Modern spectroscopy:
Saved in:
| Main Author: | |
|---|---|
| Format: | Book |
| Language: | English |
| Published: |
Chichester [u.a.]
Wiley
2004
|
| Edition: | 4. ed., reprint. |
| Subjects: | |
| Online Access: | Inhaltsverzeichnis |
| Physical Description: | XXVII, 452 S. Ill., graph. Darst. |
| ISBN: | 0470844167 9780470844168 0470844159 |
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| 100 | 1 | |a Hollas, John Michael |e Verfasser |4 aut | |
| 245 | 1 | 0 | |a Modern spectroscopy |c J. Michael Hollas |
| 250 | |a 4. ed., reprint. | ||
| 264 | 1 | |a Chichester [u.a.] |b Wiley |c 2004 | |
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| adam_text | Titel: Modern spectroscopy
Autor: Hollas, John Michael
Jahr: 2004
Contents
Preface to first edition xiii
Preface to second edition xv
Preface to third edition xvii
Preface to fourth edition xix
Units, dimensions and conventions xxi
Fundamental constants xxiii
Useful conversion factors xxv
1 Some important results in quantum mechanics 1
1.1 Spectroscopy and quantum mechanics 1
1.2 The evolution of quantum theory 2
1.3 The Schrodinger equation and some of its solutions 8
1.3.1 The Schrodinger equation 9
1.3.2 The hydrogen atom 11
1.3.3 Electron spin and nuclear spin angular momentum 17
1.3.4 The Born-Oppenheimer approximation 19
1.3.5 The rigid rotor 21
1.3.6 The harmonic oscillator 23
Exercises 25
Bibliography 26
2 Electromagnetic radiation and its interaction with atoms
and molecules 27
2.1 Electromagnetic radiation 27
2.2 Absorption and emission of radiation 27
2.3 Line width 34
2.3.1 Natural line broadening 34
2.3.2 Doppler broadening 35
2.3.3 Pressure broadening 36
2.3.4 Power, or saturation, broadening 36
2.3.5 Removal of line broadening 37
2.3.5.1 Effusive atomic or molecular beams 37
2.3.5.2 Lamb dip spectroscopy 37
V
VI
CONTENTS
Exercises
Bibliography
3 General features of experimental methods
3.1 The electromagnetic spectrum
3.2 General components of an absorption experiment
3.3 Dispersing elements
3.3.1 Prisms
3.3.2 Diffraction gratings
3.3.3 Fourier transformation and interferometers
3.3.3.1 Radiofrequency radiation
3.3.3.2 Infrared, visible and ultraviolet radiation
3.4 Components of absorption experiments in various regions of the spectrum
3.4.1 Microwave and millimetre wave
3.4.2 Far-infrared
3.4.3 Near-infrared and mid-infrared
3.4.4 Visible and near-ultraviolet
3.4.5 Vacuum- or far-ultraviolet
3.5 Other experimental techniques
3.5.1 Attenuated total reflectance spectroscopy and
reflection-absorption infrared spectroscopy
3.5.2 Atomic absorption spectroscopy
3.5.3 Inductively coupled plasma atomic emission spectroscopy
3.5.4 Flash photolysis
3.6 Typical recording spectrophotometers for the near-infrared, mid-infrared,
visible and near-ultraviolet regions
Exercise
Bibliography
4 Molecular symmetry
4.1 Elements of symmetry
4.1.1 w-Fold axis of symmetry, C„
4.1.2 Plane of symmetry, a
4.1.3 Centre of inversion, i
4.1.4 n-Fold rotation-reflection axis of symmetry, Sn
4.1.5 The identity element of symmetry, I (or E)
4.1.6 Generation of elements
4.1.7 Symmetry conditions for molecular chirality
4.2 Point groups
4.2.1 C„ point groups
4.2.2 Sn point groups
4.2.3 Cnv point groups
4.2.4 £ „ point groups
4.2.5 Cnh point groups
4.2.6 Dnd point groups
Dnh point groups
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CONTENTS vii
4.2.8 Td point group 85
4.2.9 Oh point group 85
4.2.10 Kh point group 86
4.2.11 ffj point group 86
4.2.12 Other point groups 87
4.3 Point group character tables 87
4.3.1 C2v character table 87
4.3.2 C$v character table 92
4.3.3 character table 96
4.3.4 Ih character table 97
4.4 Symmetry and dipole moments 97
Exercises 102
Bibliography 102
5 Rotational spectroscopy 103
