
276
21
The molecular beam method: basic concepts and examples
of bimolecular reaction studies
279
21.1
Basic concepts
279
21.2
Interpretation of spatial and energy distributions: dynamics of a two-body collision
283
21.3
Interpretation of spatial and energy distributions: product angular and velocity distributions
as a route to the reaction mechanism
289
22
Chemical reactions with laser-prepared reagents
295
22.1
Energy selectivity: mode-selective chemistry
295
22.2
Energy selectivity: electronic excitation
296
22.3
Stereodynamical effects with laser-prepared reagents
300
23
Laser probing of chemical reaction products
307
23.1
Where does the energy of a chemical reaction go?
307
23.2
Probing the product state distribution of a chemical reaction
307
23.3
Crossed-beam techniques and laser
spectroscopie
detection: towards the state-to-state
differential reaction cross-section measurements
309
PART
6
LASER STUDIES OF CLUSTER AND
SURFACE REACTIONS
323
24
Laser studies of complexes: Van
der Waals
and
cluster reactions
327
24.1.
Experimental set-ups and methodologies
327
24.2.
Metal-containing complexes
332
24.3.
Non-metal van
der Waals
complexes
339
25
Solvation dynamics: elementary reactions in solvent cages
349
25
Л
.
Dissociation of clusters containing
Ig 349
25.2.
Dissociation of clusters containing
Ę"
350
25.3.
Proton-transfer reactions
353
CONTENTS ix
26
Laser studies of surface reactions: an introduction
357
26.1.
Resume of metal surface properties and electronic structure
357
26.2.
Particle-surface interaction
360
26.3.
Surface reaction mechanisms
364
26.4.
Experimental methods to investigate laser-induced surface reactions
367
27
Laser studies of surface reactions: photochemistry in the adsorbed state
371
27.1.
Adsórbate-
versus substrate-mediated processes
371
27.2.
Examples of photoinduced reactions in adsorbates
378
27.3.
Femto-chemistry at surfaces: the ultrafast reaction CO/O—[RuiOOOl)]
387
PART
7
SELECTED APPLICATIONS
391
28
Environmental and other analytical applications
393
28.1
Atmospheric gas monitoring using tuneable diode laser absorption spectroscopy
394
28.2
Closed-path tuneable diode laser absorption spectroscopy applications
398
28.3
Open-path tuneable diode laser absorption spectroscopy applications
403
28.4
The
lidar
technique for remote analysis
409
28.5
Lidar
in the study of atmospheric chemistry: tropospheric measurements
412
28.6
Lidar
in the study of atmospheric chemistry: stratospheric measurements
419
28.7
Laser desorption and ionization: laser-induced breakdown spectroscopy, matrix-assisted
laser desorption and ionization, and aerosol time-of-flight mass spectrometry
422
29
Industrial monitoring and process control
433
29.1
Laser-spectroscopic analysis of internal combustion engines
433
29.2
Laser-spectroscopic analysis of burners and incinerators
438
29.3
Laser-chemical processes at surfaces: nanoscale patterning
444
30
Laser applications in medicine and biology
449
30.1
Photodynamic therapy
449
30.2
Intra-cell mapping of drug delivery using Raman imaging
453
30.3
Breath diagnostics using laser spectroscopy
455
30.4
From photons to plant defence mechanisms
460
30.5
Application to volatile compounds: on-line detection of plant stress
461
30.6
Laser applications to the study of non-volatile compounds in fruits
463
References
471
References grouped by chapter
471
Further reading grouped by part
482
Web pages
483
Appendix
485
Common abbreviations and acronyms
485
Physical constants
486
Useful conversions and other relationships
486
Energy conversion factors
486
Index
487 |
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| id | DE-604.BV022448025 |
| illustrated | Illustrated |
| index_date | 2024-07-02T17:35:18Z |
| indexdate | 2025-05-28T06:00:11Z |
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| physical | XIV, 502 S. Ill., graph. Darst. |
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| spelling | Telle, Helmut H. Verfasser aut Laser chemistry spectroscopy, dynamics and applications Helmut H. Telle ; Angel González Ureña ; Robert J. Donovan Chichester [u.a.] Wiley 2007 XIV, 502 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Lasers in chemistry Laserchemie (DE-588)4034613-4 gnd rswk-swf Laserspektroskopie (DE-588)4034620-1 gnd rswk-swf Laserchemie (DE-588)4034613-4 s DE-604 Laserspektroskopie (DE-588)4034620-1 s Ureña, Angel González Verfasser aut Donovan, Robert J. 1912-2003 Verfasser (DE-588)123674239 aut Digitalisierung UB Regensburg https://bvbr.bib-bvb.de:443/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=015655961&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Telle, Helmut H. Ureña, Angel González Donovan, Robert J. 1912-2003 Laser chemistry spectroscopy, dynamics and applications Lasers in chemistry Laserchemie (DE-588)4034613-4 gnd Laserspektroskopie (DE-588)4034620-1 gnd |
| subject_GND | (DE-588)4034613-4 (DE-588)4034620-1 |
| title | Laser chemistry spectroscopy, dynamics and applications |
| title_auth | Laser chemistry spectroscopy, dynamics and applications |
| title_exact_search | Laser chemistry spectroscopy, dynamics and applications |
| title_exact_search_txtP | Laser chemistry spectroscopy, dynamics and applications |
| title_full | Laser chemistry spectroscopy, dynamics and applications Helmut H. Telle ; Angel González Ureña ; Robert J. Donovan |
| title_fullStr | Laser chemistry spectroscopy, dynamics and applications Helmut H. Telle ; Angel González Ureña ; Robert J. Donovan |
| title_full_unstemmed | Laser chemistry spectroscopy, dynamics and applications Helmut H. Telle ; Angel González Ureña ; Robert J. Donovan |
| title_short | Laser chemistry |
| title_sort | laser chemistry spectroscopy dynamics and applications |
| title_sub | spectroscopy, dynamics and applications |
| topic | Lasers in chemistry Laserchemie (DE-588)4034613-4 gnd Laserspektroskopie (DE-588)4034620-1 gnd |
| topic_facet | Lasers in chemistry Laserchemie Laserspektroskopie |
| url | https://bvbr.bib-bvb.de:443/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=015655961&sequence=000002&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
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