Photosynthetic excitons:
Saved in:
| Main Authors: | , , |
|---|---|
| Format: | Book |
| Language: | English |
| Published: |
Singapore [u.a.]
World Scientific
2000
|
| Subjects: | |
| Online Access: | Inhaltsverzeichnis |
| Physical Description: | XIV, 590 S. Ill., graph. Darst. |
| ISBN: | 9810232802 |
Staff View
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| 245 | 1 | 0 | |a Photosynthetic excitons |c Herbert van Amerongen ; Leonas Valkunas ; Rienk van Grondelle |
| 264 | 1 | |a Singapore [u.a.] |b World Scientific |c 2000 | |
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| 650 | 7 | |a Excitonen |2 gtt | |
| 650 | 7 | |a Fotosynthese |2 gtt | |
| 650 | 4 | |a Electronic excitation | |
| 650 | 4 | |a Energy transfer | |
| 650 | 4 | |a Exciton theory | |
| 650 | 4 | |a Molecular spectroscopy | |
| 650 | 4 | |a Photosynthesis | |
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Record in the Search Index
| _version_ | 1804128235874680832 |
|---|---|
| adam_text | PHOTOSYNTHETIC EXCITONS HERBERT VAN AMERONGEN VRIJE UNIVERSITEIT, THE
NETHERLANDS LEONAS VALKUNAS INSTITUTE OF PHYSICS, LITHUANIA RIENK VAN
GRONDELLE VRIJE UNIVERSITEIT, THE NETHERLANDS Y|B WORLD SCIENTIFIC
SINAADORE* NEW JERSEV L SINGAPORE * NEW JERSEY LONDON * HONG KONG
CONTENTS PREFACE V CHAPTER 1. INTRODUCTION: STRUCTURAL ORGANIZATION,
SPECTRAL PROPERTIES 1 AND EXCITATION ENERGY TRANSFER IN PHOTOSYNTHESIS
1. INTRODUCTION 1 /. / DISORDERED VS. ORDERED LIGHT-HARVESTING SYSTEMS 2
2. THE PHOTOSYNTHETIC PIGMENTS: CHLOROPHYLLS, 2 BACTERIOCHLOROPHYLLS AND
CAROTENOIDS 2.1 THE CHLOROPHYLLS 3 2.2 THE BACTERIOCHLOROPHYLLS 6 2.3
THE CAROTENOIDS 8 3. THE STRUCTURE AND FUNCTION OF IMPORTANT
PHOTOSYNTHETIC 11 PIGMENT-PROTEIN COMPLEXES 3.1 THE BACTERIAL
PHOTOSYNTHETIC REACTION CENTER 12 3.2 THE REACTION CENTERS OF
PHOTOSYSTEM II AND PHOTOSYSTEM I 1 5 3.3 THE PERIPHERAL LIGHT-HARVESTING
COMPLEX (LH2) OF 15 PHOTOSYNTHETIC PURPLE BACTERIA 3.4 THE
FENNA*MATTHEWS-OLSON PROTEIN OF GREEN SULPHUR 18 BACTERIA 3.5 LHCII, THE
MAJOR CHLOROPHYLL BINDING LIGHT-HARVESTING 19 COMPLEX OF PLANTS 3.6 THE
CORE ANTENNA AND REACTION CENTER OF PHOTOSYSTEM I 21 4. MECHANISM OF
ENERGY TRANSFER AND TRAPPING IN PHOTOSYNTHESIS 22 4.1 THE FOERSTER
EQUATION 22 4.2 TRAPPING BY THE REATION CENTER 23 5. ENERGY TRANSFER IN
SOME PHOTOSYNTHETIC SYSTEMS 28 5.1 ENERGY TRANSFER IN THE PERIPHERAL AND
CORE ANTENNAE OF 28 PHOTOSYNTHETIC PURPLE BACTERIA 5.2 ENERGY TRANSFER
IN THE FENNA*MATTHEWS*OLSON COMPLEX 32 5.3 ENERGY TRANSFER IN THE MAJOR
PERIPHERAL PLANT LIGHT- 33 HARVESTING COMPLEX LHCII 5.4 ENERGY TRANSFER
IN PHOTOSYSTEM I 35 6. CONCLUSIONS 37 VLLL CONTENTS REFERENCES 38
CHAPTER 2. THE EXCITON CONCEPT 47 1 . HISTORICAL OVERVIEW 47 2.
