Ultrafast response of inter- and intramolecular hydrogen bonds in liquids: vibrational quantum beats and dephasing
Gespeichert in:
| 1. Verfasser: | |
|---|---|
| Format: | Buch |
| Sprache: | English |
| Veröffentlicht: |
Berlin
Logos-Verl.
2002
|
| Schlagworte: | |
| Online-Zugang: | Inhaltsverzeichnis |
| Beschreibung: | Zugl.: Berlin, Humboldt-Univ., Diss., 2002 |
| Beschreibung: | 125 S. graph. Darst. : 21 cm |
| ISBN: | 3897229471 |
Internformat
MARC
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| 003 | DE-604 | ||
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| 020 | |a 3897229471 |c kart. : EUR 40.50, sfr 72.10 |9 3-89722-947-1 | ||
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| 100 | 1 | |a Stenger, Jens |e Verfasser |4 aut | |
| 245 | 1 | 0 | |a Ultrafast response of inter- and intramolecular hydrogen bonds in liquids |b vibrational quantum beats and dephasing |c Jens Stenger |
| 264 | 1 | |a Berlin |b Logos-Verl. |c 2002 | |
| 300 | |a 125 S. |b graph. Darst. : 21 cm | ||
| 336 | |b txt |2 rdacontent | ||
| 337 | |b n |2 rdamedia | ||
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| 500 | |a Zugl.: Berlin, Humboldt-Univ., Diss., 2002 | ||
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Datensatz im Suchindex
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|---|---|
| adam_text |
CONTENTS
1
INTRODUCTION
5
2
FUNDAMENTAL
ASPECTS
AND
VIBRATIONAL
SPECTROSCOPY
OF
HYDROGEN
BONDS
9
2.1
LINEAR
IR-SPECTROSCOPY
AND
ANHARMONIC
COUPLING
.
9
2.2
NONLINEAR
ULTRAFAST
VIBRATIONAL
SPECTROSCOPY
ON
HYDROGEN
BONDS
.
12
3
THEORY
OF
NONLINEAR
OPTICAL
RESPONSE
AND
DEPHASING
15
3.1
THE
NONLINEAR
OPTICAL
RESPONSE
.
16
3.1.1
FEYNMAN
DIAGRAMS
.
16
3.2
DEPHASING
AND
THE
BROWNIAN
OSCILLATOR
.
18
3.3
LIMITING
CASES
OF
THE
BROWNIAN
OSCILLATOR
.
21
3.3.1
THE
UNDERDAMPED
OSCILLATOR:
COHERENT
VIBRATIONS
.
21
3.3.2
THE
OVERDAMPED
BROWNIAN
OSCILLATOR,
KUBO
'
S
THEORY
AND
THE
BLOCH
MODEL
.
21
3.4
VIBRATIONAL
DEPHASING
IN
HYDROGEN
BONDS
.
23
3.5
THEORY
OF
VIBRATIONAL
THIRD-ORDER
NONLINEAR
SPECTROSCOPY
.
24
3.5.1
PUMP-PROBE
SPECTROSCOPY
AND
QUANTUM
BEATS
.
25
3.5.2
PHOTON
ECHO
SPECTROSCOPY
.
28
4
EXPERIMENTAL
33
4.1
INTRODUCTION
.
33
4.2
THE
LASER
SYSTEM
.
34
4.3
NONLINEAR
PARAMETRIC
PROCESSES
.
34
4.4
MID
INFRARED
LIGHT
PULSES
OBTAINED
WITH
BBO
AND
AGGASJ
.
35
4.5
OPTICAL
PARAMETRIC
AMPLIFICATION
IN
KTP
.
36
4.6
PUMP-PROBE
EXPERIMENTS
.
36
4.7 FOUR-WAVE
MIXING
EXPERIMENTS
.
39
4.8
PULSE
CHARACTERIZATION
.
41
5
PHOTON
ECHO
SPECTROSCOPY
ON
LIQUID
WATER
43
5.1
INTRODUCTION
.
43
5.2
EXPERIMENTAL
.
46
5.3
RESULTS
.
47
5.4
THE
FAST
DEPHASING
PROCESS
.
52
5.4.1
ANALYSIS
.
52
5.4.2
DISCUSSION
.
54
5.5
TRANSIENT
GRATING
AND
ECHO
PEAK
SHIFT
.
55
5.5.1
ANALYSIS
.
55
CONTENTS
5.5.2
DISCUSSION
.
67
5.6
SUMMARY
AND
CONCLUSIONS
.
69
6
VIBRATIONAL
QUANTUM
BEATS
IN
INTRAMOLECULAR
HYDROGEN
BONDS
71
6.1
THE
MODEL
SYSTEM
PMME
AND
ITS
VIBRATIONAL
SPECTRUM
.
71
6.2
PUMP
PROBE
SPECTROSCOPY
AND
COHERENT
WAVE
PACKET
PROPAGATION
.
75
6.2.1
EXPERIMENTAL
.
75
6.2.2
RESULTS
.
75
6.2.3
ANALYSIS
.
81
6.2.4
DISCUSSION
.
85
6.3
THREE
PULSE
PHOTON
ECHO
SPECTROSCOPY
AND
DEPHASING
.
