Four-wave mixing techniques applied to the investigation of non-adiabatic dynamics in polyatomic molecules:
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| Format: | Book |
| Language: | English German |
| Published: |
2002
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| Subjects: | |
| Online Access: | Inhaltsverzeichnis |
| Item Description: | Zsfassung in dt. Sprache. - Würzburg, Univ., Diss., 2002 |
| Physical Description: | X, 146 S. Ill., graph. Darst. |
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Record in the Search Index
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CONTENTS
LIST OF FIGURES. VII
1 INTRODUCTION AND MOTIVATION 1
2 THEORY 7
2.1 TIME-RESOLVED, THIRD-ORDER OPTICAL SPECTROSCOPY. 7
2.1.1 PERTURBATION THEORY FOR THIRD-ORDER INTERACTIONS 8
2.1.2 INDUCTION AND PROPAGATION OF A FIRST-ORDER POLARIZATION . 10
2.1.3 FORMATION AND PROPAGATION OF A POPULATION GRATING. 13
2.1.4 INDUCTION OF A THIRD-ORDER POLARIZATION AND BRAGG SCATTERING 17
2.2 CLASSIFICATION OF FOUR-WAVE MIXING TECHNIQUES . . 22
2.2.1 TIME-RESOLVED COHERENT ANTI-STOKES RAMAN SCATTERING
. 23
2.2.2 TIME-RESOLVED COHERENT STOKES RAMAN SCATTERING. 27
2.2.3 TRANSIENT GRATINGS. 29
2.3 THEORETICAL TREATMENT OF ELEMENTARY MOLECULAR DYNAMICS. 33
2.3.1 WAVE-PACKET FORMALISM OF COHERENT VIBRATIONAL STATES . 33
2.3.2 INTERNAL CONVERSION IN POLYATOMIC MOLECULES. 35
3 EXPERIMENTAL SETUP
T 45
3.1 GENERATION AND CHARACTERIZATION OF
FEMTOSECOND LASER PULSES. 45
3.1.1 1 KHZ LASER SYSTEM. 46
3.1.2 100 KHZ LASER SYSTEM. 48
3.2 PHASE-MATCHING FOR FOUR-WAVE MIXING SCHEMES.Y. 50
3.3 CCD BROADBAND DETECTION. 53
4 THE STATE SELECTIVITY OF FS TIME-RESOLVED FOUR-WAVE MIXING 57
4.1 METHODOLOGY OF TIME-RESOLVED DEGENERATE FOUR-WAVE MIXING . 58
4.2 EXPERIMENTAL RESULTS: CCD-BROADBAND DETECTION OF TIME-RESOLVED
FOUR-WAVE MIXING . 60
4.3 DISCUSSION: STATE-SELECTIVITY OF DIFFERENT FWM PROCESSES. 66
V
BIBLIOGRAFISCHE INFORMATIONEN
HTTP://D-NB.INFO/965107558
VI
CONTENTS
5 NON-ADIABATIC TRANSITIONS IN POLYATOMIC MOLECULES 71
5.1 THE SYSTEM: /3-CAROTENE. 72
5.2 THE ROLE OF SPECIFIC VIBRATIONAL MODES DURING AN INTERNAL CONVERSION
PROCESS. 75
5.2.1 METHODOLOGY OF THE
PUMP-CARS SCHEME. 79
5.2.2 EXPERIMENTAL RESULTS: CARS AS A MODE-SELECTIVE PROBE PRO
CESS IN A PUMP-PROBE SCHEME. 86
5.2.3 DISCUSSION: NUCLEAR MOTION INVOLVED IN THE SI/SO INTERNAL CON-'
VERSION OF /3-CAROTENE. 97
5.3 THE BEHAVIOR OF VIBRATIONALLY HOT MODES DURING INTERNAL CONVERSION
106
5.3.1 METHODOLOGY OF POPULATION GRATINGS IN /3-CAROTENE. 107
5.3.2 EXPERIMENTAL RESULTS: PROBING VIBRATIONALLY HOT MODES IN
ELECTRONIC DARK STATES. 109
5.3.3 DISCUSSION: VIBRATIONAL COOLING AND THE INCREASING RATE OF IN
TERNAL CONVERSION. 118
6 CONCLUSION - ZUSAMMENFASSUNG 125
6.1 CONCLUSION. 125
6.2 ZUSAMMENFASSUNG. 129
BIBLIOGRAPHY 133
ACKNOWLEDGEMENTS 143
LEBENSLAUF (CURRICULUM VITAE) 145 |
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| spelling | Siebert, Torsten Uwe 1969- Verfasser (DE-588)124032931 aut Four-wave mixing techniques applied to the investigation of non-adiabatic dynamics in polyatomic molecules von Torsten Uwe Siebert 2002 X, 146 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Zsfassung in dt. Sprache. - Würzburg, Univ., Diss., 2002 Provitamin A (DE-588)4233586-3 gnd rswk-swf Vierwellenmischung (DE-588)4232554-7 gnd rswk-swf Polyatomare Verbindungen (DE-588)4175110-3 gnd rswk-swf Spektroskopie (DE-588)4056138-0 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Provitamin A (DE-588)4233586-3 s Vierwellenmischung (DE-588)4232554-7 s DE-604 Polyatomare Verbindungen (DE-588)4175110-3 s Spektroskopie (DE-588)4056138-0 s DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=009938276&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Siebert, Torsten Uwe 1969- Four-wave mixing techniques applied to the investigation of non-adiabatic dynamics in polyatomic molecules Provitamin A (DE-588)4233586-3 gnd Vierwellenmischung (DE-588)4232554-7 gnd Polyatomare Verbindungen (DE-588)4175110-3 gnd Spektroskopie (DE-588)4056138-0 gnd |
| subject_GND | (DE-588)4233586-3 (DE-588)4232554-7 (DE-588)4175110-3 (DE-588)4056138-0 (DE-588)4113937-9 |
| title | Four-wave mixing techniques applied to the investigation of non-adiabatic dynamics in polyatomic molecules |
| title_auth | Four-wave mixing techniques applied to the investigation of non-adiabatic dynamics in polyatomic molecules |
| title_exact_search | Four-wave mixing techniques applied to the investigation of non-adiabatic dynamics in polyatomic molecules |
| title_full | Four-wave mixing techniques applied to the investigation of non-adiabatic dynamics in polyatomic molecules von Torsten Uwe Siebert |
| title_fullStr | Four-wave mixing techniques applied to the investigation of non-adiabatic dynamics in polyatomic molecules von Torsten Uwe Siebert |
| title_full_unstemmed | Four-wave mixing techniques applied to the investigation of non-adiabatic dynamics in polyatomic molecules von Torsten Uwe Siebert |
| title_short | Four-wave mixing techniques applied to the investigation of non-adiabatic dynamics in polyatomic molecules |
| title_sort | four wave mixing techniques applied to the investigation of non adiabatic dynamics in polyatomic molecules |
| topic | Provitamin A (DE-588)4233586-3 gnd Vierwellenmischung (DE-588)4232554-7 gnd Polyatomare Verbindungen (DE-588)4175110-3 gnd Spektroskopie (DE-588)4056138-0 gnd |
| topic_facet | Provitamin A Vierwellenmischung Polyatomare Verbindungen Spektroskopie Hochschulschrift |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=009938276&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
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