INTERACTIONS BETWEEN MOLECULES 48 3. THE EXCITONICALLY COUPLED DIMER 50
3.1 NON-EQUIVALENT SITE ENERGIES 5 3 3.2 TRANSITION DIPOLE MOMENT 55 4.
EXCITONIC INTERACTIONS IN LARGER SYSTEMS 62 5. MOLECULAR CRYSTALS 68 6.
MOLECULAR AND LATTICE VIBRATIONS AND LOSS OF EXCITON COHERENCE 69
REFERENCES 71 CHAPTER 3. SOME OPTICAL PROPERTIES OF THE EXCITONICALLY
COUPLED DIMER 73 1. INTRODUCTION 73 2. LINEAR DICHROISM 74 3. CIRCULAR
DICHROISM 79 3.1 THE CD OF A DIMER 81 4. FLUORESCENCE 81 5. FLUORESCENCE
ANISOTROPY 85 6. TRANSIENT ABSORPTION (PUMP-PROBE) 89 7.
TRIPLET-MINUS-SINGLET SPECTROSCOPY 95 8. STARK SPECTROSCOPY 96 9. A
HYPOTHETICAL DIMER 100 10. B820: AN EXCITONICALLY COUPLED DIMER FROM
PHOTOSYNTHETIC 104 PURPLE BACTERIA 11. SPECTROSCOPIC PROPERTIES OF *820
105 APPENDIX 3.1 DERIVATION OF EXPRESSIONS FOR LINEAR DICHROISM 113
APPENDIX 3.2 DERIVATION OF EXPRESSION FOR ANISOTROPY 115 REFERENCES 117
CHAPTER 4. MIXING WITH HIGHER EXCITED STATES 119 1. INTRODUCTION 119 2.
ABSORPTION 119 2.1 GROUND-STATE ABSORPTION 119 2.2 EXCITED-STATE
ABSORPTION AND TRANSIENT ABSORPTION 122 2.3 NON-DEGENERATE DIMER 126
PHOTOSYNTHETIC EXCITONS IX 3. CIRCULAR DICHROISM 129 4. CIRCULAR
DICHROISM OF B820 135 REFERENCES 138 CHAPTER 5. SPECTRAL SHAPES:
HOMOGENEOUS AND INHOMOGENEOUS 139 BROADENING 1. INTRODUCTION 139 2. THE
COUPLING OF VIBRATIONS AND PHONONS TO ELECTRONIC 139 TRANSITIONS 2.1
ADIABATIC APPROACH 140 2.2 TRANSITION DIPOLE MOMENT 144 2.3 ABSORPTION
SPECTRUM 147 2.4 ELECTRON-PHONON COUPLING 150 2.5 BROWNIAN OSCILLATOR
MODEL 151 3. HOMOGENEOUS AND INHOMOGENEOUS BROADENING 153 4. EXCITON
COUPLING AND SPECTRAL BROADENING 156 5. SPECTRAL MOMENTS 159 6. HOLE
BURNING 164 7. FLUORESCENCE LINE NARROWING 168 8. SEPARATION OF THE
BROADENING CONTRIBUTIONS FOR THE FMO 169 COMPLEX APPENDIX 5.1 THE
HARMONIC OSCILLATOR 176 APPENDIX 5.2 THE RESPONSE FUNCTION 184 APPENDIX
5.3 SPECTRAL MOMENTS FOR INHOMOGENEOUSLY BROADENED EXCITONIC 188 SPECTRA
APPENDIX 5.4 SPECTRAL MOMENTS FOR HOMOGENEOUSLY BROADENED EXCITONIC 190
SPECTRA REFERENCES 195 CHAPTER 6. SPECTROSCOPY OF EXCITONS IN MOLECULAR
CRYSTALS AND 197 AGGREGATES 1. INTRODUCTION 197 2. MOLECULAR CRYSTALS
197 3. CYCLIC MOLECULAR AGGREGATES 203 4. LINEAR MOLECULAR AGGREGATES
(J-AGGREGATES) 207 5. EFFECT OF DISORDER ON THE EXCITON SPECTRUM 208 6.