88
6.3.1
INTRODUCTION
.
88
6.3.2
EXPERIMENTAL
.
89
6.3.3
RESULTS
.
89
6.3.4
DISCUSSION
.
93
6.4
COHERENT
VIBRATIONAL
GROUND
STATE
DYNAMICS
IN
HBT
.
95
6.4.1
EXPERIMENTAL
.
96
6.4.2
RESULTS
AND
DISCUSSION
.
96
6.5
SUMMARY
AND
CONCLUSION
.
101
7
SUMMARY
AND
CONCLUSIONS
105
REFERENCES
109
ZUSAMMENFASSUNG
122
ACKNOWLEDGEMENTS
125
4 |
| any_adam_object | 1 |
| author | Stenger, Jens |
| author_facet | Stenger, Jens |
| author_role | aut |
| author_sort | Stenger, Jens |
| author_variant | j s js |
| building | Verbundindex |
| bvnumber | BV014309858 |
| ctrlnum | (OCoLC)52048256 (DE-599)BVBBV014309858 |
| dewey-full | 541.226 |
| dewey-hundreds | 500 - Natural sciences and mathematics |
| dewey-ones | 541 - Physical chemistry |
| dewey-raw | 541.226 |
| dewey-search | 541.226 |
| dewey-sort | 3541.226 |
| dewey-tens | 540 - Chemistry and allied sciences |
| discipline | Chemie / Pharmazie |
| format | Book |
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| id | DE-604.BV014309858 |
| illustrated | Illustrated |
| indexdate | 2024-08-23T00:34:30Z |
| institution | BVB |
| isbn | 3897229471 |
| language | English |
| oai_aleph_id | oai:aleph.bib-bvb.de:BVB01-009816824 |
| oclc_num | 52048256 |
| open_access_boolean | |
| owner | DE-29T DE-11 |
| owner_facet | DE-29T DE-11 |
| physical | 125 S. graph. Darst. : 21 cm |
| publishDate | 2002 |
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| publisher | Logos-Verl. |
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| spelling | Stenger, Jens Verfasser aut Ultrafast response of inter- and intramolecular hydrogen bonds in liquids vibrational quantum beats and dephasing Jens Stenger Berlin Logos-Verl. 2002 125 S. graph. Darst. : 21 cm txt rdacontent n rdamedia nc rdacarrier Zugl.: Berlin, Humboldt-Univ., Diss., 2002 Femtosekundenspektroskopie (DE-588)4276916-4 gnd rswk-swf Photonenecho (DE-588)4326486-4 gnd rswk-swf Wasserstoffbrückenbindung (DE-588)4064787-0 gnd rswk-swf Schwingungsspektroskopie (DE-588)4128960-2 gnd rswk-swf (DE-588)4113937-9 Hochschulschrift gnd-content Wasserstoffbrückenbindung (DE-588)4064787-0 s Femtosekundenspektroskopie (DE-588)4276916-4 s Schwingungsspektroskopie (DE-588)4128960-2 s Photonenecho (DE-588)4326486-4 s DE-604 DNB Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=009816824&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Stenger, Jens Ultrafast response of inter- and intramolecular hydrogen bonds in liquids vibrational quantum beats and dephasing Femtosekundenspektroskopie (DE-588)4276916-4 gnd Photonenecho (DE-588)4326486-4 gnd Wasserstoffbrückenbindung (DE-588)4064787-0 gnd Schwingungsspektroskopie (DE-588)4128960-2 gnd |
| subject_GND | (DE-588)4276916-4 (DE-588)4326486-4 (DE-588)4064787-0 (DE-588)4128960-2 (DE-588)4113937-9 |
| title | Ultrafast response of inter- and intramolecular hydrogen bonds in liquids vibrational quantum beats and dephasing |
| title_auth | Ultrafast response of inter- and intramolecular hydrogen bonds in liquids vibrational quantum beats and dephasing |
| title_exact_search | Ultrafast response of inter- and intramolecular hydrogen bonds in liquids vibrational quantum beats and dephasing |
| title_full | Ultrafast response of inter- and intramolecular hydrogen bonds in liquids vibrational quantum beats and dephasing Jens Stenger |
| title_fullStr | Ultrafast response of inter- and intramolecular hydrogen bonds in liquids vibrational quantum beats and dephasing Jens Stenger |
| title_full_unstemmed | Ultrafast response of inter- and intramolecular hydrogen bonds in liquids vibrational quantum beats and dephasing Jens Stenger |
| title_short | Ultrafast response of inter- and intramolecular hydrogen bonds in liquids |
| title_sort | ultrafast response of inter and intramolecular hydrogen bonds in liquids vibrational quantum beats and dephasing |
| title_sub | vibrational quantum beats and dephasing |
| topic | Femtosekundenspektroskopie (DE-588)4276916-4 gnd Photonenecho (DE-588)4326486-4 gnd Wasserstoffbrückenbindung (DE-588)4064787-0 gnd Schwingungsspektroskopie (DE-588)4128960-2 gnd |
| topic_facet | Femtosekundenspektroskopie Photonenecho Wasserstoffbrückenbindung Schwingungsspektroskopie Hochschulschrift |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=009816824&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
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