5.1 Linear, symmetric rotor, spherical rotor and asymmetric rotor molecules 103
5.2 Rotational infrared, millimetre wave and microwave spectra 105
5.2.1 Diatomic and linear polyatomic molecules 105
5.2.1.1 Transition frequencies or wavenumbers 105
5.2.1.2 Intensities 110
5.2.1.3 Centrifugal distortion 111
5.2.1.4 Diatomic molecules in excited vibrational states 112
5.2.2 Symmetric rotor molecules 113
5.2.3 Stark effect in diatomic, linear and symmetric rotor molecules 115
5.2.4 Asymmetric rotor molecules 116
5.2.5 Spherical rotor molecules 117
5.2.6 Interstellar molecules detected by their radioffequency, microwave
or millimetre wave spectra 119
5.3 Rotational Raman spectroscopy 122
5.3.1 Experimental methods 122
5.3.2 Theory of rotational Raman scattering 124
5.3.3 Rotational Raman spectra of diatomic and linear polyatomic
molecules 126
5.3.4 Nuclear spin statistical weights 128
5.3.5 Rotational Raman spectra of symmetric and asymmetric rotor
molecules 131
5.4 Structure determination from rotational constants 131
Exercises 134
Bibliography 135
6 Vibrational spectroscopy 137
6.1 Diatomic molecules 137
6.1.1 Infrared spectra 138
6.1.2 Raman spectra 140
6.1.3 Anharmonicity 142
6.1.3.1 Electrical anharmonicity 142
6.1.3.2 Mechanical anharmonicity 142
via
CONTENTS
6.1.4 Vibration-rotation spectroscopy
6.1.4.1 Infrared spectra 4
6.1.4.2 Raman spectra
6.2 Polyatomic molecules
6.2.1 Group vibrations
6.2.2 Number of normal vibrations of each symmetry species
6.2.2.1 Non-degenerate vibrations
6.2.2.2 Degenerate vibrations
6.2.3 Vibrational selection rules
6.2.3.1 Infrared spectra
6.2.3.2 Raman spectra
6.2.4 Vibration-rotation spectroscopy
6.2.4.1 Infrared spectra of linear molecules
6.2.4.2 Infrared spectra of symmetric rotors
6.2.4.3 Infrared spectra of spherical rotors
6.2.4.4 Infrared spectra of asymmetric rotors
6.2.5 Anharmonicity
6.2.5.1 Potential energy surfaces
6.2.5.2 Vibrational term values
6.2.5.3 Local mode treatment of vibrations
6.2.5.4 Vibrational potential functions with more than one minimum
6.2.5.4(a) Inversion vibrations
6.2.5.4(b) Ring-puckering vibrations
6.2.5.4(c) Torsional vibrations
Exercises
Bibliography
7 Electronic spectroscopy 199
7.1 Atomic spectroscopy 199
7.1.1 The periodic table 199
7.1.2 Vector representation of momenta and vector coupling approximations 201
7.1.2.1 Angular momenta and magnetic moments 201
7.1.2.2 Coupling of angular momenta . 205
7.1.2.3 Russell-Saunders coupling approximation 206
7.1.2.3(a) Non-equivalent electrons ¦ 206
7.1.2.3(b) Equivalent electrons 210
7.1.3 Spectra of alkali metal atoms 213
7.1.4 Spectrum of the hydrogen atom 216
7.1.5 Spectra of helium and the alkaline earth metal atoms 219
7.1.6 Spectra of other polyelcctronic atoms 222
7.2 Electronic spectroscopy of diatomic molecules 225
7.2.1 Molecular orbitals 225
7.2.1.1 Homonuclear diatomic molecules 225
7.2.1.2 Hetcronuclear diatomic molecules 232
7.2.2 Classification of electronic states 233
7.2.3 Electronic selection rules 236
7.2.4 Derivation of states arising from configurations 237
7.2.5 Vibrational coarse structure 240
7.2.5.1 Potential energy curves in excited electronic states 240
7.2.5.2 Progressions and sequences 242
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CONTENTS ix
7.2.5.3 The Franck-Condon principle 246
7.2.5.4 Deslandres tables 250
7.2.5.5 Dissociation energies 250
7.2.5.6 Repulsive states and continuous spectra 253
7.2.6 Rotational fine structure 254
7.2.6.1 I - I electronic and vibronic transitions 254
7.2.6.2 /7 — *2 electronic and vibronic transitions 257
7.3 Electronic spectroscopy of polyatomic molecules 260
7.3.1 Molecular orbitals and electronic states 260
7.3.1.1 AH2 molecules 261
7.3.1.1(a) /HAH =180° 261
7.3.1.1(b) /HAH —90 263