EXCITON-PHONON INTERACTION AND EXCITON SELF-TRAPPING 216 X CONTENTS 7.
OPTICAL TRANSITIONS 220 7. 1 TRANSITION DIPOLE STRENGTH AND SELECTION
RULES 220 7.2 EXCITON ABSORPTION BANDSHAPE 230 8. EXCITON MIGRATION 231
APPENDIX 6.1 EIGENFUNCTIONS OF LINEAR AGGREGATES 237 REFERENCES 238
CHAPTER 7. EXCITONIC INTERACTIONS IN PHOTOSYNTHETIC SYSTEMS: 241
SPECTROSCOPIC EVIDENCE 1. INTRODUCTION 241 2. CORRELATION OF STRUCTURAL
AND SPECTROSCOPIC PROPERTIES OF 241 PHOTOSYNTHETIC REACTION CENTERS 2.1
THE BACTERIAL REACTION CENTER 241 2.2 POLARIZED SPECTROSCOPY OF CRYSTALS
OF THE REACTION CENTER 243 OF RHODOPSEUDOMONAS VIRIDIS 2.3 CALCULATION
OF THE ABSORPTION SPECTRA 245 2.4 VIBRONIC COUPLING IN THE BACTERIAL
REACTION CENTER 248 2.5 CHARGE-TRANSFER STATES 252 2.6 THE TNULTIMERIC
EXCITON MODEL FOR THE PHOTOSYSTEM II 261 REACTION CENTER 2. 7
THEORETICAL METHODS 263 2.8 EXCITON CALCULATIONS 264 2.9 EXCITON
DEREALIZATION AND ENERGETIC DISORDER 265 2.10 THE MULTIMER MODEL OF
P680: COMPARISON WITH 267 EXPERIMENT 2.11 P680 268 2.12 PHOTOSYSTEM I
270 3. EXCITONIC INTERACTIONS IN LIGHT-HARVESTING PIGMENT-PROTEINS 273
3.1 LH2 273 3.2 THE STRUCTURE OFLH2 OF RHODOPSEUDOMONAS ACIDOPHILA 274
AND RHODOSPIRILLUM MOLISCHIANUM 3.3 SPECTROSCOPIC PROPERTIES OFLHL AND
LH2 276 3.4 CALCULATION OF THE SPECTROSCOPIC PROPERTIES OF LH2 AND LH 1
279 3.5 DIAGONAL DISORDER AND THE DIPOLE STRENGTH OF THE LOWEST 281
EXCITON STATEOF LH2 3.6 LOCALIZATION OF THE EXCITON IN THE PRESENCE OF
STATIC AND 283 DYNAMIC DISORDER PHOTOSYNTHETIC EXCITONS XI 3.7
CALCULATION OF THE LH2 CD SPECTRUM USING EXCITON THEORY 285 3.8 THE BCHL
A BINDING PROTEIN OF GREEN PHOTOSYNTHETIC SULPHUR 288 BACTERIA (THE
FENNA*MATTHEWS-OLSON COMPLEX) 4. THE MAJOR CHI A-CHL B LIGHT-HARVESTING
COMPLEX OF GREEN 297 PLANTS (OR LHCII) APPENDIX 7.1
CAROTENOID-CHLOROPHYLL INTERACTIONS IN LHCII 304 REFERENCES 305 CHAPTER
8. EXCITON DYNAMICS 311 1. INTRODUCTION 311 2. COHERENT VS. INCOHERENT
EXCITONS 311 3. STOCHASTIC LIOUVILLE EQUATION 316 4. DEPOLARIZATION FOR
A DIMER AS DESCRIBED BY THE STOCHASTIC 323 LIOUVILLE EQUATION 5.
MIGRATION OF LOCALIZED EXCITATIONS: THE FOERSTER EQUATION 329 6.
GENERALIZED MASTER EQUATION 333 7. EXCITON RELAXATION 337 REFERENCES 344
CHAPTER 9. EXCITON DYNAMICS IN DIFFERENT ANTENNA COMPLEXES. 347
COHERENCE AND INCOHERENCE 1. INTRODUCTION 347 2. C-PHYCOCYANIN 347 3.
ALLOPHYCOCYANIN 352 4. PERIDININ-CHLOROPHYLL-A-PROTEIN FROM
DINOFLAGELLATES 357 5. THE FMO COMPLEX FROM GREEN BACTERIA 363 6.
LIGHT-HARVESTING COMPLEX II FROM GREEN PLANTS 372 7. DYNAMICS OF ENERGY
TRANSFER IN LH1 AND LH2 OF 375 PHOTOSYNTHETIC PURPLE BACTERIA 7. 1
ENERGY TRANSFER AMONG THE B800 BACTERIOCHLOROPHYLLS IN 376 LH2 7.2 B800
TO B850 ENERGY TRANSFER 379 7. 3 ENERGY TRANSFER WITHIN THE STRONGLY
COUPLED B850 RING 3 81 7.4 INTERACTIONS AND ENERGY TRANSFER BETWEEN
CAROTENOID AND 387 BACTERIOCHLOROPHYLL MOLECULES OFLH2 REFERENCES 393
XLL CONTENTS CHAPTER 10. MIGRATION OF LOCALIZED EXCITONS: FOERSTER
EXCITATION ENERGY 401 TRANSFER AND TRAPPING BY REACTION CENTERS 1.
INTRODUCTION 401 2. EXCITATION TRAPPING BY REACTION CENTERS 402 2.1
KINETIC MODEL 404 2.2 AVERAGE-LIFETIME APPROACH 40 5 2.3
LONGEST-DECAY-TIME APPROACH 408 2.4 PERTURBED-TWO-LEVEL MODEL 409 2.5
COMPARISON OF THE MODELS 412 3. APPLICATION TO BACTERIAL PHOTOSYNTHESIS
415 3.1 LOCAL-TRAP APPROXIMATION 416 3.2 PERTURBED TWO-LEVEL
APPROXIMATION ALL 3.3 INTERPRETATION OF THE EFFECTIVE TRAPPING RATE 419
3.4 COMPARISON TO STANDARDIZED MODELS 421 4. APPLICATION TO PLANT
SYSTEMS 424 4.1 EXCITATION TRAPPING IN PSI 424 4.2 APPLICATION TO PSII
430 5. CONCLUDING REMARKS 434 APPENDIX 10.1 THE TRAP AS A LOCAL
PERTURBATION OF A LATTICE 437 APPENDIX 10.2 THE PERTURBED TWO-LEVEL
MODEL 440 APPENDIX 10.3 AVERAGED ORIENTATION FACTOR IN EXCITON TRANSFER
444 REFERENCES 445 CHAPTER 11. EXCITATION ENERGY TRANSFER AND TRAPPING.
EXPERIMENTS 449 1. INTRODUCTION 449 2. THE BACTERIAL PSU * ENERGY
TRANSFER OVER THE ANTENNA 449 NETWORK AND TRAPPING BY THE REACTION
CENTER 3. PHOTOSYSTEM II 453 3.1 ORGANIZATION 453 3.2 TRAPPING IN PSII
CORES 455 4. ENERGY TRANSFER DYNAMICS AND TRAPPING IN INTACT PSII 456 5.
ENERGY TRANSFER AND TRAPPING IN THE CORE ANTENNA OF 458 PHOTOSYSTEM I
5.1 ORGANIZATION AND STRUCTURE 459 5.2 STEADY-STATE SPECTROSCOPIC
PROPERTIES 460 5.3 TIME-RESOLVED EXCITATION DECAY AT ROOM TEMPERATURE
461 5.4 TRAPPING IN THE PHOTOSYSTEM I CORE COMPLEX 462 PHOTOSYNTHETIC
EXCITONS XLLL 5.5 TRAPPING IN LARGE PHOTOSYSTEM I COMPLEXES 465 5.6
EXCITATION DECAY IN INTACT PHOTOSYSTEM I 465 5.7 SPECTRAL AND SPATIAL
EQUILIBRATION IN PHOTOSYSTEM I 465 5.8 ENERGY TRANSFER IN PHOTOSYSTEM I
AT LOW TEMPERATURES 467 6. CONCLUDING REMARKS 470 REFERENCES 472 CHAPTER
12. NONLINEAR ANNIHILATION OF EXCITONS. THEORY 479 1. INTRODUCTION 479
2. ANNIHILATION IN LARGE AGGREGATES 480 2.1 MATHEMATICAL FORMULATION OF
THE KINETIC EQUATIONS 481 2.2 ANALYSIS OF KINETIC EQUATIONS 483 2.3
NONLINEAR EXCITATION QUENCHING 485 2.4 QUASI-LINEAR EXCITATION QUENCHING
487 2.5 FRACTAL MODEL FOR SPECTRALLY INHOMOGENEOUS AGGREGATES 488 3.