7.3.1.2 Formaldehyde (H2CO) 265
7.3.1.3 Benzene 267
7.3.1.4 Crystal field and ligand field molecular orbitals 270
7.3.1.4(a) Crystal field theory 271
7.3.1.4(b) Ligand field theory 273
7.3.1.4(c) Electronic transitions 275
7.3.2 Electronic and vibronic selection rules 275
7.3.3 Chromophorcs 278
7.3.4 Vibrational coarse structure 278
7.3.4.1 Sequences 278
7.3.4.2 Progressions 279
7.3.4.2(a) Totally symmetric vibrations 279
7.3.4.2(b) Non-totally symmetric vibrations 279
7.3.5 Rotational fine structure 283
7.3.6 Diffuse spectra 284
Exercises 287
Bibliography 288
8 PhotoeJectron and related spectroscopies 289
8.1 Photoelectron spectroscopy 289
8.1.1 Experimental methods 291
8.1.1.1 Sources of monochromatic ionizing radiation 291
8.1.1.2 Electron velocity analysers 294
8.1.1.3 Electron detectors 294
8.1.1.4 Resolution 294
8.1.2 Ionization processes and Koopmans theorem 295
8.1.3 Photoelectron spectra and their interpretation 297
8.1.3.1 Ultraviolet photoelectron spectra of atoms 297
8.1.3.2 Ultraviolet photoelectron spectra of molecules 298
8.1.3.2(a) Hydrogen 298
8.1.3.2(b) Nitrogen 300
8.1.3.2(c) Hydrogen bromide 302
8.1.3.2(d) Water 305
8.1.3.2(e) Benzene 305
8.1.3.3 X-ray photoelectron spectra of gases 307
8.1.3.4 X-ray photoelectron spectra of solids 313
8.2 Auger electron and X-ray fluorescence spectroscopy 315
8.2.1 Auger electron spectroscopy 317
8.2.1.1 Experimental method 317
CONTENTS
318
8.2.1.2 Processes in Auger electron ejection ^9
8.2.1.3 Examples of Auger electron spectra ^
8.2.2 X-ray fluorescence spectroscopy ^22
8.2.2.1 Experimental method ^24
8.2.2.2 Processes in X-ray fluorescence ^5
8.2.2.3 Examples of X-ray fluorescence spectra
8.3 Extended X-ray absorption fine structure ^ ^
Exercises ^35
Bibliography
9 Lasers and laser spectroscopy
9.1 General discussion of lasers
9.1.1 General features and properties
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9.1.2 Methods of obtaining population inversion 340
9.1.3 Laser cavity modes
9.1.4 (7-switching
9.1.5 Mode locking
9.1.6 Harmonic generation
9.2 Examples of lasers 346
9.2.1 The ruby and alexandrite lasers 346
9.2.2 The titanium-sapphire laser 348
9.2.3 The neodymium-YAG laser 349
9.2.4 The diode or semiconductor laser 350
9.2.5 The helium-neon laser 352
9.2.6 The argon ion and krypton ion lasers 354
9.2.7 The nitrogen (N2) laser 355
9.2.8 The excimer and exciplex lasers 356
9.2.9 The carbon dioxide laser 358
9.2.10 The dye lasers 359
9.2.11 Laser materials in general 362
9.3 Uses of lasers in spectroscopy 362
9.3.1 Hyper Raman spectroscopy 363
9.3.2 Stimulated Raman spectroscopy 365
9.3.3 Coherent anti-Stokes Raman scattering spectroscopy 367
9.3.4 Laser Stark (or laser electron resonance) spectroscopy 368
9.3.5 Two-photon and multiphoton absorption 371
9.3.6 Multiphoton dissociation and laser separation of isotopes 374
9.3.7 Single vibronic level, or dispersed, fluorescence 377
9.3.8 Light detection and ranging (LIDAR) 379
9.3.9 Cavity ring-down spectroscopy 382
9.3.10 Femtosecond spectroscopy 387
9.3.11 Spectroscopy of molecules in supersonic jets 393
9.3.11.1 Properties of a supersonic jet 393
9.3.11.2 Fluorescence excitation spectroscopy 396
9.3.11.3 Single vibronic level, or dispersed, fluorescence
spectroscopy 4QQ
9.3.11.4 Zero kinetic energy photoelectron spectroscopy 402
Exercises
Bibliography
404
405
CONTENTS
Appendix
A Character tables
B Symmetry species of vibrations
Index of Atoms and Molecules
Subject Index
|
| any_adam_object | 1 |
| author | Hollas, John Michael |
| author_facet | Hollas, John Michael |
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| author_sort | Hollas, John Michael |
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| dewey-full | 535.8/4 543.0858 |