SMALL AGGREGATES 490 3.1 DISTRIBUTION FUNCTION APPROACH 490 3.2
STATISTICAL APPROACH 491 3.3 COHERENT EXCITONS 494 4. SINGLET-TRIPLET
ANNIHILATION 495 4.1 SINGLET EXCITATION TRAPPING BY TRIPLETS 495 4.2
FLUORESCENCE INDUCTION AND S-T ANNIHILATION 497 5. LOCAL HEATING DURING
ANNIHILATION 503 5.1 DISSIPATION OF VIBRATIONAL-MODE ENERGY 503 5.2
MODULATION OF THE NUCLEAR MOTION 505 6. EXCITATION ANNIHILATION STUDIED
BY PUMP-PROBE SPECTROSCOPY 506 6.1 HIGHER EXCITED STATE RELAXATION 507
6.2 EXCITATION CORRELATION EFFECTS 508 6.3 LOCAL TEMPERATURE EFFECT 509
APPENDIX 12.1 KINETIC EQUATIONS OF THE S-S ANNIHILATION 510 APPENDIX
12.2 DISTRIBUTION FUNCTION APPROACH FOR THREE-MOLECULAR 516 AGGREGATE
REFERENCES 519 CHAPTER 13. NONLINEAR ANNIHILATION OF EXCITONS.
EXPERIMENTAL 523 1. INTRODUCTION 523 2. FLUORESCENCE QUANTUM YIELD
MEASUREMENTS 523 XIV CONTENTS 3. ANNIHILATION KINETICS IN CHROMATOPHORES
530 4. FENNA-MATTHEWS-OLSON COMPLEX 535 5. ANNIHILATION KINETICS IN
LHCII COMPLEX 538 6. THE EFFECT OF S-T ANNIHILATION ON FLUORESCENCE
INDUCTION IN 546 PSII REFERENCES 548 CHAPTER 14. NONLINEAR SPECTROSCOPY
551 1. INTRODUCTION 551 /./ LINEAR RESPONSE 552 1.2 MULTI-WAVE MIXING
557 1.3 NONLINEAR OPTICAL RESPONSE 560 2. RESPONSE FUNCTIONS IN
MULTILEVEL SYSTEMS 568 3. EXPERIMENTS ON ENERGY TRANSFER AND ELECTRON
TRANSFER IN 575 PHOTOSYNTHESIS APPLYING NONLINEAR FEMTOSECOND
SPECTROSCOPY 3.1 THE 3PEPS METHOD 575 3.2 3PEPS EXPERIMENTS ON LH1
ANDLH2 COMPLEXES OF 578 RHODOBACTER SPHAEROIDES 3.3 3PEPS EXPERIMENTS ON
THE ACCESSORY PIGMENTS IN THE RC 580 OF RHODOBACTER SPHAEROIDES APPENDIX
14.1 FOURIER TRANSFORMATION 582 REFERENCES 583 SUBJECT INDEX 585
|
| any_adam_object | 1 |
| author | Amerongen, Herbert van 1959- Valkunas, Leonas Grondelle, Rienk van 1949- |
| author_GND | (DE-588)1154567192 (DE-588)1038699983 (DE-588)1154566358 |
| author_facet | Amerongen, Herbert van 1959- Valkunas, Leonas Grondelle, Rienk van 1949- |
| author_role | aut aut aut |
| author_sort | Amerongen, Herbert van 1959- |
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| ctrlnum | (OCoLC)45133895 (DE-599)BVBBV013443797 |
| dewey-full | 572.6 |
| dewey-hundreds | 500 - Natural sciences and mathematics |
| dewey-ones | 572 - Biochemistry |
| dewey-raw | 572.6 |
| dewey-search | 572.6 |
| dewey-sort | 3572.6 |
| dewey-tens | 570 - Biology |
| discipline | Physik Biologie |
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| id | DE-604.BV013443797 |
| illustrated | Illustrated |
| indexdate | 2024-07-09T18:46:02Z |
| institution | BVB |
| isbn | 9810232802 |
| language | English |
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| open_access_boolean | |
| owner | DE-19 DE-BY-UBM DE-703 DE-29T DE-355 DE-BY-UBR DE-20 DE-11 DE-188 |