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| dewey-search | 535.8/4 543.0858 |
| dewey-sort | 3535.8 14 |
| dewey-tens | 530 - Physics 540 - Chemistry and allied sciences |
| discipline | Chemie / Pharmazie Physik Chemie |
| edition | 4. ed., reprint. |
| format | Book |
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| genre | (DE-588)4123623-3 Lehrbuch gnd-content |
| genre_facet | Lehrbuch |
| id | DE-604.BV019645534 |
| illustrated | Illustrated |
| indexdate | 2024-07-09T20:02:03Z |
| institution | BVB |
| isbn | 0470844167 9780470844168 0470844159 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-012974321 |
| oclc_num | 54817480 |
| open_access_boolean | |
| owner | DE-20 DE-19 DE-BY-UBM |
| owner_facet | DE-20 DE-19 DE-BY-UBM |
| physical | XXVII, 452 S. Ill., graph. Darst. |
| publishDate | 2004 |
| publishDateSearch | 2004 |
| publishDateSort | 2004 |
| publisher | Wiley |
| record_format | marc |
| spelling | Hollas, John Michael Verfasser aut Modern spectroscopy J. Michael Hollas 4. ed., reprint. Chichester [u.a.] Wiley 2004 XXVII, 452 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Analyse spectrale Análise espectral larpcal Foto-elektronspectrometrie gtt Física moderna larpcal Kwantummechanica gtt Laser spectrometrie gtt Molecuulstructuur gtt Rotatiespectra gtt Spectrometrie gtt Vibratiespectra gtt Spectrum analysis Spektroskopie (DE-588)4056138-0 gnd rswk-swf Molekülspektroskopie (DE-588)4128850-6 gnd rswk-swf Theorie (DE-588)4059787-8 gnd rswk-swf Atomspektroskopie (DE-588)4143333-6 gnd rswk-swf (DE-588)4123623-3 Lehrbuch gnd-content Molekülspektroskopie (DE-588)4128850-6 s DE-604 Atomspektroskopie (DE-588)4143333-6 s Spektroskopie (DE-588)4056138-0 s Theorie (DE-588)4059787-8 s 1\p DE-604 HBZ Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=012974321&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis 1\p cgwrk 20201028 DE-101 https://d-nb.info/provenance/plan#cgwrk |
| spellingShingle | Hollas, John Michael Modern spectroscopy Analyse spectrale Análise espectral larpcal Foto-elektronspectrometrie gtt Física moderna larpcal Kwantummechanica gtt Laser spectrometrie gtt Molecuulstructuur gtt Rotatiespectra gtt Spectrometrie gtt Vibratiespectra gtt Spectrum analysis Spektroskopie (DE-588)4056138-0 gnd Molekülspektroskopie (DE-588)4128850-6 gnd Theorie (DE-588)4059787-8 gnd Atomspektroskopie (DE-588)4143333-6 gnd |
| subject_GND | (DE-588)4056138-0 (DE-588)4128850-6 (DE-588)4059787-8 (DE-588)4143333-6 (DE-588)4123623-3 |
| title | Modern spectroscopy |
| title_auth | Modern spectroscopy |
| title_exact_search | Modern spectroscopy |
| title_full | Modern spectroscopy J. Michael Hollas |
| title_fullStr | Modern spectroscopy J. Michael Hollas |
| title_full_unstemmed | Modern spectroscopy J. Michael Hollas |
| title_short | Modern spectroscopy |
| title_sort | modern spectroscopy |
| topic | Analyse spectrale Análise espectral larpcal Foto-elektronspectrometrie gtt Física moderna larpcal Kwantummechanica gtt Laser spectrometrie gtt Molecuulstructuur gtt Rotatiespectra gtt Spectrometrie gtt Vibratiespectra gtt Spectrum analysis Spektroskopie (DE-588)4056138-0 gnd Molekülspektroskopie (DE-588)4128850-6 gnd Theorie (DE-588)4059787-8 gnd Atomspektroskopie (DE-588)4143333-6 gnd |
| topic_facet | Analyse spectrale Análise espectral Foto-elektronspectrometrie Física moderna Kwantummechanica Laser spectrometrie Molecuulstructuur Rotatiespectra Spectrometrie Vibratiespectra Spectrum analysis Spektroskopie Molekülspektroskopie Theorie Atomspektroskopie Lehrbuch |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=012974321&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT hollasjohnmichael modernspectroscopy |