| owner_facet | DE-19 DE-BY-UBM DE-703 DE-29T DE-355 DE-BY-UBR DE-20 DE-11 DE-188 |
| physical | XIV, 590 S. Ill., graph. Darst. |
| publishDate | 2000 |
| publishDateSearch | 2000 |
| publishDateSort | 2000 |
| publisher | World Scientific |
| record_format | marc |
| spelling | Amerongen, Herbert van 1959- Verfasser (DE-588)1154567192 aut Photosynthetic excitons Herbert van Amerongen ; Leonas Valkunas ; Rienk van Grondelle Singapore [u.a.] World Scientific 2000 XIV, 590 S. Ill., graph. Darst. txt rdacontent n rdamedia nc rdacarrier Excitonen gtt Fotosynthese gtt Electronic excitation Energy transfer Exciton theory Molecular spectroscopy Photosynthesis Photosynthese (DE-588)4045936-6 gnd rswk-swf Exziton (DE-588)4016091-9 gnd rswk-swf Photosynthese (DE-588)4045936-6 s Exziton (DE-588)4016091-9 s DE-604 Valkunas, Leonas Verfasser (DE-588)1038699983 aut Grondelle, Rienk van 1949- Verfasser (DE-588)1154566358 aut GBV Datenaustausch application/pdf http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=009176548&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA Inhaltsverzeichnis |
| spellingShingle | Amerongen, Herbert van 1959- Valkunas, Leonas Grondelle, Rienk van 1949- Photosynthetic excitons Excitonen gtt Fotosynthese gtt Electronic excitation Energy transfer Exciton theory Molecular spectroscopy Photosynthesis Photosynthese (DE-588)4045936-6 gnd Exziton (DE-588)4016091-9 gnd |
| subject_GND | (DE-588)4045936-6 (DE-588)4016091-9 |
| title | Photosynthetic excitons |
| title_auth | Photosynthetic excitons |
| title_exact_search | Photosynthetic excitons |
| title_full | Photosynthetic excitons Herbert van Amerongen ; Leonas Valkunas ; Rienk van Grondelle |
| title_fullStr | Photosynthetic excitons Herbert van Amerongen ; Leonas Valkunas ; Rienk van Grondelle |
| title_full_unstemmed | Photosynthetic excitons Herbert van Amerongen ; Leonas Valkunas ; Rienk van Grondelle |
| title_short | Photosynthetic excitons |
| title_sort | photosynthetic excitons |
| topic | Excitonen gtt Fotosynthese gtt Electronic excitation Energy transfer Exciton theory Molecular spectroscopy Photosynthesis Photosynthese (DE-588)4045936-6 gnd Exziton (DE-588)4016091-9 gnd |
| topic_facet | Excitonen Fotosynthese Electronic excitation Energy transfer Exciton theory Molecular spectroscopy Photosynthesis Photosynthese Exziton |
| url | http://bvbr.bib-bvb.de:8991/F?func=service&doc_library=BVB01&local_base=BVB01&doc_number=009176548&sequence=000001&line_number=0001&func_code=DB_RECORDS&service_type=MEDIA |
| work_keys_str_mv | AT amerongenherbertvan photosyntheticexcitons AT valkunasleonas photosyntheticexcitons AT grondellerienkvan photosyntheticexcitons |